检索结果-南通市图书馆

Proton‑Prompted Ligand Exchange to Achieve High‑Efficiency CsPbI_(3) Quantum Dot Light‑Emitting Diodes

在线全文

学校读者我要写书评

暂无评论

Nano-Micro Letters 2024年第6期16卷 53-62页

作者： Yanming Li Ming Deng Xuanyu Zhang Lei qian Chaoyu xiang Laboratory of Advanced Nano‑Optoelectronic Materials and Devices Qianwan Institute of CNITECHNingbo 315300People’s Republic of China Division of Functional Materials and Nanodevices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201People’s Republic of China Zhejiang Provincial Engineering Research Center of Energy Optoelectronic Materials and Devices Ningbo Institute of Materials Technology&EngineeringChinese Academy of SciencesNingbo 315201People’s Republic of China Faculty of Electrical Engineering and Computer Science Ningbo UniversityNingbo 315211ZhejiangPeople’s Republic of China University of Nottingham Ningbo China Ningbo 315100People’s Republic of China

CsPbI_(3)perovskite quantum dots(QDs)are ideal materials for the next generation of red light-emitting ***,the low phase stability of CsPbI_(3)QDs and long-chain insulating capping ligands hinder the improvement of device *** in-situ ligand replacement and ligand exchange after synthesis were often difficult to ***,we proposed a new ligand exchange strategy using a proton-prompted insitu exchange of short 5-aminopentanoic acid ligands with long-chain oleic acid and oleylamine ligands to obtain stable small-size CsPbI_(3)*** exchange strategy maintained the size and morphology of CsPbI_(3)QDs and improved the optical properties and the conductivity of CsPbI_(3)QDs *** a result,high-efficiency red QD-based light-emitting diodes with an emission wavelength of 645 nm demonstrated a record maximum external quantum efficiency of 24.45%and an operational half-life of 10.79 h.

关键词： CsPbI_(3) perovskite quantum dots Light-emitting diodes Ligand exchange Proton-prompted in-situ exchange

Deformation mechanism and limit support pressure of cutting steel plate during connection between pipes in large spacing using pipe curtain structure method

在线全文

学校读者我要写书评

暂无评论

Underground Space 2024年第5期18卷 83-96页

作者： xiang Liu Rui Zhang Jun Huang Guang Zhao qian Fang Annan Jiang Liaoning Key Laboratory of Marine Environmental Bridge and Tunnel Engineering Dalian Maritime UniversityDalian 116026China JSTI Group Nanjing 210017China Key Laboratory for Urban Underground Engineering of Ministry of Education Beijing Jiaotong UniversityBeijing 100044China

The pipe curtain structure method(PSM)is a novel construction method to control ground deformation *** with the traditional pipe-roofing and pipe jacking method,the connection between pipes in large spacings using PSM is widely acknowledged as a unique construction *** study on this connection procedure is needed to resolve similar cases in that the pipes are inevitably constructed on both sides of existing *** the steel plate during the connection procedure is the first step,which is crucial to control the safety and stability of the surrounding environment and existing *** deformation mechanism and limit support pressure of the cutting steel plate during the connection between pipes in large spacings are studied in this paper,relying on the undercrossing Yifeng gate tower project of Jianning West Road River Crossing Channel in Nanjing,China.A modified 3D wedge-prism failure model is proposed using the 3D discrete element *** with Terzaghi loose earth pressure theory and the limit equilibrium theory,the analytical solutions for the limit support pressure of the excavation face of the cutting steel plate are *** modified 3D wedge-prism failure model and corresponding analytical solutions are categorised into two cases:(a)unilateral cutting scheme,and(b)bilateral cutting *** analytical solutions for the two cases are verified from the numerical simulation and in-situ data and compared with the previous *** comparative analysis between the unilateral and bilateral cutting schemes indicates that the bilateral cutting scheme can be adopted as a *** bilateral cutting scheme saves more time and induces less ground deformation than the unilateral one due to the resistance generated from the superimposed *** addition,the parametric sensitivity analysis is carried out using an orthogonal experimental *** main influencing factors arranged from high to low are the pipe sp

关键词： Pipe curtain structure method Wedge-prism failure model Limit support pressure Discrete element method Connection between pipes

