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In^(3+)-doped Sr_(2)Fe_(1.5)Mo_(0.5)O_(6−δ)cathode with improved performance for an intermediate-temperature solid oxide fuel cell

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Nano Research 2024年第1期17卷 407-415页

作者： Yumei Ma Lijie Zhang Kang zhu Binze Zhang Ranran peng Changrong Xia Ling Huang State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830046China Department of Materials Science and Engineering University of Science and Technology of ChinaHefei 230026China

Promoting the oxygen reduction reaction(ORR)is critical for commercialization of intermediate-temperature solid oxide fuel cells(IT-SOFCs),where Sr_(2)Fe_(1.5)Mo_(0.5)O_(6)−δ(SFM)is a promising cathode by working as a mixed ionic and electronic *** this work,doping of In^(3+)greatly increases the oxygen vacancy concentration and the content of adsorbed oxygen species in Sr_(2)Fe_(1.5)Mo_(0.5−x)InxO_(6−δ)(SFMInx),and thus effectively promotes the ORR *** a typical example,SFMIn_(0.1)reduces the polarization resistance(R_(p))from 0.089 to 0.046Ω∙cm^(2)at 800°C,which is superior to those doped with other metal *** addition,SFMIn0.1 increases the peak power density from 0.92 to 1.47 W∙cm^(−2)at 800°C with humidified H_(2)as the fuel,indicating that In3+doping at the Mo site can effectively improve the performance of SOFC cathode material.

关键词： solid oxide fuel cell cathode In3+doping oxygen reduction reaction(ORR) Sr_(2)Fe_(1.5)Mo_(0.5)O_(6-δ)

Automatic detection and assessment of crack development in ultra-high performance concrete in the spatial and Fourier domains

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Frontiers of Structural and Civil Engineering 2024年第3期18卷 350-364页

作者： Jixing CAO Yao ZHANG Haijie HE Weibing peng Weigang ZHAO zhiguo YAN Hehua zhu School of Safety Engineering and Emergency Management Shijiazhuang Tiedao UniversityShijiazhuang 050043China College of Civil Engineering and Architecture Zhejiang UniversityHangzhou 310058China College of Civil and Architectural Engineering Taizhou UniversityTaizhou 318000China College of Civil Engineering and Architecture Zhejiang University of TechnologyHangzhou 310014China Department of Geotechnical Engineering Tongji UniversityShanghai 200092China

Automatic detection and assessment of surface cracks are beneficial for understanding the mechanical performance of ultra-high performance concrete(UHPC).This study detects crack evolution using a novel dynamic mode decomposition(DMD)*** this method,the sparse matrix‘determined’from images is used to reconstruct the foreground that contains cracks,and the global threshold method is adopted to extract the crack *** application of the DMD method to the three-point bending test demonstrates the efficiency in inspecting cracks with high ***,the geometric features,including the area and its projection in two major directions,are evaluated over *** relationship between the geometric properties of cracks and load-displacement curves of UHPC is *** to the irregular shape of cracks in the spatial domain,the cracks are then transformed into the Fourier domain to assess their *** indicate that crack patterns in the Fourier domain exhibit a distinct concentration around a central ***,the power spectral density of cracks exhibits an increasing trend over *** investigation into crack evolution in both the spatial and Fourier domains contributes significantly to elucidating the mechanical behavior of UHPC.

