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Effect of the anionic composition of sulfolane based electrolytes on the performances of lithium-sulfur batteries

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Journal of Energy Chemistry 2024年第8期95卷 231-240页

作者： Elena V.Karaseva Elena V.Kuzmina Bo-quan li qiang Zhang Vladimir S.Kolosnitsyn Ufa Institute of Chemistry of the Ufa Federal Research Centre of the Russian Academy of Science Advanced Research Institute of Multidisciplinary Science Beijing Institute of Technology Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical Engineering Tsinghua University

In lithium-sulfur batteries,cell design,specifically electrolyte design,has a key impact on the battery performance.The effect of lithium salt anion donor number（DN）(DN[PF6]-=2.5,DN[N（SO2CF3）2]-=5.4,DN[ClO4]-=8.4,DN[SO3CF3]-=16.9,and DN[NO3]-=21.1) on the patterns of lithium-sulfur batteries and lithium metal electrode performances with sulfola ne-based electrolytes is investigated.An increase in DN of lithium salt anions leads to an increase in the depth and rate of electrochemical reduction of sulfur and long-chain lithium polysulfides and to a decrease in those for medium-and short-chain lithium polysulfides.DN of lithium salt anions has weak effect on the discharge capacity of lithium-sulfur batteries and the Coulomb efficiency during cycling,with the exception of liSO3CF3and liNO3.An increase in DN of lithium salt anions leads to an increase in the cycling duration of lithium metal anodes and to a decrease in the presence of lithium polysulfides.In sulfolane solutions of liNO3and liSO3CF3,lithium polysulfides do not affect the cycling duration of lithium metal anodes.

关键词： Donor number Electrolyte lithium metal electrode lithium polysulfide lithium salt lithium-sulfur battery Sulfolane

Severe pediatric COVID‑19:a review from the clinical and immunopathophysiological perspectives

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World Journal of Pediatrics 2024年第4期20卷 307-324页

作者： Yi‑Kan Sun Can Wang Pei‑quan lin Lei Hu Jing Ye Zhi‑Gang Gao Ru lin Hao‑Min li qiang Shu li‑Su Huang lin‑Hua Tan Children's Hospital Zhejiang University School f MedicineHangzhou 310052China The Second Affiliated Hospital Zhejiang University School of MedicineHangzhou 310030China Surgical Intensive Care Unit Children’s HospitalZhejiang University School of MedicineHangzhou 310052China Department of General Surgery Children’s HospitalZhejiang University School of MedicineHangzhou 310052China Department of Cardiopulmonary and Extracorporeal life Support Children’s HospitalZhejiang University School of MedicineHangzhou 310052China Clinical Data Center Children’s HospitalZhejiang University School of MedicineHangzhou 310052China Department of Cardiac Surgery Children’s HospitalZhejiang University School of MedicineHangzhou 310052China National Clinical Research Center for Child Health Children’s HospitalZhejiang University School of MedicineHangzhou 310052China Department of Infectious Diseases Children’s HospitalZhejiang University School of MedicineHangzhou 310052China

Background Coronavirus disease 2019(COVID-19)tends to have mild presentations in children.However,severe and critical cases do arise in the pediatric population with debilitating systemic impacts and can be fatal at times,meriting further attention from clinicians.Meanwhile,the intricate interactions between the pathogen virulence factors and host defense mechanisms are believed to play indispensable roles in severe COVID-19 pathophysiology but remain incompletely understood.Data sources A comprehensive literature review was conducted for pertinent publications by reviewers independently using the PubMed,Embase,and Wanfang databases.Searched keywords included“COVID-19 in children”,“severe pediatric COVID-19”,and“critical illness in children with COVID-19”.Results Risks of developing severe COVID-19 in children escalate with increasing numbers of co-morbidities and an unvaccinated status.Acute respiratory distress stress and necrotizing pneumonia are prominent pulmonary manifestations,while various forms of cardiovascular and neurological involvement may also be seen.Multiple immunological processes are implicated in the host response to COVID-19 including the type I interferon and inflammasome pathways,whose dysregulation in severe and critical diseases translates into adverse clinical manifestations.Multisystem inflammatory syndrome in children(MIS-C),a potentially life-threatening immune-mediated condition chronologically associated with COVID-19 exposure,denotes another scientific and clinical conundrum that exemplifies the complexity of pediatric immunity.Despite the considerable dissimilarities between the pediatric and adult immune systems,clinical trials dedicated to children are lacking and current management recommendations are largely adapted from adult guidelines.Conclusions Severe pediatric COVID-19 can affect multiple organ systems.The dysregulated immune pathways in severe COVID-19 shape the disease course,epitomize the vast functional diversity of the pediatric immune system and highlight the immun

关键词： Immunopathophysiology MIS-C Pediatric critical care Severe pediatric COVID-19

KnowledgeMapping of Hybrid Solar PV andWind Energy Standalone Systems: A Bibliometric Analysis

