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Facile and effective synthesis strategy for terbium-doped hydroxyapatite toward photoelectric devices and flexible functional fibers

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Rare Metals 2024年第4期43卷 1713-1723页

作者： Xiao-Dong Zhang Kun Nie Zi-Yao Hu ran-ran Zhou Xiu-Qiang Duan Wu-Bin Dai Song-Song Nie Song-Jun Yao Luo-Xin Wang Le-Fu Mei Hua Wang Yi-Yi Yao Xiao-Xue Ma Hubei Key Laboratory for New Textile Materials and Applications and State Key Laboratory of New Textile Materials and Advanced Processing Technology School of Materials Science and EngineeringWuhan Textile UniversityWuhan430200China Key Laboratory of Testing and Tracing of Rare Earth Products for State Market Regulation Jiangxi University of Science and TechnologyGanzhou341000China Hubei Key Laboratory of Plasma Chemistry and Advanced Materials and Key Laboratory of Green Chemical Engineering Process of Ministry of Education Wuhan Institute of TechnologyWuhan430205China

As a material with good biocompatibility,hydroxyapatite(HAP)can have optical properties after doping with various rare earth *** a biocompatible fluorescent material,doped HAP could have broad applications in biological probes,drug delivery,optoelectronic materials,fluorescence anti-counterfeiting,and other *** this paper,we put forward the preparation of HAP doped with terbium(Ⅲ)ions(Tb^(3+))by hydrothermal *** controlling the Tb^(3+)doping content in reaction and the reaction time,the changes in HAP's structure,morphology,and luminescence properties under different conditions were *** the doping amount of Tb^(3+)reached an optimal value,the dipole-quadrupole would occur and the concentration would be *** control experiment showed that the optimal Tb3+content was 7.5×10^(-5)mol,which showed the best fluorescence ***,a non-luminous material,was rarely used in the field of fluorescent anti-counterfeiting and photoelectric *** proposed to prepare a luminescent aramid/polyphenylene sulfide(ACFs/PPS)fiber paper and a new light-emitting diode(LED)using the Tb-doped HAP *** composite sample exhibited an excellent stability and fluorescence performance,which also demonstrated a possibility of HAP applications in anticounterfeiting and *** introduction of Tb3+dopant HAP was done to give HAP optical properties and broaden the application range of HAP.

关键词： Hydroxyapatite Rare earth luminescence Photoelectric device Aramid Polyphenylene sulfide fiber paper Luminescent fiber

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An in-situ polymerized interphase engineering for high-voltage allsolid- state lithium-metal batteries

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Nano Research 2024年第4期17卷 2687-2692页

作者： Lu Nie Shaojie Chen Mengtian Zhang Tianyi Gao Yuyao Zhang ran Wei Yining Zhang Wei Liu School of Physical Science and Technology ShanghaiTech UniversityShanghai 201210China Tsinghua-Berkeley Shenzhen Institute&Tsinghua Shenzhen International Graduate School Tsinghua UniversityShenzhen 518055China

All-solid-state lithium batteries(ASSLBs)have attracted great interest due to their promising energy density and strong ***,the interface issues,including large interfacial resistance between electrode and electrolyte and low electrochemical stability of solid-state electrolytes against high-voltage cathodes,have restricted the development of high-voltage ***,we report an ASSLB with stable cycling by adopting a conformal polymer interlayer in-situ formed at the Li_(6.4)La_(3)Zr_(1.4)Ta_(0.6)O_(12)(LLZTO)–cathode *** polymer can perfectlyﬁll the voids and create a stable interface contact between LLZTO and *** addition,the electric field across the polymer interlayer is reduced compared with pure solid polymer electrolyte(SPE),which facilitates the electrochemical stability with high-voltage *** all-solid-state Li|LLZTO-SPE|LiFe_(0.4)Mn_(0.6)PO_(4)(LMFP)cells achieve a low interface impedance,high specific capacity,and excellent cycling *** work presents an effective and practical strategy to rationally design the electrode–electrolyte interface for the application of high-voltage ASSLBs.

关键词： all-solid-state lithium batteries interface contact electric field electrochemical stability

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Practical Synthesis of Valbenazine via 1,3-Dipolar Cycloaddition

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Chinese Journal of Chemistry 2024年第8期42卷 841-845页

作者： Yalan Peng Zuming Lin Lili Zhu Shiqing Han Sha-Hua Huang ran Hong College of Biotechnology and Pharmaceutical Engineering Nanjing Tech UniversityNanjingJiangsu211816 China School of Environmental and Chemical Engineering Shanghai Institute of TechnologyShanghai201418 China State Key Laboratory of Chemical Biology Shanghai Institute of Organic ChemistryChinese Academy of SciencesShanghai200032 China Innovation Research Institute of Traditional Chinese Medicine(IRI) Shanghai University of Traditional Chinese Medicine1200 Cailun RoadShanghai201203 China

