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Design and fabrication of self-suspending aluminum-plastic/semiconductor photocatalyst devices for solar energy conversion

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Journal of Environmental Sciences 2024年第2期136卷 615-625页

作者： Zhi-Ang Zhao Jingyun Mao Chengjing lu Shuangqiao Yang Qingrong Qian qinghua Chen Hun Xue Xiaoli Sun Min-Quan Yang College of Environmental and Resource Sciences College of Carbon Neutral Modern IndustryFujian Key Laboratory of Pollution Control and Resource ReuseFujian Normal UniversityFuzhou 350007China State Key Laboratory of Polymer Materials Engineering Polymer Research Institute of Sichuan UniversityChengdu 610065China

The design and synthesis of self-suspending photocatalyst device with easy recyclability is important for practical application.Here,this work utilizes aluminum-plastic package waste as raw material to prepare an aluminum-plastic supported TiO_(2)(AP-TiO_(2))photocatalyst device through 3D printing design and surface deposition method.A series of characterizations were carried out to explore the structure,morphology and performance of the AP-TiO_(2)device.Under UV light illumination,the AP-TiO_(2)-50 efficiently degrade 93.6%tetracycline hydrochloride(THC)after 4 hr,which increases by 8.3%compared with that of TiO_(2)powder suspension system with the same catalyst amount.Based on it,AP-ZnO,AP-CdS,AP-g-C_3N_4and AP-Pt-TiO_(2)are also fabricated,and applied in photocatalytic degradation and hydrogen evolution,which all exhibit higher photoactivities than powder suspension systems.This work provides a new avenue for the fabrication of advanced recyclable photocatalyst device.Moreover,the work offers a novel sight for the high-value utilization of aluminum-plastic package waste,which has positive implications for environmental protection.

关键词： TiO_(2) Self-suspending Photocatalyst device Aluminum plastic

A Deep Learning-Enabled Skin-Inspired Pressure Sensor for Complicated Recognition Tasks with Ultralong Life

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Research 2024年第1期2023卷 443-454页

作者： Yingxi Xie Xiaohua Wu Xiangbao Huang qinghua Liang Shiping Deng Zeji Wu Yunpeng Yao Longsheng lu School of Mechanical&Automotive Engineering South China University of TechnologyGuangzhouChina

Flexible full-textile pressure sensor is able to integrate with clothing directly,which has drawn extensive attention from scholars recently.But the realization of flexible full-textile pressure sensor with high sensitivity,wide detection range,and long working life remains challenge.Complex recognition tasks necessitate intricate sensor arrays that require extensive data processing and are susceptible to damage.The human skin is capable of interpreting tactile signals,such as sliding,by encoding pressure changes and performing complex perceptual tasks.Inspired by the skin,we have developed a simple dip-and-dry approach to fabricate a full-textile pressure sensor with signal transmission layers,protective layers,and sensing layers.The sensor achieves high sensitivity(2.16 kPa^(−1)),ultrawide detection range(0 to 155.485 kPa),impressive mechanical stability of 1 million loading/unloading cycles without fatigue,and low material cost.The signal transmission layers that collect local signals enable real-world complicated task recognition through one single sensor.We developed an artificial Internet of Things system utilizing a single sensor,which successfully achieved high accuracy in 4 tasks,including handwriting digit recognition and human activity recognition.The results demonstrate that skin-inspired full-textile sensor paves a promising route toward the development of electronic textiles with important potential in real-world applications,including human–machine interaction and human activity detection.