Post-traumatic cauda equina nerve calcification:A case report

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

World Journal of Clinical Cases 2023年第6期11卷 1356-1364页

作者： Yan-Dong Liu qiang Deng Jun-Jie Li Hai-Yun Yang Xian-Fu Han Kai-Dong Zhang Ran-Dong Peng qian-qian xiang Graduate School Gansu University of Traditional Chinese MedicineLanzhou 730000Gansu ProvinceChina Spinal Disease Diagnosis and Treatment Center Gansu Provincial Hospital of Traditional Chinese MedicineLanzhou 730050Gansu ProvinceChina First Orthopedic Department Lanzhou Traditional Chinese Medicine Orthopedic HospitalLanzhou 730050Gansu ProvinceChina Department of Osteomyelitis Gansu Provincial Hospital of Traditional Chinese MedicineLanzhou 730000Gansu ProvinceChina

BACKGROUND Post-traumatic cauda equina nerve calcification is extremely rare in clinical practice,and its etiology,pathogenesis,treatment and prognosis are *** are few studies and reports on Post-traumatic cauda equina nerve calci-fication,and this review reports a case of Post-traumatic cauda equina nerve calcification for *** SUMMARY A 52-year-old patient presented to our hospital with a history of lumbar spinal stenosis and a lumbar vertebral fracture caused by *** patient's right lower limb had weakness in hip flexion,knee extension and plantarflexion with muscle strength grade 3,right ankle dorsiflexion and thumb dorsiflexion with muscle strength grade *** patient's skin sensation below the right knee plane *** patient's Computed tomography(CT)data showed signs of cauda equina nerve calcification and the terminal filaments in the plane of the third to fifth lumbar *** treatment the patient's symptoms were slightly *** We provide an extremely rare case of Post-traumatic cauda equina nerve calcification and offer a conservative treatment ***,the etiology,mechanism and treatment of Post-traumatic cauda equina nerve calcification are still *** requires scholars to conduct more research and exploration in this area.

关键词： Post-traumatic Calcification Cauda equina nerve Spinal Cord Injury Case report

Root-derived long-distance signals trigger ABA synthesis and enhance drought resistance in Arabidopsis

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Genetics and Genomics 2024年第7期51卷 749-761页

作者： qian-qian Liu Jin-Qiu Xia Jie Wu Yi Han Gui-Quan Zhang Ping-Xia Zhao Cheng-Bin xiang Division of Life Sciences and Medicine Division of Molecular&Cell BiophysicsHefei National Science Center for Interdisciplinary Sciences at the MicroscaleUniversity of Science and Technology of ChinaThe Innovation Academy of Seed DesignChinese Academy of SciencesHefeiAnhui 230027China College of Life Sciences Anhui Agricultural UniversityHefeiAnhui 230036China College of Agronomy South China Agricultural UniversityGuangzhouGuangdong 510642China School of Biology and Basic Medical Sciences Soochow UniversitySuzhouJiangsu 215123China

Vascular plants have evolved intricate long-distance signaling mechanisms to cope with environmental stress,with reactive oxygen species(ROS)emerging as pivotal systemic signals in plant stress ***,the exact role of ROS as root-to-shoot signals in the drought response has not been *** this study,we reveal that compared with wild-type plants,ferric reductase defective 3(frd3)mutants exhibit enhanced drought resistance concomitant with elevated NINE-CIS-EPOXYCAROTENOID DIOXYGENASE 3(NCED3)transcript levels and abscisic acid(ABA)contents in leaves as well as increased hydrogen peroxide(H_(2)O_(2))levels in roots and *** experiments distinctly illustrate that drought resistance can be conferred by the frd3 rootstock regardless of the scion genotype,indicating that long-distance signals originating from frd3 roots promote an increase in ABA levels in ***,the drought resistance conferred by the frd3 mutant rootstock is weakened by the CAT2-overexpressing scion,suggesting that H_(2)O_(2)may be involved in long-distance ***,the results of comparative transcriptome and proteome analyses support the drought resistance phenotype of the frd3 *** together,our findings substantiate the notion that frd3 root-derived long-distance signals trigger ABA synthesis in leaves and enhance drought resistance,providing new evidence for root-to-shoot long-distance signaling in the drought response of plants.

