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Exploring one material for dual applications:A red-emitting Mg2GeO4:Eu3+ nanophosphor for future generation energy efficient WLEds and dosimetric applications

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Journal of Rare Earths 2024年第10期42卷 1835-1845页

作者： Akshay Arjun G.P.darshan S.C.Sharma H.Nagabhushana d.V.Sunitha H.B.Premkumar department of Physics Faculty of Mathematical and Physical SciencesM.S.Ramaiah University of Applied Sciences Jain University C.N.R.Rao Centre for Advanced Materials Tumkur University School of Applied Sciences (Physics) REVA University

The envisaged design and developme nt of individual mate rials to excavate a broader spectrum of desired properties and offer multiple applications are highly *** this in mind,a series of forsterite-structured Mg2GeO4:Eu3+（1 mol%-9 mol%） nanophosphors was synthesized via a solution combustion method using oxalyl dihydrazide as a *** X-ray.diffraction patterns confirm the orthorhombic crystal system with a Puma space *** results clearly show irregularly shaped cluster-like structures with aggregation of the *** diffuse reflectance spectra,the optical energy band gap of the Mg2GeO4:Eu3+（1 mol%-9 mol%） nanophosphors was estimated and obtained to be～4.12-4.32 *** photoluminescence emission spectra exhibit intense peaks at ～579,589,610,661,and 707 nm,which are due to characteristic5d0→7F0,5d0→7F1,5do→7F2,5d0→7F3and5d0→7F4transitions of Eu3+ions,*** Commission International de L'Eclairage color coordinates are gradually tuned from pale red（0.5980,0.4012） to a pure red（0.6385,0.3611） *** glow peaks showcase excellent super-linear response at low doses of γ-irradiations,indicating that the prepared phosphor can be used in thermoluminescent personal dosimetry which is a biological tissue *** aforementioned results demonstrate that the prepared Mg2GeO4:Eu3+（1 mol%-9 mol%） nanophosphors are considered an excellent candidate for dual applications,i.e.,red component in future generation white-light-emitting diodes（WLEds） and personal dosimetric applications.

关键词： Nanophosphors Photoluminescence Thermoluminescence dosimetry Photometric properties

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Preparation and elements analysis of porous fluorescent glasses

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中国有色金属学会会刊：英文版 2006年第B01期16卷 79-81页

作者：朱冬梅罗发周万城 d.E.dAY C.S.ray State Key Laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an 710072China Graduate Center for Materials Research University of Missouri-RollaRollaMissouri 65409-1170USA

A large variety of porous fluorescent glasses were prepared and the concentration of different elements in these glasses was analyzed. The start porous glasses were soaked in a solution containing soluble salts and then heated at 650 ℃ for 3 h to decompose the salts in the pores into oxides. Fluorescent agents, such as UO3, Eu2O3, were impregnated into the porous glasses to prepare the fluorescent glasses. The results show that soaking is a feasible method to prepare the glass sphere with compositions distinguishable from each other and easy to be located in a complicated background. Six or more components can be impregnated together into one glass sample and the concentration of them can be analyzed accurately. UO3 and Eu2O3 can be impregnated into porous glass to make the glass strongly fluorescent. Higher concentration of Eu2O3 produces stronger fluorescence while higher concentration of UO3 reduces the fluorescence intensity because of the concentration quenching effect.

关键词：多孔荧光玻璃制备元素分析发光性质可变成分

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Insights into chondrule formation process and shock-thermal history of the dergaon chondrite (H4-5)

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Geoscience Frontiers 2017年第3期8卷 413-423页

作者： d. ray S. Ghosh T.K. Goswami M.J. Jobin PLANEX Physical Research Laboratory Ahmedabad 380 009 India department of Applied Geology Dibrugarh University Assam India department of Applied Geology Pondicherry University India