关键词： Deep Skin utilizing

Thoughts on the system construction of digital Chinese medicine

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Digital Chinese Medicine 2024年第1期7卷 1-2页

作者： lu Shan PENG qinghua Editorial Office of Digital Chinese Medicine Hunan University of Chinese MedicineChangshaHunan 410208China Chinese Medicine Diagnostic Institute Hunan University of Chinese MedicineChangshaHunan 410208China

Digital Chinese medicine refers to a comprehensive system that utilizes unified scientific technologies to fully explore and reproduce human phenomenology, patterns of physical changes, and related human experiences. ... 详细信息

关键词： (TCM) system utilize

Three-phase interface induced charge modulation on MoO_(2)/Mo_(2)Ccarbon tube for enhanced hydrogen evolution

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Nano Research 2023年第4期16卷 4706-4714页

作者： Zhijie Zhang Jing Zhao Mengchen Wu qinghua lu Rui Liu Shanghai Key Laboratory of Development and Application for Metal-Functional Materials School of Materials Science and EngineeringTongji UniversityShanghai 201804China School of Chemical Science and Engineering Tongji UniversityShanghai 200092China

Exploring superior electrocatalyst for hydrogen evolution reaction(HER)is an urgent need for hydrogen production based on water splitting.The redistribution of electrons and the increase of active sites through multi-interface designing of electrocatalyst are powerful strategies to improve the catalytic efficiency.Herein,a three-phase interface structure of N,P co-doped carbon tube embedded with MoO_(2)/Mo_(2)C(MoO_(2)/Mo_(2)C-CT)was fabricated via a cooperative polymerizing-embedding and pyrolysis strategy.Work function and X-ray photoelectron spectroscopy(XPS)verified that the interfacial charge was quantificationally modulated,achieving an intrinsically enhanced charge transfer by an induced built-in electric field.Theoretical study of density functional theory(DFT)illustrated that triple-interface structure showed a lower energy for H*+H2O*than that of single-interface counterparts.The triple-interface MoO_(2)/Mo_(2)C-CT delivered a lower overpotential of 129 mV at 10 mA·cm^(−2)than that of either single-interface MoO_(2)-CT or Mo_(2)C-CT catalyst.This work may put forward an attractive approach for modulating electronic structure and provide insights into the understanding of triple-interface structure towards HER.

关键词： triple-interface Mo carbon tube hydrogen evolution reaction density functional theory

Au(Ⅰ)-BSA nanocomposites with assembling-induced excitation-dependent multicolor emission for dynamic cell imaging

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Science China Chemistry 2023年第1期66卷 174-184页

作者： Xuejuan Wang Guofeng Liu Kuo Fu Xuping Li Mengting Yao qinghua lu Liangliang Zhu Xiang Ma Shanghai Key Laboratory of Chemical Assessment and Sustainability Advanced Research Institute School of Chemical Science and EngineeringTongjiUniversityShanghai200092China Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering Frontiers Science Center for Materiobiology and Dynamic ChemistrySchool of Chemistry and Molecular EngineeringEast China University of Scienceand TechnologyShanghai 200237China State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular ScienceFudan University Shanghai 200438China

Excitation wavelength dependent(Ex-De) luminescent materials have attracted intense attention due to their great potential in multicolor bioimaging,dynamic anti-counterfeiting,and light emitting devices.However,it remains a formidable challenge to construct an Ex-De luminescent biomaterial with green starting materials,excellent biocompatibility,good water solubility,and multiple color emission for dynamic cell imaging.In this work,nanocomposites based on the facile self-assembly strategy of bovine serum albumin(BSA) and Au(Ⅰ)-complex are rationally designed and synthesized to simultaneously present Ex-De fluorescence(429–516 nm) and decent phosphorescence(~615 nm) in a dilute aqueous solution.Combinatory analyses of spectroscopic and microscopic results reveal that the luminescent mechanism of Au(Ⅰ)-BSA nanocomposites is cluster-induced Ex-De fluorescence and metal-to-ligand charge transition(MLCT) based phosphorescence.Importantly,based on the excellent biocompatibility,water-solubility and color-tunable emission over the entire visible region(360–800 nm),the Au(Ⅰ)-BSA nanocomposites are successfully used for cell imaging with multiple and switchable colors on demand.What is more,the solid tablets of Au(Ⅰ)-BSA nanoparticles showed pressure-responsive luminescence and decent room temperature phosphorescence.This work provides an assembling-induced emission strategy for the design of water-soluble,non-cytotoxic,and color-tunable luminescent biomaterials based on the composite of protein and Au nanoparticles.

