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The effect of adsorbent textural and functional properties on model naphthenic acid adsorption

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Journal of Environmental Sciences 2025年第2期148卷 27-37页

作者： Tyler m.roy Elmira Nazari Oliver K.l.Strong Paul r.Pede Andrew J.Vreugdenhil material Science Department of ChemistryTrent University1600 West BankPeterboroughOntario K9L 0G2Canada Carbonix 690 Mountain RdSuite 200Fort William First NationOntario P7J 1G8Canada

Naphthenic acids,NAs,are a major contaminant of concern and a focus of much research around remediation of oil sand process affected waters,*** activated carbon adsorbents are an attractive option given their low cost of fabrication and im.l.mentation.A deeper evaluation of the effect NA structural differences have on uptake affinity is *** we provide an in-depth exploration of NA adsorption including many more model NA species than have been assessed previously with evaluation of adsorption kinetics and isotherms at the relevant alkaline pH of OSPW using several different carbon adsorbents with pH buffering to sim.l.te the behaviour of real *** for the NA varied considerably regardless of the activated carbon used,ranging from 350 mg/g to near zero highlighting recalcitrant *** equilibrium data was explored to identify structural features of these species and key physiochemical properties that influence *** found that certainNAwill be resistant to adsorptionwhen hydrophobic adsorbents are *** isotherm modelling helped explore interactions occurring at the interface between NA and adsorbent *** identified the importance of NA hydrophobicity for activated carbon *** is also presented that indicates favorable hydrogen bonding between certain NA and surface site hydroxyl groups,demonstrating the importance of adsorbent surface functionality for NA *** research highlights the challenges associated with removing NAs from OSPW through adsorption and also identifies howadsorbent surface chemistry modification can be used to increase the removal efficiency of recalcitrant NA species.

关键词： Adsorption Activated carbon model naphthenic acids Isotherm modelling

Notes on linear Gossip Algorithms:Potentials and Challenges Dedicated to Peter E. Caines in honour of his 80th birthday

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Journal of Systems Science & Com.l.xity 2025年第01期 98-128页

作者： GErENCSér Balázs GErENCSér lászló HUN-rEN Alfréd rényi Institute of mathematics E?tv?s loránd University Department of Probability and Statistics HUN-rEN SZTAKI Institute for Computer Science and Control

The authors consider the problem of reaching consensus over a communication network via asynchronous interaction between pairs of agents. A well-known method is the linear gossip algorithm due to Tsitsiklis(1984). Extension of this, allowing the selection of a strictly stationary sequence of communicating pairs, was given in Picci and Taylor(2013). Extension of the linear gossip algorithm to directed communication networks, retaining the linear dynamics, was proposed by Cai and Ishii(2012),later extended by Silvestre, et al.(2018). A definite novelty of these algorithms is that l2-convergence with exponential rate can be established. The authors attend the above issues, extending the result of Picci and Taylor(2013) motivated by features of algorithms for directed networks. The authors present and discuss the algorithm of Silvestre, et al.(2018), together with systematic sim.l.tion results based on 5m randomly chosen parameter settings. The core of the proposed mathematical technology is a set of sim.l. observations, presented with a tutorial aspect, by which the authors can conveniently establish various results on the almost sure convergence of products of strictly stationary sequences of matrices to a rank-1 matrix.

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Getting physical with medical education:Exercise based virtual anatomy review classes for medical students

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World Journal of methodology 2025年第1期15卷 20-25页

作者： Nadeesha r Samarasinghe Taniya S Nagpal michele l Barbeau Charys m martin Division of General Surgery Faculty of MedicineUniversity of British ColumbiaVancouver V6T 1Z3BCCanada Faculty of Kinesiology Sport and RecreationUniversity of AlbertaEdmonton T6G 2R3ABCanada Anatomy and Cell Biology University of Western OntarioLondon N6A 3K7ONCanada Department of Anatomy and Cell Biology Schulich School of Medicine and DentistryThe University of Western OntarioLondon N6A 3K7ONCanada