The dergaon fall represents a shock-melted H4-5 （S5） ordinary chondrite which includes at least ten textural varieties of chondrules and belongs to the high chondrule-matrix ratio type. Our study reveals that the chondrules are of diverse mineralogy with variable olivine-pyroxene ratios （Type Ⅱ）, igneous melt textures developed under variable cooling rates and formed through melt fractionations from two different melt reservoirs. Based on the experimental analogues, mineralogical associations and phase compositions, it is suggested that the dergaon chondrules reflect two contrasting environments： a hot, dust-enriched and highly oxidized nebular environment through melting, without significant evapora- tion, and an arrested reducing environment concomitant with major evaporation loss of alkali and highly volatile trace elements. Coexistence of chlorapatite and merrillite suggests formation of the dergaon matrix in an acidic accretionary environment. Textural integration and chemical homogenization occurred at - I atmospheric pressure and a mean temperature of 765 ℃ mark the radiogenic thermal event. Equilibrated shock features （olivine mosaicism, diaplectic plagioclase, polycrystalline troilite） due to an impact-induced thermal event reflect a shock pressure 〉45 GPa and temperature of 600 ℃. By contrast, the local disequilibrium shock features （silicate melt veins comprising of olivine crystallites, troilite melt veins and metal droplets） correspond to a shock pressure up to 75 GPa and temperature 〉950 ℃.

关键词： dergaon chondrite Chondrule Thermal metamorphism Shock metamorphism

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Glass and Mineral Chemistry of Northern Central Indian Ridge Basalts:Compositional diversity and Petrogenetic Significance

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Acta Geologica Sinica(English Edition) 2009年第6期83卷 1122-1135页

作者： dwijesh ray Ranadip BANERJEE Sridhar d IYER Basavaraju BASAVALINGU Subir MUKHOPAdHYAY4 National Centre for Antarctic and Ocean Research National Institute of Oceanography CSIR department of Studies in Geology University of Mysore department of Geological Sciences Jadavpur University

The glass and mineral chemistry of basaits examined from the northern central Indian ridge （NCIR） provides an insight into magma genesis around the vicinity of two transform faults： Vityaz （VT） and Vema （VM）. The studied mid-ocean ridge basalts （MORBs） from the outer ridge flank （VT area） and a near-ridge seamount （VM area） reveal that they are moderately phyric plagioclase basalts composed of plagioclase （phenocryst [An60-90] and groundmass [An35-79]）, olivine （Fo81-88）, diopside （Wo45-51, En25-37, Fs14-24）, and titanomagnetite （FeOt -63.75 wt% and TiO2 -22.69 wt%）. The wholerock composition of these basalts has similar Mg# [mole Mg/mole（Mg＋Fe2＋）] （VT basalt： -0.56-0.58; VM basalt： -0.57）, but differ in their total alkali content （VT basalt： -2.65; VM basalt： -3.24）. The bulk composition of the magma was gradually depleted in MgO and enriched in FeOt, TiO2, P2O5, and Na2O with progressive fractionation, the basalts were gradually enriched in Y and Zr and depleted in Ni and Cr. In addition, the ∑REE of magma also increased with fractionation, without any change in the （La/ Yb）N value. Glass from the VM seamount shows more fractionated characters （Mg#： 0.56-0.57） compared to the outer ridge flank lava of the VT area （Mg#： 0.63-0.65）. This study concludes that present basalts experienced low-pressure crystallization at a relatively shallow depth. The geochemical changes in the NCIR magmas resulted from fractional crystallization at a shallow depth. As a consequence, spinel was the first mineral to crystallize at a pressure 〉10 kbar, followed by Fe-rich olivine at 〈10 kbar pressure.

关键词： mineral chemistry fractional crystallization petrogenesis northern central Indian ridge

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A Petrogenetic Model of Basalts from the Northern Central Indian Ridge:3-11°S

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Acta Geologica Sinica(English Edition) 2007年第1期81卷 99-112页

作者： dwijesh ray Sridhar d. IYER Ranadip BANERJEE Saumitra MISRA M. WIddOWSON Geological Oceanography division National Institute of Oceanography Goa-403 004 India department of Geology and Geophysics Indian Institute of Technology Kharagpur-721 302 India department of Earth Sciences Open University Milton Keynes MK7 6AA U.K.