关键词： nanocomposites excitation wavelength-dependent emission room temperature phosphorescence assembling-induced emission dynamic cell imaging

Durable superamphiphobic silica aerogel surfaces for the culture of 3D cellular spheroids

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National Science Review 2019年第6期6卷 1255-1265页

作者： Lianyi Xu Shuangshuang Chen Xuemin lu qinghua lu School of Materials Science Institute of Energy Equipment Materials Shanghai Dianji University School of Chemical Science and Engineering Tongji University School of Chemistry and Chemical Engineering State Key Laboratory of Metal Matrix Composite Shanghai Jiao Tong University

The 3D multicellular spheroids with intact cell–cell junctions have major roles in biological research by virtue of their unique advantage of mimicking the cellular physiological environments. In this work, a durable superamphiphobic silica aerogel surface(SSAS) has been fabricated for the upward culture of 3D multicellular spheroids. Poly(3,4-ethylenedioxythiophene)(PEDOT) was first electrodeposited on a conductive steel mesh as a first template for porous silica coating. Soot particles were then applied as a second template to construct a cauliflower-like silica aerogel nanostructure. After fluorination, a hierarchical structure with re-entrant curvature was finally fabricated as a durable superamphiphobic surface. This superamphiphobic surface also presented excellent antifouling towards biomacromolecules and cells, which has been demonstrated by the successful upward culture of cell spheroids. The upward culture makes the observation of cellular behavior in situ possible, holding great potential for 3D cellular evaluation in vitro.

关键词： cell spheroids superamphiphobicity durability electrochemistry silica aerogel

Predictive value of T cell receptor repertoire profiling for immunosuppressive therapy in severe aplastic anemia

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Genes & Diseases 2024年第1期11卷 95-98页

作者： Cunte Chen Yuling Zhang Dongpei lu Zelong Zhang Jun Yang Xiaowei Chen Ming Zhou Wenjian Mo Caixia Wang qinghua Cai Yumiao Li Ruiqing Zhou Shilin Xu Wei Zhou Tingfen Deng Shiyi Pan Yanli Xu Shunqing Wang Yuping Zhang Department of Hematology Guangzhou First People's HospitalSouth China University of TechnologyGuangzhouGuangdong 510180China Guangzhou Junruikang Biotechnology Co. LtdGuangzhouGuangdong 510700China

Increasing evidence supports the hypothesis of autologous immune attack in severe aplastic anemia(SAA):the predominant role of activated cytotoxic T cells(CTL)expressing-interferon in inhibiting the growth of bone marrow(BM)cells,putative autoantigens,and oligoclonal expansion of CD8+T cells.1 For SAA patients,the definitive therapies are immunosuppressive therapy(IST)or hematopoietic stem transplantation(HSCT).

关键词： anemia aplastic interferon

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基于多特征融合的露天矿区道路负障碍检测

煤炭学报 2024年第5期49卷 2561-2572页

作者：阮顺领鄢盛钰顾清华卢才武西安建筑科技大学资源工程学院陕西西安710055 西安建筑科技大学矿山系统工程研究所陕西西安710055 西安市智慧工业感知计算与决策重点实验室陕西西安710055

随着智慧矿山概念的逐步落实,智能化、无人化逐渐在矿区落实,露天矿卡车无人驾驶日益成为矿山智能化建设的主要内容,为解决露天矿区复杂多变的道路因坑洼、塌陷等路面小部分下陷出现的非规则负障碍而导致矿区无人车、重载卡车侧翻等安... 详细信息

