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A BODIPY analogue from the tautomerization of sodium 3-oxide BODIPY

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Chinese Chemical Letters 2015年第6期26卷 631-635页

作者： peng-zhong chen Hai-Rong Zheng Li-Ya Niu Yu-Zhe chen Li-Zhu Wu chen-Ho Tung Qing-Zheng Yang Key Laboratory of Photochemical Conversion and Optoelectronic Materials Technical Institute of Physics and ChemistryChinese Academy of Sciences University of the Chinese Academy of Sciences College of Chemistry Beijing Normal University

The introduction of hydroxy group to the 3- or 5-position of 4,4-difluoro-4-bora-3aAa-diazaindacene （BODIPY） results in unexpected tautomerization to BDPONa with interesting structural and photophysical properties. The core of BDPONa is an anion with sodium cation as counter-ion. BDPONa displays strong fluorescence in organic solvents.

关键词： Bodipy Substitution reaction Tautomerization Sodium salt

Discrete element modeling and verification of the simulation parameters for chopped hybrid Broussonetia papyrifera stems

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International Journal of Agricultural and Biological Engineering 2024年第1期17卷 23-32页

作者： Caiwang peng Junwei chen Xi He Songlin Sun Yulong Yin zhong chen College of Mechanical and Electrical Engineering Hunan Agricultural UniversityChangsha 410128China College of Animal Science and Technology Hunan Agricultural UniversityChangsha 410128China Rongcheng Gouyang Modern Agriculture(Chongqing)Co. LtdChongqing 500153China

In this study,the discrete element software EDEM was applied to establish a simulation model of non-uniform-sized particle units for Broussonetia papyrifera stalks,which aimed to address the low utilization rate of existing Broussonetia papyrifera harvesting machinery,the significant variation between the simulated model of Broussonetia papyrifera stalks and their actual appearance,as well as the absence of contact parameter *** a combination of the free-fall collision method,inclined plane sliding method,and inclined plane rolling method,numerical simulation was conducted to analyze the pattern of variations in contact parameters between Broussonetia papyrifera stalks and the steel material of the ***,these parameters were *** results showed that the coefficient of restitution between Broussonetia papyrifera stalks and steel materials was 0.321,the static friction factor was 0.589,and the rolling friction factor was *** the parameters of contact between Broussonetia papyrifera stalks as variables and the experimentally measured pile angle as the objective of optimization,the steepest ascent experiment and the three-factor five-level rotation combination experiment were *** this way,a second-order response model was constructed to analyze the relationship between the contact parameters and the pile *** the optimization analysis of experimental data,it was determined that the coefficient of restitution between Broussonetia papyrifera stalks was 0.21,the static friction factor was 0.24,and the rolling friction factor was ***,the calibration results were validated through experimentation to show that the relative error between the obtained pile angle under the context of optimal parameter combination and the actual one was 4.11%.In addition,the relative error of mass flow rate in spiral transport was within a reasonable range,this study lays a foundation both theoretically and statistic

关键词： hybrid Broussonetia papyrifera stem discrete element method repose angle contact parameters calibration

Some Rotundities of Orlicz–Lorentz Spaces

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Acta Mathematica Sinica,English Series 2024年第8期40卷 1893-1919页

作者： Wan zhong GONG peng WANG Department of Mathematics Anhui Normal UniversityWuhu 241000P.R.China

K-UR,K-LUR and K-R are the generalizations of UR,LUR and R respectively,which are of great significance in Banach space *** in Orlicz–Lorentz function spaceΛ_(ϕ,ω)^(◦)[0,γ)equipped with the Orlicz norm,the research methods of K-UR,K-LUR and K-R are much more complicated than those of UR,LUR and *** this paper we obtain some criteria of K-UR,K-LUR and K-R ofΛ_(ϕ,ω)^(◦)[0,γ)by means of the norm of dual space and H_(μ)property ofΛ_(ϕ,ω)^(◦)[0,γ).

关键词： Orlicz-Lorentz space Orlicz norm k-uniform rotundity locally k-uniform rotundity krotundity

CrossLinkNet: An Explainable and Trustworthy AI Framework for Whole-Slide Images Segmentation

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Computers, Materials & Continua 2024年第6期79卷 4703-4724页

作者： peng Xiao Qi zhong Jingxue chen Dongyuan Wu Zhen Qin Erqiang Zhou Network and Data Security Key Laboratory of Sichuan Province University of Electronic Science and Technology of ChinaChengdu610054China Faculty of Data Science City University of MacaoMacao999078China

