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Ion dynamics into different pore size distributions in supercapacitors under compression

journal of Energy Chemistry 2023年第5期80卷 110-119,I0004页

作者： joão Pedro Aguiar dos Santos Cesar j.B.Pagan rafael Vicentini Reinaldo F.Teófilo Renato Beraldo Leonardo M.Da Silva Hudson Zanin Brazilian Renewable Energies Center for Innovation on New EnergiesSchool of Electrical and Computer EngineeringUniversity of CampinasAv.Albert Einstein 40CampinasSP13083-852Brazil School of Electrical and Computer Engineering University of CampinasSP 13083-852Brazil multivariate Chemical Data Analysis Laboratory Department of ChemistryUniversidade Federal de Viçosa36570-900 ViçosaMGBrazil Department of Chemistry Laboratory of Fundamental and Applied ElectrochemistryFederal University of Jequitinhonha and Mucuri's ValleyRodovia MGT 367km 5835000 Alto da Jacuba39100-000DiamantinaMGBrazil

Compressing supercapacitor(SCs)electrode is essential for improving the energy storage characteristics and minimizing ions’distance travel,faradaic reactions,and overall ohmic *** comprising the ion dynamics in SC electrodes under compression are still ***,the ionic dynamics of five aqueous electrolytes in electrodes under compression were studied in this work for tracking electrochemical and structural changes under mechanical stress.A superionic state is formed when the electrode is compressed until the micropores match the dimensions with the electrolyte’s hydrated ion sizes,which increases the *** excessive compression is applied,the accessible pore regions decrease,and the capacitance ***,as the studied hydrated ions have different dimensions,the match between ion/pore sizes *** the LiOH and NaClO4electrolytes,increasing the pressure from 60 to 120 and 100 PSI raised the capacitance from 13.5 to 35.2 F g^(-1)and 30.9 to 39.0 F g^(-1),***,the KOH electrolyte with the lowest and LiCl with the biggest combination of hydrated ion size have their point of maximum capacitance(39.5 and 36.7F g^(-1))achieved at 140 and 80 PSI,*** LiCl and KCl electrolytes,overcompression causes a drop in capacitance higher than 23%.

关键词： Mechanic compression Pore size distribution lon dynamics Activated carbon Supercapacitors

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Gourds and Tendrils of Cucurbitaceae: How Their Shape Diversity, Molecular and Morphological Novelties Evolved via Whole-Genome Duplications

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Molecular Plant 2020年第8期13卷 1108-1110页

作者： josuéBarrera-Redondo rafael Lira-Saade Luis E.Eguiarte Departamento de Ecología Evolutiva Instituto de EcologíaUniversidad Nacional Autónoma de MéxicoCircuito Exterior s/n Anexo al Jardín BotánicoCiudad de México 04510Mexico UBIPRO Facultad de Estudios Superiores IztacalaUniversidad Nacional Autónoma de MéxicoAvenido de los Barrios#1Col.Los Reyes IztacalaTlalnepantlaEstado de México 54090Mexico

Whole-genome duplications(WGDs)are regarded as important drivers of macroevolution in plants(Clark and Donoghue,2018).However,there are few studies that test a connection between WGDs and evolutionary *** proper study of evolutionary patterns related to WGDs needs a well-resolved phylogeny,accurate dates of the WGD events,and historical reconstructions of the evolutionary novelties(Clark and Donoghue,2018).The advent of exhaustive phylogenomic studies is becoming a promising way to solve these issues,as wholegenome data can help clarify obscure phylogenetic relationships,evaluate patterns associated with WGDs,and track down the evolution of life-history traits that shaped plant lineages(Bellot et al.,2020).

关键词： Whole phylogeny traits

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A Technical Review of Hydro-Project Development in China

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Engineering 2016年第3期2卷 302-312页

作者： rafael Duarte António Pinheiro Anton j. Schleiss Laboratory of Hydraulic Constructions (LCH) école polytechnique fédérale de Lausanne (EPFL) Civil Engineering Research and Innovation for Sustainability (CERIS) Instituto Superior Técnico Universidade de Lisboa

This paper summarizes the development of hydro-projects in China,blended with an international *** expounds major technical progress toward ensuring the safe construction of high dams and river harnessing,and covers the theorization of uneven non-equilibrium sediment transport,inter-basin water diversion,giant hydro-generator units,pumped storage power stations,underground caverns,ecological protection,and so on.