Comprehensive Summary,Valbenazine(Ingrezza),a potent and highly selective inhibitor of vesicular monoamine transporter type 2(VMAT2)through the active metabolite hydrotetrabenazine(HTBZ),has been approved for the treatment of tardive dyskinesia and,very recently,for chorea,which is associated with Huntington's *** numerous synthetic efforts dedicated to the synthesis of HTBZ,the industrial preparation of valbenazine uses dihydroisoquinoline as a starting material and the chiral resolution of racemic HTBZ derived from ketone ***,we present a practical synthesis of HTBZ and valbenazine featuring a highly stereoselective 1,3-dipolar cycloaddition and enzymatic kinetic *** cascade process includes cycloaddition,N—O bond cleavage,and lactamization,which proved to be operationally *** allure of the enzymatic resolution developed in this work offers a rapid access toward affording tetrahydroisoquinoline(THIQ)-fused piperidine in the production of medically significant compounds,such as yohimbine and reserpine.

关键词： Cycloaddition Chemoenzymatic Kinetic resolution Prodrugs VMAT2 inhibitor

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Experimental study on the effect of unloading rate on gneiss rockburst

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第6期16卷 2064-2076页

作者： Dongqiao Liu Jie Sun ran Li Manchao He Binghao Cao Chongyuan Zhang Wen Meng State Key Laboratory for Tunnel Engineering China University of Mining and TechnologyBeijing100083China Key Laboratory of Active Tectonics and Geological Safety Ministry of Natural ResourcesInstitute of GeomechanicsChinese Academy of Geological SciencesBeijing100081China School of Mechanics and Civil Engineering China University of Mining and TechnologyBeijing100083China

Rockburst are often encountered in tunnel construction due to the complex geological *** study the influence of unloading rate on rockburst,gneiss rockburst experiments were conducted under three groups of unloading rates.A high-speed photography system and acoustic emission(AE)system were used to monitor the entire process of rockburst process in *** results show that the intensity of gneiss rockburst decreases with decrease of unloading rate,which is manifested as the reduction of AE energy and fragments ejection *** mechanisms are proposed to explain this effect:(i)The reduction of unloading rate changes the crack propagation mechanism in the process of *** makes the rockbursts change from the tensile failure mechanism at high unloading rate to the tension-shear mixed failure mechanism at low unloading rate,and more energy released in the form of shear crack ***,less strain energy is converted into kinetic energy of fragments ejection.(ii)Less plate cracking degree of gneiss has taken shape due to decrease of unloading rate,resulting in the destruction of rockburst incubation *** enlightenments of reducing the unloading rate for the project are also described *** rockburst magnitude is reduced from the medium magnitude at the unloading rate of 0.1 MPa/s to the slight magnitude at the unloading rate of 0.025 MPa/s,which was judged by the ejection velocity.

关键词： Rockburst Unloading rate Crack propagation Influence mechanisms

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Delayed-measurement one-way quantum computing on cloud quantum computer

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Chinese Physics B 2024年第9期33卷 125-131页

作者： Zhi-Peng Yang Yu-ran Zhang Fu-Li Li Heng Fan Beijing Academy of Quantum Information Science Beijing 100193China Ministry of Education Key Laboratory for Nonequilibrium Synthesis and Modulation of Condensed Matter Shaanxi Province Key Laboratory of Quantum Information and Quantum Optoelectronic DevicesSchool of PhysicsXi’an Jiaotong UniversityXi’anShaanxi 710049China School of Physics and Optoelectronics South China University of TechnologyGuangzhou 510640China Institute of Physics China Academy of SciencesBeijing 100190China

One-way quantum computation focuses on initially generating an entangled cluster state followed by a sequence of measurements with classical communication of their individual ***,a delayed-measurement approach has been applied to replace classical communication of individual measurement *** this work,by considering the delayed-measurement approach,we demonstrate a modified one-way CNOT gate using the on-cloud superconducting quantum computing platform:*** modified protocol for one-way quantum computing requires only three qubits rather than the four used in the standard *** this modified cluster state decreases the number of physical qubits required to implement one-way computation,both the scalability and complexity of the computing process are *** to previous work,this modified one-way CNOT gate is superior to the standard one in both fidelity and resource *** have also numerically compared the behavior of standard and modified methods in large-scale one-way quantum *** results suggest that in a noisy intermediate-scale quantum(NISQ)era,the modified method shows a significant advantage for one-way quantum computation.

