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Synergistic integration of self-supported 1T/2h-WS_(2) and nitrogendoped rGO on carbon cloth for ph-universal electrocatalytic hydrogen evolution

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Nano Research 2024年第3期17卷 1267-1280页

作者： Feng ming Yap Jian Yiing Loh Wee-Jun ong School of Energy and Chemical Engineering Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia Center of Excellence for NaNo Energy&Catalysis Technology(CONNECT) Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia State Key Laboratory of physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Gulei Innovation Institute Xiamen UniversityZhangzhou 363200China Shenzhen Research Institute of Xiamen University Shenzhen 518057China

hydrogen economy based on electrochemical water splitting exemplified one of the most promising means for overcoming the rapid consumption of fossil fuels and the serious deterioration of global *** development of earth-abundant,efficient,and durable electrocatalysts for hydrogen evolution reaction(hER)plays a vital role in the commercialization of water ***,the self-supported electrode with unique nitrogen-doped reduced graphene oxide(N-rGO)nanoflakes and WS_(2) hierarchical nanoflower that were grown directly on carbon cloth(CC)substrate(WS_(2)/N-rGO/CC)was successfully synthesized using a facile dual-step hydrothermal *** as-synthesized 50%1T/2h-WS_(2)/N-rGO/CC(WGC),which possessed high metallic 1T phase of 57%not only efficiently exposed more active sites and accelerated mass/charge diffusion,but also endowed excellent structural lustiness,robust stability,and durability at a high current *** a result,the 50%WGC exhibited lower overpotentials and Tafel slopes of 21.13 mV(29.55 mV∙dec^(-1))and 80.35 mV(137.02 mV∙dec^(-1))as compared to 20%Pt-C/CC,respectively for catalyzing acidic and alkaline hydrogen evolution ***,the as-synthesized 50%WGC also depicted long-term stability for more than 8 h in the high-current-density regions(100 and 220 mA∙cm^(-2)).In brief,this work reveals a self-supported electrode as an extraordinary alternative to Pt-based catalysts for hER in a wide ph range,while paving a facile strategy to develop advanced electrocatalysts with abundant heterointerfaces for practical applications in energy-saving hydrogen production.

关键词： self-supported electrocatalyst carbon-based substrate phase engineering ph-universal water splitting

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Implementation and evaluation of Exercise is medicine in primary care clinics within a large academic health system

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Family medicine and Community health 2024年第1期12卷 16-27页

作者： John Kevin ong Dayao Caroline E L Duffy Amalia m Cristiano Gene'Rusty'Kallenberg Sarah E Linke University of California San Diego School of medicine La JollaCaliforniaUSA milken Institute of Public health The George Washington UniversityWashingtonDistrict of ColumbiaUSA The University of Texas medical Branch at Galveston School of medicine GalvestonTexasUSA Scripps Family medicine Residency Scripps Mercy Hospital Chula VistaChula VistaCaliforniaUSA herbert Wertheim School of Public health&human Longevity Science University of California San DiegoLa JollaCaliforniaUSA Department of Family medicine University of California San DiegoLa JollaCaliforniaUSA Omada health San FranciscoCaliforniaUSA

Objective Exercise is medicine(EIm)is a global initiative encouraging healthcare providers to routinely assess and promote physical activity(PA)among *** objective of this study was to evaluate the feasibility,adoption,implementation and effectiveness of EIm from patient,clinician and healthcare staff perspectives using a combination of electronic health record(EhR),survey and interview *** This study used a combination of the Practical Robust Implementation and Sustainability model(PRISm)and the Learning Evaluation model to implement *** captured from the EhR,including physical Activity Vital Sign(PAVS)scores,and data collected from qualitative surveys and interviews were used to evaluate the programme’s Reach,Effectiveness,Adoption,Implementation,maintenance(RE-AIm,which is embedded within PRISm)from provider,staff and patient *** Five primary care clinics within a large academic health *** A total of 24443 patients from all participating clinics had at least one PAVS score during the study period.A total of 17 clinicians completed surveys,and 4 clinicians,8 medical assistants and 9 patients completed *** Implementation fidelity metrics varied widely between components and across clinics but were generally consistent over time,indicating a high degree of programme *** was highest during the first 6 months of the COVID-19 pandemic when most visits were *** PAVS scores increased from 57.7(95%CI:56 to 59.4)to 95.2(95%CI:91.6 to 98.8)min per week at 6 months for patients not meeting PA guidelines at baseline and decreased from 253.84(95%CI:252 to 255.7)to 208.3(95%CI:204.2 to 212.4)min per week at 6 months for patients meeting PA guidelines at *** EIm implementation,clinician-estimated time spent discussing PA with patients increased for 35%of providers and stayed the same for 53%.Conclusion Overall,this study established EIm’s feasibility,adoption,implementation