In the intelligent medical diagnosis area,Artificial Intelligence(AI)’s trustworthiness,reliability,and interpretability are critical,especially in cancer *** neural networks,while excellent at processing natural images,often lack interpretability and adaptability when processing high-resolution digital pathological *** limitation is particularly evident in pathological diagnosis,which is the gold standard of cancer diagnosis and relies on a pathologist’s careful examination and analysis of digital pathological slides to identify the features and progression of the ***,the integration of interpretable AI into smart medical diagnosis is not only an inevitable technological trend but also a key to improving diagnostic accuracy and *** this paper,we introduce an innovative Multi-Scale Multi-Branch Feature Encoder(MSBE)and present the design of the CrossLinkNet *** MSBE enhances the network’s capability for feature extraction by allowing the adjustment of hyperparameters to configure the number of branches and *** CrossLinkNet Framework,serving as a versatile image segmentation network architecture,employs cross-layer encoder-decoder connections for multi-level feature fusion,thereby enhancing feature integration and segmentation *** quantitative and qualitative experiments on two datasets demonstrate that CrossLinkNet,equipped with the MSBE encoder,not only achieves accurate segmentation results but is also adaptable to various tumor segmentation tasks and scenarios by replacing different feature ***,CrossLinkNet emphasizes the interpretability of the AI model,a crucial aspect for medical professionals,providing an in-depth understanding of the model’s decisions and thereby enhancing trust and reliability in AI-assisted diagnostics.

关键词： Explainable AI security trustworthy CrossLinkNet whole slide images

Amphoteric Supramolecular Nanofiber Separator for High-Performance Sodium-Ion Batteries

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Energy & Environmental Materials 2024年第5期7卷 118-125页

作者： Yuping Zhang Hongzhi Zheng Xing Tong Hao Zhuo Wu Yang Yuling chen Ge Shi Zehong chen Linxin zhong Xinwen peng State Key Laboratory of Pulp and Paper Engineering South China University of Technology Department of Chemistry UBC Faculty of Science Vancouver Campus Department of Mechanical Engineering National University of Singapore

The separator is an essential component of sodium-ion batteries （SIBs） to determine their electrochemical performances. However, the separator with high mechanical strength, good electrolyte wettability and excellent electrochemical performance remains an open challenge. Herein, a new separator consisting of amphoteric nanofibers with abundant functional groups was fabricated through supramolecular assembly of natural polymers for SIB. The uniform nanoporous structure, remarkable mechanical properties and abundant functional groups （e.g.-COOH,-NH2and-OH）endow the separator with lower dissolution activation energy and higher ion migration numbers. These metrics enable the separator to lower the barrier for desolvation of Na+, accelerate the migration of Na+, and generate more stable solid electrolyte interphase （SEI） and cathode electrolyte interphase（CEI）. The battery assembled with the amphoteric nanofiber separator shows higher specific capacity and better stability than that assembled with glass fiber （GF） separator.

关键词： amphoteric nanofiber self-assembly Separator sodium-ion batteries

Promising interlayer sensitization strategy for the construction of high-performance blue hyperfluorescence OLEDs

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Light(Science & Applications) 2024年第7期13卷 1372-1382页

作者： Jianghui Wang peng Zou Letian chen Zhentao Bai Hao Liu Wen-cheng chen Yanping Huo Ben zhong Tang Zujin Zhao State Key Laboratory of Luminescent Materials and Devices Guangdong Provincial Key Laboratory of Luminescence from Molecular AggregatesSouth China University of TechnologyGuangzhou 510640China. School of Chemical Engineering and Light Industry Guangdong University of TechnologyGuangzhou 510006China. School of Science and Engineering Shenzhen Institute of Aggregate Science and TechnologyThe Chinese University of Hong KongShenzhenGuangdong 518172China

Multi-resonance thermally activated delayed fluorescence(MR-TADF)materials are promising candidates for organic light-emitting diodes(OLEDs)with narrow electroluminescence(EL)*** researches focus on fabricating hyperfluorescence OLEDs to improve EL efficiencies of MR-TADF emitters by co-doping them with TADF sensitizers in a single host ***,in many cases,the polarity of the single host could be not suitable for both blue MRTADF emitters and blue TADF sensitizers,resulting in broadened EL spectra in high-polar hosts or decreased EL efficiencies in low-polar ***,we wish to report an efficient sensitization strategy for blue MR-TADF emitters by constructing an interlayer-sensitizing configuration,in which the blue TADF sensitizers and blue MR-TADF emitters are separated into two closely aligned host layers with high polarity and low polarity,*** on this strategy,efficient blue hyperfluorescence OLEDs are realized and verified by employing various TADF sensitizers and different MR-TADF emitters,furnishing outstanding external quantum efficiencies of up to 38.8%and narrow EL *** results validate the feasibility and universality of this interlayer sensitization strategy,which provides an effective alternative to high-performance blue hyperfluorescence OLEDs.

