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Chinese Journal of Polymer Science 2024年第5期42卷 570-578,I0005页

作者： Xiao-Fei Sun Xu Zha.g Shu-Ping song Ya-Qun Yao Yan Zha.g Cheng-Liang Wang Jing-Jiang Sun qing-Fu Wang Key Laboratory of Rubber-plastics Ministry of EducationSchool of Polymer Science and EngineeringQingdao University of Science and TechnologyQingdao266042China qingdao Research Academy of Environmental Science Qingdao266012China

L-glutamic acid(LA)is a bio-based,non-toxic,environmentally friendly material derived from *** present study reports the application of Passerini three-component polymerization(P-3CP)for the straightforward preparation of LA-based light-responsive polyesters(PLTDs)under mild *** with molar masses up to 8500 g/mol and high yields exceeding 90%are *** chemical structures and light-responsive self-immolative beha.ior of PLTDs are comprehensively cha.acterized by employing ultraviolet-visible(UV-Vis)spectroscopy,size exclusion chromatography(SEC),nuclear magnetic resonance(NMR)spectroscopy,and liquid chromatography mass spectrometry(LC-MS).Meanwhile,monodisperse PLTD-based doxorubicin-loaded nanoparticles(PLTD-DOX-NP)(size=193 nm,PDI=0.018)are formulated by nanoprecipitation *** light-induced depolymerization,the PLTD-DOX-NP undergoes rapid decomposition,resulting in a burst release of 80%cargo within 13 ***,according to biological toxicity tests,the PLTD-NP possesses adequate biosafety,both before and after ***,the incorporation of P-3CP with biorenewable LA-based monomer adheres to the principles of green chemistry,significantly simplifying the synthetic pathway of light-responsive polymers.

关键词： L-glutamic acid Passerini three-component polymerization Light-responsive Polyester Nanoparticles

Rational design multi-color-emissive chemiluminescent carbon nanodots in a single solvothermal reaction

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Nano Research 2024年第6期17卷 4651-4660页

作者： Guang-song Zheng Cheng-Long Shen Yuan Deng Kai-Kai Liu Jin-ha. Zang Lin Dong qing Lou Chong-Xin Sha. Henan Key Laboratory of Diamond Optoelectronic Materials and Devices Key Laboratory of Materials PhysicsMinistry of Educationand School of Physics and MicroelectronicsZhengzhou UniversityZhengzhou 450052China

Recently,the chemiluminescence(CL)induced by carbon nanodots(CDs)ha. intrigued researchers’extensive interests in various applications due to its special light emission ***,the difficulty of synthesizing chemiluminescent CDs with full-spectrum emission severely hinders the further regulation of the CL emission ***,the multi-color-emissive chemiluminescent CDs are rational designed and further synthesized by regulating the sp2-hybrid core and sp3-hybrid surface from the citrate-ammonia molecular in a single solvothermal *** experimental cha.acterizations and density functional theory calculations reveal tha. the higher temperature can promote the crosslinking polymerization/carbonization of carbon core and the higher protonation of solvent can determine the core size of final CDs,resulting in the variant CL emission from molecular-,crosslinking-and ***,the CL emission of the CDs can be further synthesized by tuning the luminescence chromophores in the formation process via regulating the temperature and solvent,enabling the applications of the CL CDs in illumination and information *** study paves a new technology to understand the luminescence of CDs and affords an industry translational potential over traditional chemiluminescent molecular.

关键词： carbon nanodots chemiluminescence regulation energy level alignment mecha.ism

Enrichment of Chemical Element ^(7)Li in the Rotating Red Clump Star

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Chinese Physics Letters 2024年第8期41卷 121-125页

作者： Fang-Wen Wu ha.-Feng song qing-Li Li Yun He Xin-Yue Qu Zhuo ha. College of Physics Guizhou UniversityGuiyang 550025China Geneva Observatory University of GenevaCH-1290 SauvernySwitzerland

About 2 percent of red clump stars are found to be the lithium-rich and thus the surface lithium increases obviously in some red clump *** physical mecha.ism of the lithium enrichment in these stars ha. not yet been explained satisfactorily by the evolutionary models of single *** flash induced internal gravity wave mixing(i.e.,IGW)could play a primary role in explaining the red clump star with lithium enrichment and it ha. a very significant impact on the internal structure and surface compositions of a *** can significantly increase the mixing efficiency of the internal gravity wave because the timescale for the enrichment event ha. been *** mixing can explain the observed beha.ior of lithium on red giant stars tha. are more luminosity tha. the RGB ***,it ha. a very small effect on the diffusion of elements because its diffusion coefficient is much smaller tha. the one of IGW induced mixing after the core helium flash.

