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Polymer-to-Monomers Chemically Recyclable Poly(imide-imine)Plastics with Extreme-Condition Resistance and Flame Retardancy

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Chinese Journal of Polymer Science 2024年第10期42卷 1525-1535,I0012页

作者： zhen-Yu wang Xiao-Kong Liu State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchun130012China

Polyimides are a family of high-tech plastics that have irreplaceable applications in the fields of aerospace,defense,and opto-electronics,but polyimides are difficult to be reprocessed and recycled at the end of their service life,resulting in a significant waste of ***,it is of great significance to develop recyclable polyimides with comparable properties to the commercial ***,we report a novel polymer-to-monomers chemically recyclable poly(imide-imine)(PtM-CR-PII)plastic,synthesized by cross-linking the amine-terminated aromatic bisimide monomer and the hexa-vanillin terminated cyclophosphazene monomer via dynamic imine *** PtM-CR-PII plastic exhibits comparable mechanical and thermal properties as well as chemical stability to the commercial *** PtM-CR-PII plastic possesses a high Young’s modulus of≈3.2 GPa and a tensile strength as high as≈108 MPa,which also exhibits high thermal stability with a glass transition temperature of≈220℃.Moreover,the PtM-CR-PII plastic exhibits outstanding waterproofness,acid/alkali-resistance,and solvent-resistance,its appearance and mechanical properties can be well maintained after long-term soaking in water,highly concentrated acid and base,and various organic ***,the cyclophosphazene moieties endow the PtM-CR-PII plastic with excellent flame *** PtM-CR-PII plastic exhibits the highest UL-94 flame-retarding rating of V-0 and a limiting oxygen index(LOI)value of 45.5%.Importantly,the PtM-CR-PII plastic can be depolymerized in an organic solvents-acid mixture medium at room temperature,allowing easy separation and recovery of both monomers in high *** recovered pure monomers can be used to regenerate new PtM-CR-PII plastics,enabling sustainable polymer-monomers-polymer circulation.

关键词： Chemical recyclability Polyimides Polyimines Dynamic imine bonds Mechanical properties Chemical stability

Effect of Calcination Temperature on the Microstructure and Surface Properties of a Cu/ZnO Catalyst Derived from Zn_(3)Cu_(2)(OH)_(6)(CO_(3))_(2)

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China Petroleum Processing & Petrochemical Technology 2024年第2期26卷 46-56页

作者： qiu Shiming wang Shengjie School of Chemistry and Chemical Engineering Guangxi Minzu Normal UniversityChongzuo 532200GuangxiChina Guangxi Key Laboratory for High-value Utilization of Manganese Resources Chongzuo 532200GuangxiChina

The Cu/ZnO catalyst formed upon the calcination of aurichalcite has a uniform distribution of ZnO,which can delay the sintering of Cu species at high *** this study,aurichalcite possessing a nearly pure phase was prepared using the ammonium complex dissociation precipitation method,and the effect of calcination temperature on the structure and surface properties of the derived Cu/ZnO catalyst was *** results show that the calcination temperature determines the particle size and crystallization degree of the Cu/ZnO catalyst and the surface properties of the corresponding copper oxide and reduced ***-temperature calcination is more conducive to reducing the particle size of the Cu/ZnO catalyst,increasing the specific surface area,and generating abundant defect characteristics on the surface,which is key to obtaining highly dispersed copper and copper-specific surface area catalysts by subsequent ***,the Cu/ZnO catalyst derived using a 300℃or 400℃calcination proved to have a higher specific activity per gram of copper than a commercial Cu/Zn/Al *** discovery in this study opens up a new method for the convenient preparation of a high-temperature resistant Cu/Zn methanol reforming catalyst.

关键词： methanol reforming copper zinc oxide lattice defect

Novel intelligent reasoning system for tool wear prediction and parameter optimization in intelligent milling

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Advances in Manufacturing 2024年第1期12卷 76-93页

作者： Long-Hua Xu Chuan-zhen Huang zhen wang Han-Lian Liu Shui-Quan Huang Jun wang School of Mechanical Engineering Yanshan UniversityQinhuangdao066004HebeiPeople’s Republic of China Center for Advanced Jet Engineering Technologies(CaJET) Key Laboratory of High-efficiency and Clean Mechanical Manufacture(Ministry of Education)National Experimental Teaching Demonstration Center for Mechanical Engineering(Shandong University)School of Mechanical EngineeringShandong UniversityJinan250061People’s Republic of China Institute of Manufacturing Technology Guangdong University of TechnologyGuangzhou510006People’s Republic of China

Accurate intelligent reasoning systems are vital for intelligent *** this study,a new intelligent reasoning system was developed for milling processes to accurately predict tool wear and dynamically optimize machining *** developed system consists of a self-learning algorithm with an improved particle swarm optimization(IPSO)learning algorithm,prediction model determined by an improved case-based reasoning(ICBR)method,and optimization model containing an improved adaptive neural fuzzy inference system(IANFIS)and *** results showed that the IPSO algorithm exhibited the best global convergence *** ICBR method was observed to have a better performance in predicting tool wear than standard CBR *** IANFIS model,in combination with IPSO,enabled the optimization of multiple objectives,thus generating optimal milling *** paper offers a practical approach to developing accurate intelligent reasoning systems for sustainable and intelligent manufacturing.

