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Heat transfer enhanced inorganic phase change material compositing carbon nanotubes for battery thermal management and thermal runaway propagation mitigation

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Journal of Energy Chemistry 2024年第2期89卷 226-238,I0006页

作者： Xinyi Dai ping ping Depeng Kong Xinzeng Gao Yue Zhang Gongquan Wang Rongqi Peng Center for Offshore Engineering and Safety Technology China University of Petroleum(East China)Qingdao 266580ShandongChina College of Chemistry and Chemical Engineering China University of Petroleum(East China)Qingdao 266580ShandongChina

Developing technologies that can be applied simultaneously in battery thermal management(BTM)and thermal runaway(TR)mitigation is significant to improving the safety of lithium-ion battery *** phase change material(PCM)with nonflammability has the potential to achieve this dual *** study proposed an encapsulated inorganic phase change material(EPCM)with a heat transfer enhancement for battery systems,where Na_(2)HPO_(4)·12H_(2)O was used as the core PCM encapsulated by silica and the additive of carbon nanotube(CNT)was applied to enhance the thermal *** microstructure and thermal properties of the EPCM/CNT were analyzed by a series of characterization *** different incorporating methods of CNT were compared and the proper CNT adding amount was also *** preparation,the battery thermal management performance and TR propagation mitigation effects of EPCM/CNT were further investigated on the battery *** experimental results of thermal management tests showed that EPCM/CNT not only slowed down the temperature rising of the module but also improved the temperature uniformity during normal *** peak battery temperature decreased from 76℃to 61.2℃at 2 C discharge rate and the temperature difference was controlled below 3℃.Moreover,the results of TR propagation tests demonstrated that nonflammable EPCM/CNT with good heat absorption could work as a TR barrier,which exhibited effective mitigation on TR and TR *** trigger time of three cells was successfully delayed by 129,474 and 551 s,respectively and the propagation intervals were greatly extended as well.

关键词： Inorganic phase change material Carbon nanotube Battery thermal management Thermal runaway propagation Fire resistance Encapsulation

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Advances in noble metal-modified g-C3N4 heterostructures toward enhanced photocatalytic redox ability

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International Journal of Minerals, Metallurgy and Materials 2024年第11期31卷 2368-2389页

作者： Zhang, Xiao Yang, ping Faculty of Chemical Engineering and Technology Cracow University of Technology Krakow Poland School of Material Science & Engineering University of Jinan Jinan China

The photocatalytic activity of catalysts depends on the energy-harvesting ability and the separation or transport of photogenerated carriers. The light absorption capacity of graphitic carbon nitride (g-C3N4)-based composites can be enhanced by adjusting the surface plasmon resonance (SPR) of noble metal nanoparticles (e.g., Cu, Au, and Pd) in the entire visible region. Adjustments can be carried out by varying the nanocomponents of the materials. The SPR of noble metals can enhance the local electromagnetic field and improve interband transition, and resonant energy transfer occurs from plasmonic dipoles to electron–hole pairs via near-field electromagnetic interactions. Thus, noble metals have emerged as relevant nanocomponents for g-C3N4 used in CO2 photoreduction and water splitting. Herein, recent key advances in noble metals (either in single atom, cluster, or nanoparticle forms) and composite photocatalysts based on inorganic or organic nanocomponent-incorporated g-C3N4 nanosheets are systematically discussed, including the applications of these photocatalysts, which exhibit improved photoinduced charge mobility in CO2 photoconversion and H2 production. Issues related to the different types of multi-nanocomponent heterostructures (involving Schottky junctions, Z-/S-scheme heterostructures, noble metals, and additional semiconductor nanocomponents) and the adjustment of dimensionality of heterostructures (by incorporating noble metal nanoplates on g-C3N4 forming 2D/2D heterostructures) are explored. The current prospects and possible challenges of g-C3N4 composite photocatalysts incorporated with noble metals (e.g., Au, Pt, Pd, and Cu), particularly in water splitting, CO2 reduction, pollution degradation, and chemical conversion applications, are summarized.