关键词： flash stars lithium

Development of a scintillating-fiber-based beam monitor for the coherent muon-to-electron transition experiment

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Nuclear Science and Techniques 2024年第4期35卷 156-164页

作者： Yu Xu Yun-song Ning Zhi-Zhen Qin Yao Teng Cha.g-qing Feng Jian Tang Yu Chen Yoshinori Fukao Satoshi Miha.a Kou Oishi School of Physics Sun Yat-sen UniversityGuangzhou 510275China State Key Laboratory of Particle Detection and Electronics University of Science and Technology of ChinaHefei 230026China Department of Modern Physics University of Science and Technology of ChinaHefei 230026China High Energy Accelerator Research Organization(KEK) Ibaraki 305‑0801Japan Department of Physics Imperial College LondonLondon SW72AZUK

The coherent muon-to-electron transition(COMET)experiment is a leading experiment for the coherent conversion of μ^(-)N→e^(-)N using a high-intensity pulsed muon beamline,produced using innovative slow-extraction ***,it is critical to measure the muon beam *** set up a muon beam monitor(MBM),where scintillating fibers woven in a cross sha.e were coupled to silicon photomultipliers to measure the spatial profile and timing structure of the extracted muon beam for the *** MBM detector was tested successfully with a proton beamline at the China Spallation Neutron Source and took data with good performance in the commissioning *** development of the MBM,including its mecha.ical structure,electronic readout,and beam measurement results,are discussed.

关键词： Beam instrumentation Profile monitor Scintillating fiber Silicon photomultipliers

Co-occurrence of per- and polyfluoroalkyl substances, heavy metals and polycyclic aromatic hydrocarbons and their composite impacts on microbial consortium in soil: A field study

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Pedosphere 2024年第4期34卷 736-748页

作者： Meng Zha.G qing WANG Xin song Mukhtiar ALI Zhiwen TANG Xin LIU Zhuanxia Zha.G Shurong MA Jinhui BI Zhongyuan LI Key Laboratory of Saline-Alkali Vegetation Ecology Restoration Northeast Forestry UniversityHarbin 150040China Key Laboratory of Soil Environment and Pollution Remediation Institute of Soil ScienceChinese Academy of SciencesNanjing 210008China University of Chinese Academy of Sciences Beijing 100049China Center International Group Co. Ltd.Beijing 101160China China Construction Eighth Engineering Division Corp. Ltd.Shanghai 200122China

This is the first study to report the co-occurrence of per-and polyfluoroalkyl substances(PFASs),heavy metals,and polycyclic aromatic hydrocarbons(PAHs)and their impacts on the native microbial consortium in soil due to the long-term *** PFASs,heavy metals,and PAHs were detected in soil samples collected at 2–6 m below the ground surface at different sampling locations in a steel-making *** total concentrations of PFASs varied from 6.55 to 19.79 ng g^(-1),with perfluorooctane sulfonate(PFOS),perfluorobutane sulfonate,and 6:2 chlorinated polyfluorinated ether sulfonate(alternative of PFOS)being the predominant *** concentrations of arsenic,cadmium,and lead were detected in the ranges of 4.40–1270.00,0.01–8.67,and 18.00–647.00 mg kg^(-1),respectively,and the concentration of total PAHs was detected in the range of 1.02–131.60 mg kg^(-1).The long-term exposure to mixed contaminants of PFASs,heavy metals,and PAHs led to lower richness and diversity of microbial communities in *** soil bacterial communities were mainly composed of Pseudomonas,norank_p_GAL15,Leptothrix,norank_o_Rokubacteriales,and *** between soil environmental factors and microbial communities indicated tha. cation excha.ge capacity and total phosphorus were two key factors in sha.ing the composition of native microbial ***,Arthrobacter,Leptothrix,and Sphingobium were found to be significantly positively correlated with PFAS concentrations,indicating tha. these genera could tolerate the stress exerted by PFASs,along with the stress imposed due to the presence of heavy metals or/and PAHs.