Mid-Ocean Ridge Basalts （MORB） from the Northern Central Indian Ridge （NCIR） were recovered between latitudes 3° and 11° S and are olivine tholeiite with higher abundances of K and Rb. They are of typical transitional MORB （T-MORB） variety and appear to have been generated from an enriched-mantle peridotite source. The primitive NCIR MORBs having Mg^# 〉 0.68 are the product of partial melting at an estimated pressure of - 1 GPa. It is inferred that the magma was subsequently modified at a pressure 〉 1 GPa by crystal fractionation and spinel was the first mineral to crystallize followed by separation of relatively Fe-rich olivine with subsequent decrease in pressure. during progressive fractionation at lower pressure （between 1-0.5 GPa）, the bulk composition of the magma became systematically depleted in MgO, and enriched in ∑FeO, TiO2, P2Os and Na20. There was, however, limited gradual depletion in Al2O3 and CaO and concomitant enrichment in K20. With the progressive fractionation these basalts became gradually enriched in V, Co, Y, Zr and to some extent in Sr, and depleted in Ni and Cro In addition, the T_JtEE of the magma also increased with fractionation, without any change in （La/Yb）n value.

关键词： MORB NCIR geochemistry petrogenesis Indian Ocean mid-ocean ridge

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Cu/TiO_(2) Photocatalysts for CO_(2) Reduction: Structure and Evolution of the Cocatalyst Active Form

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Transactions of Tianjin University 2024年第2期30卷 140-151页

作者： Andrey A.Saraev Anna Yu.Kurenkova denis d.Mishchenko Alexandr L.Trigub Evgeniy Yu.Gerasimov Ekaterina A.Kozlova Boreskov Institute of Catalysis Lavrentieva Ave 5Novosibirsk 630090Russia Synchrotron Radiation Facility SKIF Boreskov Institute of CatalysisNikol’skiy Ave 1Kol’tsovo 630559Russia National Research Center “Kurchatov Institute”Kurchatova Sq 1Moscow 123182Russia

Extensive work on a Cu-modified TiO_(2) photocatalyst for CO_(2) reduction under visible light irradiation was conducted. The structure of the copper cocatalyst was established using UV-vis diff use refl ectance spectroscopy, high-resolution transmis- sion electron microscopy, X-ray absorption spectroscopy, and X-ray photoelectron spectroscopy. It was found that copper exists in different states (Cu 0 , Cu^(+) , and Cu^(2+) ), the content of which depends on the TiO_(2) calcination temperature and copper loading. The optimum composition of the cocatalyst has a photocatalyst based on TiO_(2) calcined at 700℃ and modified with 5 wt% copper, the activity of which is 22 μmol/(h·g cat ) (409 nm). Analysis of the photocatalysts after the photocatalytic reaction disclosed that the copper metal on the surface of the calcined TiO_(2) was gradually converted into Cu_(2) O during the photocatalytic reaction. Meanwhile, the metallic copper on the surface of the noncalcined TiO_(2) did not undergo any trans- formation during the reaction.

关键词： Photocatalysis Photocatalytic CO_(2)conversion Visible light Titanium dioxide Copper Copper oxides Methane formation Photocatalyst transformation

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SMILE soft X-ray Imager flight model CCd370 pre-flight device characterisation

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Earth and Planetary Physics 2024年第1期8卷 25-38页

作者： S.Parsons d.J.Hall O.Hetherington T.W.Buggey T.Arnold M.W.J.Hubbard A.Holland Centre for Electronic Imaging the Open UniversityMilton KeynesMK76AAUK

Throughout the SMILE mission the satellite will be bombarded by radiation which gradually damages the focal plane devices and degrades their *** order to understand the changes of the CCd370s within the soft X-ray Imager,an initial characterisation of the devices has been carried out to give a baseline performance *** CCds have been characterised,the two flight devices and the flight spa *** has been carried out at the Open University in a bespo ke cleanroom measure ment *** results show that there is a cluster of bright pixels in the flight spa re which increases in size with tempe *** at the nominal ope rating tempe rature(-120℃) it is within the procure ment ***,the devices meet the specifications when ope rating at -120℃ in 6 × 6 binned frame transfer science *** se rial charge transfer inefficiency degrades with temperature in full frame *** any charge losses are recovered when binning/frame transfer is implemented.