关键词： routine qualitative completed

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甘肃省熊蜂分布特征及其影响因素

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中国蜂业 2024年第8期15卷 13-13页

作者：安建东 Naeem m Chen h Li W hughes AC Williams ph Bashir Nh miao Z huang J An J 中国农业科学院蜜蜂研究所

近日，中国农业科学院蜜蜂研究所联合曲靖师范学院等单位科研人员发现甘肃省熊蜂呈现四大生物地理区系，净初级生产力是影响熊蜂多样性分布的最主要因素。该研究成果在线发表在《昆虫(Insects)》上。熊蜂是众多植物的传粉者，在陆地生... 详细信息

近日，中国农业科学院蜜蜂研究所联合曲靖师范学院等单位科研人员发现甘肃省熊蜂呈现四大生物地理区系，净初级生产力是影响熊蜂多样性分布的最主要因素。该研究成果在线发表在《昆虫(Insects)》上。熊蜂是众多植物的传粉者，在陆地生态系统中发挥着十分重要的作用。明确影响熊蜂分布的因素对于熊蜂多样性保护至关重要。

关键词： Gansu biodiversity biogeographic regionalization bumblebees canonical correspondence analysis

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magnesium oxide(mgO)nanoadsorbents in wastewater treatment:A comprehensive review

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Journal of magnesium and Alloys 2024年第5期12卷 1709-1773页

作者： h.C.S.Perera V.Gurunanthanan Anoop Singh m.m.m.G.P.G.mantilaka G.Das Sandeep Arya Department of physics Khalifa UniversityAbu Dhabi12788United Arab Emirates Postgraduate Institute of Science University of PeradeniyaPeradeniyaSri Lanka Department of humanities and Sciences Guru Nanak Institutions Technical CampusIbrahimpatnamHyderabad501506India Centre for Global health Research Saveetha Medical College and HospitalsSaveetha Institute of Medical and Technical SciencesChennai602105Tamil NaduIndia Department of physics University of JammuJammu and Kashmir180006India

Wastewater contamination by heavy metals and synthetic dyes presents a significant environmental challenge,necessitating effective and sustainable separation *** review article provides a detailed examination of magnesium oxide(mgO)nanoparticles as an innovative nanoadsorbent for wastewater treatment,with a specific focus on heavy metal and dye *** review comprehensively explores various aspects of mgO nanoparticles,including their structural characteristics and synthesis *** article delves into the morphology and crystallographic arrangement of mgO nanoparticles,offering insights into their structural *** the complexity of adsorption processes,the review identifies and analyzes parameters influencing the adsorption efficiency of mgO nanoparticles,such as temperature,ph,contact time,initial concentration,and co-existing *** interplay between these parameters and the adsorption capability of mgO nanoparticles emphasizes the importance of optimizing operational ***,the review assesses various synthesis methods for mgO nanoparticles,including sol-gel,hydrothermal,precipitation,green synthesis,solvothermal,and template-assisted *** discusses the advantages,limitations,and resulting nanoparticle characteristics of each method,enabling readers to grasp the implications of synthesis processes on adsorption *** comprehensive review consolidates current insights into the effectiveness of mgO nanoparticles as a potent nanoadsorbent for removing heavy metals and dyes from wastewater covering a wide spectrum of aspects related to mgO ***,there is a need to investigate the use of mgO in the treatment of actual wastewater or river water,in order to leverage its cost-effectiveness and high efficiency for practical water treatment applications in real-time.

关键词： mgO nanoparticles Nanoadsorbent Wastewater treatment heavy metals Dye separation Adsorption Synthesis methods

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New Breakdown Electric Field Calculation for SF6 high Voltage Circuit Breaker Applications

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Plasma Science and Technology 2007年第6期9卷 690-694页

作者： ph.ROBIN-JOUAN m.YOUSFI AREVA T & D high Voltage Switchgear Research Centre 130 rue L.BLUM 69611 VilleurbanneFrance University of Toulouse LAPLACE-UMR 5213 CNRSUPS118 Route de Narbonne31062 Toulouse Cedex 9France

The critical electric fields of hot SF6 are calculated including both electron and ion kinetics in wide ranges of temperature and pressure, namely from 300 K up to 4000 K and 2 atmospheres up to 32 atmospheres respectively. Based on solving a multi-term electron Boltz- mann equation the calculations use improved electron-gas collision cross sections for twelve SF6 dissociation products with a particular emphasis on the electron-vibrating molecule interactions. The ion kinetics is also considered and its role on the critical field becomes non negligible as the temperature is above 2000 K. These critical fields are then used in hydrodynamics simulations which correctly predict the circuit breaker behaviours observed in the case of breaking tests.