关键词： dynamic mode decomposition ultra-high performance concrete crack detection geometric features Fourier domain

Towards carbon neutrality of calcium carbide-based acetylene production with sustainable biomass resources

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Green Energy & Environment 2024年第6期9卷 1068-1078页

作者： peng Jiang Guanhan Zhao Hao Zhang Tuo Ji Liwen Mu Xiaohua Lu Jiahua zhu State Key Laboratory of Materials-oriented Chemical Engineering College of Chemical EngineeringNanjing Tech UniversityNanjing211816China

Acetylene is produced from the reaction between calcium carbide(CaC_(2))and water,while the production of CaC_(2) generates significant amount of carbon dioxide not only because it is an energy-intensive process but also the raw material for CaC_(2) synthesis is from ***,a comprehensive biomass-to-acetylene process was constructed that integrated several units including biomass pyrolysis,oxygen-thermal CaC_(2) fabrication and calcium *** comparison,a coal-to-acetylene process was also established by using coal as *** carbon efficiency,energy efficiency and environmental impacts of the bio-based calcium carbide acetylene(BCCA)and coal-based calcium carbide acetylene(CCCA)processes were systematically ***,the environmental impacts were further evaluated by applying thermal integration at system level and energy substitution in CaC_(2) *** though the BCCA process showed lower carbon efficiency and energy efficiency than that of the CCCA process,life cycle assessment demonstrated the BCCA(1.873 kgCO_(2eq) kg-prod^(-1))a lower carbon footprint process which is 0.366 kgCO_(2eq) kg-prod^(-1) lower compared to the CCCA *** sustainable energy(biomass power)substitution in CaC_(2) furnace,an even lower GWP value of 1.377 kgCO_(2eq) kg-prod^(-1) can be achieved in BCCA *** work performed a systematic analysis on integrating biomass into industrial acetylene production,and revealed the positive role of biomass as raw material(carbon)and energy supplier.

关键词： Biomass pyrolysis CO_(2)mitigation Calcium carbide Acetylene Calcium loop

A review of ^(17)O isotopic labeling techniques for solid-state NMR structural studies of metal oxides in lithium-ion batteries

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Magnetic Resonance Letters 2024年第2期4卷 46-53页

作者： Xiaoli Xia Lei zhu Weiping Tang Luming peng Junchao Chen School of Chemistry and Chemical Engineering Shanghai Jiao Tong University800 Dongchuan RoadShanghai200240China Key Laboratory of Mesoscopic Chemistry of Ministry of Education and Collaborative Innovation Center of Chemistry for Life Sciences School of Chemistry and Chemical EngineeringNanjing University163 Xianlin RoadNanjing210023China State Key Laboratory of Space Power-Sources Technology Shanghai Institute of Space Power-SourcesShanghai200245China

Recent advances in utilizing ^(17)O isotopic labeling methods for solid-state nuclear magnetic resonance(NMR)investigations of metal oxides for lithium-ion batteries have yielded extensive insights into their structural and dynamic ***,we commence with a brief introduction to recent research on lithium-ion battery oxide materials studied using ^(17)O solid-state NMR *** we delve into a review of ^(17)O isotopic labeling methods for tagging oxygen sites in both the bulk and surfaces of metal *** last,the unresolved problems and the future research directions for advancing the ^(17)O labeling technique are discussed.

关键词： ^(17)O solid-state NMR ^(17)O isotopic labeling methods Bulk and surfaces of metal oxides DFT calculation

High-chromium vanadium-titanium magnetite all-pellet integrated burden optimization and softening-melting behavior based on flux pellets

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International Journal of Minerals,Metallurgy and Materials 2024年第3期31卷 498-507页

作者： Bojian Chen Tao Jiang Jing Wen Guangdong Yang Tangxia Yu Fengxiang zhu peng Hu School of Metallurgy Northeastern UniversityShenyang 110819China Key Laboratory for Ecological Metallurgy of Multimetallic Mineral(Ministry of Education) Northeastern UniversityShenyang 110819China Liaoning Key Laboratory for Metallurgical Sensor and Technology Shenyang 110819China State key laboratory of vanadium and titanium resources comprehensive utilization Panzhihua 617000China