关键词： arsenic cation excha.ge capacity mixed contaminant native microbial community perfuorooctane sulfonate total phosphorus

Phosphorus-silicon-integrated electrolyte additive boosts cycling performance and safety of high-voltage lithium-ion batteries

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Chinese Chemical Letters 2024年第8期35卷 418-424页

作者： Mei-Chen Liu qing-song Liu Yi-Zhou Quan Jia-Ling Yu Gang Wu Xiu-Li Wang Yu-Zhong Wang The Collaborative Innovation Center for Eco-Friendly and Fire-Safety Polymeric Materials(MoE) National Engineering Laboratory of Eco-Friendly Polymeric Materials(Sichuan)State Key Laboratory of Polymer Materials EngineeringCollege of ChemistrySichuan UniversityChengdu 610064China

Safety and energy density are significant for lithium-ion batteries(LIBs),and the flammable organic elec-trolyte is one of the most critical causes of the safety problem of *** LiNi0.8 Co 0.1 Mn 0.1 O 2(NCM811)cathode with high capacity can improve the energy density,the interface stability between NCM811 cathode and electrolytes needs to be ***,we report a multifunctional additive,diethyl(2-(triethoxysilyl)ethyl)phosphonate(DETSP),which can suppress the flammability of the elec-trolyte and enha.ce the cycling stability of NCM811 cathode with a capacity retention of 89.9%after 400 cycles at 1 C,while tha. of the blank electrolyte is merely 61.3%.In addition,DETSP is compati-ble well with the graphite anode without impairing the electrochemical ***,the performance and safety of NCM811/graphite full cells are also *** and theoretical re-sults demonstrate tha. DETSP can scavenge acidic byproducts and is beneficial to form a stable cathode-electrolyte interface(CEI).Accordingly,DETSP can potentially be an effective solution to ameliorating the safety of the commercial electrolyte and improving the stability of high-voltage cathodes.

关键词： Electrolyte additive NCM Lithium-ion batteries Safety Cathode-electrolyte interface

Enha.ced Electrical Properties of Styrene-grafted Polypropylene Insulation for Bulk Power Transmission HVDC Cables

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 361-370页

作者： ha. Yuan Shixun Hu Yao Zhou Cha. Yuan Wenbo song qing Sha. Hongwei Shi Juan Li Jun Hu Qi Li Jinliang He SINOPEC Beijing Research Institute of Chemical Industry Beijing 100013China State Key Laboratory of Power Systems Department of Electrical EngineeringTsinghua UniversityBeijing 100084China

Polypropylene(PP)is considered to be a rather promising material for HVDC cable *** modification ha. proved to be an effective method on the electrical property improvements of *** paper reports on the highlyenha.ced electrical properties of styrene-grafted polypropylene(PP-g-St)and their related *** influence of grafting styrene on crystallization structures,thermal properties and electrical properties of PP-g-St are cha.acterized and *** results show tha. PP-g-St exhibits remarkably enha.ced DC volume resistivity,suppressed space cha.ge accumulation and improved DC breakdown strengths as compared to *** observation shows PP-g-St ha. small,imperfect spherulites with indistinct boundaries,which is strongly correlated to enha.ced electrical *** study provides an effective grafting strategy to design high-performance HVDC cable insulation materials for bulk power transmission systems.

关键词： Electrical properties grafting modification polypropylene styrene

Sensitive humidity sensor based on moisture-driven energy generation

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Nano Research 2024年第6期17卷 5578-5586页

作者： qingcha. Ni qing Lou Chenglong Shen Guangsong Zheng Runwei song Jingnan ha. Jialu Liu Jinyang Zhu Jinha. Zang Lin Dong Chong-Xin Sha. Henan Key Laboratory of Diamond Optoelectronic Materials and Devices Key Laboratory of Materials PhysicsMinistry of Educationand School of Physics and MicroelectronicsZhengzhou UniversityZhengzhou 450052China State Centre for International Cooperation on Designer Low-Carbon&Environmental Materials and School of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China

The emergence of novel self-powered humidity sensors ha. attracted considerable attention in the fields of smart electronic devices and personal ***,self-powered humidity sensors ha.e been fabricated using a moisture-driven energy generation(MEG)device based on asymmetric tubular graphitic carbon nitride(g-CN)films prepared on anodized aluminum(AAO)*** a relative humidity(RH)of 96%,the MEG device can provide an open-circuit voltage of 0.47 V and a short-circuit current of 3.51μA,with a maximum output power of 0.08μ*** inherent self-powered ability and humidity response via current variation,an extraordinary response of 1.78×106%(41%-96%RH)can be gained from the MEG *** possible power generation mecha.ism is tha. g-CN/AAO heterostructure can form ion gradient and diffusion under the action of moisture to convert chemical potential into electrical potential,evoking a connaturally sensitive response to ***-powered respiration monitoring device based on the sensor is designed to monitor human movement(sitting,warming up,and running)and sleep status(normal,snoring,and apnea),maintaining excellent stability during cumulative 12-h respiration *** self-powered humidity sensing technology ha. promising potential for extensive integration into smart electronic and round-the-clock health monitoring devices.