关键词： CCd soft X-ray imager characterisation SMILE

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One-neutron stripping process in the^(209)Bi(^(6)Li,^(5)Li)^(210)Bi*reaction reaction

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Nuclear Science and Techniques 2024年第6期35卷 120-129页

作者： Gao-Long Zhang Zhen-Wei Jiao Guang-Xin Zhang E.N.Cardozo B.Paes Shi-Peng Hu Jian-Qiang Qian daniele Mengoni Wei-Wei Qu Cong-Bo Li Yun Zheng Huan-Qiao Zhang Hui-Bin Sun Nan Wang Chun-Lei Zhang J.J.Valiente-dobón d.Testov M.Mazzocco A.Gozzelino C.Parascandolo d.Pierroutsakou M.La Commara A.Goasduff d.Bazzacco d.R.Napoli F.Galtarossa F.Recchia A.Illana S.Bakes I.Zanon S.Aydin Gde Angelis M.Siciliano R.Menegazzo S.M.Lenzi S.Akkoyun L.F.Canto J.Lubian School of Physics Beihang UniversityBeijing 100191China Sino-French Institute of Nuclear Engineering and Technology Sun Yat-Sen UniversityZhuhai 519082China Instituto de Física Universidade Federal Fluminense24210-340 NiteróiRio de JaneiroBrazil Laboratorio TANdAR Comisión Nacional de Energía AtómicaBKNA1650 San MartíınArgentina Institute for Advanced Study in Nuclear Energy and Safety Shenzhen UniversityShenzhen 518060China Shenzhen Key Laboratory of Research and Manufacture of High Purity Germanium Materials and Fetectors Shenzhen UniversityShenzhen 518060China INFN Sezione di PadovaPaduaItaly dipartimento di fisica Astronomia dell’Universita di padova PaduaItaly State Key Laboratory of Radiation Medicine and Protection School of Radiation Medicine and ProtectionSoochow UniversitySuzhou 215123China China Institute of Atomic Energy Beijing 102413China The Key Laboratory of Beam Technology and Material Modification of Ministry of Education College of Nuclear Science and TechnologyBeijing Normal UniversityBeijing 100875China Laboratori Nazionali di Legnaro INFN35020 LegnaroItaly INFN Sezione di Napoli80126 NaplesItaly dipartimento di Farmacia Universitàdi Napoli“Federico II”80131 NaplesItaly department of Natural and Mathematical Sciences Faculty of EngineeringTarsus University33480 MersinTurkey Physics division Argonne National LaboratoryLemontILUSA department of Physics Sivas Cumhuriyet UniversitySivasTurkey Instituto de Física Universidade Federal do Rio de JaneiroRio de Janeiro CP 6852821941-972Brazil

One-neutron stripping process between^(6)Li and^(209)Bi was studied at 28,30,and 34 MeV using the in-beamγ-ray spectroscopy ***γ-γcoincident analysis clearly identified twoγ-rays feeding the ground and long-lived isomeric states,which were employed to determine the cross *** one-neutron stripping cross sections were similar to the cross sections of complete fusion in the^(6)Li+^(209)Bi system,but the one-neutron stripping cross sections decreased more gradually at the sub-barrier region.A coupled-reaction-channel calculation was performed to study the detailed reaction mechanism of the one-neutron stripping process in^(6)*** calculations indicated that the first excited state of 5 Li is critical in the actual one-neutron transfer mechanism,and the valence proton of 209Bi can be excited to the low-lying excited state in(^(6)Li,^(5)Li)reaction,unlike in the(d,p)reaction.

