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A mixed-valence polyoxometalate-based 3D inorganic framework cathode material for high-efficiency rechargeable AZIBs

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Rare Metals 2024年第8期43卷 3677-3691页

作者： Qing Han Hao-ran xiao Tao Zhou Bing-Chuan Li Liu Yang Ling-Ling Xie Xue-Jing Qiu Xian-Yong Wu Li-Min Zhu xiao-Yu Cao School of Chemistry and Chemical Engineering Henan University of TechnologyZhengzhou 450001China Key Laboratory of High Specific Energy Materials for Electrochemical Power Sources of Zhengzhou City Zhengzhou 450001China College of Materials Engineering Henan University of EngineeringZhengzhou450007China School of Environmental Engineering Henan University of TechnologyZhengzhou 450001China Department of Chemistry University of Puerto Rico-Rio Piedras CampusSan JuanPR 00925USA

The global trend towards new energy storage systems has stimulated the development of electrochemical energy storage *** these technologies,rechargeable aqueous zinc-ion batteries(AZIBs)have attracted considerable interest as a potential alternative to lithium-ion batteries(LIBs)due to their affordable cost,environmental compatibility and high safety *** this study,a high-quality electrode for AZIBs has been successfully developed using a dehydrated mixed-valence polyoxometalate-based three-dimensional(3D)inorganic framework material known as[H_6Mn_(3)V^Ⅳ_(15)V-^Ⅴ_(4O)_(46)(H_2O)_(12)](3D-MnVO).This innovative 3D-MnVO material is built from the alternate connections of{V_(19)O_(46)}"sphere-shaped"clusters andμ_(2)-{Mn(H_(2)O)_(4)}bridges,where each{V_(19)O_(46)}cluster is surrounded by three pairs of vertically distributed{Mn(H_(2)O)_(4)}units,thus resulting in the 3D interpenetrating grid-like network from the infinite[-{V_(19)O_(46)}-μ_(2)-Mn(H_(2)O)_(4)-{V_(19)O_(46)}]_∞chains in three mutually perpendicular *** 3D framework structure of 3D-MnVO possesses abundant oxygen vacancies,spacious and multi-level interconnected channels for ion transport,which facilitates the efficient intercalation/deintercalation of hydrated Zn^(2+)into the pores of the primary structure via the intercalation capacitance *** a result,the 3D-MnVO electrode exhibits excellent diffusion rates and minimal interfacial *** a current density of 0.1 A·g^(-1),the 3D-MnVO cathode delivers a commendable discharge capacity of170.5 mAh·g^(-1)with 81.6%capacity retention after100 charge/discharge ***,even at a high current density of 1.0 A·g^(-1),the 3D-MnVO electrode delivers a remarkable reversible capacity of198.9 mAh·g^(-1).Our research results provide valuable insights into the development of advanced polyoxometalate-based 3D inorganic framework electrode materials for high-performance rechargeable AZIBs.

关键词： Cathode Polyoxometalate 3D inorganic framework Zinc-ion batteries Energy storage mechanism

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Simultaneous multiplex genome loci editing of Halomonas bluephagenesis using an engineered CRISPR-guided base editor

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Synthetic and Systems Biotechnology 2024年第3期9卷 586-593页

作者： Yulin Zhang Yang Zheng Qiwen Hu Zhen Hu Jiyuan Sun Ping Cheng Xiancai Rao xiao-ran Jiang Medical Research Institute Southwest UniversityChongqing400716China Department of Microbiology College of Basic Medical SciencesArmy Medical University(Third Military Medical University)Chongqing400038China

Halomonas bluephagenesis TD serves as an exceptional chassis for next generation industrial biotechnology to produce various ***,the simultaneous editing of multiple loci in *** TD remains a significant ***,we report the development of a multiple loci genome editing system,named CRISPR-deaminase-assisted base editor(CRISPR-BE)in *** *** system comprises two components:a cytidine(CRISPR-cBE)and an adenosine(CRISPR-aBE)deaminase-based base ***-cBE can introduce a cytidine to thymidine mutation with an efficiency of up to 100%within a 7-nt editing window in *** ***,CRISPR-aBE demonstrates an efficiency of up to 100%in converting adenosine to guanosine mutation within a 7-nt editing ***-cBE has been further validated and successfully employed for simultaneous multiplexed editing in *** *** findings reveal that CRISPR-cBE efficiently inactivated all six copies of the IS1086 gene simultaneously by introducing stop *** system achieved an editing efficiency of 100%and 41.67%in inactivating two genes and three genes,*** substituting the Pcas promoter with the inducible promoter PMmp1,we optimized CRISPR-cBE system and ultimately achieved 100%editing efficiency in inactivating three *** conclusion,our research offers a robust and efficient method for concurrently modifying multiple loci in *** TD,opening up vast possibilities for industrial applications in the future.

