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Magnetron sputtered nickel oxide with suppressed interfacial defect states for efficient inverted perovskite solar cells

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Journal of Energy Chemistry 2025年第1期100卷 348-355页

作者： Guoqiang Ma qin Tan Zhaoning li Jingwei Xiu Jiafeng Wang Tianle Cheng Dong He Qiang Sun Xuhang Ma Francesco Lamberti Zhubing He Department of Materials Science and Engineering Institute of Innovative Materials (I2M) Shenzhen Key Laboratory of Full Spectral Solar Electricity Generation (FSSEG)Southern University of Science and Technology (SUSTech) Core Research Facilities Southern University of Science and Technology Department of Chemical Sciences Department of Industrial Engineering University of Padova

Widely used spin-coated nickle oxide （NiOx） based perovskite solar cells often suffer from severe interfacial reactions between the NiOxand adjacent perovskite layers due to surface defect states,which inherently impair device performance in a long-term view,even with surface molecule *** this study,we developed high-quality magnetron-sputtered NiOxthin films through detailed process optimization,and compared systematically sputtered and spin-coated NiOxthin film surfaces from materials to *** sputtered NiOxfilms exhibit improved crystallinity,smoother surfaces,and significantly reduced Ni3+or Ni vacancies compared to their spin-coated ***,the interface between the perovskite and sputtered NiOxfilm shows a substantially reduced density of defect *** solar cells （PSCs） fabricated with our optimally sputtered NiOxfilms achieved a high power conversion efficiency （PCE） of up to 19.93%and demonstrated enhanced stability,maintaining 86.2% efficiency during 500 h of maximum power point tracking under one standard sun ***,with the surface modification using (4-(2,7-dibromo-9,9-dimethylacridin-10（9H）-yl)butyl)p hosphonic acid （DMAcPA）,the device PCE was further promoted to 23.07%,which is the highest value reported for sputtered NiOxbased PSCs so far.

关键词： Nickle oxide Magnetron sputter Defect Stability Perovskite solar cell

High‑Entropy Electrode Materials:Synthesis,Properties and Outlook

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Nano-Micro Letters 2025年第1期17卷 472-506页

作者： Dongxiao li Chang liu Shusheng Tao Jieming Cai Biao zhong Jie li Wentao Deng Hongshuai Hou Guoqiang Zou Xiaobo Ji College of Chemistry and Chemical Engineering Central South UniversityChangsha 410083People’s Republic of China School of Chemistry and Chemical Engineering Hunan Institute of EngineeringXiangtan 411104People’s Republic of China

High-entropy materials represent a new category of high-performance materials,first proposed in 2004 and extensively investigated by researchers over the past two *** definition of high-entropy materials has continuously *** the last ten years,the discovery of an increasing number of high-entropy materials has led to significant advancements in their utilization in energy storage,electrocatalysis,and related domains,accompanied by a rise in techniques for fabricating high-entropy electrode ***,the research emphasis has shifted from solely improving the performance of high-entropy materials toward exploring their reaction mechanisms and adopting cleaner preparation ***,the current definition of high-entropy materials remains relatively vague,and the preparation method of high-entropy materials is based on the preparation method of single metal/low-or medium-entropy *** should be noted that not all methods applicable to single metal/low-or medium-entropy materials can be directly applied to high-entropy *** this review,the definition and development of high-entropy materials are briefly ***,the classification of high-entropy electrode materials is presented,followed by a discussion of their applications in energy storage and catalysis from the perspective of synthesis ***,an evaluation of the advantages and disadvantages of various synthesis methods in the production process of different high-entropy materials is provided,along with a proposal for potential future development directions for high-entropy materials.

关键词： High-entropy Energy storage Electrode materials

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第14届世锦赛中国女篮实力分析

延边大学学报（自然科学版） 2005年第1期31卷 67-70页

作者：孙继新秦立忠延边大学体育学院吉林延吉133002

根据第14届世界女篮锦标赛相关技术统计数据,结合中国女篮的表现,对中国女篮的比赛能力进行分析,客观地评价其优势与不足,并提出相应的对策和建议,为今后的训练和比赛提供参考.