关键词： g-C3N4 heterostructure noble metal photocatalysis H_(2)generation CO_(2)

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Strong Subgame Consistency of the Core in Stochastic Network Formation Games

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Journal of the Operations Research Society of China 2024年第1期12卷 189-213页

作者： ping Sun Elena Parilina Faculty of Applied Mathematics and Control Processes Saint Petersburg State UniversitySaint Petersburg199034Russia

We consider a model of network formation as a stochastic game with random duration proposed initially in Sun and Parilina(Autom Remote Control 82(6):1065–1082,2021).In the model,the leader first suggests a joint project to other players,i.e.,the network connecting ***,the players are allowed to form fresh links with each other updating the initially proposed *** stage payoff of any player is defined depending on the network *** are two types of randomness in the network formation process:(i)links may fail to be formed with different probabilities although players intend to establish them,(ii)the game process may terminate at any stage or transit to the next stage with a certain probability ***,a network is formed as a result of players’decisions and realization of random *** cooperative version of the stochastic game is *** particular,we examine the properties of subgame consistency as well as strong subgame consistency of the *** provide a payment mechanism or regularization of the core elements to sustain its subgame consistency and avoid the player’s deviations from the cooperative *** addition,the distribution procedure of the core elements is regularized in case there are negative payments to achieve only nonnegative payments to the players at any *** sufficient condition of a strongly subgame consistent core is also *** illustrate our theoretical results with a numerical example.

关键词： Stochastic game Network formation Core Strong subgame consistency

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Topological and superconducting properties of monolayered CoN and CoP:A first-principles comparative study

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Science China(Physics,Mechanics & Astronomy) 2024年第5期67卷 98-108页

作者： Jiaqing Gao Zhenyu Zhang ping Cui International Center for Quantum Design of Functional Materials(ICQD) Hefei National Research Center for Physical Sciences at Microscale(HFNL)University of Science and Technology of ChinaHefei 230026China Hefei National Laboratory University of Science and Technology of ChinaHefei 230088China

Two-dimensional systems that simultaneously harbor superconductivity and nontrivial band topology may serve as appealing platforms for realizing topological superconductivity with promising applications in fault-tolerant quantum ***,based on first-principles calculations,we show that monolayered Co N and Co P with the isovalent Fe Se-like structure are stable in freestanding form,even though their known bulk phases have no resemblance to *** two systems are further revealed to display intrinsic band inversions due to crystal field splitting,and such orderings are preserved with the inclusion of spin-orbit coupling(SOC),which otherwise is able to open a curved band gap,yielding a non-zero Z2 topological invariant in each *** a mechanism of topologicalization is distinctly contrasted with that identified recently for the closely related monolayers of CoX(X=As,Sb,Bi),where the SOC plays an indispensable role in causing a nontrivial band ***,we demonstrate that,by applying equi-biaxial tensile strain,the electron-phonon coupling strength in monolayered CoN can be significantly enhanced,yielding a superconducting transition temperature(Tc)up to 7-12 K for the Coulomb pseudopotential ofμ*=0.2-0.1,while the CoP monolayer shows very low Tc even under pronounced *** different superconducting behaviors can be attributed to different variations in lattice softening and electronic density of states around the Fermi level upon *** central findings enrich the understanding of different mechanisms of band inversions and topologicalization and offer platforms for achieving the coexistence of superconductivity and nontrivial band topology based on two-dimensional systems.

关键词： topological yielding otherwise

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New Results in Cooperative Adaptive Optimal Output Regulation

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Journal of Systems Science & Complexity 2024年第1期37卷 253-272页

作者： DONG Yuchen GAO Weinan JIANG Zhong-ping State Key Laboratory of Synthetical Automation for Process Industries Northeastern UniversityShenyang 110819China Department of Electrical and Computer Engineering Tandon School of EngineeringNew York UniversityBrooklynNY 11201USA

This paper investigates the cooperative adaptive optimal output regulation problem of continuous-time linear multi-agent *** the multi-agent system dynamics are uncertain,solving regulator equations and the corresponding algebraic Riccati equations is challenging,especially for high-order *** this paper,a novel method is proposed to approximate the solution of regulator equations,i.e.,gradient descent *** is worth noting that this method obtains gradients through online data rather than model information.A data-driven distributed adaptive suboptimal controller is developed by adaptive dynamic programming,so that each follower can achieve asymptotic tracking and disturbance ***,the effectiveness of the proposed control method is validated by simulations.

