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Recent advances in the synthesis and energetic properties of potassium-based potential green primary explosives

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Defence Technology（防务技术） 2022年第11期18卷 1945-1959页

作者： qamar-un-nisa tariq Saira Manzoor Maher-un-nisa tariq Wen-Li Cao Jian-Guo Zhang State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing100081China Department of Chemistry University of OkaraOkara56300Pakistan

Primary explosives are utilized as a reliable initiator for secondary explosives in an extensive range of military and civilian operations. Heavy-metal-based primary explosives are moderate performing, more sensitive, and environmentally hazardous, posing a direct and indirect threat to health and ***, heavy-metal-based primaries have been replaced by environment-friendly metal-based primary explosives, such as potassium complexes. This review presents not only a summary of the current progress of new-generation potassium-based primary explosives and their methods of preparation, energetic properties, and applications, but also a further comparison with traditional primary explosives. In addition, this work discusses the necessity of heavy metal-free primary explosives and the major challenges faced in replacing traditional primary explosives.

关键词： Green primary explosives Heterocyclic compounds Synthesis Energetic properties

Nitro-tetrazole based high performing explosives:Recent overview of synthesis and energetic properties

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Defence Technology（防务技术） 2021年第6期17卷 1995-2010页

作者： Saira Manzoor qamar-un-nisa tariq Xin Yin Jian-Guo Zhang State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing100081China

Heterocyclic skeleton(Azoles)and different energetic groups containing high performing explosives are highly emerged in recent years to meet the challenging requirements of energetic materials in both military and civilian applications with improved *** this purpose tetrazole(Azole)is identified as an attractive heterocyclic backbone with energetic functional groups nitro(-NO_(2)),nitrato(-ONO_(2)),nitrimino(-NNO_(2)),and nitramino(eNHeNO_(2))to replace the traditionally used high performing *** tetrazole based compounds having these energetic functional groups demonstrated advanced energetic performance(detonation velocity and pressure),densities,and heat of formation(HOF)and became a potential replacement of traditional energetic compounds such as *** review presents a summary of the recently reported nitro-tetrazole energetic compounds containing poly-nitro,di/mono-nitro,nitrato/nitramino/nitrimino,bridged/bis/di tetrazole and nitro functional groups,describing their preparation methods,advance energetic properties,and further applications as highperforming explosives,especially those reported in the last *** review aims to provide a fresh concept for designing nitro-tetrazole based high performing explosives together with major challenges and perspectives.

关键词： Tetrazole Energetic materials Functional groups Heterocyclic High-performing explosives

Recent advances on the nitrogen-rich 1,2,4-oxadiazole-azoles-based energetic materials

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Defence Technology（防务技术） 2022年第3期18卷 344-367页

作者： Wen-Li Cao qamar-un-nisa tariq Zhi-Min Li Jun-Qing Yang Jian-Guo Zhang State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing100081 PR China CAS Key Laboratory of Energy Regulation Materials Shanghai200032China

This review covers recent advances in the synthesis and energetic performance of nitrogen-rich 1,2,4-oxadiazole-azoles-based energetic *** materials comprise of 1,2,4-oxadiazole subunit as a key structural motif linked to different nitrogen-rich or nitrogen-oxygen azoles:tetrazole,furazan,furoxan,1,3,4-oxadiazole,pyrazole,and *** attention is devoted to the introduction of various energetic groups including nitro,nitramino,azo,azoxy,dinitromethyl,trinitroethyl moieties,and their *** physicochemical and available performance parameters including density,decomposition temperature,heat of formation,detonation pressure,detonation velocity,impact sensitivity,and friction sensitivity of typical energetic compounds are also provided and ***,it was obtained that several screened compounds exhibit superior detonation properties and outstanding insensitivities,which can be classified as a new family of high-performance energetic ***,1,2,4-oxadiazole-azoles-based energetic materials still have many thorough works to further exploited and studied,expecting to get very promising insensitive high explosives for practical application and industrialization.

关键词： 1,2,4-Oxadiazole-azoles Triazole Tetrazole Furazan Energetic materials Furoxan

Tuning the reactivity of TiO_(2)layer with uniform distribution of Sub-5 nm Fe_(2)O_(3)particles via in situ voltage-assisted oxidation for robust catalytic reduction

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Nano Materials Science 2024年第2期6卷 223-234页

作者： nisa Nashrah Abdelkarim Chaouiki Wail Al Zoubi Young Gun Ko Integrated Materials Chemistry Laboratory School of Materials Science and EngineeringYeungnam UniversityGyeongsan38541Republic of Korea