The benefits of regular physical activity are well ***,few studies have examined the effectiveness of integrating physical activity(PA)into curricula within a post-secondary *** investigate the incorporation of PA into medical curriculum,we developed a series of optional exercise-based review sessions designed to reinforce musculoskeletal(mSK)anatomy course *** synchronous sessions were co-taught by a group fitness instructor and an anatomy *** fitness instructor would lead students through both strength and yoga style exercises,while the anatomy instructor asked questions about relevant anatomical structures related to course material previously *** the sessions,participants were asked to evaluate the classes on their self-reported exam preparedness in improving mSK anatomy knowledge,PA levels,and mental *** participants com.l.ted surveys;a majority agreed that the classes increased understanding of mSK concepts(90.0%)and activity levels(97.7%).many(70.0%)felt that the classes helped reduce *** majority of respondents(90.0%)agreed that the classes contributed to increased feelings of social ***,medical students saw benefit in PA based interventions to supplement mSK course *** with increasing activity levels and promoting health behaviours,integrating PA into medical curriculum may improve comprehension of learning material,alleviate stress and foster social connectivity among medical students.

关键词： medical education musculoskeletal Anatomy Exercise Online learning

Assessment of the heartwood contribution to carbon accum.l.tion in Pinus sylvestris l. trees under different forest site conditions

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FOrEST ECOSYSTEmS 2025年第1期12卷 159-175页

作者： Galibina, Natalia A. Nikerova, Kseniya m. moshnikov, Sergey A. Kryshen, Alexander m. russian Acad Sci Forest Res Inst Karelian Res Ctr 11 Pushkinskaya St Petrozavodsk 185910 Karelia Russia

Background: The heartwood (HW) proportion in the trunk of mature trees is an important characteristic not only for wood quality but also for assessing the role of forests in carbon sequestration. We have for the first time studied the proportion of HW in the trunk and the distribution of carbon and extractives in sapwood (SW) and HW of 70-80 year old Pinus sylvestris l. trees under different growing conditions in the pine forests of North-West russia. method: We have examined the influence of conditions and tree position in stand (dominant, intermediate and suppressed trees) in the ecological series: blueberry pine forest (Blu) - lingonberry pine forest (lin) - lichen pine forest (lic). We have analyzed the influence of climate conditions in the biogeographical series of lin: the middle taiga subzone - the northern taiga subzone - the transition area of the northern taiga subzone and tundra. results: We found that the carbon concentration in HW was 1.6%-3.4% higher than in SW, and the difference depended on growing conditions. Carbon concentration in HW increased with a decrease in stand productivity (Blu-lin-lic). In medium-productive stands, the carbon concentration in SW was higher in intermediate and supressed trees compared to dominant trees. In the series from south to north, carbon concentration in HW increased by up to 2%, while in SW, it rose by 2.7%-3.8%. Conclusions: Our results once again emphasized the need for an empirical assessment of the accurate carbon content in aboveground wood biomass, including various forest growing conditions, to better understand the role of boreal forests in carbon storage.

关键词： Scots pine Blueberry pine forest lingonberry pine forest lichen pine forest Tree social class Climate Carbon content Extractives Cellulose lignin

Hunting for a viral proxy in bioaerosols of swine buildings using m.l.cular detection and metagenomics

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Journal of Environmental Sciences 2025年第2期148卷 69-78页

作者： Valérie létourneau marie-Josée Gagné Jonathan m.Vyskocil Vincent Brochu Kim robitaille martin Gauthier Julie Brassard Caroline Duchaine Quebec Heart and lung Institute research Centre-Universitélaval 2725 Chemin Sainte-FoyQuebecG1V 4G5Canada Saint-Hyacinthe research and Development Centre Agriculture and Agri-Food Canada3600 Casavant Boulevard WestSaint-HyacintheJ2S 8E3Canada Department of Biochemistry Microbiologyand Bio-informaticsFaculty of Science and EngineeringUniversitéLaval1045 Avenue de la MédecineQuebecG1V 0A6Canada The Swine and Poultry Infectious Diseases research Centre Faculty of Veterinary Medicine of Universitéde Montréal3200 Rue SicotteSaint-HyacintheJ2S 2M2Canada