关键词： Base editor Gene editing Multiplex Halomonas bluephagenesis

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Tragic Beauty of Faulkner’s Villain Characters

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Journal of Literature and Art Studies 2024年第9期14卷 774-777页

作者： LIU xiao-ran Faculty of English Language and Culture Guangdong University of Foreign StudiesGuangzhouChina

This paper applies the theory of“Sphinx Factor”to examine the characters such as Sutpen,Emily and Jason in Faulkner’s fiction who are filled with brutal *** is found that although these characters are generally con... 详细信息

关键词： tragic beauty bestial elements Sphinx Factor Faulkner’s fiction Ethics

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Spatiotemporal distribution,environmental risk and carbon emission reduction potential of livestock manure in Shaanxi Province,China

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Frontiers of Agricultural Science and Engineering 2024年第3期11卷 381-396页

作者： Mengyuan QIAO Jianchun ZHU Ronghua LI Junting PAN ran xiao Hailong WANG Kuok Ho Daniel TANG Zengqiang ZHANG College of Humanities&Social Development Northwest A&F UniversityYangling 712100China College of Natural Resources and Environment Northwest A&F UniversityKey Laboratory of Low-carbon Green Agriculture in Northwestern ChinaMinistry of Agriculture and Rural AffairsYangling 712100China Key Laboratory of Non-point Source Pollution of Ministry of Agricultural and Rural Affairs Institute of Agricultural Resources and Regional PlanningChinese Academy of Agricultural SciencesBeijing 100081China Interdisciplinary Research Center for Agriculture Green Development in Yangtze River Basin College of Resources and EnvironmentSouthwest UniversityChongqing 400715China Biochar Engineering Technology Research Center of Guangdong Province School of Environmental and Chemical EngineeringFoshan UniversityGuangdong 528000China Department of Environmental Science University of ArizonaTucsonAZ 85721USA

Shaanxi is a leading province in animal husbandry(AH)in ***,the lack of provincial information on the characteristics and utilization potential of livestock manure(LM)hinders crucial management ***,we investigated the spatiotemporal distribution,availability and biogas potential of LM in Shaanxi,and examine the carbon emission reduction potential of *** has been a 1.26-fold increase in LM quantities in Shaanxi over the past 35 years,reaching 4635.6×10^(4)t by *** was mainly concentrated in northern Shaanxi and the eastern part of *** and pig manure were the primary sources of LM,with the average LM land-load of 14.57 t·ha^(−1)in *** the overall AH in Shaanxi has not exceeded the environmental capacity,the actual scales of AH in Ankang and Hanzhong have already surpassed the respective environmental capacities,posing a higher risk of N and P *** 2021,the estimated biogas energy potential of LM was 1.2×10^(11)*** 2012 to 2021,the average carbon emission reduction potential in Shaanxi was 22%,with an average potential scale of 10%.The results of this research provide valuable data and policy recommendations for promoting the intensive use of LM and reducing carbon emissions in Shaanxi.

关键词： Livestock manure emission estimation N and P loads biogas potential carbon emission reduction

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围绝经期血管舒缩症状非激素治疗药物fezolinetant

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中国新药杂志 2024年第8期33卷 752-755页

作者：肖然杜小莉中国医学科学院北京协和医院药剂科北京100730

fezolinetant(商品名:Veozah^(TM))是美国FDA批准的第1款用于治疗围绝经期血管舒缩症状(vasomotor symptoms,VMS)的选择性神经激肽3受体(neurokinin 3 receptor,NK3R)拮抗剂。与传统的雌激素疗法相比,fezolinetant降低了心血管不良事件及乳腺癌的发生风险。临床研究证实,fezolinetant可显著降低中重度VMS的发生频率与严重程度,且安全性良好。本文就fezolinetant的作用机制、药动学、药效学、临床疗效、安全性、药物相互作用等方面进行介绍。

关键词： fezolinetant 血管舒缩症状神经激肽3受体拮抗剂围绝经期

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Multiple pollutants from crop and livestock production in the Yangtze River: status and challenges

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Frontiers of Agricultural Science and Engineering 2024年第1期11卷 134-139,I0005页

