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Effects of zero-valent iron added in the flooding or drainage process on cadmium immobilization in an acid paddy soil

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Journal of Environmental Sciences 2024年第4期138卷 19-31页

作者： Hanbing Meng Shiwen Hu Zebin Hong Wenting Chi Guojun Chen Kuan Cheng qiwang Tongxu Liu Fangbai Li Kexue Liu Yang Yang Guangzhou Institute of Geochemistry Chinese Academy of SciencesGuangzhou 510640China National-Regional Joint Engineering Research Center for Soil Pollution Control and Remediation in South China Guangdong Key Laboratory of Integrated Agro-environmental Pollution Control and ManagementInstitute of Eco-environmental and Soil SciencesGuangdong Academy of SciencesGuangzhou 510650China School of Resources and Planning Guangzhou Xinhua UniversityGuangzhou 510310China University of Chinese Academy of Sciences Beijing 100049China

Zero-valent iron(ZVI)is a promising material for the remediation of Cd-contaminated paddy ***,the effects of ZVI added during flooding or drainage processes on cadmium(Cd)retention remain ***,Cd-contaminated paddy soil was incubated for 40days of flooding and then for 15 days of drainage,and the underlying mechanisms of Cd immobilization coupled with Fe/S/N redox processes were *** addition of ZVI to the flooding process was more conducive to Cd *** potential available Cd was detected by adding ZVI before flooding,which may be due to the increase in paddy soil pH and newly formed secondary Fe ***,the reductive dissolution of Fe minerals promoted the release of soil colloids,thereby increasing significantly the surface sites and causing Cd ***,the addition of ZVI before flooding played a vital role in Cd retention after soil *** contrast,the addition of ZVI in the drainage phase was not conducive to Cd retention,which might be due to the rapid decrease in soil pH that inhibited Cd adsorption and further immobilization on soil *** findings of this study demonstrated that Cd availability in paddy soil was largely reduced by adding ZVI during the flooding period and provide a novel insight into the mechanisms of ZVI remediation in Cd-contaminated paddy soils.

关键词： Paddy soil Zero-valent iron Cadmium Flooding and drainage Remediation

Nanodiamond/Ti_(3)C_(2) MXene-coated quartz crystal microbalance humidity sensor with high sensitivity and high quality factor

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Rare Metals 2024年第6期43卷 2719-2729页

作者： Yao Yao Qiao Chen Yan-Qi Li Xian-He Huang Wei-Wei Ling Zhe-MiaoXie Jia-qiwang Chang-Ming Chen College of Communication Engineering Chengdu University of Information TechnologyChengdu 610225China School of Automation Chongqing University of Posts and TelecommunicationsChongqing 400065China School of Automation Engineering University of Electronic Science and Technology of ChinaChengdu 611731China Advanced Micro-/Nano-Devices Lab Department of Systems Design EngineeringUniversity of WaterlooWaterlooON N2L 3GlCanada

To address the challenge of achieving both high sensitivity and a high quality factor in quartz crystal microbalance(QCM)humidity sensors,a nanodiamond(ND)/Ti_(3)C_(2)MXene composite-coated QCM humidity sensor was *** material characteristics of ND,Ti_(3)C_(2)MXene,and ND/Ti_(3)C_(2)MXene composite were analyzed by transmission electron microscopy(TEM)and Fourier transform infrared(FTIR)*** experimental results demonstrated that the hydrophilic ND nanoparticles coated on Ti_(3)C_(2) MXene nanosheet prevented the self-stacking of Ti_(3)C_(2)MXene and enhanced the sensitivity of Ti_(3)C_(2) MXene-based QCM humidity ***,the high mechanical modulus of Ti_(3)C_(2) MXene material helped ND/Ti_(3)C_(2)MXene composite-coated QCM humidity sensor to achieve a high quality factor(>20,000).ND/Ti_(3)C_(2)MXene compositecoated QCM humidity sensor exhibited a sensitivity of 82.45 Hz/%RH,a humidity hysteresis of 1.1%RH,fast response/recovery times,acceptable repeatability,and good stability from 11.3%RH to 97.3%*** response mechanism of ND/Ti_(3)C_(2) MXene composite-coated QCM humidity sensor was analyzed in combination with a bi-exponential kinetic adsorption ***,the potential application of ND/Ti_(3)C_(2)MXene composite-coated QCM humidity sensor was demonstrated through its frequency response to wooden blocks with different moisture contents.

