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The genesis and resource potential of gold deposits in the Liaodong Peninsula

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Science China Earth Sciences 2024年第3期67卷 657-672页

作者： Rixiang ZHU Jin-Hui YANG Gongwen WANG Qingdong ZENG Guoqiang XUE Tao XU Xinghui LI peng zhang Da LEI Guang ZHU State Key Laboratory of Lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China School of Earth Sciences and Resources China University of GeosciencesBeijing 100083China Shenyang Center China Geological SurveyShenyang 110034China School of Resources and Environmental Engineering Hefei University of TechnologyHefei 230009China

Plenty of gold deposits related to Late Mesozoic craton destruction are widely distributed in eastern North China Craton. However, significant differences in research degrees, ore-forming characteristics, and proven reserves exist among different regions in the North China Craton. The Liaodong Peninsula has similar regional geological characteristics to those of the Jiaodong Peninsula, with both experiencing craton destruction during Late Mesozoic, but the two areas have substantial differences in terms of gold mineralization and the proven gold resources. Based on regional geology, Mesozoic magmatictectonic evolution and ore geology, combined with integrated geophysical exploration and big data AI resource prediction, in this paper, we propose that the ore-forming materials of Late Mesozoic gold deposits in Liaodong were mainly originated from mantle-derived melts and/or fluids induced by craton destruction. The gold deposits were primarily controlled by NE-NNEtrending faults, mainly classified as fracture-controlled altered rock-type and sulfide-bearing quartz vein-type. Moreover, our study predicts that the Yalu River fault zone and its related secondary faults, as well as the periphery and deeper parts of known goldfields, are the important regions for future gold resource exploration. The Yalu River metallogenic belt has an enormous potential for gold resources, and the Liaodong Peninsula has a potential to add thousands of tons of gold resources.

关键词： Liaodong Peninsula Gold deposit Integrated geophysical exploration Prospecting potential Direction for prospecting breakthroughs

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Eco-Friendly Encapsulation of Metal Clusters in Porous Organic Cages for Engineerable Microenvironment and Enhanced Catalysis

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CCS Chemistry 2024年第9期6卷 2186-2197页

作者： Siyu Ren Liangxiao Tan Jun-Hao Zhou Jian Sun peng zhang Xingzhong Cao Yun-Hong zhang Jian-Ke Sun MOE Key Laboratory of Cluster Science Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion MaterialsSchool of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 102488 Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049

Developing artificial catalysts that mimic the functionality of enzymes and adapt to the surrounding microenvironment to achieve specific activity and selectivity is a fascinating research area yet remains a great *** this work,we present a meticulously designed strategy for the successful encapsulation of ultrasmall metal clusters(MCs)within an amine-type porous organic cage(POC)through electrostatic complexation,phase transfer,and alcohol reduction *** amine cage showcases an intriguing and customizable feature that allows for the regulation of the surrounding microenvironment of the confined MCs through a feasible postmodifi-cation *** functionalization of cage skeleton further facilitates precise adjustment to the surface electronic state of Pd cluster,thereby influencing the adsorption behavior of ***,this controlled regulation leads to modified activity and chemoselectivity in the catalytic hydrogenation of halogenated ***,the investigation of the correlation between the surrounding microenvironment,substrate adsorption,and catalytic performance in the POC-immobilized MCs system has not been previously *** anticipate that our research will provide valuable insights in this field.

关键词： metal cluster porous organic cage encapsulation microenvironment catalysis

Pollution source identification methods and remediation technologies of groundwater: A review

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China Geology 2024年第1期7卷 125-137页

作者： Ya-ci Liu Yu-hong Fei Ya-song Li Xi-lin Bao peng-wei zhang Fujian Provincial Key Laboratory of Water Cycling and Eco-Geological Processes Institute of Hydrogeology and Environmental GeologyChinese Academy of Geological SciencesXiamen 361000China Key Laboratory of Water and Soil Resources Conservation and Restoration in the Middle and Lower Reaches of Yellow River Basin MNRZhengzhou 450016China

Groundwater is an important source of drinking *** pollution severely endangers drinking water safety and sustainable social *** the case of groundwater pollution,the top priority is to identify pollution sources,and accurate information on pollution sources is the premise of efficient ***,an appropriate pollution remediation scheme should be developed according to information on pollution sources,site conditions,and economic *** methods for identifying pollution sources mainly include geophysical exploration,geochemistry,isotopic tracing,and numerical *** these identification methods,only the numerical modeling can recognize various information on pollution sources,while other methods can only identify a certain aspect of pollution *** remediation technologies of groundwater can be divided into in-situ and ex-situ remediation technologies according to the remediation *** in-situ remediation technologies enjoy low costs and a wide remediation range,but their remediation performance is prone to be affected by environmental conditions and cause secondary *** ex-situ remediation technologies boast high remediation efficiency,high processing capacity,and high treatment concentration but suffer high *** methods for pollution source identification and remediation technologies are applicable to different *** achieve the expected identification and remediation results,it is feasible to combine several methods and technologies according to the actual hydrogeological conditions of contaminated sites and the nature of ***,detailed knowledge about the hydrogeological conditions and stratigraphic structure of the contaminated site is the basis of all work regardless of the adopted identification methods or remediation technologies.