关键词： breakdown electric field hot dissociated SF6 high voltage gas-circuit-breaker

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Biosynthesized CS-mgO/zeolite hybrid material:An efficient adsorbent for chlorpyrifos removal-Kinetic studies and response surface methodology

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Emerging Contaminants 2024年第3期10卷 304-317页

作者： mohammed T.m.h.hamad Belal N.A.mahran Central Laboratory for Environmental Quality monitoring National Water Research CenterEgypt

The prevalence of organophosphate pesticides in aquatic environments raises severe concerns on a global ***,an insecticide,is included in a class of organophosphate *** is widely used on agricultural lands to control pests in cotton,fruit,and *** acute toxicity of chlorpyrifos is still dangerous to all aquatic living *** the treatment of water contaminated with chlorpyrifos is an important *** recent decade has witnessed adsorption technology emerging as an advanced organophosphate pesticide wastewater treatment with great potential and a grand blueprint,in which the specific surface area and active sites of the adsorbent are considered to be the two most important characteristics largely impacting the adsorption *** this study,a CS-mgO/Zeolite composite was prepared by the microbial method as an effective adsorbent for the removal of chlorpyrifos from an aqueous *** adsorbent's properties were carefully characterized using Xray diffraction,scanning electron microscopy,and Fourier-transform infrared *** refinement of experimental conditions,encompassing variations in adsorbent dosage,contact time,and chlorpyrifos concentration at five discrete levels,was systematically undertaken through the utilization of a composite central design rooted in response surface *** solution ph played a key role in chlorpyrifos removal,and a ph of 7.0 was selected according to its high adsorption *** highest removal(80.9%)of chlorpyrifos by CS-mgO/Zeolite was obtained at an optimum ph of 7,a contact time of 40 min,an adsorbent dosage of 0.4 g/L,and a chlorpyrifos concentration of 5 mg/L^(-1).The adsorption results were highly fitted with the Freundlich adsorption isotherm model,and the maximum adsorption was 83.3 mg/*** studies indicate that the removal of chlorpyrifos followed the pseudo-secondorder model of adsorption(0.994).The thermodynamic parameters indicate the sponta

关键词： Chlorpyrifos adsorption CS-mgO/Zeolite Response surface methodology

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Study on Cytokines IL-2,IL-6,IL-10 in Patients of Chronic Allergic Rhinitis Treated with Acupuncture

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Journal of Traditional Chinese medicine 2002年第2期22卷 104-111页

作者： FILOmENA BAngRAZI PETTI m.Sc.ph.D. ALDO LIGUORI m.D. FLORA IPPOLITI m.D.ph.D. Paracelso Chair

OBJECTIVES: To observe the plasmatic concentration of IL-6, IL-10 and IL-2 in the patient of chronic allergic rhinitis before and after acupuncture therapy. mEThODS: Cytokine levels were determined before and after treatment in 30 healthy volunteers (Group A) and 90 patients of chronic allergic rhinitis (Group B) with an increased plasma IL-10 level. Group B was then divided into 3 subgroups: 30 patients treated with real acupuncture (Group B1); 30 patients treated with sham acupuncture (Group B2); 30 non-treated patients (Group B3). RESULTS: The allergic subjects of group B1, compared with controls, showed a significant reduction of IL-10 after a specific treatment with acupuncture (P

关键词： Acupuncture Therapy Adult CD4-Positive T-Lymphocytes Female humans Interleukin-10 Interleukin-2 Interleukin-6 male middle Aged Rhinitis, Allergic, Perennial

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Biorhythms and the Biological Clock Involvement of melatonin and the Pineal Gland in Life and Disease

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Biomedical and Environmental Sciences 1995年第2期8卷 90-105页