There are limited biosecurity measures directed at preventing airborne transmission of viruses in *** effectiveness of dust mitigation strategies such as oil sprinkling,to decrease risk of airborne virus transmission are *** and qPCr for common fecal viruses were used to hunt for a ubiquitous virus to serve as a proxy when evaluating the efficiency of mitigation strategies against airborne viral infectious *** particles were collected from swine buildings using high-volume air *** DNA and rNA were used to perform specific rT-qPCr and qPCr and analyzed by highthroughput *** astroviruses group 2 were common(from 102 to 105 genomic copies per cubic meter of air or gc/m^(3),93%positivity)while no norovirus genogroup II was recovered from air *** torque teno sus virus were detected by qPCr in low concentrations(from 101 to 102 gc/m^(3),47%positivity).Among the identified viral fam.l.es by metagenomics analysis,Herelleviridae,microviridae,myoviridae,Podoviridae,and Siphoviridae were *** phage vB_Avim_AVP of Aerococcus was present in all air sam.l.s and a newly designed qPCr revealed between 101 and 105 gc/m^(3) among the sam.l.s taken for the present study(97%positivity)and banked sam.l.s from5-and 15-year old studies(89%positivity).According to the present study,both the porcine astrovirus group 2 and the phage vB_Avim_AVP of Aerococcus could be proxy for airborne viruses of swine buildings.

关键词： Bioaerosols Viral metagenomics Astrovirus Aerococcus phage Swine buildings

Hybrid and enhanced electrokinetic system for soil remediation from heavy metals and organic matter

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Journal of Environmental Sciences 2025年第1期147卷 424-450页

作者： Faris m.Hamdi Namuun Ganbat Ali Altaee Akshaya K.Sam.l.Ibrar Ibrar John l.Zhou Adel O.Sharif Centre for Green Technology School of Civil and Environmental EngineeringThe University of Technology Sydney15 BroadwayNSW 2007Australia Department of Civil Engineering Jazan UniversityJazan 82822Saudi Arabia Centre for Nano and material Sciences Jain UniversityRamanagaraBangaloreKarnataka 562112India School of mechanical Sciences Faculty of Engineering and Physical SciencesUniversity of SurreyAustralia

The electrokinetic(EK)process has been proposed for soil decontamination from heavy metals and organic *** advantages of the EK process include the low operating energy,suitability for fine-grained soil decontamination,and no need for *** the last three decades,enhanced and hybrid EK systems were developed and tested for improving the efficiency of contaminants removal from *** enhanced-EK processes exhibited excellent efficiency in removing contaminants by controlling the soil pH or the chemical reaction of *** hybrid systems were tested to overcome environmental hurdles or technical drawbacks of decontamination *** of the EK process with phytoremediation,bioremediation,or reactive filtermedia(rFm)improved the remediation process performance by capturing contaminants or facilitating biological agents’movement in the ***,EK process coupling with solar energy was proposed to treat off-grid contaminated soils or reduce the EK energy *** study reviews recent advancements in the enhancement and hybrid EK systems for soil remediation and the type of contaminants targeted by the *** study also covered the impact of operating parameters,imperfect pollution separation,and differences in the physicochemical characteristics and microstructure of soil/sediment on the EK ***,a comparison between various remediation processes was presented to highlight the pros and cons of these technologies.