关键词： measurement-based quantum computing quantum entanglement quantum gates

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A Bitcoin Address Multi-Classification Mechanism Based on Bipartite Graph-Based Maximization Consensus

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Computer Modeling in Engineering & Sciences 2024年第4期139卷 783-800页

作者： Lejun Zhang Junjie Zhang Kentaroh Toyoda Yuan Liu Jing Qiu Zhihong Tian ran Guo College of Information Engineering Yangzhou UniversityYangzhou225127China Cyberspace Institute Advanced Technology Guangzhou UniversityGuangzhou510006China Research and Development Center for E-Learning Ministry of EducationBeijing100039China Institute of High Performance Computing(IHPC) Agency for ScienceTechnology and Research(A∗STAR)Singapore138632Singapore School of Physics and Materials Science Guangzhou UniversityGuangzhou510006China

Bitcoin is widely used as the most classic electronic currency for various electronic services such as exchanges,gambling,marketplaces,and also scams such as high-yield investment *** the services operated by a Bitcoin address can help determine the risk level of that address and build an alert model *** engineering can also be used to flesh out labeled addresses and to analyze the current state of Bitcoin in a small *** this paper,we address the problem of identifying multiple classes of Bitcoin services,and for the poor classification of individual addresses that do not have significant features,we propose a Bitcoin address identification scheme based on joint multi-model prediction using the mapping relationship between addresses and *** innovation of the method is to(1)Extract as many valuable features as possible when an address is given to facilitate the multi-class service identification task.(2)Unlike the general supervised model approach,this paper proposes a joint prediction scheme for multiple learners based on address-entity mapping ***,after obtaining the overall features,the address classification and entity clustering tasks are performed separately,and the results are subjected to graph-basedmaximization *** final result ismade to baseline the individual address classification results while satisfying the constraint of having similarly behaving entities as far as *** testing and evaluating over 26,000 Bitcoin addresses,our feature extraction method captures more useful *** addition,the combined multi-learner model obtained results that exceeded the baseline classifier reaching an accuracy of 77.4%.

关键词： Bitcoin multi-service classification graph maximization consensus data security

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Numerical investigation on ball-sealers transport and diversion performance in shale gas horizontal well based on semi-resolved CFDDEM

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PARTICUOLOGY 2024年第10期93卷 137-153页

作者： Huang, Yinjian Zhao, Jinzhou Ren, Lan Lin, ran Wu, Jianfa Shen, Cheng Wu, Jianjun Li, Bing Southwest Petr Univ Natl Key Lab Oil & Gas Reservoir Geol & Exploitat Chengdu 610500 Peoples R China Tianfu Yongxing Lab Chengdu 610213 Peoples R China PetroChina Southwest Oil & Gas Field Co Shale Gas Res Inst Chengdu 610056 Peoples R China PetroChina Coalbed Methane Co Ltd Xian 710082 Peoples R China

In the staged multi-cluster fracturing of shale gas horizontal wells, ball sealers are used to ensure uniform fluid distribution among clusters, a strategy that is both cost-effective and operationally beneficial. Despite these advantages, comprehending the ball sealers' dynamics within the wellbore and their plugging behavior at perforations is still challenging. This complexity results in prediction difficulties regarding their diversion efficiency. To address this, our study utilized a semi-resolved CFD-DEM model based on kernel approximation to simulate the behavior of medium-sized ball sealers in single and multiple cluster scenarios. Our findings from a single cluster scenario reveal that the plugging probability is co-determined by velocity gradients in the fluid ingestion area near the perforation, backflow region, and inertial forces of the ball sealers. As the critical flow rate is achieved, the plugging probability negatively correlated with fluid viscosity and displacement, and positively correlated with the perforation flow ratio (PFR), the difference in particle-fluid density, ball sealer 's diameter, and the ball sealer 's offset from the pipeline center. Temporary plugging control efficiency was used to evaluate the flow balance effect among multiple clusters. The results indicate that an increased number of ball sealers enhances the fault tolerance during the temporary plugging process. Nevertheless, excessive ball sealers might undermine the temporary plugging control efficiency, as perforations with lower fluid inflow rates are unexpectedly plugging. Higher differences in fluid injection rates between clusters led to increased efficiency in temporary plugging control. Premature deployment of ball sealers cannot effectively plug perforations with marginally higher fluid inflow rates, but instead accidently plug intermediate clusters with lower fluid inflow rates. These findings offer a theoretical basis for optimizing the design of ball sealers. (c

关键词： Gas shale Horizontal wells Ball sealer Semi-resolved CFD-DEM Diversion DEM SIMULATION PARTICLES FLOW MODEL EFFICIENCY

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Transparent micropatterned conductive films based on highlyordered nanowire network

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Nano Research 2024年第5期17卷 4288-4297页

作者： Xin-ran Zhang Hai-Tao Deng Xu Zeng Yi-Lin Wang Peng Huang Xiao-Sheng Zhang School of Integrated Circuit Science and Engineering University of Electronic Science and Technology of ChinaChengdu 611731China