作者： ISAACNIR m.D ph.D Departmentofpharmacology HebrewUniversity-HadassahMedicalSchoolP.O.B.12065JerusalemIsraelDepartmentofPharmacologyHebrewUniversity-HadassahMedicalSchoolP.O.B.12065JerusalemIsraelDepartmentofPharmacologyHebrewUniversity-HadassahMedicalSchoolP.O.B

humanbeing***'dothesedaiIyandseasonalenvironmentalch.ngeshaveanyeffectsonourbodilyandmentalfunctionsandhowdoesthelivingorganismadaptitselftothem?Areoursleep-wakerhythmscasualcircadianchronobiologicalevents,ordoweresIX)ndandreassessourbiologicalfunctiontothenaturalIight/darkcycle?moreover,couldsomedisordersinourbOdybeinducedbyshiftingthephotoperiod,especiallytoitsextIemesofcontinuousIightordarkness?DoesthebodyPossessacircadianpace...

关键词： SNAT SAD Biorhythms and the Biological Clock Involvement of melatonin and the Pineal Gland in Life and Disease

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Biodiversity Assessment of Avifauna in the Forest Reservation of Aurora State College of Technology (ASCOT), philippines

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Open Journal of Ecology 2024年第4期14卷 292-308页

作者： Afed S. Daiwey heherson B. ong Emerson V. Barcellano Edmundo C. Gumpal michelle Ann m. Calubaquib Rafael J. Padre School of Forestry and Environmental Sciences Aurora State College of Technology Baler Philippines College of Forestry and Environmental Science Isabela State University Cabagan Philippines College of Agriculture Isabela State University Cabagan Philippines College of Engineering Isabela State University Echague Philippines

The research study was conducted to assess and quantify the current status of avifauna biodiversity assets of Aurora State College of Technology’s Forest Reservation in Baler, Aurora, philippines. Assessment of avifaunal diversity was undertaken by traversing the four established circular plots having a radius of 125 meters or 250 meters diameters each as permanent monitoring stations. Study revealed a total number of 151 Individual species, classified into 23 genera and 21 families. Eighteen of these species are endemic while the remaining five were fully migrated birds. All birds observed were classified as Least Concern (LC) species according to the International Union for Conservation of Nature’s Red List of Threatened Species and the updated list of the Birds of the World online. Its abundance, richness and diversity index were calculated using Shannon Diversity Index (h') while Pielou’s evenness (J') for distribution of species. Forest reservation of ASCOT has more even (0.756 J') and moderate diversity (2.812 h') observation on avifauna in general. however, this avian population evaluation was threatened into a verge of extinction due to natural and anthropological threats that causes forest deforestation. Such deforestation of habitat causes dwindling of wildlife territory leading to the scarcity of bird’s population. Thus, the assessment was conducted to aid ASCOT administration find significant plans to ensure sustainable conservation and protection of the remaining avifauna species in the reservation area.

关键词： Biodiversity Avifauna Abundance Species Richness Species Diversity

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Effect of Ag substitution on structural,magnetic and magnetocaloric properties of Pr_(0.6)Sr_(0.4–x)Ag_xmnO_3 manganites

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Journal of Rare Earths 2017年第9期35卷 875-882页

作者： R.Thaljaoui m.Pekala J.-F.Fagnard ph.Vanderbemden SUPRATECS Department of Electrical Engineering and Computer Science(B28)University of LiegeBelgium Department of Chemistry University of WarsawAl.Zwirki i Wigury 10102-089Poland Faculty of physics Warsaw University of TechnologyKoszykowa 7500-662 WarsawPoland

A systematic investigation on the structural, magnetic and magnetocaloric properties of Pr_（0.6）Sr_（0.4-x）Ag_xmnO_3（x=0.05 and 0.1） manganites was reported. Rietveld refinements of the X-ray diffraction patterns confirmed that all samples were single phase and crystallized in the orthorhombic structure with Pnma space group. magnetic measurements in a magnetic applied field of 0.01T revealed that the ferromagnetic-paramagnetic transition temperature T_C decreased from about 293 to 290 K with increasing silver content from x=0.05 to 0.1. The reported magnetocaloric entropy ch.nge and relative cooling power for both samples were considerably remarkable with a △S_（max） value of 1.9 J/（kg·K）and maximum RCP values of 100 J/kg, under a magnetic field ch.nge（？μ0h） equal to 1.8T. The analysis of the universal curves gave an evidence of a second order magnetic transition for the studied samples. The magnetic field influence on both the magnetic entropy ch.nge and the relative cooling power was also studied and discussed.

关键词： monovalent doped manganite XRD SEm ZFC and FC curves mgnetocaloric effect universal curves relative cooling power critical exponents

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