The trade-off between efficiency and stability has limited the application of TiO_(2)as a catalyst due to its poor surface ***,we present a modification of a TiO_(2)layer with highly stable Sub-5 nm Fe_(2)O_(3)nanoparticles(NP)by modulating its structure-surface reactivity relationship to attain efficiency-stability balance via a voltage-assisted oxidation *** situ simultaneous oxidation of the Ti substrate and Fe precursor using high-energy plasma driven by high voltage resulted in uniform distribution of Fe_(2)O_(3)NP embedded within porous TiO_(2)*** surface characterizations with density functional theory demonstrated an improved electronic transition in TiO_(2)due to the presence of surface defects from reactive oxygen species and possible charge transfer from Ti to Fe;it also unexpectedly increased the active site in the TiO_(2)layer due to uncoordinated electrons in Sub-5 nm Fe_(2)O_(3)NP/TiO_(2)catalyst,thereby enhancing the adsorption of chemical functional groups on the *** unique embedded structure exhibited remarkable improvement in reducing 4-nitrophenol to 4-aminophenol,achieving approximately 99%efficiency in 20 min without stability decay after 20 consecutive cycles,outperforming previously reported TiO_(2)-based *** finding proposes a modified-electrochemical strategy enabling facile construction of TiO_(2)with nanoscale oxides extandable to other metal oxide systems.

关键词： Titanium dioxide Oxide nanoparticle Electrochemical oxidation Surface reactivity Efficiency Stability

Leveraging a new thermosensor for heat-smart future agriculture

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Plant Communications 2024年第9期5卷 1-4页

作者： Ali Raza qamar U.Zaman Zhangli Hu Guangdong Key Laboratory of Plant Epigenetics College of Life Sciences and OceanographyShenzhen UniversityShenzhen 518060China College of Physics and Optoelectronic Engineering Shenzhen UniversityShenzhen 518060China Shenzhen Engineering Laboratory for Marine Algal Biotechnology Guangdong Technology Research Center for Marine Algal BiotechnologyCollege of Life Sciences and OceanographyShenzhen UniversityShenzhen 518060China Shenzhen Collaborative Innovation Public Service Platform for Marine Algae Industry Longhua Innovation Institute for BiotechnologyCollege of Life Sciences and OceanographyShenzhen UniversityShenzhen 518060China School of Breeding and Multiplication(Sanya Institute of Breeding and Multiplication) Hainan Yazhou-Bay Seed LaboratoryHainan UniversitySanya 572025China Collaborative Innovation Center of Nanfan and High-Efficiency Tropical Agriculture School of Tropical CropsHainan UniversityHaikou 570228China

As global temperatures rise owing to climate change,crops are increasingly subjected to conditions that surpass their optimal temperature ranges,leading to heat stress(HS).HS impacts many morpho-physiological,biochemical,and molecular mechanisms in plants,ultimately affecting sustainable agricultural production worldwide(Ding et al.,2020;Kan et al.,2023;Raza et al.,2024).

关键词： smart pass crops

Impact of the Brink-Axel hypothesis on unique first-forbiddenβ-transitions for r-process nuclei

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Chinese Physics C 2024年第3期48卷 148-168页

作者： Fakeha Farooq Jameel-un Nabi Ramoona Shehzadi Department of Physics University of the PunjabQuaid-e-Azam Campus 54590LahorePakistan university of Wah Quaid AvenueWah Cantt 47040PunjabPakistan

Key nuclear inputs for the astrophysical r-process simulations are the weak interaction ***,the accuracy of these inputs directly affects the reliability of nucleosynthesis *** majority of the stellar rates,used in simulation studies are calculated by invoking the Brink-Axel(BA)*** BA hypothesis assumes that the strength functions of all parent excited states are the same as for the ground state,only shifted in ***,the BA hypothesis has to be tested against microscopically calculated state-by-state *** this project,we study the impact of the BA hypothesis on calculated stellarβ^(-)-decay and electron capture *** investigation include both unique first forbidden(U1F)and allowed transitions for 106 neutron-rich trans-iron nuclei([27,77]≤[Z,A]≤[82,208]).The calculations were performed using the deformed proton-neutron quasiparticle random-phase approximation(pn-QRPA)model with a simple plus quadrupole separable and schematic ***-point and several key r-process nuclei lie within the considered mass region of the nuclear *** computed electron capture andβ^(-)-decay rates using two different prescriptions for strength *** was based on invoking the BA hypothesis and the other was the state-by-state calculation of strength functions,under stellar density and temperature conditions([10,1]≤[ρYe(g/cm^(3)),T(GK)]≤[10^(11),30]).Our results show that the BA hypothesis invoked U1Fβ^(-)rates are overestimated by 4–5 orders of magnitude as compared to microscopic *** capture rates,more than two orders of magnitude differences were noted when applying the BA *** was concluded that the BA hypothesis is not a reliable approximation,especially forβ^(-)-decay forbidden transitions.