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Energy Engineering 2024年第7期121卷 1781-1803页

作者： quan Zhou Haiyang li School of Mechanical and Electrical Engineering Central South University of Forestry and TechnologyChangsha410004China

Renewable energy is becoming more attractive as traditional fossil fuels are rapidly depleted and expensive,and their use would release pollutants.Power systems that use both wind and solar energy are more reliable and efficient than those that utilize only one energy.Hybrid renewable energy systems(HRES)are viable for remote areas operating in standalone mode.This paper aims to present the state-of-the-art research on off-grid solar-wind hybrid energy systems over the last two decades.More than 1500 published articles extracted from the Web of Science are analyzed by bibliometric methods and processed by CiteSpace to present the results with figures and tables.Productive countries and highly cited authors are identified,and hot topics with hotspot articles are shown in landscape and timeline views.Emerging trends and new developments related to techno-economic analysis and microgrids,as well as the application of HOMER software,are predicted based on the analysis of citation bursts.Furthermore,the opportunities of hybrid energy systems for sustainable development are discussed,and challenges and possible solutions are proposed.The study of this paper provides researchers with a comprehensive understanding and intuitive representation of standalone solar-wind hybrid energy systems.

关键词： Wind energy solar PV standalone citation bursts emerging trends

Object Helps U-Net Based Change Detectors

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IEEE/CAA Journal of Automatica Sinica 2024年第2期11卷 548-550页

作者： Lan Yan qiang li Kenli li College of Computer Science and Electronic Engineering Hunan UniversityChangsha 410082China State Key Laboratory for Management and Control of Complex Systems Institute of AutomationChinese Academy of SciencesBeijing 100190China

Dear Editor,This letter focuses on leveraging the object information in images to improve the performance of the U-Net based change detector.Change detection is fundamental to many computer vision tasks.Although exist... 详细信息

关键词： Net computer networks

Weak type(1, 1) of the Riesz transform on some direct product manifolds with exponential volume growth

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Science China Mathematics 2024年第7期67卷 1599-1622页

作者： Hong-quan li Jie-Xiang Zhu School of Mathematical Sciences Fudan UniversityShanghai200433China Center for Applied Mathematics Tianjin UniversityTianjin300072China

In this paper, we are concerned with the Riesz transform on the direct product manifold H^(n)× M,where H^(n) is the n-dimensional real hyperbolic space, and M is a connected complete non-compact Riemannian manifold satisfying the volume doubling property and generalized Gaussian or sub-Gaussian upper estimates for the heat kernel. We establish its weak type(1, 1) property. In addition, we obtain the weak type(1, 1) of the heat maximal operator in the same setting. Our arguments also work for a large class of direct product manifolds with exponential volume growth. Particularly, we provide a simpler proof of weak type(1, 1) boundedness of some operators considered in the work of li et al.(2016).

关键词： Riesz transform heat kernel direct product real hyperbolic space

Protective Effects of Phellodendron Species on Bone Health: A Novel Perspective on Their Potentials in Treating Osteoporosis and Osteoarthritis

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Chinese Journal of Integrative Medicine 2024年第4期30卷 379-384页

作者： XIN li TAN Guo-yao ZHANG qiang ZHANG Qun Good Clinical Practice Development Guangdong Provincial Key Laboratory of Bone and Joint Degeneration DiseasesThe Third Affiliated Hospital of Southern Medical UniversityGuangzhou(510630)China Department of Pharmacy Sun Yat-sen Memorial HospitalSun Yat-sen UniversityGuangzhou(510120)China

Phellodendron(PN)species,traditionally used in Chinese medicine for centuries,hold promise as a potential treatment for osteoporosis(OP)and osteoarthritis(OA)due to their bioactive compounds.The bioactive compounds,including berberine and palmatine,exhibit anti-inflammatory,antioxidant,and bone-protective properties,contributing to their potential therapeutic benefits in promoting bone health and preventing bone loss.However,challenges such as the need for standardized preparation and dosing,limited clinical studies,and potential interactions with other medications hinder their clinical use.Nonetheless,the rich history of PN species in Chinese medicine provides a promising foundation for future investigation into their potential as alternative treatments for OP and OA.Further research is needed to fully understand the underlying mechanisms of action and explore the clinical implications of PN for bone health.