随着智慧矿山概念的逐步落实,智能化、无人化逐渐在矿区落实,露天矿卡车无人驾驶日益成为矿山智能化建设的主要内容,为解决露天矿区复杂多变的道路因坑洼、塌陷等路面小部分下陷出现的非规则负障碍而导致矿区无人车、重载卡车侧翻等安全难题,提升矿区安全驾驶系数,提出一种多特征融合的露天矿区道路负障碍检测方法。该方法使用BiFPN特征融合模块,提高小型负障碍检测权重占比;引入空间和通道双注意力机制提高对负障碍边缘的特征提取和特征融合能力,从而提高对道路小尺度负障碍的检测精度;采用SIoU Loss作为模型边界框损失函数并使用K-means++方法优化Anchor以提高负障碍检测模型的收敛速度和边界框定位效果,并基于遗传算法优化超参数让模型更贴合矿区场景,最终实现对矿区道路负障碍的快速精准识别。实验表明该检测模型能快速准确识别复杂背景下露天矿区道路负障碍目标,对道路负障碍目标的检测精度、召回率、平均精确度均值分别达到了96.9%、89.9%、95.3%,且该模型大小仅有12.7 MB。对比其他主流检测网络,该网络模型更适合复杂环境下露天矿区非结构化道路行驶安全需求,且该检测模型的鲁棒性好,可适配于多种情况的露天矿区,为实际环境复杂多变的露天矿区非结构化道路负向障碍检测提供了可行的方法,为露天矿无人卡车安全生产运输提供安全预警。

关键词：露天矿区无人卡车负障碍检测特征融合安全预警

Jianpi qinghua Formula Alleviates Diabetic Myocardial Injury Through Inhibiting JunB/c-Fos Expression

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Current Medical Science 2024年第1期44卷 144-155页

作者： Lin WANG Qing-guang CHEN Hao lu Department of Endocrinology Shuguang Hospital Affiliated to Shanghai University of Traditional Chinese MedicineShanghai 201203China Department of Traditional Chinese Medicine Naval Medical UniversityShanghai 200433China

Objective Diabetic cardiomyopathy(DCM)represents a substantial risk factor for heart failure and increased mortality in individuals afflicted with diabetes mellitus(DM).DCM typically manifests as myocardial fibrosis,myocardial hypertrophy,and impaired left ventricular diastolic function.While the clinical utility of the Jianpi qinghua(JPQH)formula has been established in treating diabetes and insulin resistance,its potential efficacy in alleviating diabetic cardiomyopathy remains uncertain.This study aims to investigate the impact and underlying molecular mechanisms of the JPQH formula(JPQHF)in ameliorating myocardial injury in nonobese diabetic rats,specifically focusing on apoptosis and inflammation.Methods Wistar rats were assigned as the normal control group(CON),while Goto-Kakizaki(GK)rats were randomly divided into three groups:DM,DM treated with the JPQHF,and DM treated with metformin(MET).Following a 4-week treatment regimen,various biochemical markers related to glucose metabolism,cardiac function,cardiac morphology,and myocardial ultrastructure in GK rats were assessed.RNA sequencing was utilized to analyze differential gene expression and identify potential therapeutic targets.In vitro experiments involved high glucose to induce apoptosis and inflammation in H9c2 cells.Cell viability was evaluated using CCK-8 assay,apoptosis was monitored via flow cytometry,and the production of inflammatory cytokines was measured using quantitative real-time PCR(qPCR)and ELISA.Protein expression levels were determined by Western blotting analysis.The investigation also incorporated the use of MAPK inhibitors to further elucidate the mechanism at both the transcriptional and protein levels.Results The JPQHF group exhibited significant reductions in interventricular septal thickness at end-systole(IVSs)and left ventricular internal diameter at end-systole and end-diastole(LVIDs and LVIDd).JPQHF effectively suppressed high glucose-induced activation of IL-1βand caspase 3 in cardiomyocytes.Furthermore,JPQHF downregulated

关键词： Jianpi qinghua formula diabetic cardiomyopathy AP-1 transcription factor apoptosis inflammation