关键词： Humidity sensor Quartz crystal microbalance Nanodiamond Ti_(3)C_(2)MXene High quality factor

Impact of short-term ambient air pollution exposure on the risk of severe COVID-19

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Journal of Environmental Sciences 2024年第1期135卷 610-618页

作者： Baihuan Feng Jiangshan Lian Fei Yu Dan Zhang Weizhen Chen qiwang Yifei Shen Guoliang Xie Ruonan Wang Yun Teng Bin Lou Shufa Zheng Yida Yang Yu Chen Department of Laboratory Medicine The First Affiliated HospitalZhejiang University School of MedicineHangzhou 310000China Key Laboratory of Clinical In Vitro Diagnostic Techniques of Zhejiang Province Hangzhou 310000China Institute of Laboratory Medicine Zhejiang UniversityHangzhou 310000China Department of Infectious Diseases The First Affiliated HospitalZhejiang University School of MedicineHangzhou 310000China State Key Laboratory for Diagnosis and Treatment of Infectious Diseases National Clinical Research Center for Infectious DiseasesCollaborative Innovation Center for Diagnosis and Treatment of Infectious Diseasesthe First Affiliated HospitalZhejiang University School of MedicineHangzhou 310000China

Ecological studies suggested a link between air pollution and severe COVID-19 outcomes,while studies accounting for individual-level characteristics are *** the present study,we aimed to investigate the impact of short-term ambient air pollution exposure on disease severity among a cohort of 569 laboratory confirmed COVID-19 patients admitted to designated hospitals in Zhejiang province,China,from January 17 to March 3,2020,and elucidate the possible biological processes involved using *** with mild cases,severe cases had higher proportion of medical conditions as well as unfavorable results in most of the laboratory tests,and manifested higher air pollution exposure *** exposure to air pollutants was associated with increased risk of severe COVID-19 with odds ratio(OR)of 1.89(95%confidence interval(CI):1.01,3.53),2.35(95%CI:1.20,4.61),2.87(95%CI:1.68,4.91),and 2.01(95%CI:1.10,3.69)for PM_(2.5),PM_(10),NO_(2)and CO,*** for NO_(2)remained significant in two-pollutant models after adjusting for other *** analysis showed 884 differentially expressed genes which mainly were enriched in virus clearance related biological processes between patients with high and low NO_(2)exposure levels,indicating that compromised immune response might be a potential underlying mechanistic *** findings highlight the impact of shortterm air pollution exposure,particularly for NO_(2),on COVID-19 severity,and emphasize the significance in mitigating the COVID-19 burden of commitments to improve air quality.

关键词： Air pollution COVID-19 Severity Transcriptomics Immune response

协同双小区下行协作NOMA-SWIPT中断性能分析

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信号处理 2024年第6期40卷 1052-1061页

作者：张煜贺玉成张彦陈启望华侨大学厦门市移动多媒体通信重点实验室福建厦门361021

本文研究了在毫微微蜂窝网络(femtocell network,FN)中,协同双小区系统的非正交多址接入(non-orthogonal multiple access,NOMA)与无线携能通信(simultaneous wireless information and power transfer,SWIPT)下行协作通信的中断性能,提出了一种边缘用户在邻基站及源基站随机中心用户共同协作的下行接入方案。所提方案共分为两个时隙:第一时隙内由两基站向所有用户广播叠加信号,提供中继服务的中心用户对其所接收的叠加信号逐级解码并收集能量。第二时隙,中心用户将其第一时隙内所收集的能量作为额外功率资源,在优先保证自身通信质量的前提下对成功解码的边缘用户信息进行再编码转发。基于空间均质泊松点过程(Poisson point process,PPP)中心用户的位置模型,推导了中心用户与边缘用户平均中断概率的表达式,进行了蒙特卡罗仿真验证,同时分析了各仿真参数(中心用户分布半径、用户阈值速率、路径损耗指数等)与中心用户、边缘用户平均中断概率的关系。结果表明:所提方案可以改善边缘用户的下行接入中断性能和系统吞吐量。

关键词：非正交多址接入无线携能通信协作通信下行中断概率泊松点过程

Elevated-temperature properties of one long-life high-strength gun steel

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Journal of University of Science and Technology Beijing 2004年第1期11卷 62-66页

作者： MaoqiuWang HanDong qiwang DivisionofStructuralMaterials CentralIron＆SteelResearchInstituteBeijing100081China

The hardness, tensile strength and impact toughness of one quenched andtempered steel with nominal composition of Fe-0.25C-3.0Cr-3.0Mo-0.6Ni-0.1Nb (mass fraction) both atroom temperature and at elevated temperatures were investigated in order to develop high-strengthsteel for long-life gun barrel use. It is found that the steel has lower decrease rate of tensilestrength at elevated temperature in comparison with the commonly used G4335V high-strength gunsteel, which contains higher Ni and lower Cr and Mo contents. The high elevated-temperature strengthof the steel is attributed to the strong secondary hardening effect and high tempering softeningresistance caused by the tempering precipitation of fine Mo-rich M_2C carbides in the α-Fe *** experimental steel is not susceptible to secondary hardening embrittlement, meanwhile, itsroom-temperature impact energy is much higher than the normal requirement of impact toughness forhigh strength gun steels. Therefore, the steel is suitable for production of long-life high-strengthgun barrels with the combination of superior elevated-temperature strength and good impacttoughness.