关键词： Phellodendron species bone health osteoporosis osteoarthritis review

Distributed Harmonic Power Sharing with Voltage Distortion Suppression in Islanded Microgrids Considering Non-linear Loads

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 117-128页

作者： Guannan Lou Shanlin li Wei Gu quan Yang School of Electrical Engineering Southeast UniversityNanjingJiangsu 210096China the Jiangsu Provincial Key Laboratory of Smart Grid Technology and Equipment Southeast University Dongguan Power Supply Bureau of Guangdong Power Grid Company Guangdong 523000China

In contemporary power grids or microgrids,harmonic distortion has emerged as one of the critical power quality issues for utility power grids,which has escalated especially due to the high penetration of power-electronic-converter-interfaced distributed generation(DG).This paper first illustrates the prevalent dispute revolving around the harmonic power sharing and distortion restraint,and subsequently proposes a consensusbased framework that facilitates an accurate sharing of harmonics among multi-DGs connected in parallel,with an effective suppression of the output voltage distortion.Compared with the majority of existing studies addressing the issue of voltage harmonics at the point of common coupling(PCC),our method primarily emphasizes on the output voltage distortion since the power quality requirement for certain local critical loads is often known to be high.With the help of adaptive regulation,the overall distortion produced at the output terminals of DGs can be retained within an acceptable range.The working principle of the proposed control method,which is not only easy to implement but also independent of model parameters,is further described in detail.Employing the small-signal dynamic model,the system stability and robustness are analyzed.The hardware-in-the-loop(HIL)simulations aid in determining the outcome of the proposed strategy in microgrid control.

关键词： Distributed generation droop control harmonic power sharing microgrid voltage distortion mitigation

In Situ Atomic Reconstruction Engineering Modulating Graphene-like MXene-Based Multifunctional Electromagnetic Devices Covering Multi-Spectrum

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Nano-Micro Letters 2024年第9期16卷 247-261页

作者： Ting‑Ting liu Qi Zheng Wen‑qiang Cao Yu‑Ze Wang Min Zhang quan‑liang Zhao Mao‑Sheng Cao School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081People’s Republic of China Department of Physics Beijing Technology and Business UniversityBeijing 100048People’s Republic of China School of Mechanical and Materials Engineering North China University of TechnologyBeijing 100144People’s Republic of China

With the diversified development of big data,detection and precision guidance technologies,electromagnetic(EM)functional materials and devices serving multiple spectrums have become a hot topic.Exploring the multispectral response of materials is a challenging and meaningful scientific question.In this study,MXene/TiO_(2)hybrids with tunable conduction loss and polarization relaxation are fabricated by in situ atomic reconstruction engineering.More importantly,MXene/TiO_(2)hybrids exhibit adjustable spectral responses in the GHz,infrared and visible spectrums,and several EM devices are constructed based on this.An antenna array provides excellent EM energy harvesting in multiple microwave bands,with|S11|up to−63.2 dB,and can be tuned by the degree of bending.An ultra-wideband bandpass filter realizes a passband of about 5.4 GHz and effectively suppresses the transmission of EM signals in the stopband.An infrared stealth device has an emissivity of less than 0.2 in the infrared spectrum at wavelengths of 6-14μm.This work can provide new inspiration for the design and development of multifunctional,multi-spectrum EM devices.

关键词： Graphene-like MXene hybrids Multi-spectral response Multi-function antenna Ultra-wideband bandpass filter Electromagnetic device

Achieving high carrier mobility and low lattice thermal conductivity in GeTe-based alloys by cationic/anionic co-doping

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Rare Metals 2024年第6期43卷 2784-2795页

作者： Xiao-qiang Wang Xiao-quan Hu Jun-Yan lin Chu-Bin li Xiao-Tong Yu Qi-Yong Chen li-li Xi Qi-Shuo Yang Han li Ji-Ye Zhang Shuan-Kui li Kai Guo School of Physics and Materials Science Guangzhou University Research Center for Advanced Information Materials (CAIM) Huangpu Research & Graduate School of Guangzhou University School of Materials Science and Engineering Shanghai University Materials Genome Institute Shanghai University School of Mechanical and Mining Engineering University of Queensland Key Laboratory of Si-Based Information Materials & Devices and Integrated Circuits Design Department of Education of Guangdong Province

The Ⅳ-Ⅵ compound GeTe is considered as a promising alternative to the toxic PbTe for high-efficiency mid-temperature thermoelectric applications.However,pristine GeTe suffers from a high concentration of Ge vacancies,resulting in an excessively high hole concentration(> 1 × 1021cm-3),which greatly limits its thermoelectric enhancement.To address this issue,CuBiTe2alloying is introduced to increase the formation energy of Ge vacancies in GeTe,thereby inhibiting the high carrier concentration.The carrier scattering caused by the electronegativity difference between different elements is suppressed due to the similar electronegativity of Cu and Ge atoms.A relatively high hole mobility is obtained,which ultimately leads to a high power factor.Additionally,by introducing Se as an alloying element at the anionic site in GeTe,dense point defects with mass/strainfield fluctuations are induced.This contributes to the strengthening of phonon scattering,thereby reducing the lattice thermal conductivity from 1.44 W·m-1·K-1for pristine GeTe to 0.28 W·m-1·K-1for Ge0.95Cu0.05Bi0.05Te0.9Se0.15compound at 623 K.

关键词： GeTe Carrier mobility CuBiTe 2 alloying Lattice thermal conductivity Thermoelectric properties