作者： Lihua MA Shiyang LI Linfa FANG Xuanjing CHEN ran xiao xiaoxuan SU Zhaolei LI Zhaohai BAI Lin MA Prakash LAKSHMANAN Xinping CHEN Interdisciplinary Research Center for Agriculture Green Development in Yangtze River Basin College of Resources and EnvironmentSouthwest UniversityChongqing 400715China Water Systems and Global Change Group Wageningen University&Research6708 PB Wageningenthe Netherlands Key Laboratory of Agricultural Water Resources Center for Agricultural Resources ResearchInstitute of Genetic and Developmental BiologyChinese Academy of SciencesShijiazhuang 050021China Key Laboratory of Sugarcane Biotechnology and Genetic Improvement(Guangxi) Ministry of Agriculture and Rural AffairsGuangxi Key Laboratory of Sugarcane Genetic ImprovementSugarcane Research InstituteGuangxi Academy of Agricultural SciencesNanning 530007China Queensland Alliance for Agriculture and Food Innovation University of QueenslandSt Lucia 4067Australia

The rapid increase in the proportion of cash crops and livestock production in the Yangtze River Basin has led to commensurate increases in fertilizer and pesticide inputs. Excessive application of chemical fertilizer, organophosphorus pesticides and inappropriate disposal of agricultural waste induced water pollution and potentially threaten Agriculture Green Development(AGD). To ensure food security and the food supply capacity of the Yangtze River Basin, it is important to balance green and development, while ensuring the quality of water bodies. Multiple pollutants affect the transfer, adsorption, photolysis and degradation of each other throughout the soil-plant-water system. This paper considers the impact of multi-pollutants on the nitrogen and phosphorus cycles especially for crops, which are related to achieving food security and AGD. It presents prospective on theory, modeling and multi-pollutant control in the Yangtze River Basin for AGD that are of potential value for other developing regions.

关键词： Agriculture Green Development crop production livestock production multi-pollutant models multiple pollutants Yangtze River Basin

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大学生主动性社交网站使用与友谊质量的关系:线上积极反馈和社交自我效能感的中介作用

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中国临床心理学杂志 2024年第2期32卷 446-450,456页

作者：李笑燃内蒙古师范大学心理学院呼和浩特010022

目的:探讨大学生主动性社交网站使用、线上积极反馈、社交自我效能感与友谊质量的关系。方法:采用主动性社交网站使用问卷、线上积极反馈量表、社交自我效能感量表和友谊质量问卷对687名大学生进行调查。结果:(1)主动性社交网站使用、... 详细信息

目的:探讨大学生主动性社交网站使用、线上积极反馈、社交自我效能感与友谊质量的关系。方法:采用主动性社交网站使用问卷、线上积极反馈量表、社交自我效能感量表和友谊质量问卷对687名大学生进行调查。结果:(1)主动性社交网站使用、线上积极反馈、社交自我效能感与友谊质量两两间均呈显著正相关;(2)主动性社交网站使用不仅对友谊质量有直接正向预测作用,而且还能通过线上积极反馈、社交自我效能感的链式中介作用间接影响大学生的友谊质量。结论:研究揭示了线上积极反馈和社交自我效能感在主动性社交网站使用与大学生友谊质量关系间的中介作用机制,对正确引导大学生合理利用社交网站来发展良好的友谊关系有一定的借鉴和启示。

关键词：社交网站线上积极反馈社交自我效能感友谊质量

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高校“有组织科研”的碎片化困境与突破路径

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科学学研究 2024年第10期42卷 2122-2129页

作者：黄巨臣萧然兰州大学高等教育研究院甘肃兰州730000 广西医科大学信息与管理学院广西南宁530021

高校“有组织科研”以提升自主创新能力和服务国家战略需求为主要目标,但在开展过程中存在的碎片化困境影响了目标实现。本文借助整体性治理理论思想,关照现实情况,构建“价值—制度—技术—主体”的四维度分析框架,并基于实际调查和深... 详细信息

高校“有组织科研”以提升自主创新能力和服务国家战略需求为主要目标,但在开展过程中存在的碎片化困境影响了目标实现。本文借助整体性治理理论思想,关照现实情况,构建“价值—制度—技术—主体”的四维度分析框架,并基于实际调查和深度访谈发现,当前高校实施“有组织科研”面临的困境主要体现在学术信念的“疏离”、管理政策的“脱嵌”、数据信息的“孤岛”以及主体参与的“悬浮”等,实则反映出了价值、制度、技术以及行动主体的碎片化问题。从整体性治理思维出发,应从坚持“以学术作为志业”的价值理念、实现“联动式攥指成拳”的政策协同、打通“共享最后一公里”的技术壁垒和探寻“利益最大公约数”的集体行动来协同破解既存困境,高质量推进高校“有组织科研”。