关键词： Groundwater pollution Identification of pollution sources Geophysical exploration identification Geochemistry identification Isotopic tracing Numerical modeling Remediation technology Hydrogeological conditions Hydrogeological survey engineering

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Angiotensin-converting enzyme 2 alleviates liver fibrosis through the renin-angiotensin system

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World Journal of Gastroenterology 2024年第6期30卷 607-609页

作者： Bai-Wei Zhao Ying-Jia Chen Ruo-peng zhang Yong-Ming Chen Bo-Wen Huang Department of Gastric Surgery Sun Yat-sen University Cancer CenterState Key Laboratory of Oncology in South ChinaGuangdong Provincial Clinical Research Center for CancerGuangzhou 510060Guangdong ProvinceChina Health Science Center Peking UniversityBeijing 100191China

The present letter to the editor is related to the study titled‘Angiotensin-converting enzyme 2 improves liver fibrosis in mice by regulating autophagy of hepatic stellate cells’.Angiotensin-converting enzyme 2 can alleviate liver fibrosis by regulating autophagy of hepatic stellate cells and affecting the renin-angiotensin system.

关键词： Angiotensin-converting enzyme 2 Hepatic stellate cells Liver fibrosis Angiotensin II Angiotensin 1-7 Renin-angiotensin system

Association between glucose-lowering drugs and circulating insulin antibodies induced by insulin therapy in patients with type 2 diabetes

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World Journal of Diabetes 2024年第7期15卷 1489-1498页

作者： peng zhang Qing Jiang Bo Ding Reng-Na Yan Yun Hu Jian-Hua Ma Department of Endocrinology Nanjing First HospitalNanjing Medical UniversityNanjing 210000Jiangsu ProvinceChina Department of Endocrinology The Affiliated Wuxi People's Hospital of Nanjing Medical UniversityWuxi Medical CenterWuxi 214000Jiangsu ProvinceChina

BACKGROUND Insulin antibodies(IAs)affect blood glucose control in patients receiving insulin *** To investigate the relationship between different hypoglycemic treatments and IAs in patients with type 2 diabetes mellitus(T2DM).METHODS This cross-sectional,retrospective study included 1863 patients with T2DM who were receiving exogenous insulin *** patients received stable antidiabetic therapy in the last 3 months and IA levels were measured using an iodine-125 *** A total of 1863 patients were *** were 902(48.4%)patients who had positive IAs(IA level>5%),with a mean IA level of 11.06%(10.39%-11.72%).IA levels were positively correlated with high fasting blood glucose(odds ratio=1.069,P<0.001).The proportion of positive IAs was lowest in patients using glargine only(31.9%)and highest in patients using human insulin only(70.3%),P<*** IA levels in patients using sulfonylureas/glinides(8.3%),metformin(9.6%),and dipeptidyl peptidase-4 inhibitors(8.2%)were all lower than in patients without these drugs(all P<0.05).CONCLUSION Nearly half of patients on insulin therapy have positive IA antibodies,and IA antibody levels are associated with blood glucose *** glargine and a combination of oral glucose-lowering drugs were correlated with lower IA levels.

关键词： Insulin antibodies Insulin therapy Glucose-lowering drugs Glargine Type 2 diabetes

Sustainable electrochemical dearomatization for the synthesis of diverse 2,3-functionalized indolines

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Green Synthesis and Catalysis 2024年第1期5卷 25-30页

作者： Jun Chen Rong zhang Caiyan Ma peng zhang Yonghong zhang Bin Wang Fei Xue Weiwei Jin Yu Xia Chenjiang Liu Urumqi Key Laboratory of Green Catalysis and Synthesis Technology Key Laboratory of Oil and Gas Fine ChemicalsMinistry of Education&Xinjiang Uygur Autonomous RegionState Key Laboratory of Chemistry and Utilization of Carbon Based Energy ResourcesCollege of ChemistryCollege of Future TechnologyXinjiang UniversityUrumqi 830017China

Herein,we achieved a green and efficient dearomatization for the synthesis of 2,3-functionalized polycyclic indolines in an electrochemical *** avoiding of external oxidants and metals approach allowed various nucleophilic sources(Nu¼anilines,TMSN3 and ROH)to perform the products,representing an environmentally benign ***,the continuous flow electrosynthesis and synthetic transformations also reveal the strong practicality of electrochemistry in organic synthesis.