关键词： graphitic carbon nitride moisture-driven energy generation humidity sensor respiration monitoring

Disruption of cyclin D1 degradation leads to the development of mantle cell lymphoma

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Acta Pha.maceutica Sinica B 2024年第7期14卷 2977-2991页

作者： Ke Lu Ming Zha.g Hongyu Qin Siyu Shen ha.qing song Hua Jiang Chunxiang Zha.g Guozhi Xiao Liping Tong qing Jiang Di Chen Research Center for Computer-aided Drug Discovery Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China Faculty of Pha.maceutical Sciences Shenzhen Institute of Advanced TechnologyShenzhen 518055China Oncology Department Johns Hopkins University School of MedicineBaltimoreMD 21205USA Division of Spine Surgery the First Affiliated Hospital of Guangxi Medical UniversityNanning 530021China Division of Sports Medicine and Adult Reconstructive Surgery Department of Orthopedic SurgeryNanjing Drum Tower HospitalAffiliated Hospital of Medical SchoolState Key Laboratory of Pharmaceutical BiotechnologyNanjing UniversityNanjing 210008China Wenzhou Institute University of Chinese Academy of SciencesWenzhou 325000China Department of Cardiology Basic Medicine Innovation Center for Cardiometabolic Diseases of Ministry of EducationInstitute of Cardiovascular Researchthe Affiliated HospitalSouthwest Medical UniversityLuzhou 646000China School of Medicine Southern University of Science and TechnologyShenzhen 518055China

Cyclin D1 ha. been recognized as an oncogene due to its abnormal upregulation in different types of ***,we demonstrated tha. cyclin D1 is SUMOylated,and we identified Itch as a specific E3 ligase recognizing SUMOylated cyclin D1 and mediating SUMO-induced ubiquitination and proteasome degradation of cyclin *** generated cyclin D1 mutant mice with mutations in the SUMOylation site,phosphorylation site,or both sites of cyclin D1,and found tha. double mutant mice developed a Mantle cell lymphoma(MCL)-like *** showed tha. arsenic trioxide(ATO)enha.ces cyclin D1 SUMOylation-mediated degradation through inhibition of cyclin D1 deSUMOylation enzymes,leading to MCL cell *** of severe combined immunodeficiency(SCID)mice grafted with MCL cells with ATO resulted in a significant reduction in tumor *** this study,we provide novel insights into the mecha.isms of MCL tumor development and cyclin D1 regulation and discover a new strategy for MCL treatment.

关键词： Cyclin D1 SUMOylation Mantle cell lymphoma Arsenic trioxide SENP2 Proteasome degradation

Pachymic acid exerts antitumor activities by modulating the Wnt/β-catenin signaling pathway via targeting PTP1B

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Asian Pacific Journal of Tropical Biomedicine 2024年第4期14卷 170-180页

作者： ha. Zha.g Kun Zhu Xue-Feng Zha.g Yi-Hui Ding Bing Zhu Wen Meng qing-song Ding Fan Zha.g Department of Emergency Affiliated Hangzhou First People’s HospitalZhejiang University School of MedicineHangzhou 310006ZhejiangChina Department of Cardiothoracic Surgery The Third Affiliated Hospital of Qiqihar Medical CollegeQiqihar 161000HeilongjiangChina Department of Cardiothoracic Surgery The Affiliated Heilongjiang Provincial Hospital of Harbin Institute of TechnologyHarbin 150036HeilongjiangChina

Objective:To determine the inhibitory effects of pachymic acid on lung adenocarcinoma(LUAD)cells and elucidate its underlying ***:CCK-8,wound healing,Transwell,Western blot,tube formation,and immunofluorescence assays were carried out to measure the effects of various concentrations of pachymic acid on LUAD cell proliferation,metastasis,angiogenesis as well as ***,molecular docking technology was used to detect the potential targeted binding association between pachymic acid and protein tyrosine phospha.ase 1B(PTP1B).Moreover,PTP1B was overexpressed in A549 cells to detect the specific mecha.isms of pachymic ***:Pachymic acid suppressed LUAD cell viability,metastasis as well as angiogenesis while inducing cell *** also targeted PTP1B and lowered PTP1B ***,PTP1B overexpression reversed the effects of pachymic acid on metastasis,angiogenesis,and autopha.y as well as the expression of Wnt3a andβ-catenin in LUAD ***:Pachymic acid inhibits metastasis and angiogenesis,and promotes autopha.y in LUAD cells by modulating the Wnt/β-catenin signaling pathway via targeting PTP1B.

关键词： Pachymic acid Lung adenocarcinoma Protein tyrosine phospha.ase 1B Wnt/β-catenin signaling pathway Metastasis Angiogenesis Autopha.y