关键词： frd3 Drought resistance Root-to-shoot long-distance signals Reactive oxygen species(ROS) H_(2)O_(2) Iron ABA

Quantum weak force sensing with squeezed magnomechanics

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Science China(Physics,Mechanics & Astronomy) 2024年第10期67卷 23-32页

作者： qian Zhang Jie Wang Tian-xiang Lu Ran Huang Franco Nori Hui Jing Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education Department of Physics and Synergetic Innovation Center for Quantum Effects and ApplicationsHunan Normal UniversityChangsha 410081China Theoretical Quantum Physics Laboratory Cluster for Pioneering ResearchRIKENWako-shi 351-0198Japan Center for Quantum Computing RIKENWako-shi 351-0198Japan Department of Physics University of MichiganAnn Arbor 48109-1040USA College of Physics and Electronic Information Gannan Normal UniversityGanzhou 341000China Academy for Quantum Science and Technology Zhengzhou University of Light IndustryZhengzhou 450002China

Cavity magnomechanics,exhibiting remarkable experimental tunability,rich magnonic nonlinearities,and compatibility with various quantum systems,has witnessed considerable advances in recent ***,the potential benefits of using cavity magnomechanical(CMM)systems in further improving the performance of quantum-enhanced sensing for weak forces remain largely *** we show that,by squeezing the magnons,the performance of a quantum CMM sensor can be significantly enhanced beyond the standard quantum limit(SQL).We find that,for comparable parameters,two orders of magnitude enhancement in the force sensitivity can be achieved in comparison with the case without magnon ***,we obtain the optimal parameter regimes of homodyne angle for minimizing the added quantum *** findings provide a promising approach for highly tunable and compatible quantum force sensing using hybrid CMM devices,with potential applications ranging from quantum precision measurements to quantum information processing.

关键词： quantum force sensing cavity magnomechanics magnon Kerr effect

Metal-organic framework hybrid materials of ZIF-8/RGO for immobilization of D-amino acid dehydrogenase

在线全文

学校读者我要写书评

暂无评论

Nano Research 2024年第1期17卷 290-296页

作者： Hangbin Lei qian Zhang Xiaoyan xiang Liang Jiang Shiyan Wang Lingxuan Duan Shizhen Wang Department of Chemical and Biochemical Engineering College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Xiamen Key Laboratory of Synthetic Biotechnology Xiamen UniversityXiamen 361005China

Immobilization of D-amino acid dehydrogenase(DAADH)by the assembly of peptide linker was studied for the biosynthesis of *** material of zeolitic imidazolate framework-8(ZIF-8)combined with reduced graphene oxide(RGO)was applied for the immobilization of DAADH from Ureibacillus *** recovery rate of DAADH/ZIF-8/RGO was 165.6%.DAADH/ZIF-8/RGO remained 53.4%of its initial activity at 50°C for 10 h while the free enzyme was ***/ZIF-8/RGO maintained 70.5%activity in hyperalkaline solution with pH *** parameters indicated that DAADH/ZIF-8/RGO had greater affinity of phenylpyruvate as V_(max)/K_(m)of DAADH/ZIF-8/RGO was 1.27-fold than free *** seven recycles,the activity of DAADH/ZIF-8/RGO remained 64.3%.Furthermore,one-step separation and in situ immobilization of DAADH by ZIF-8/RGO/Ni was carried out with 1.5-fold activity *** peptide linker and metal-organic framework(MOF)immobilization,thermostability and activity of the immobilized DAADH were significantly improved.

关键词： D-Amino acid dehydrogenase immobilization metal-organic frameworks zeolitic imidazolate framework-8(ZIF-8) reduced graphene oxide

Investigation on cavitating turbulent flow for the twisted NACA66 hydrofoil using a PANS model with helicity modification

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Hydrodynamics 2024年第2期36卷 219-231页

作者： Chen Geng Zhao-hui qian Ke-xin Zheng Wei-xiang Ye Xian-wu Luo State Key Laboratory of Hydroscience cand Engineering Deparment of Energy and Power EngineeringTsinghua UniversityBeijing 100084China Institute of Nuclear and New Energy Technology Tsinghua UniversityBeijing 100084China