关键词： Adaptive dynamic programming cooperative output regulation gradient descent method multi-agent systems.

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Dark Localized Waves in Shallow Waters:Analysis within an Extended Boussinesq System

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Chinese Physics Letters 2024年第4期41卷 32-37页

作者： Zhengping Yang Wei-ping Zhong Milivoj Belic Department of Medical Science Shunde PolytechnicShunde 528300China Department of Electronic Engineering Shunde PolytechnicShunde 528300China Division of Arts and Sciences Texas A&M University at Qatar23874 DohaQatar

We study dark localized waves within a nonlinear system based on the Boussinesq approximation,describing the dynamics of shallow water *** symbolic calculus,we apply the Hirota bilinear method to transform an extended Boussinesq system into a bilinear form,and then use the multiple rogue wave method to obtain its dark rational *** the first-and second-order dark solutions,we examine the conditions under which these localized solutions exist and their spatiotemporal *** the selection of various parameters and by utilizing different visualization techniques(intensity distributions and contour plots),we explore the dynamical properties of dark solutions found:in particular,the first-and second-order dark rogue *** also explore the methods of their *** findings presented here not only deepen the understanding of physical phenomena described by the(1+1)-dimensional Boussinesq equation,but also expand avenues for further *** method can be extended to other nonlinear systems,to conceivably obtain higher-order dark rogue waves.

关键词： Boussinesq bilinear nonlinear

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Prediction of chemical short-range order in high-/medium-entropy alloys

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Journal of Materials Science & Technology 2024年第2期169卷 115-123页

作者： Pei-Yu Cao Jing Wang ping Jiang Yun-Jiang Wang Fu-ping Yuan Xiao-Lei Wu State Key Laboratory of Nonlinear Mechanics Institute of MechanicsChinese Academy of ScienceBeijing 100190China School of Engineering Science University of Chinese Academy of SciencesBeijing 100049China

Chemical short-range orders(CSROs),as the built-in sub-nanoscale entities in a high-/medium-entropy alloy(H/MEA),have aroused an ever-increasing *** multi-principal elements in an H/MEA to form a complex concentrated solution,a variety of sub-systems of species exist to induce the metastable ordered compounds as candidates for ultimate *** issues remain pending on the origin of CSROs as to how to judge if CSRO will form in an H/MEA and particularly,what kind of CSROs would be stably produced if there were multiple ***,the first-principles method,along with the proposed local formation energy calculation in allusion to the atomic-scale chemical heterogeneities,is used to predict the CSRO formation based on the mechanical stability,thermodynamic formation energy,and electronic *** simulations are detailed in an equiatomic ternary VCoNi MEA with three kinds of potential compounds,i.e.,L1_(1),L1_(2),and B2,in the face-centered cubic *** turns out that L1_(1)is stable but hard to grow up so as to become the final CSRO.L1_(1)is further predicted as CSROs in CrCoNi,but unable to form in FeCoNi and CrMnFeCoNi *** predictions are consistent with the experimental *** findings shed light on understanding the formation of *** method is applicable to other H/MEAs to design and tailor CSROs by tuning chemical species/contents and thermal processing for high performance.