关键词： OLEDs interlayer sensitization

A Transparent Photoresist Made of Titanium Dioxide Nanoparticle-Embedded Acrylic Resin with a Tunable Refractive Index for UV-Imprint Lithography

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Engineering 2024年第6期37卷 96-104页

作者： Yinglu Liu Dan Wang Changlin Liu Qianqian Hao Jian Li Jie-Xin Wang Xiuyun chen peng zhong Xibin Shao Jian-Feng chen State Key Laboratory of Organic–Inorganic Composites Beijing University of Chemical TechnologyBeijing 100029China Research Center of the Ministry of Education for High Gravity Engineering and Technology Beijing University of Chemical TechnologyBeijing 100029China BOE Technology Group Co. Ltd.Beijing 100176China

Transparent photoresists with a high refractive index(RI)and high transmittance in visible wavelengths have promising functionalities in optical *** work reports a kind of tunable optical material composed of titanium dioxide nanoparticles embedded in acrylic resin with a high RI for ultraviolet(UV)-imprint *** hybrid film exhibits a tunable RI of up to 1.67(589 nm)after being cured by UV light,while maintaining both a high transparency of over 98%in the visible light range and a low haze of less than 0.05%.The precision machining of optical microstructures can be imprinted easily and efficiently using the hybrid resin,which acts as a light guide plate(LGP)to guide the light from the side to the top in order to conserve the energy of the display *** preliminary studies based on both laboratory and commercial experiments pave the way for exploiting the unparalleled optical properties of nanocomposite resins and promoting their industrial application.

关键词： Photoresist Tunable refractive index Hanson solubility Ultraviolet imprint Organic-inorganic composites

Optical detection method of discharge mode transition of inductively coupled plasma in an atmosphere-breathing electric propulsion system

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Chinese Journal of Aeronautics 2024年第10期37卷 172-183页

作者： Yuxuan zhong Yu ZHANG Jianjun WU peng ZHENG College of Aerospace Science and Engineering National University of Defense TechnologyChangsha 410073China

Plasma discharge stability is an important problem in atmosphere-breathing electric propulsion system when maintaining long-term missions at ultra-low earth *** paper designed an inductively coupled plasma source to imitate the ionization *** effect of inflow rate and Radio Frequency(RF)power on the plasma discharge mode transition is experimentally studied.A discharge mode detection method is proposed,which determines the discharge mode by identifying the morphology of the plasma *** using the method,the discharge mode transition is quantified and a control model based on the parameter sensitivity is *** verify the method,the spectra are measured and the electron temperature spatial distribution is *** the method has been proven *** results show that the inductively coupled discharge contains capacitive components affected by the mass flow rate and the radio frequency *** plasma characteristics can be maintained stably by controlling the radio frequency power when the mass flow rate randomly changes in a certain *** is demonstrated that the application of detection method effectively identifies the discharge mode,which is a promising active control method for the plasma discharge mode.

关键词： Atmosphere-breathing electric propulsion Inductively coupled plasma Discharge mode transition Optical diagnosis Ultra-low earth orbit

Construction of core@double-shell structured energetic composites with simultaneously enhanced thermal stability and safety performance

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Defence Technology（防务技术） 2024年第4期34卷 134-142页

作者： peng Wang Wen Qian Ruolei zhong Fangfang He Xin Li Jie chen Li Meng Yinshuang Sun Guansong He Institute of Chemical Materials China Academy of Engineering PhysicsMianyang 621900China State Key Laboratory of Environment-friendly Energy Materials School of Materials and ChemistrySouthwest University of Science and TechnologyMianyang 621010China

The poor thermal stability and high sensitivity severely hinder the practical application of hexanitrohexaazaisowurtzitane(CL-20).Herein,a kind of novel core@double-shell CL-20 based energetic composites were fabricated to address the above *** coordination complexes which consist of natural polyphenol tannic acid(TA) and Fe~Ⅲ were chosen to construct the inner shell,while the graphene sheets were used to build the outer *** resulting CL-20/TA-Fe~Ⅲ/graphene composites exhibited simultaneously improved thermal stability and safety performance with only 1 wt% double-shell content,which should be ascribed to the intense physical encapsulation effect from inner shell combined with the desensitization effect of carbon nano-materials from outer *** phase transition(ε to γ) temperature increased from 173.70 ℃ of pure CL-20 to 191.87℃ of CL-20/TA-Fe~Ⅲ/graphene ***,the characteristic drop height(H_(50)) dramatically increased from 14.7 cm of pure CL-20 to112.8 cm of CL-20/TA-Fe~Ⅲ/graphene composites,indicating much superior safety performance after the construction of the double-shell *** general,this work has provided an effective and versatile strategy to conquer the thermal stability and safety issues of CL-20 and contributes to the future application of high energy density energetic materials.

关键词： CL-20 Double-shell structure Thermal stability Safety performance Tannic acid Graphene sheets