关键词： secondary hardening steel elevated-temperature strength hot hardness impact toughness

Molecular Simulation on Transport Properties of Confined Water

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Chinese Chemical Letters 2004年第7期15卷 879-882页

作者： YingChunLIU GuoZhenXIAO qiwang DepartmentofChemistry ZhejiangUniversityHangzhou310027 DepartmentofComputerScience ZhejiangUniversityHangzhou310027

The diffusivity and viscosity of water confined in micropores were studied by molecular dynamics simulations. The effects of pore width and density were analyzed at pore widths from 0.9 to 2.6 nm. The diffusivity in micropores is lower than that of the bulk, and it decreases as pore width decreases and as density increases. But the viscosity in micropores is much larger than that of the bulk, and it increases as pore width decreases and as density increases. The diffusivity in channel parallel direction is obviously larger than that in channel perpendicular directions.

关键词： Micropore transport property molecular dynamics simulation.

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油菜直播组合式埋茬防堵装置设计与试验

农业工程学报 2024年第5期40卷 60-70页

作者：杜文斌周国威张青松边祺旺廖庆喜廖宜涛华中农业大学工学院武汉430070 农业农村部长江中下游农业装备重点实验室武汉430070

针对长江中下游地区油菜机械化种植时土壤黏重板结、前茬秸秆留茬高、残留量大,致使油菜直播机旋耕及深施肥部件易出现秸秆缠绕、壅土堵塞等问题,导致秸秆埋覆率低、种床厢面起伏不平,影响种床质量的生产现状,该研究设计了一种适用于高... 详细信息

针对长江中下游地区油菜机械化种植时土壤黏重板结、前茬秸秆留茬高、残留量大,致使油菜直播机旋耕及深施肥部件易出现秸秆缠绕、壅土堵塞等问题,导致秸秆埋覆率低、种床厢面起伏不平,影响种床质量的生产现状,该研究设计了一种适用于高茬黏重稻茬田的油菜直播机组合式埋茬防堵装置。该装置主要包括埋茬弯刀和双刃旋耕刀,刀片在筒状刀轴上整体呈人字型排布,通过埋茬弯刀和双刃旋耕刀配合作业,可防止旋耕及深施肥部件秸秆缠绕和黏附堵塞,实现黏重土壤细碎、高茬秸秆埋覆和厢面平整。开展理论分析与EDEM仿真,确定了埋茬弯刀回转半径为245 mm,正切面弯折线角为27°、弯折角为125°,作业幅宽为75 mm,防堵直刀回转半径为275 mm,刃磨角为15°。田间对比试验结果表明:装有组合式埋茬防堵装置的油菜直播机在高茬黏重地表作业通过性好,未出现秸秆缠绕和黏土堵塞,厢面平整度为19.19~22.14 mm,相较于普通旋耕装置,秸秆埋覆率至少提高27.19个百分点,埋茬防堵性能良好,种床质量满足油菜直播农艺要求。研究结果可为高茬黏重工况下的种床整备装置开发提供参考。

关键词：农业机械试验油菜埋茬防堵种床制备

A New Efficient Synthesis of p-Nitrocalix[4]arene

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Chinese Chemical Letters 2004年第4期15卷 400-403页

作者： YongLI JiaSongWANG qiwang DeShanLI DepartmentofChemistry TsinghuaUniversityBeijing100084

A new efficient synthesis of p-nitrocalix[4]arene from calix[4]arene by using nitrogen dioxide is described. The compound is an useful intermediates for the introduction of other functional groups to obtain N containi... 详细信息

关键词： Nitration calixarene nitrogen dioxide.

改进注意力机制嵌入PR-Net模型的水稻病害识别仿真

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系统仿真学报 2024年第6期36卷 1322-1333页

作者：路阳刘鹏飞许思源刘启旺顾福谦王鹏黑龙江八一农垦大学信息与电气工程学院黑龙江大庆163319 东北石油大学黑龙江省网络化与智能控制重点实验室黑龙江大庆163318 东北石油大学人工智能能源研究院黑龙江大庆163318 东北石油大学三亚海洋油气研究院海南三亚572024

针对现有的CNN模型在水稻叶部病害的识别中准确率较低的问题,提出了一种结合并行结构和残差结构的混合卷积神经网络模型PRC-Net(parallel residual with coordinate attention network)。引入并行结构,提高卷积的感受野;结合残差结构,... 详细信息

针对现有的CNN模型在水稻叶部病害的识别中准确率较低的问题,提出了一种结合并行结构和残差结构的混合卷积神经网络模型PRC-Net(parallel residual with coordinate attention network)。引入并行结构,提高卷积的感受野;结合残差结构,使特征信息完整的连续传递;在骨干模型PR-Net中嵌入改进的空间注意力机制,增强对不同尺度病斑特征信息的凝聚程度;为进一步提升病害识别的准确率,并减少模型的训练时间和推理时间,通过改变加权方式对模型结构进行优化。仿真结果表明:与InceptionResNetV2等分类模型相比,PRC-Net具有更少的训练参数、更短的训练时间和更高的识别精度,性能优于其他作物病害识别模型。

关键词：水稻叶部病害 PRC-Net(parallel residual with coordinate attention network) 卷积神经网络注意力机制图像识别