关键词： DamRiver harnessingWater diversionPumped storage power stationUnderground cavernEcological protection

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Association between urinary concentrations of bisphenol A substitutes and diabetes in adults

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World journal of Diabetes 2022年第7期13卷 521-531页

作者： rafael Moreno-Gómez-Toledano Esperanza Vélez-Vélez María I Arenas Marta Saura Ricardo j Bosch Universidad de Alcalá Department of Biological Systems/Physiology UnitAlcaláde Henares 28871Spain Fundación jiménez Díaz School of Nursing Jiménez Díaz FoundationAutonomous University of MadridMadrid 28040Spain Universidad de Alcalá Department of Biomedicine and BiotechnologyAlcaláde Henares 28871Spain Centro de Investigación en Red de Enfermedades Cardiovasculares Instituto Ramón y Cajal de Investigación SanitariaMadrid 28034Spain

BACKGROUND Due to new restrictions on the use of bisphenol A(BPA),industries are beginning to replace it with derived molecules such as bisphenol S and F(BPS and BPF).There is extensive evidence in the academic literature on the potential health effects of BPA,which is known to be a diabetogenic ***,there are few publications related to new compounds derived from *** To perform an epidemiological study of urinary BPS and BPF in the American National Health and Nutrition Examination Survey(NHANES)cohort,and analyze their possible relationship with diabetes *** NHANES datasets from 2013 to 2016 were used due to the urinary BPF and BPS *** from 3658 adults were analyzed to perform regression analysis exploring the possible relationship between BPA-derived compounds and *** Descriptive statistics,linear regression modeling,and logistic regression analysis revealed a significant relationship between urinary BPS,but not BPF,and diabetes ***,a relationship was observed between both compounds and hypertension and a slight relationship between BPF and *** In the present study,a strong relationship between urinary BPS,not BPF,and diabetes risk has been *** substitute molecules do not exempt the population from potential health risks.

关键词： Bisphenol S Bisphenol F Diabetes mellitus National Health and Nutrition Examination Survey Urine

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Optimal laser intensity profiles for a uniform target illumination in direct-drive inertial confinement fusion

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High Power Laser Science and Engineering 2014年第4期2卷 62-67页

作者： Mauro Temporal Benoit Canaud Warren j.Garbett rafael Ramis Centre de Mathématiques et de Leurs Applications ENS Cachan and CNRS 61 Av.du President WilsonF-94235 Cachan Cedex France CEA DIF F-91297 Arpajon Cedex France AWE plc Aldermaston ReadingBerkshire RG7 4PR United Kingdom ETSI Aeronuticos Universidad Polit'ecnica de Madrid28040 Madrid Spain

A numerical method providing the optimal laser intensity profiles for a direct-drive inertial confinement fusion scheme has been developed. The method provides an alternative approach to phase-space optimization studies, which can prove computationally expensive. The method applies to a generic irradiation configuration characterized by an arbitrary number NBof laser beams provided that they irradiate the whole target surface, and thus goes beyond previous analyses limited to symmetric configurations. The calculated laser intensity profiles optimize the illumination of a spherical *** paper focuses on description of the method, which uses two steps: first, the target irradiation is calculated for initial trial laser intensities, and then in a second step the optimal laser intensities are obtained by correcting the trial intensities using the calculated illumination. A limited number of example applications to direct drive on the Laser Mega joule(LMj) are described.