关键词： Transfer reaction Weakly bound nuclei Cross section

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ZnO/CeO_(2)/carbon xerogel composites with direct Z-scheme heterojunctions:Enhancing photocatalytic remediation of 4-chlorophenol under visible light

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Journal of Rare Earths 2024年第2期42卷 314-322,I0003页

作者： Nicolas Perciani de Moraes Maite Birkett de Campos Sanmartin Robson da Silva Rocha Abner de Siervo Marcos Roberto de Vasconcelos Lanza d.Amaranatha Reddy Lianqing Yu Liana Alvares Rodrigues Escola de Engenharia de Lorena-EEL/USP Estrada Municipal do Campinho S/NCEP 12602-810LorenaSao PauloBrazil Institute of Physics"Gleb Wataghin" Applied Physics DepartmentState University of Campinas13083-859CampinasSPBrazi Instituto de Quimica de Sao Carlos Universidade de Sao PauloAv.Trab.Sao Carlense400-Parque Arnold SchimidtSao CarlosSP13566-590Spain department of Sciences Indian Institute of Information Technology Design and ManufacturingKurnoolAndhra Pradesh518007India School of Materials Science and Engineering China University of PetroleumQingdao266580China

This paper aims to create visible light driven ternary photocatalysts using zinc oxide(ZnO),cerium(IV)oxide(CeO_(2)),and carbon xerogel(CX) as constituent *** use of CeO_(2) is based on the creation of direct-Z-scheme heterojunctions with the ZnO and the consequent diminishing of charge recombination,whereas the carbon xerogel inclusion is predicted to minimize bandgap energy,decrease electro n-hole reco mbination,and boost specific surface *** re,the choice of the black-wattle tannin as a carbonaceous precursor was targeted at the development of an environmentally friendly and affordable *** existence of the hexagonal phase of zinc oxide and cubic structure of the cerium(IV) oxide in the ternary material was confirmed by X-ray.diffractometry and X-ray photoelectron spectroscopy,with the latter also suggesting chemical bonding between the ZnO and the CX due to the creation of zinc oxycarbide *** inclusion of the carbon xerogel provokes a significant modification in the morphology of the ternary material,resulting in an increased surface area and smaller particle *** CX/ZnO-CeO_(2) ternary composite obtains the highest photocatalytic efficiency among all the materials studied,degrading 100% of 4-chlorophenol under simulated sunlight and 68% under visible radiation,after 5 *** increased photocatalytic activity can be attributed to the formation of direct Z-scheme heterojunctions between the semiconductors,higher visible light response,and higher specific surface area,as evidenced by the results obtained by active radical scavenging,chronoamperometry,diffuse reflectance spectroscopy,and N_(2) adsorption-desorption isotherms.

关键词： Zinc oxide Cerium(Ⅳ)oxide Carbon xerogel Photocatalysis direct Z-scheme heterojunction 4-Chlorophenol Rare earths

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Painlevé analysis,auto-Bäcklund transformation and new exact solutions of(2+1)and(3+1)-dimensional extended Sakovich equation with time dependent variable coefficients in ocean physics

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Journal of Ocean Engineering and Science 2023年第3期8卷 246-262页

作者： Shailendra Singh S.Saha ray National Institute of Technology Department of MathematicsRourkela 769008India

This article considers time-dependent variable coefficients(2+1)and(3+1)-dimensional extended Sakovich ***éanalysis and auto-Bäcklund transformation methods are used to examine both the considered ***éanalysis is appeared to test the integrability while an auto-Bäcklund transformation method is being presented to derive new analytic soliton solution families for both the considered *** new family of exact analytical solutions are being obtained success-fully for each of the considered *** soliton solutions in the form of rational and exponential functions are being *** results are also expressed graphically to illustrate the potential and physical behaviour of both *** the considered equations have applications in ocean wave theory as they depict new solitary wave soliton solutions by 3d and 2d graphs.

关键词： (2+1)-dimensional extended Sakovich equation (3+1)-dimensional extended Sakovich equation Auto-Bäcklund transformation Painlevéanalysis Solitary wave solution

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