关键词：中国女篮实力分析对策

The Citron homology domain of MAP4Ks improves outcomes of traumatic brain injury

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Neural Regeneration Research 2025年第11期20卷 3233-3244页

作者： Xiaoling zhong Wenjiao Tai Meng-Lu liu Shuaipeng Ma Tianjin Shen Yuhua Zou Chun-li Zhang Department of Molecular Biology University of Texas Southwestern Medical CenterDallasTXUSA Hamon Center for Regenerative Science and Medicine University of Texas Southwestern Medical CenterDallasTXUSA Peter O’Donnell Jr.Brain Institute University of Texas Southwestern Medical CenterDallasTXUSA

The mitogen-activated protein kinase kinase kinase kinases(MAP4Ks)signaling pathway plays a pivotal role in axonal regrowth and neuronal degeneration following *** targeting this pathway is beneficial to brain injury remains *** this study,we showed that adeno-associated virus-delivery of the Citron homology domain of MAP4Ks effectively reduces traumatic brain injury-induced reactive gliosis,tauopathy,lesion size,and behavioral *** inhibition of MAP4Ks replicated the ameliorative effects observed with expression of the Citron homology ***,the Citron homology domain acted as a dominant-negative mutant,impeding MAP4K-mediated phosphorylation of the dishevelled proteins and thereby controlling the Wnt/β-catenin *** findings implicate a therapeutic potential of targeting MAP4Ks to alleviate the detrimental effects of traumatic brain injury.

关键词： adeno-associated virus Citron homology Citron homology domain gene therapy mitogen-activated protein kinase kinase kinase kinases traumatic brain injury

树、单圈图和双圈图改进的第二Zagreb指标（英文）

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曲阜师范大学学报（自然科学版） 2017年第4期43卷 15-20页

作者：秦忠芳袁利赵飚新疆大学数学与系统科学学院新疆维吾尔自治区乌鲁木齐市830046

文章采用了类似Ji s等(2014)的方法,研究了树、单圈图、双圈图的改进的第二Zagreb指标,通过四个图变换(其中图变换1,2是严格增该指标的变换,图变换3,4是严格减该指标的变换)严格论证,分别得出了树、单圈图、双圈图的极大极小值.

关键词：改进的第二Zagreb指标树单圈图双圈图图变换

Porous Organic Cage‑Based Quasi‑Solid‑State Electrolyte with Cavity‑Induced Anion‑Trapping Effect for Long‑life lithium Metal Batteries

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Nano-Micro Letters 2025年第2期17卷 376-386页

作者： Wei-Min qin zhongliang li Wen‑Xia Su Jia‑Min Hu Hanqin Zou Zhixuan Wu Zhiqin Ruan Yue‑Peng Cai Kang li Qifeng Zheng School of Chemistry South China Normal UniversityGuangzhou 510006People’s Republic of China Key Laboratory of Functional Metal‑Organic Compounds of Hunan Province College of Chemistry and Material ScienceHengyang Normal UniversityHengyang 421008People’s Republic of China Guangzhou Key Laboratory of Energy Conversion and Energy Storage Materials Guangzhou 510006People’s Republic of China

Porous organic cages(POCs)with permanent porosity and excellent host–guest property hold great potentials in regulating ion transport behavior,yet their feasibility as solid-state electrolytes has never been testified in a practical ***,we design and fabricate a quasi-solid-state electrolyte(QSSE)based on a POC to enable the stable operation of li-metal batteries(LMBs).Benefiting from the ordered channels and cavity-induced anion-trapping effect of POC,the resulting POC-based QSSE exhibits a high li+transference number of 0.67 and a high ionic conductivity of 1.25×10^(−4) S cm^(−1) with a low activation energy of 0.17 *** allow for homogeneous li deposition and highly reversible li plating/stripping for over 2000 *** a proof of concept,the LMB assembled with POC-based QSSE demonstrates extremely stable cycling performance with 85%capacity retention after 1000 ***,our work demonstrates the practical applicability of POC as SSEs for LMBs and could be extended to other energy-storage systems,such as Na and K batteries.

关键词： Porous organic cage Cavity-induced anion-trapping Quasi-solid-state electrolyte Homogeneous li+flux lithium metal battery

光果甘草与乌拉尔甘草开花与传粉方式对生殖及种间关系的影响

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西北植物学报 2012年第10期32卷 2004-2008页

作者：田润炜陆嘉惠谢良碧秦忠立李学禹石河子大学生命科学学院新疆石河子832003 新疆兵团绿洲生态农业重点实验室新疆石河子832003 石河子大学甘草研究所新疆石河子832003

通过对光果甘草和乌拉尔甘草花期物候和访花昆虫行为的观察及人工授粉实验,探讨开花模式及传粉方式对生殖成功及种间关系的影响。结果表明:(1)两种甘草的种群水平花期重叠时间长达21d,均表现出"集中大量开花"模式,但乌拉尔甘草呈现分批... 详细信息