关键词： Short-range order High-entropy alloy Microstructure First-principles calculation Gibbs free energy Local electronic density of states

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Encouraging Solution to the Problem of Synthesizing Protein α-Thioester

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Chinese Journal of Chemistry 2024年第10期42卷 1114-1120页

作者： Xinliang Liu Zijun Gao Jie Zhao Farong Ye ping Huang ping Wang Center for Chemical Glycobiology Shanghai Key Laboratory for Molecular Engineering of Chiral DrugsFrontiers Science Center for Transformative MoleculesSchool of Chemistry and Chemical EngineeringZhangjiang Institute for Advanced StudyShanghai JiaoTongUniversityShanghai 200240China Shenzhen Research Institute of Shanghai Jiao Tong University ShenzhenGuangdong 518057China

Expressed protein ligation(EPL)provides a powerful tool to access large-size proteins with precise *** methods for constructing the critical protein thioester for EPL have predominantly relied on the recombinant intein fusion expressed in Escherichia coli(***).Despite its powerful applications,the expression of thioester derived from eukaryotic protein in *** inherently suffers from its limited solubility,the inactivity of intein,premature hydrolysis and low *** overcome these obstacles,we present herein the facile one-flask synthesis of inaccessible proteinα-thioester via a SUMO-protein-intein(SPI)sandwich *** utility of SUMO enhances the protein fusion yield and solubility,prevents premature hydrolysis and simplifies the purification *** inaccessible protein thioester with internal Cys residues can be readily produced and is compatible with the EPL-desulfurization protocol used to prepare complex proteins,which is otherwise difficult to obtain using traditional *** utility has been highlighted through the synthesis of human granulocyte colony-stimulating factor(G-CSF).

关键词： Desulfurization Glycoproteins Glycopeptides Protein expression Peptide thioester

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Improving Federated Learning through Abnormal Client Detection and Incentive

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Computer Modeling in Engineering & Sciences 2024年第4期139卷 383-403页

作者： Hongle Guo Yingchi Mao Xiaoming He Benteng Zhang Tianfu Pang ping ping College of Computer and Information Hohai UniversityNanjing211100China Key Laboratory ofWater Big Data Technology of Ministry ofWater Resources Hohai UniversityNanjing211100China

Data sharing and privacy protection are made possible by federated learning,which allows for continuous model parameter sharing between several clients and a central *** reliable and high-quality clients must participate in practical applications for the federated learning global model to be accurate,but because the clients are independent,the central server cannot fully control their *** central server has no way of knowing the correctness of the model parameters provided by each client in this round,so clients may purposefully or unwittingly submit anomalous data,leading to abnormal behavior,such as becoming malicious attackers or defective *** reduce their negative consequences,it is crucial to quickly detect these abnormalities and incentivize *** this paper,we propose a Federated Learning framework for Detecting and Incentivizing Abnormal Clients(FL-DIAC)to accomplish efficient and security federated *** build a detector that introduces an auto-encoder for anomaly detection and use it to perform anomaly identification and prevent the involvement of abnormal clients,in particular for the anomaly client detection *** them,before the model parameters are input to the detector,we propose a Fourier transform-based anomaly data detectionmethod for dimensionality reduction in order to reduce the computational ***,we create a credit scorebased incentive structure to encourage clients to participate in training in order tomake clients actively *** training models(CNN,MLP,and ResNet-18)and three datasets(MNIST,Fashion MNIST,and CIFAR-10)have been used in *** to theoretical analysis and experimental findings,the FL-DIAC is superior to other federated learning schemes of the same type in terms of effectiveness.

关键词： Federated learning abnormal clients incentive credit score abnormal score detection

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Direct capture and separation of CO_(2) from air

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Green Energy & Environment 2024年第3期9卷 413-416页

作者： Siew ping Teong Yugen Zhang Institute of Sustainability for Chemicals Energy and Environment(ISCE2)Agency for ScienceTechnology and Research(A*STAR)1 Pesek Road Jurong Island627833SingaporeRepublic of Singapore

Direct air capture(DAC)has attracted increasing interest and investment over the past few *** are a fast-growing number of companies that entered the field and demonstrated DAC carbon removal setups and ***,current DAC methods are still based on solid absorbents or alkali solutions approaches which have low capture efficiency and low energy *** highlight proposed a promising CO_(2) capture technology,an electric energy driven closed-loop system for the direct removal of CO_(2) from ambient air which are based on two individual technologies:Polyam-N-Cu hybrid system promoted CO_(2) capture with ocean as anthropogenic CO_(2) sink and a chloride-mediated electrochemical pH swing system to remove CO_(2) from oceanwater.

关键词： system separation companies

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