关键词： Improved particle swarm optimization(IPSO)algorithm Improved case-based reasoning(ICBR)method Adaptive neural fuzzy inference system(ANFIS)model Tool wear prediction Intelligent manufacturing

Multi-scale physics-informed neural networks for solving high Reynolds number boundary layer flows based on matched asymptotic expansions

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Theoretical & Applied Mechanics Letters 2024年第2期14卷 76-81页

作者： Jianlin Huang Rundi qiu Jingzhu wang Yiwei wang Key Laboratory for Mechanics in Fluid Solid Coupling Systems Institute of MechanicsChinese Academy of SciencesBeijing 100190China School of Future Technology University of Chinese Academy of SciencesBeijing 100049China School of Engineering Science University of Chinese Academy of SciencesBeijing 100049China Guangdong Aerospace Research Academy Guangzhou 511458China

Multi-scale system remains a classical scientific problem in fluid dynamics,biology,*** the present study,a scheme of multi-scale Physics-informed neural networks is proposed to solve the boundary layer flow at high Reynolds numbers without any *** flow is divided into several regions with different scales based on Prandtl's boundary *** regions are solved with governing equations in different *** method of matched asymptotic expansions is used to make the flow field continuously.A flow on a semi infinite flat plate at a high Reynolds number is considered a multi-scale problem because the boundary layer scale is much smaller than the outer flow *** results are compared with the reference numerical solutions,which show that the msPINNs can solve the multi-scale problem of the boundary layer in high Reynolds number *** scheme can be developed for more multi-scale problems in the future.

关键词： Physics-informed neural networks(PINNs) Multi-scale Fluid dynamics Boundary layer

Decentralized Primary Frequency Regulation for Hybrid Multi-terminal Direct Current Power Systems Considering Multi-source Enhancement

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Journal of Modern Power Systems and Clean Energy 2024年第3期12卷 958-970页

作者： Jialiang Wu zhen wang Ruixu Liu Yu Shan Chenxuan wang the College of Electrical Engineering Zhejiang UniversityHangzhou 310027China the Economic Research Institute of State Grid Zhejiang Electric Power Co. Ltd.Hangzhou 310016China

Hybrid multi-terminal direct current(MTDC)transmission technology has been a research focus,and primary frequency regulation(FR)improvement in the receiving-end system is one of the problems to be *** paper presents a decentralized primary FR scheme for hybrid MTDC power systems considering multi-source enhancement to help suppress frequency disturbance in the receiving-end *** the converters only need local frequency or DC voltage signal input to respond to system disturbance without communication or a control center,i.e.,a decentralized control *** proposed scheme can activate appropriate power sources to assist in FR in various system disturbance severities with fine-designed thresholds,ensuring sufficient utilization of each power *** better balance FR performance and FR resource participation,an evaluation index is proposed and the parameter optimization problem is further ***,the validity of the proposed scheme is verified by simulations in MATLAB/Simulink.

关键词： Decentralized control scheme primary frequency regulation(FR) rate of change of frequency(ROCOF) system frequency disturbance

A low-power Bluetooth-based wireless sensor network and its global confliction-solving impact localization method

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Chinese Journal of Aeronautics 2024年第1期37卷 153-161页

作者： Yuanjia wang Lei qiu Qiyun XU Liming SHI College of Aerospace Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China Department of Electrical and Electronic Engineering University of EdinburghEdinburgh EH89YLUK

During the whole service lifetime of aircraft structures with composite materials,impacts are inevitable and can usually cause severe but barely visible *** the occurrences of impact are random and unpredictable,it is a hotspot direction to develop an online impact monitoring system that can meet strict limitations of aerospace applications including small size,light weight,and low power ***(PZT)sensor,being able to generate impact response signals with no external power and cover a large-scale structure with only a small amount of them,is a promising ***,for real systems,networks with multiple nodes are normally required to monitor large-scale structures in a global way to identify any impact localization confliction,yet the existing studies are mostly evaluated with single nodes instead of ***,in this paper,based on a new low-power node designed,a Bluetooth-based digital impact monitoring PZT sensor network is proposed for the first time with its global confliction-solving impact localization *** of the system as a network are researched and analyzed on a complex real aircraft wing box for a global confliction-solving impact localization,showing a satisfying high accuracy.