High-chromium vanadium-titanium magnetite(HVTM)is a crucial polymetallic-associated resource to be *** allpellet operation is a blast furnace trend that aims to reduce carbon dioxide emissions in the *** referencing the production data of vanadium-titanium magnetite blast furnaces,this study explored the softening-melting behavior of high-chromium vanadium-titanium magnetite and obtained the optimal integrated burden based on flux *** results show that the burden with a composition of 70wt%flux pellets and 30wt%acid pellets exhibits the best softening-melting *** comparison to that of the single burden,the softening-melting characteristic temperature of this burden composition was *** melting interval first increased from 307 to 362℃and then decreased to 282℃.The maximum pressure drop(ΔPmax)decreased from 26.76 to 19.01 *** permeability index(S)dropped from 4643.5 to 2446.8 kPa·℃.The softening-melting properties of the integrated burden were apparently *** acid pellets played a role in withstanding load during the softening *** flux pellets in the integrated burden exhibited a higher slag melting point,which increased the melting temperature during the melting *** slag homogeneity and the TiC produced by over-reduction led to the gas permeability deterioration of the single *** segregation of the flux and acid pellets in the HVTM proportion and basicity mainly led to the better softening-melting properties of the integrated burden.

关键词： high-chromium vanadium-titanium magnetite softening-melting properties all pellets integrated burden flux pellets

Influence of multi-stage volcanic events on the Late Cretaceous-Paleogene reservoirs and its geological significance in the northern Central Myanmar Basin

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Journal of Oceanology and Limnology 2024年第4期42卷 1074-1086页

作者： Zengyuan ZHOU Weilin zhu Wenxu peng Hefeng SUN Shijie ZHAO Xiaowei FU State Key Laboratory of Marine Geology Tongji UniversityShanghai 200092China CNOOC International Ltd. Beijing 100027China

The northward subduction of the Neo-Tethys oceanic crust triggered multiple magmatic activities in the West Myanmar Arc,which in turn influenced the deposition of sedimentary pyroclastic rocks from the Cretaceous to Eocene strata in the Central Myanmar Basin(CMB).The pore structure of these lithologic reservoirs is complex and rich in tuffaceous sandstone,which plays an adverse role in reservoir development in this *** understand the development characteristics and genetic mechanism of the pyroclastic rocks within three sets of reservoirs in this area,a comprehensive analysis was conducted through borehole core observations,thin section identification,scanning electron microscope analysis,and mercury injection *** tuffaceous sandstone from the upper Cretaceous to the Eocene is dominated by intermediate-acid volcanic rock *** pyroclastic rocks exhibit evident chloritization and ironization,with residual intergranular pores being the principal type accompanied by a smaller amount of intergranular dissolved pores and intragranular dissolved *** highest porosity is observed in the Eocene tuffaceous sandstone,ranging from 8%to 12%.The Late Cretaceous to Paleocene sandstones exhibit lower porosity levels of only 4%-6%.These reservoirs are characterized by their low porosity and *** the presence of a good source rock in this area,the volcanic debris particles filling the pores,as well as their subsequent devitrification,chloritization,and limonite mineralization,result in pore throat blockage and *** reservoirs in this area are small in size,exhibit poor reservoir connectivity and lateral continuity,and fail to meet the necessary conditions for commercial-scale hydrocarbon accumulation and migration.

关键词： Central Myanmar Basin back-arc basin reservoir characteristic volcanic debris

Identification of Early Warning Signals of Infectious Diseases in Hospitals by Integrating Clinical Treatment and Disease Prevention

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Current Medical Science 2024年第2期44卷 273-280页

作者： Lei ZHANG Min-ye LI Chen zhi Min zhu Hui MA Sixth Medical Center Chinese PLA General HospitalBeijing100048China The Nursing Department Chinese PLA General HospitalBeijing 100853China

The global incidence of infectious diseases has increased in recent years,posing a significant threat to human *** typically serve as frontline institutions for detecting infectious ***,accurately identifying warning signals of infectious diseases in a timely manner,especially emerging infectious diseases,can be ***,there is a pressing need to integrate treatment and disease prevention data to conduct comprehensive analyses aimed at preventing and controlling infectious diseases within *** paper examines the role of medical data in the early identification of infectious diseases,explores early warning technologies for infectious disease recognition,and assesses monitoring and early warning mechanisms for infectious *** propose that hospitals adopt novel multidimensional early warning technologies to mine and analyze medical data from various systems,in compliance with national strategies to integrate clinical treatment and disease ***,hospitals should establish institution-specific,clinical-based early warning models for infectious diseases to actively monitor early signals and enhance preparedness for infectious disease prevention and control.