关键词： Brink-Axel hypothesis pn-QRPA model unique first forbiddenβ-transitions GT strength functions trans-iron nuclei r-process

underground communication:Long non-coding RNA signaling in the plant rhizosphere

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Plant Communications 2024年第7期5卷 28-51页

作者： Muhammad Fahad Leeza tariq Sajid Muhammad Liang Wu Hainan Institute Zhejiang UniversitySanyaHainan 572000China Zhejiang Provincial Key Laboratory of Crop Genetic Resources College of Agriculture and BiotechnologyZhejiang UniversityHangzhouZhejiang 310058China National Key Laboratory for Rice Biology Institute of BiotechnologyZhejiang UniversityHangzhou 310058China

Long non-coding RNAs(lncRNAs)have emerged as integral gene-expression regulators underlying plant growth,development,and *** adapt to the heterogeneous and dynamic rhizosphere,plants use interconnected regulatory mechanisms to optimally fine-tune gene-expression-governing interactions with soil biota,as well as nutrient acquisition and heavy metal ***,high-throughput sequencing has enabled the identification of plant lncRNAs responsive to rhizosphere biotic and abiotic ***,we examine lncRNA biogenesis,classification,and mode of action,highlighting the functions of lncRNAs in mediating plant adaptation to diverse rhizosphere *** then discuss studies that reveal the significance and target genes of lncRNAs during developmental plasticity and stress responses at the rhizobium interface.A comprehensive understanding of specific lncRNAs,their regulatory targets,and the intricacies of their functional interaction networks will provide crucial insights into how these transcriptomic switches fine-tune responses to shifting rhizosphere *** ahead,we foresee that single-cell dissection of cell-type-specific lncRNA regulatory dynamics will enhance our understanding of the precise developmental modulation mechanisms that enable plant rhizosphere *** future challenges through multi-omics and genetic approaches will more fully reveal the integral roles of lncRNAs in governing plant adaptation to the belowground environment.

关键词： biotic and abiotic cues heavy metals long non-coding RNAs nutrients phytoremediation rhizosphere microbiome

Travelling wave solutions of nonlinear conformable analytical approaches

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Applied Mathematics(A Journal of Chinese universities) 2024年第3期39卷 502-518页

作者： Hira tariq Hira Ashraf Hadi Rezazadeh Ulviye Demirbilek Department of Mathematics Government College Women UniversitySialkotPakistan Faculty of Engineering Technology Amol University of Special Modern TechnologiesAmolIran Faculty of Arts and Sciences Department of MathematicsMersin UniversityMersinTurkey

The presented study deals with the investigation of nonlinear Bogoyavlenskii equations with conformable time-derivative which has great importance in plasma physics and non-inspectoral scattering *** wave solutions of this nonlinear conformable model are constructed by utilizing two powerful analytical approaches,namely,the modified auxiliary equation method and the Sardar sub-equation *** novel soliton solutions are extracted using these ***,3D surface graphs,contour plots and parametric graphs are drawn to show dynamical behavior of some obtained solutions with the aid of symbolic software such as *** constructed solutions will help to understand the dynamical framework of nonlinear Bogoyavlenskii equations in the related physical phenomena.

关键词： nonlinear partial differential equations modified auxiliary equation method Sardar sub-equation method soliton solutions

Radiative capture of proton through the ^(14)N(p,γ)^(15)O reaction at low energy

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Chinese Physics C 2024年第4期48卷 183-192页

作者： B.F.Irgaziev Abdul Kabir Jameel-un Nabi National university of Uzbekistan Tashkent 100174Uzbekistan Space and Astrophysics Research lab National Centre of GIS and Space ApplicationsDepartment of Space ScienceInstitute of Space TechnologyIslamabad 44000Pakistan university of Wah Quaid AvenueWah Cantt 47040PunjabPakistan

The CNO cycle is the main source of energy in stars more massive than our *** process defines the energy production,the duration of which can be used to determine the lifetime of massive *** cycle is an important tool for determining the age of globular *** proton capture via p+^(14)N→^(15)O+γ,at energies of astrophysical interest,is an important process in the CNO *** this project,we apply a potential model to describe both non-resonant and resonant reactions in the channels where radiative capture occurs through electric E1 *** employed the R-matrix method to describe the ongoing reactions via M1 resonant transitions,when it was not possible to correctly reproduce the experimental data using the potential *** partial components of the astrophysical S-factor are calculated for all possible electric and magnetic dipole transitions in ^(15)*** linear extrapolated S-factor at zero energy(S(0))agrees well with earlier reported values for all transition types considered in this *** on the value of the total astrophysical S-factor,depending on the collision energy,we calculate the nuclear reaction rates for p+^(14)N→^(15)O+γ.The computed rates agree well with the results reported in the NACRE II Collaboration and most recent existing measurements.

关键词： CNO cycle potential model R-matrix method cross-section astrophysical S-factor nuclear rates.