关键词： Electrokinetic Soil remediation reactive filter media Enhanced electrokinetic Contaminants

Com.l.ment-dependent neuroinflammation in spinal cord injury:from pathology to therapeutic im.l.cations

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Neural regeneration research 2025年第5期20卷 1324-1335页

作者： Hassan Saad Bachar El Baba Ali Tfaily Firas Kobeissy Juanmarco Gutierrez Gonzalez Daniel refai Gerald r.rodts Christian mustroph David Gimbel Jonathan Grossberg Daniel l.Barrow matthew F.Gary Ali m.Alawieh Department of Neurosurgery Emory University School of MedicineAtlantaGAUSA Department of Neurology Yale UniversityNew HavenCTUSA Center for Neurotrauma Multiomics&Biomarkers(CNMB)Morehouse School of MedicineAtlantaGAUSA

Spinal cord injury remains a major cause of disability in young adults,and beyond acute decompression and rehabilitation,there are no pharmacological treatments to limit the progression of injury and optimize recovery in this *** the thorough investigation of the com.l.ment system in triggering and propagating cerebral neuroinflammation,a sim.l.r role for com.l.ment in spinal neuroinflammation is a focus of ongoing *** this work,we survey the current literature investigating the role of com.l.ment in spinal cord injury including the sources of com.l.ment proteins,triggers of com.l.ment activation,and role of effector functions in the *** study relevant data demonstrating the different triggers of com.l.ment activation after spinal cord injury including direct binding to cellular debris,and or activation via antibody binding to damage-associated m.l.cular *** effector functions of com.l.ment have been im.l.cated in spinal cord injury,and we critically evaluate recent studies on the dual role of com.l.ment anaphylatoxins in spinal cord injury while emphasizing the lack of pathophysiological understanding of the role of opsonins in spinal cord *** this pathophysiological review,we systematically review the different translational approaches used in preclinical models of spinal cord injury and discuss the challenges for future translation into human *** review emphasizes the need for future studies to dissect the roles of different com.l.ment pathways in the pathology of spinal cord injury,to evaluate the phases of involvement of opsonins and anaphylatoxins,and to study the role of com.l.ment in white matter degeneration and regeneration using translational strategies to supplement genetic models.

关键词： com.l.ment neuroinflammation neuroplasticity regeneration spinal cord injury targeted therapy

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Emerging role of A-kinase anchoring protein 5 signaling in reward circuit function

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Neural regeneration research 2025年第10期20卷 2913-2914页

作者： William J.Flerlage mark l.Dell’Acqua Brian m.Cox Fereshteh S.Nugent Uniformed Services University of the Health Sciences Department of Pharmacology and Molecular TherapeuticsBethesdaMDUSA Department of Pharmacology University of Colorado School of MedicineAnschutz Medical CampusAuroraCOUSA

There is a strong evidence supporting the hypothesis of synaptic dysfunction as a major contributor to neural circuit and network disruption underlying emotional and mood dysregulation in psychiatric disorders(Simmons et al.,2024).Diverse sets of distinct m.l.cular signaling pathways converge on the synapse to regulate synaptogenesis,synaptic function,and synaptic plasticity in brain regions and circuits through com.l.x interactions organized by numerous m.l.ivalent protein scaffolds,including the fam.l. of proteins known as A-kinase anchoring proteins(AKAPs).

关键词： function supporting

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Knotting ligands to control metal coordination geometry

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Science China Chemistry 2025年第2期68卷 403-404页

作者： Fabien B.l.Cougnon Department of Chemistry and Nanoscience Centre University of JyväskyläJyväskyläFinland

Zinc is a metal of particular importance for life[1].It is the most abundant transition metal in biological systems after iron and contributes both structural and catalytic roles to many cellular *** properties of Zn^(Ⅱ),unlike those of any other first-row transition metal ions,explain its biological *** to its filled d-shell orbitals,Zn^(Ⅱ) is redox-stable,has a ligand-field energy stabilization of zero and,consequently,no typical coordination number and *** metalloproteins exploit these features to carry a broad range of chemical reactions in m.l. *** metalloenzymes,unsaturated ZnII centres often act as redox-stable lewis *** protein backbone provides a highly preorganized environment around the metal centre and accompanies the changes in coordination geometry occurring as substrate transformation proceeds,thereby modulating the metal reactivity.

关键词： coordination geometry centre