Transparent conductive films that are based on nanowire networks are essential to construct flexible,wearable,and even stretchable ***,large-scale precise micropatterning,especially with regard to the controllability of the organizing orientation of nanowires,is a critical ***,we proposed a liquid film rupture self-assembly approach for manufacturing transparent conductive films with microstructure arrays based on a highly ordered nanowire *** large-scale microstructure conductive films were fabricated through air-liquid interface self-assembly and liquid film rupture *** typical micropattern morphologies,including square,hexagon,circle,serpentine,etc.,were prepared to reveal the universal applicability of the proposed *** homogeneity and controllability of this approach were verified for multiple *** the assembly cycles increasing,the optical transmittance decreases *** addition,theoretical model analysis is carried out,and the analytical formula of the speed of the film moving with the surface tension and the density of the liquid film is ***,the feasibility of this approach for piezoresistive strain sensors is *** fabrication approach demonstrated a cost-effective and efficient method for precisely arranging nanowires,which is useful in transparent and wearable applications.

关键词： flexible electronics transparent conductive network micropatterning nanowires micro electromechanical systems(MEMS)

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Viral-mediated gene therapy in pediatric neurological disorders

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World Journal of Pediatrics 2024年第6期20卷 533-555页

作者： Jing Peng Wei-Wei Zou Xiao-Lei Wang Zhi-Guo Zhang ran Huo Li Yang Department of Pediatrics Clinical Research Center for Chidren Neurodevelopmental disablities of Hunan ProvinceXiangya HospitalCentral South UniversityChangsha 410008China Reproductive Medicine Center Department of Obstetrics and Gynecologythe First Affiliated Hospital of Anhui Medical UniversityHefeiChina State Key Laboratory of Reproductive Medicine Nanjing Medical UniversityNanjingChina

Background Due to the broad application of next-generation sequencing,the molecular diagnosis of genetic disorders in pediatric neurology is no longer an unachievable ***,treatments for neurological genetic disorders in children remain primarily *** the other hand,with the continuous evolution of therapeutic viral vectors,gene therapy is becoming a clinical *** this perspective,we wrote this review to illustrate the current state regarding viral-mediated gene therapy in childhood neurological *** sources We searched databases,including PubMed and Google Scholar,using the keywords"adenovirus vector,""lentivirus vector,"and"AAv"for gene therapy,and"immunoreaction induced by gene therapy vectors,""administration routes of gene therapy vectors,"and"gene therapy"with"NCL,""SMA,""DMD,""congenital myopathy,""MPS""leukodystrophy,"or"pediatric metabolic disorders".We also screened the database of *** using the keywords"gene therapy for children"and then filtered the results with the ones aimed at neurological *** time range of the search procedure was from the inception of the databases to the *** We presented the characteristics of commonly used viral vectors for gene therapy for pediatric neurological disorders and summarized their merits and drawbacks,the administration routes of each vector,the research progress,and the clinical application status of viral-mediated gene therapy on pediatric neurological *** Viral-mediated gene therapy is on the brink of broad clinical ***-mediated gene therapy will dramatically change the treatment pattern of childhood neurological disorders,and many children with incurable diseases will meet the dawn of a ***,the vectors must be optimized for better safety and efficacy.

关键词： Gene therapy Neurological disorders Pediatrics Viral vectors

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Abnormal Action Recognition with Lightweight Pose Estimation Network in Electric Power Training Scene

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Computers, Materials & Continua 2024年第6期79卷 4979-4994页

作者： Yunfeng Cai ran Qin Jin Tang Long Zhang Xiaotian Bi Qing Yang State Grid Jiangsu Electric Power Co. Ltd.Research InstituteNanjing211103China School of Computer Engineering Nanjing Institute of TechnologyNanjing211167China

Electric power training is essential for ensuring the safety and reliability of the *** this study,we introduce a novel Abnormal Action Recognition(AAR)system that utilizes a Lightweight Pose Estimation Network(LPEN)to efficiently and effectively detect abnormal fall-down and trespass incidents in electric power training *** LPEN network,comprising three stages—MobileNet,Initial Stage,and Refinement Stage—is employed to swiftly extract image features,detect human key points,and refine them for accurate ***,a Pose-aware Action Analysis Module(PAAM)captures the positional coordinates of human skeletal points in each ***,an Abnormal Action Inference Module(AAIM)evaluates whether abnormal fall-down or unauthorized trespass behavior is *** fall-down recognition,three criteria—falling speed,main angles of skeletal points,and the person’s bounding box—are *** identify unauthorized trespass,emphasis is placed on the position of the *** experiments validate the effectiveness and efficiency of the proposed system in ensuring the safety and reliability of electric power training.

关键词： Abnormal action recognition action recognition lightweight pose estimation electric power training

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