关键词： Bluetooth-based low-power design Confliction-solving evaluation Complex composites Piezoelectric sensors Wireless impact monitoring network

Partition-based Network Equivalent Method for Power System Subsynchronous Oscillation Analysis

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Journal of Modern Power Systems and Clean Energy 2024年第1期12卷 313-320页

作者： Chenxuan wang Weimin zheng zhen wang Yangqing Dan Ping Ju the Department of Electrical Engineering Zhejiang UniversityHangzhou 310027China the Economic Research Institute of State Grid Zhejiang Electric Power Co. Ltd.Hangzhou 310016China the College of Energy and Electrical Engineering Hohai UniverstiyNanjing 211100China

Given large-scale modern power systems with pow er electronic converters,the numerical simulation with subsyn chronous oscillation(SSO)faces great challenges in engineering practice due to sharply enlarged modeling scale and high com putational *** reduce the modeling scale,network parti tion and equivalent becomes a vital technique in numerical sim *** several methods have been developed for net work equivalent,a generally accepted rule for network parti tion is still *** paper proposes that the system can be partitioned into three parts,i.e.,the internal,the middle,and the external subsystems,in which the internal subsystem consists of all power electronic components,the middle subsys tem includes those selected AC dynamic components with de tailed models,and the remaining components and buses consti tute the external *** external subsystem is further represented by an equivalent RLC network determined by the frequency dependent network equivalent(FDNE)*** the proposed method,the observability index and the electrical distance index are used to identify the interface between the middle and the external *** studies based on a modified Hydro-Quebec system are used to verify the effective ness of the proposed method.

关键词： Electrical distance network equivalent subsyn chronous oscillation observability index

∞-Tilting Subcategories in Extriangulated Categories

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Chinese Annals of Mathematics,Series B 2024年第1期45卷 151-160页

作者： zhen ZHANG Jiaqun WEI Shance wang Department of Mathematics Qilu Normal UniversityJinan 250200China Institution of Mathematics School of Mathematics ScienceNanjing Normal UniversityNanjing 210023China

In this paper, the authors introduce a new definition of ∞-tilting(resp. cotilting) subcategories with infinite projective dimensions(resp. injective dimensions) in an extriangulated category. They give a Bazzoni characterization of ∞-tilting(resp. cotilting)subcategories. Also, they obtain a partial Auslander-Reiten correspondence between ∞-tilting(resp. cotilting) subcategories and coresolving(resp. resolving) subcategories with an E-projective generator(resp. E-injective cogenerator) in an extriangulated category.

关键词： Extriangulated category ∞-Tilting subcategory Auslander-Reiten correspondence Bazzoni characterization

B Vitamins Can Reduce Body Weight Gain by Increasing Metabolism-related Enzyme Activities in Rats Fed on a High-Fat Diet

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Journal of Huazhong University of Science and Technology(Medical Sciences) 2018年第1期38卷 174-183页

作者： Ying zhenG Ai-guo MA Ming-ci zhenG qiu-zhen wang Hui LIANG Xiu-xia HAN Evert G.Schouten Department of Nutrition Guangdong General HospitalGuangdong Academy of Medical SciencesGuangzhou 510080China Institute of Human Nutrition Medical College of Qingdao UniversityQingdao 266021China Department of Pediatrics Guilin Medical College Affiliated HospitalGuilin 541001China Division of Human Nutrition Wageningen UniversityWageningen 6700 EVThe Netherland

B vitamins are enzyme cofactors that play an important role in energy *** aim of this study was to elucidate whether B vitamin administration can reduce body weight(BW)gain by improving energy metabolism-related enzyme activities in rats fed on a highfat *** rats were randomly assigned to one of the following five groups:control group(C),including rats fed on standard rat chow;four treatment groups(H0,H1,H2,and H3),in which rats were fed on a high-fat *** in the H1 group were treated daily with 100 mg/kg BW thiamine(VB1),100 mg/kg BW riboflavin(VB2),and 250 mg/kg BW niacin(VPP);rats in the H2 group were treated daily with 100 mg/kg BW pyridoxine(VB6),100 mg/kg BW cobalamin(VB12),and 5 mg/kg BW folate(FA);and rats in the H3 group were treated daily with all of the B vitamins administered to the H1 and H2 *** 12 weeks,the BW gains from the initial value were 154.5±58.4 g and 159.1±53.0 g in the H1 and C groups,respectively,which were significantly less than the changes in the H0 group(285.2±14.8 g,P〈0.05).In the H0 group,the plasma total cholesterol(CHO)and triglyceride(TG)levels were 1.59±0.30 mmol/L and 1.55±0.40 mmol/L,respectively,which were significantly greater than those in the H1 group(1.19±0.18 mmol/L and 0.76±0.34 mmol/L,respectively,P〈0.05).The activities of transketolase(TK),glutathione reductase,and Na^+/K^+adenosine triphosphatase were significantly increased in the B vitamin-treated groups and were significantly greater than those in the H0 group(P〈0.05).Furthermore,the glucose-6-phosphate dehydrogenase,pyruvic acid kinase,and succinate dehydrogenase activities also were increased after treatment with B *** with B vitamins could effectively reduce BW gain and plasma levels of lipids by improving energy metabolism-related enzyme activities in rats,thus possibly providing potential benefits to humans.

关键词： B vitamins obesity body weight gain enzyme activities rats