关键词： direct drive inertial confinement fusion laser system

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Anthropogenic impacts to the sediment budget of São Francisco River navigation channel using SWAT

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International journal of Agricultural and Biological Engineering 2015年第3期8卷 140-157页

作者： Calvin T.Creech rafael Brito Siqueira james P.Selegean Carol Miller Wayne State University DetroitMichigan 48202United States Com panhia de Desenvolvimento dos Vales do São Francisco e do Parnaíba(CODEVASF) Brasília 70830Brazil United States Army Corps of Engineers Detroit DistrictDetroitMichigan 48226United States United States Army Corps of Engineers Mobile Di strictMobile 36628AlabamaUnited States

The São Francisco River Basin,located in eastern Brazil,has undergone a significant amount of anthropogenic changes in the last several decades,such as agricultural expansion,irrigation activities,mining,and the construction of large ***,these changes have altered the historic sediment budget and have led to an aggradation of sediments in the navigation channel,impacting the ability to efficiently ship agricultural commodities to regional *** an effort to aid decision makers in future waterway navigation planning,an international partnership between the Brazilian government agency CODEVASF and the US Army Corps of Engineers(USACE)was *** this partnership a SWAT model of the 630000 km2 São Francisco River basin was developed to better understand both the historic and current sediment budget within the navigation *** SWAT model of the São Francisco River Basin was calibrated for hydrology and sediment *** discharges were calibrated at 17 Agência Nacional deÁguas(ANA)gages,with Nash-Sutcliffe efficiency(NSE)values ranging from 0.42 to 0.75 for an eleven year *** loads were calibrated to an ANA sediment gage located in the Middle São Francisco River Navigation Channel,with a PBIAS(Percent Bias)of *** on model results,the aggradation rate of sediment in the São Francisco River and major tributaries has increased by approximately 20 Mt since Pre-European settlement of the basin(from approximately 7 Mt/a to 27 Mt/a).This increase has contributed to an impaired navigation channel due to shoaling of sandy sediments in the navigation channel.

关键词： sediment budget aggradation rate São Francisco River anthropogenic impact SWAT

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Procedural modeling applied to the 3D city model of Bogota:A case study

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Virtual Reality & Intelligent Hardware 2021年第5期3卷 423-433页

作者： Gustavo ALOMÍA Diego LOAIZA Claudia ZÙÑIGA Xun LUO rafael ASOREyCACHEDA Department of Engineering Universidad Santiago de CaliCO 760001Colombia Department of Engineering Tianjin University of TechnologyTianjin 300384China Department of Information&Communications Technologies Universidad Politécnica de CartagenaES 30202Spain

Background Computer Generated Animations(CGA),when applied to three-dimensional(3D)city models(3DCM),can be used as powerful tools to support urban *** leads to a new paradigm,based on procedural modeling,that allows the integration of known urban *** This paper introduces a new workflow for the development of high-quality approximations of urban models in a short time and enables facilities to be imported from other cities into a given city model,following specific generation *** Thus,this workflow provides a very simple approach to observe,study,and simulate the implementation of models already developed in other cities,in a city where they are not yet *** of these models include all types of mobility systems and urban *** This allows us to perceive the environmental impact of certain decisions in the real world,as well as to carry out simple simulations to determine the changes that can occur in the flows of people,traffic,and other city activities.

关键词： Computer Generated Animations Geographical information system Urban planning 3D City Modeling

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Carbon stock estimation in halophytic wooded savannas of Uruguay:An ecosystem approach

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Forest Ecosystems 2024年第4期11卷 580-589页

作者： Andres Baietto Andres Hirigoyen Carolina Toranza Franco Schinato Maximiliano Gonzalez rafael Navarro Cerrillo Forest Department Faculty of AgronomyUniversity of the RepublicMontevideoPO 12900Uruguay National Research Program of Forest Production National Agriculture Research InstituteTacuaremboPO 97000Uruguay Soil and Water Department Faculty of AgronomyUniversity of the RepublicMontevideoPO 12900Uruguay Department of Forestry Engineering University of CordobaCordobaPO 14014Spain