关键词： Green synthesis Organic electrochemistry Indole Dearomatization Cyclization

Data-Driven Design of Single-Atom Electrocatalysts with Intrinsic Descriptors for Carbon Dioxide Reduction Reaction

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Transactions of Tianjin University 2024年第5期30卷 459-469页

作者： Xiaoyun Lin Shiyu Zhen Xiaohui Wang Lyudmila V.Moskaleva peng zhang Zhi-Jian Zhao Jinlong Gong Key Laboratory for Green Chemical Technology of Ministry of Education School of Chemical Engineering and Technology Tianjin University Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) School of Economics and Management Tianjin University of Technology and Education Department of Chemistry University of the Free State Haihe Laboratory of Sustainable Chemical Transformations National Industry-Education Platform of Energy Storage Tianjin University Joint School of National University of Singapore and Tianjin University International Campus of Tianjin University

The strategic manipulation of the interaction between a central metal atom and its coordinating environment in single-atom catalysts（SACs） is crucial for catalyzing the CO2reduction reaction（CO2RR）. However, it remains a major challenge. While density-functional theory calculations serve as a powerful tool for catalyst screening, their time-consuming nature poses limitations. This paper presents a machine learning（ML） model based on easily accessible intrinsic descriptors to enable rapid, cost-effective, and high-throughput screening of efficient SACs in complex systems. Our ML model comprehensively captures the influences of interactions between 3 and 5d metal centers and 8 C, N-based coordination environments on CO2RR activity and selectivity. We reveal the electronic origin of the different activity trends observed in early and late transition metals during coordination with N atoms. The extreme gradient boosting regression model shows optimal performance in predicting binding energy and limiting potential for both HCOOH and CO production. We confirm that the product of the electronegativity and the valence electron number of metals, the radius of metals, and the average electronegativity of neighboring coordination atoms are the critical intrinsic factors determining CO2RR activity. Our developed ML models successfully predict several high-performance SACs beyond the existing database, demonstrating their potential applicability to other systems. This work provides insights into the low-cost and rational design of high-performance SACs.

关键词： CO2 reduction reaction Density functional theory Electrocatalysts High-throughput screening Machine learning

Effects and fate of metal-based engineered nanomaterials in soil ecosystem: A review

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Pedosphere 2024年第5期34卷 843-852页

作者： Qibin WANG peng zhang Weichen ZHAO Shakoor NOMAN Adeel MUHAMMAD Guikai ZHU Yi SUN Quanlong WANG Yaqi JIANG Yukui RUI Beijing Key Laboratory of Farmland Soil Pollution Prevention and Remediation College of Resources and Environmental Sciences China Agricultural University Department of Environmental Science and Engineering University of Science and Technology of China School of Geography Earth and Environmental Sciences University of Birmingham BNU-HKUST Laboratory of Green Innovation Advanced Institute of Natural Sciences Beijing Normal University at Zhuhai China Agricultural University Professor Workstation of Yuhuangmiao Town China Agricultural University Professor Workstation of Sunji Town

Metal-based engineered nanomaterials (MENMs) are increasingly being used in people’s working lives. Although MENMs have important effects on soil ecosystem and play an important role in solving soil environmental problems, the hazards associated with MENMs cannot be ignored. Therefore, more and more scholars have studied the behavior and effects of nanomaterials in soils in recent years. In this review, we explore the articles on MENMs and soil ecosystem retrieved from various databases from 2013 to 2022. We discuss the mechanisms of MENM toxicity, the current state of soil ecosystem, the ecological effects of MENMs on soil microbes, earthworms, and plants, and the ways by which soil organisms take up MENMs. We now know that although MENMs have positive effects on soil ecosystem, their potential hazards are not negligible. Therefore, it is necessary to investigate the effects of MENMs on soil organisms. Meanwhile, we should pay more attention to the negative effects of MENMs on soil ecosystem while exploring their positive effects on soil ecosystem in future research.

关键词： earthworm nanomaterial migration and transformation nanotechnology plant soil microorganism toxicity

Temperature field calculation of rail flash welding

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High-Speed Railway 2024年第2期2卷 116-121页

作者： Rui Xu Min zhang Zhenkun Gao Guo Zhao Wei Ding Shouming Wang peng zhang Xiang Liu Jingjing Li Material Science&Engineering Research Center School of MechanicalElectronic and Control EngineeringBeijing Jiaotong UniversityBeijing 100044China Institute of Metals and Chemistry China Academy of Railway Sciences Group Co.Ltd.Beijing 100081China Department of Industrial and Manufacturing Engineering Pennsylvania State UniversityUniversity ParkPA 16802USA

The forging stage of rail flash welding has a decisive influence on joint strength,and the study of the temperature distribution in the process has an important role in further improving joint *** this paper,three calculation methods for the temperature field are ***,the finite element model of the temperature field before forging rail flash welding is established by using the transient heat module of Ansys software and verified by infrared temperature ***,the temperature distribution of different parts of the rail before flash welding is obtained by using infrared thermal imaging ***,Matlab software is used to calculate the temperature of the non-measured ***,the temperature distribution function along the rail axis is fitted through the temperature measurement *** temperature distribution before the top forging of the rail flash welding can be used to analyze the joint and heat-affected zone organization and properties effectively and to guide the parameter setting and industrial production.

关键词： Flash welding Temperature field Joint strength Software calculation