In the present paper,the unsteady cavitating turbulent flow over the twisted NACA66 hydrofoil is investigated based on an modified shear stress transfer k-ωpartially averaged Navier-Stokes(MSST PANS)model,i.e.,new MSST PANS(NMSST PANS)model,where the production term of kinetic energy in the turbulence model is modified with *** with the experimental data,cavitation evolution and its characteristic frequency are satisfactorily predicted by the proposed NMSST PANS *** is revealed that the interaction among the main flow,the reentrant jets,and sheet cavitation causes the formation of the primary shedding cavity near the mid-span and the secondary shedding cavity at each side of the twisted hydrofoil,and further induces the remarkable pressure gradient around shedding *** with the development of the primary and the secondary shedding cavities,the great pressure gradient associated with large cavity volume variation promotes the vortical flow generation and the spatial deformation of vortex structure during cavitation evolution,and results in the primary and the secondary U-type ***,dynamic mode decomposition(DMD)analysis is utilized to confirm the interaction among the main flow,the main reentrant jet and two side reentrant jets,and *** results indicate that the proposed NMSST PANS model is suitable to simulate the complicated cavitating turbulent flow for various engineering applications.

关键词： Cavitating turbulent flow partially averaged Navier-Stokes(PANS)model hydrofoil numerical simulation

Numerical Study on the Effect of Gap Diffraction on the Hydrodynamic Performance of A Floating Breakwater

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

China Ocean Engineering 2024年第4期38卷 663-675页

作者： BIAN xiang-qian JI Chun-yan XU Sheng GUO Jian-ting HUO Fa-li School of Naval Architecture and Ocean Engineering Jiangsu University of Science and TechnologyZhenjiang 212100China

Two-dimensional(2D)flume experiments are useful in investigating the performances of floating breakwaters(FBs),including hydrodynamic performances,motion responses,and mooring *** a reasonable gap between the flume wall and the FBs is a critical step in 2D flume ***,research on the effect of the gap on the accuracy of 2D FB experimental results is *** address this issue,a numerical wave tank is developed using CFD to estimate the wave-FB interaction of a moored dual-cylindrical FB,and the results are compared to experimental data from a previously published *** is good agreement between them,indicating that the numerical model is sufficiently *** numerical model is then applied to explore the effect of gap diffraction on the performance of FBs in2D *** was discovered that the nondimensional gap length L_(Gap)/W_(Pool)should be smaller than 7.5%to ensure that the relative error of the transmission coefficient is smaller than 3%.The influence of the gap is also related to the entering wave properties,such as the wave height and period.

关键词： floating breakwater diffraction effect gap hydrodynamic performance model experiments CFD numerical simulation

Three‑dimensional numerical simulation of dynamic strength and failure mode of a rock mass with cross joints

在线全文

学校读者我要写书评

暂无评论

International Journal of Coal Science & Technology 2024年第2期11卷 35-52页

作者： Tingting Liu Wenxu Huang Chang xiang qian Dong Xinping Li Chao Zhang Hubei Key Laboratory of Blasting Engineering Jianghan UniversityWuhan 430056China School of Civil Engineering and Architecture Wuhan University of TechnologyWuhan 430070China Hainan Institute Wuhan University of TechnologySanya 572025China

To study the dynamic mechanical properties and failure characteristics of intersecting jointed rock masses with different joint distributions under confining pressure,considering the cross angleαand joint persistence ratioη,a numerical model of the biaxial Hopkinson bar test system was established using the finite element method–discrete-element model coupling *** validity of the model was verified by comparing and analyzing it in conjunction with laboratory test ***-static combined impact tests were conducted on specimens under various conditions to investigate the strength characteristics and patterns of crack initiation and *** study revealed the predominant factors influencing intersecting joints with different angles and penetrations under impact *** results show that the peak stress of the specimens decreases first and then increases with the increase of the cross ***α<60°,regardless of the value ofη,the dynamic stress of the specimens is controlled by the main ***α≥60°,the peak stress borne by the specimens decreases with increasingη.Whenα<60°,the initiation and propagation of cracks in the cross-jointed specimens are mainly controlled by the main joint,and the final failure surface of the specimens is composed of the main joint and wing ***α≥60°orη≥0.67,the secondary joint guides the expansion of the wing cracks,and multiple failure surfaces composed of main and secondary joints,wing cracks,and co-planar cracks are *** lateral confinement significantly increases the dynamic peak stress able to be borne by the *** triaxial conditions,the degree of failure of the intersecting jointed specimens is much lower than that under uniaxial and biaxial conditions.

关键词： Cross joints Joint distribution form Dynamic failure characteristics FEM–DEM BHPB