Savannas constitute a mixture of trees and shrub patches with a more continuous herbaceous *** contribution of this biome to the soil organic carbon(SOC)and above-ground biomass(AGB)carbon(C)stock globally is ***,they are frequently subjected to land use changes,promoting increases in CO_(2) *** Uruguay,subtropical wooded savannas cover around 100,000 ha,of which approximately 28%is circumscribed to sodic soils(i.e.,subtropical halophytic wooded savannas).Nevertheless,there is little background about the contribution of each ecosystem component to the C stock as well as site-specific allometric *** study was conducted in 5 ha of subtropical halophytic wooded savannas of the national protected area Esteros y Algarrobales del Rio *** work aimed to estimate the contribution of the main ecosystem components(e.g.,soil,trees,shrubs,and herbaceous plants)to the C ***-specific allometric equations for the most frequent tree species and shrub genus were fitted based on basal diameter(BD)and total height(H).The fitted equations accounted for between 77%and 98%of the aerial biomass variance of Netuma affinis and Vachellia *** shrubs(Baccharis sp.),the adjusted equation accounted for 86%of total aerial biomass.C stock for the entire system was 116.71±11.07 Mg·ha^(-1),of which 90.7%was allocated in the soil,8.3%in the trees,0.8%in the herbaceous plants,and 0.2%in the *** results highlight the importance of subtropical halophytic wooded savannas as C sinks and their relevance in the mitigation of global warming under a climate change scenario.

关键词： Carbon stock Climate change Biomass modeling Sodic soils

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Neuronal photoactivation through secondharmonic near-infrared absorption by gold nanoparticles

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Light(Science & Applications) 2018年第1期7卷 79-91页

作者： Wieteke D.A.M.de Boer jan j.Hirtz Antonio Capretti Tom Gregorkiewicz Mercè Izquierdo-Serra Shuting Han Christophe Dupre yuriy Shymkiv rafael yuste NeuroTechnology Center Department of Biological SciencesColumbia UniversityNew YorkNY 10027USA Van der Waals–Zeeman Institute University of Amsterdam1098 XH AmsterdamNetherlands Present address:Laboratori de Fisiologia Molecular Departament de Ciències Experimentals i de la SalutUniversitat Pompeu FabraBarcelonaSpain

Optical activation of neurons requires genetic manipulation or the use of chemical photoactivators with undesirable side *** a solution to these disadvantages,here,we demonstrate optically evoked neuronal activity in mouse cortical neurons in acute slices and in vivo by nonlinear excitation of gold *** addition,we use this approach to stimulate individual epitheliomuscular cells and evoke body contractions in Hydra *** achieve this,we use a low-power pulsed near-infrared excitation at the double-wavelength of the plasmon resonance of gold nanoparticles,which enables optical sectioning and allows for high spatial precision and large penetration *** effect is explained by second-harmonic Mie scattering,demonstrating light absorption by a second-order nonlinear process,which enables photothermal stimulation of the *** approach also minimizes photodamage,demonstrating a major advancement towards precise and harmless photoactivation for neuroscience and human therapeutics.

关键词： activation harmonic absorption

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Rock mass structural recognition from drill monitoring technology in underground mining using discontinuity index and machine learning techniques

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International journal of Mining Science and Technology 2023年第5期33卷 555-571页

作者： Alberto Fernández joséA.Sanchidrián Pablo Segarra Santiago Gómez Enming Li rafael Navarro Universidad Politécnica de Madrid–ETSI Minas y Energía Spain Universidad de Salamanca–GIR Charrock Spain

A procedure to recognize individual discontinuities in rock mass from measurement while drilling(MWD)technology is developed,using the binary pattern of structural rock characteristics obtained from in-hole images for *** from two underground operations with different drilling technology and different rock mass characteristics are considered,which generalizes the application of the methodology to different sites and ensures the full operational integration of MWD data *** approaches are followed for site-specific structural model building:a discontinuity index(DI)built from variations in MWD parameters,and a machine learning(ML)classifier as function of the drilling parameters and their *** prediction ability of the models is quantitatively assessed as the rate of recognition of discontinuities observed in borehole *** between the parameters involved in the models for each site,and differences in their weights,highlight the site-dependence of the resulting *** ML approach offers better performance than the classical DI,with recognition rates in the range 89%to 96%.However,the simpler DI still yields fairly accurate results,with recognition rates 70%to 90%.These results validate the adaptive MWD-based methodology as an engineering solution to predict rock structural condition in underground mining operations.

关键词： Drill monitoring technology Rock mass characterization Underground mining Similarity metrics of binary vectors Structural rock factor Machine learning

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