关键词：高校 “有组织科研” 碎片化整体性治理

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Extracellular vesicles derived from mesenchymal stem cells mediate extracellular matrix remodeling in osteoarthritis through the transport of microRNA-29a

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World Journal of Stem Cells 2024年第2期16卷 191-206页

作者： Fan Yang Wan-Qi Xiong Chen-Zhi Li Ming-Jian Wu Xiu-Zhi Zhang Chun-xiao ran Zhen-Hao Li Yan Cui Bao-Yi Liu De-Wei Zhao Department of Orthopedics Affiliated Zhongshan Hospital of Dalian UniversityDalian 116001Liaoning ProvinceChina

BACKGROUND Knee osteoarthritis(KOA)is a common orthopedic condition with an uncertain etiology,possibly involving genetics and *** like changes in chondrocyte microenvironment,oxidative stress,inflammation,and immune responses affect KOA ***-stage treatment options primarily target symptom *** stem cells(MSCs)show promise for treatment,despite *** research highlights microRNAs(miRNAs)within MSC-released extracellular vesicles that can potentially promote cartilage regeneration and hinder KOA *** suggests exosomes(Exos)as a promising avenue for future *** these findings emphasize the need for effective KOA progression management,further safety and efficacy validation for Exos is *** To explore miR-29a’s role in KOA,we’ll create miR-29a-loaded vesicles,testing for early treatment in rat *** Extraction of bone marrow MSC-derived extracellular vesicles,preparation of engineered vesicles loaded with miR-29a using ultrasonication,and identification using quantitative reverse transcription polymerase chain reaction;after establi-shing a rat model of KOA,rats were randomly divided into three groups:Blank control group injected with saline,normal extracellular vesicle group injected with normal extracellular vesicle suspension,and engineered extrace-llular vesicle group injected with engineered extracellular vesicle *** three groups evaluation,histological detection,and immunohistochemical detection to compare and evaluate the progress of various forms of *** General behavioral observation results showed that the extracellular vesicle group and engineered extracellular vesicle group had better performance in all four indicators of pain,gait,joint mobility,and swelling compared to the blank control ***,the engineered extracellular vesicle group had better pain relief at 4 wk and better knee joint mobility at 8 wk compared to the nor

关键词： Exosomes Osteoarthritis Mesenchymal stem cells MicroRNA-29a Intra-articular injection

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Growth and Interactions of Multi-Source Perturbations in Convection-Allowing Ensemble Forecasts

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Journal of Tropical Meteorology 2024年第2期30卷 118-131页

作者：张璐闵锦忠庄潇然王世璋魏莉青 Key Laboratory of Meteorological Disaster of Ministry of Education/Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University of Information Science and TechnologyNanjing 210044 China Jiangsu Meteorological Observatory Jiangsu Meteorological ServiceNanjing 210008 China Nanjing Joint Institute for Atmospheric Sciences Nanjing 210000 China

This study investigated the growth of forecast errors stemming from initial conditions(ICs),lateral boundary conditions(LBCs),and model(MO)perturbations,as well as their interactions,by conducting seven 36 h convectionallowing ensemble forecast(CAEF)*** cases,one with strong-forcing(SF)and the other with weak-forcing(WF),occurred over the Yangtze-Huai River basin(YHRB)in East China,were selected to examine the sources of uncertainties associated with perturbation growth under varying forcing backgrounds and the influence of these backgrounds on *** perturbations exhibited distinct characteristics in terms of temporal evolution,spatial propagation,and vertical distribution under different forcing backgrounds,indicating a dependence between perturbation growth and forcing background.A comparison of the perturbation growth in different precipitation areas revealed that IC and LBC perturbations were significantly influenced by the location of precipitation in the SF case,while MO perturbations were more responsive to convection triggering and dominated in the WF *** vertical distribution of perturbations showed that the sources of uncertainties and the performance of perturbations varied between SF and WF cases,with LBC perturbations displaying notable case ***,the interactions between perturbations were considered by exploring the added values of different source *** the SF case,the added values of IC,LBC,and MO perturbations were reflected in different forecast periods and different source uncertainties,suggesting that the combination of multi-source perturbations can yield positive *** the WF case,MO perturbations provided a more accurate estimation of uncertainties downstream of the Dabie Mountain and need to be prioritized in the research on perturbation development.

关键词： convection-allowing ensemble forecast forcing background perturbation growth interactions added value

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