通过对光果甘草和乌拉尔甘草花期物候和访花昆虫行为的观察及人工授粉实验,探讨开花模式及传粉方式对生殖成功及种间关系的影响。结果表明:(1)两种甘草的种群水平花期重叠时间长达21d,均表现出"集中大量开花"模式,但乌拉尔甘草呈现分批渐次开花趋势,这对提高生殖成功率,避免近交衰退,维持物种的稳定具有重要意义。(2)两种甘草的访花昆虫在种类和数量上有所不同,但具有共同传粉者——宽板尖腹蜂、意大利蜂和紫木蜂。(3)以乌拉尔甘草为母本、光果甘草为父本的种间杂交结实率为48.3%;以光果甘草为母本、乌拉尔甘草为父本的种间杂交结实率为39.4%,说明种间杂交亲和,不存在生殖障碍。研究认为,花期重叠、共有传粉昆虫及种间杂交亲和使光果甘草与乌拉尔甘草自然种群杂交种的形成成为可能。

关键词：甘草属开花模式传粉方式生殖成功种间关系

滴灌种植药用甘草对盐碱地土壤微生物及盐分的影响

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新疆农业科学 2012年第10期49卷 1920-1925页

作者：秦忠立陆嘉惠陆爽田中平阎平包芳石河子大学生命科学学院新疆石河子832000

【目的】研究滴灌种植胀果甘草和乌拉尔甘草对盐碱地土壤微生物及盐分的影响。【方法】设置4种种植处理(无处理对照组,深耕(40～60 cm)+沙子(3～5 cm),深耕+沙子+胀果甘草,深耕+沙子+乌拉尔甘草),每一处理4 m×4 m,3个随机重复,共占地19... 详细信息

【目的】研究滴灌种植胀果甘草和乌拉尔甘草对盐碱地土壤微生物及盐分的影响。【方法】设置4种种植处理(无处理对照组,深耕(40～60 cm)+沙子(3～5 cm),深耕+沙子+胀果甘草,深耕+沙子+乌拉尔甘草),每一处理4 m×4 m,3个随机重复,共占地192 m^2,对滴灌一年后的各处理土壤进行测定。【结果】种植乌拉尔甘草处理土壤电导率亦显著下降(P<0.05);乌拉尔甘草种植土壤微生物在不同土层种植前后差异显著(P<0.05)。【结论】土壤盐分的降低可能是因为庞大根系的生长改善了土壤的结构和渗透性能,从而明显降低了土壤积返盐的速度。随着土壤盐分的降低,土壤微生物的数量也显著改变。总之,种植盐生植物既改变了土壤的盐分,又改变了土壤的微生物群落组成,从而对土壤肥力、理化性质产生影响。

关键词：滴灌甘草盐碱地土壤微生物盐分

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关于维生素C大剂量静脉给药问题的讨论

儿科药学杂志 2006年第2期12卷 64-64,I0001页

作者：秦立忠胡晓红河南省开封市儿童医院河南开封475000

目前临床应用VitC(VC)静脉给药治疗某些疾病越来越多,如大剂量用于治疗克山病心源性休克、亚硝酸盐中毒和病毒性心肌炎、缺氧缺血性脑病、多器官功能衰竭等的辅助治疗等,尚有将VC广泛、大量地应用于许多效果并未得到证实的疾病,且为1次/... 详细信息

目前临床应用VitC(VC)静脉给药治疗某些疾病越来越多,如大剂量用于治疗克山病心源性休克、亚硝酸盐中毒和病毒性心肌炎、缺氧缺血性脑病、多器官功能衰竭等的辅助治疗等,尚有将VC广泛、大量地应用于许多效果并未得到证实的疾病,且为1次/d大剂量静脉给药。根据VC的药理作用和药动学规律,大剂量临床给药争议颇多,许多问题尚无定论,有待进一步研究和临床验证。本文旨在对目前临床及某些文献中的一些用法提出意见或建议,供大家讨论。1剂量过大缺乏依据人体VC的需要量,就其缺乏而言,每日补充100￣300 mg已足。尽管VC的消耗量随其体内的饱和程度而增加,对VC饱和者,每日消耗VC仅1.4￣1.8mg/kg。VC体内储存能力有限,总量约为2 500 mg(成人),血浆含量平均约为14μg/mL[1]。目前儿科临床中常用静脉给药剂量几乎均在100 mg/(kg·d)以上,常常1次给予,因此,给药后血浆中VC的含量约为其正常浓度的50倍以上,即使VC缺乏患者,以此剂量首次给药后亦已满足机体组织细胞储存并超过其血浆饱和度(1.4 mg/100 mL),故再给予则大部分自尿中排出[2]。笔者临床研究发现,以100 mg/kg剂量给药,...

关键词：静脉给药治疗大剂量维生素C 缺氧缺血性脑病多器官功能衰竭病毒性心肌炎亚硝酸盐中毒临床应用心源性休克辅助治疗