关键词： infectious disease disease prevention and control medical data warning signals

Thermal comfort in a building with Trombe wall integrated with phase change materials in hot summer and cold winter region without air conditioning

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Energy and Built Environment 2024年第1期5卷 58-69页

作者： Jie Li Yuan Zhang Ziyang zhu Jiangtian zhu Jing Luo Fen peng Xiaoqin Sun School of Energy and Power Engineering Changsha University of Science and TechnologyChangshaHunan 410114PR China

Trombe wall and phase change materials(PCMs)are two effective ways to regulate indoor thermal ***,Trombe wall surfers from overheating in summer and PCMs suffer from low heat transfer rate caused by the limited thermal *** compensate the shortcomings of the two methods,this paper proposed a Trombe wall system integrated with *** on a light-weight building envelope in Changsha,China,the thermal comfort of 10 kinds of Trombe wall systems with PCMs with a melting temperature of 18-28℃ were *** the integrated indoor discomfort duration(I_(D)),integrated indoor discomfort degree-hour(I_(DH)),indoor air temperature(T_(in)),PCM liquid fraction(γ)and heat flux across wall(q)as evaluation indexes,the indoor thermal comfort was assessed in hot summer and cold winter *** show that the Trombe wall helped PCMs complete the phase change process *** wall with PCM25 next to the wall inner surface possessed the lowest annual I_(D) and I_(DH),as 2877 h and 12,974℃·h,*** with the values in a traditional building,the I_(D) and I_(DH) were reduced by 7.01% and 14.14%.In order to give full play to the heat storage and heat release of the Trombe wall with PCMs,PCMs with phase change temperature 7℃ lower than the peak ambient temperature in summer or 8℃ higher than the winter night temperature was recommended according to regional climate conditions.

关键词： Trombe wall Phase change materials Integrated indoor discomfort duration Integrated discomfort degree-hour Liquid fraction

Atmospheric transmission algorithm for pulsed X-rays from high-altitude nuclear detonations based on scattering correction

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Nuclear Science and Techniques 2024年第3期35卷 40-52页

作者： Ding-Han zhu Xiong Zhang Xiao-Qiang Li peng Li Yan-Bin Wang Shuang Zhang State Key Laboratory of NBC Protection for Civilian Beijing 102205China

In high-altitude nuclear detonations,the proportion of pulsed X-ray energy can exceed 70%,making it a specific monitoring signal for such *** pulsed X-rays can be captured using a satellite-borne X-ray detector following atmospheric *** quantitatively analyze the effects of different satellite detection altitudes,burst heights,and transmission angles on the physical processes of X-ray transport and energy fluence,we developed an atmospheric transmission algorithm for pulsed X-rays from high-altitude nuclear detonations based on scattering *** proposed method is an improvement over the traditional analytical method that only computes direct-transmission *** traditional analytical method exhibits a maximum relative error of 67.79% compared with the Monte Carlo *** improved method reduces this error to within 10% under the same conditions,even reaching 1% in certain ***,its computation time is 48,000 times faster than that of the Monte Carlo *** results have important theoretical significance and engineering application value for designing satellite-borne nuclear detonation pulsed X-ray detectors,inverting nuclear detonation source terms,and assessing ionospheric effects.

关键词： High-altitude nuclear detonation Atmospheric transmission Pulsed X-rays Scattering correction Analytical method Monte Carlo method