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ZIF-8 modified by isocyanate as a photocatalytic antibacterial agent

Rare Metals 2024年第6期43卷 2708-2718页

作者： Yi-Ning zhang Zhen pei Zi-Hao Wang Chong-En Wang fen-fen Liang Li-Qiao Wei College of Architecture Taiyuan University of TechnologyTaiyuan 030024China Key Laboratory of Interface Science and Engineering in Advanced Materials of Taiyuan University of Technology Ministry of EducationTaiyuan 030024China Department of Materials Science and Engineering Shanxi Institute of TechnologyYangquan 045000China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030000China

Zeolite imidazole skeleton(ZIF-8)is a promising option for self-cleaning of building exterior walls due to its large specific surface area,high antibacterial activity and low ***,it suffers from low antibacterial efficiency and yield under visible light *** address the issues,we developed the photocatalytic materials T-ZIF-8-TDI(thermally treated-ZIF-8-toluene 2,4-diisocyanate)by modifying ZIF-8 with thermal oxygen sensitization and chemical *** results show that the yield of T-ZIF-8-TDI photocatalytic antibacterial agent is increased to 11.5 times of that of T-ZIF-8,while maintaining the crystal structure of T-ZIF-8 and thermal stability up to 60℃.Furthermore,T-ZIF-8-TDI exhibits extended optical response range to the nearinfrared region,significantly narrowed band gap,improved photogenerated elec tron-hole separation efficiency,reduced recombination rate,and excellent photocatalytic *** the concentration of antibacterial agent is 600 mg·L^(-1),the antibacterial rate of Escherichia coli(***)reaches 99.99%irradiated by visible light for30 min,and when the concentration of antibacterial agent is 200 mg·L^(-1),the antibacterial rate of Staphylococcus aureus(***)reaches 99.99%irradiated by visible light for 25 *** also analyzed the reasons in detail from the aspects of bacterial species and antibacterial mechanism,and proposed the antibacterial mechanism of·O_(2)^(-)and h^(+)as the main active *** findings suggest that T-ZIF-8-TDI photocatalytic antibacterial agent has potential for use in self-cleaning of building exterior walls.

关键词： ZIF-8 Hot oxygen sensitization Modified by isocyanate Antimicrobial performance Photocatalytic antibacterial mechanism

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Nasopharyngeal brushing: a convenient and feasible sampling method for nucleic acid-based nasopharyngeal carcinoma research

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Cancer Communications 2018年第1期38卷 95-104页

作者： pei-fen zhang Xiao-Hui Zheng Xi-Zhao Li Tian Tian Shao-Dan zhang Ye-Zhu Hu Wei-Hua Jia Tumor Resource Bank State Key Laboratory of Oncology in South ChinaCollaborative Innovation Center for Cancer MedicineSun Yat-sen University Cancer Center651 Dongfeng East RoadGuangzhou 510060Guang-dongP.R.China Affiliated Tumor Hospital of Xinjiang Medical University Ürümqi 830000XinjiangP.R.China

Background:Tissue specimens for nasopharyngeal carcinoma(NPC)research are scarce because of sampling *** studies have suggested non-invasive nasopharyngeal brushing as an effective sampling method for NPC *** present study aimed to evaluate the feasibility of nasopharyngeal brushing in the acquisition of NPC nucleic acids for ***:Nasopharyngeal brushing samples were acquired from 24 healthy individuals and 48 NPC *** from 48 NPC and 18 nasopharyngitis patients were collected by endoscopic *** expression levels of tumor suppressor genes(TSGs)and Epstein-Barr virus(EBV)-encoded microRNAs as well as EBV DNA copy number were measured by quantitative polymerase chain reaction in both types of ***:Among six TSGs examined,the expression levels of two genes were significantly decreased in nasopharyn-geal brushing and tissue samples from NPC patients as compared with those from healthy/nasopharyngitis *** EBV-encoded microRNAs,mir-bart1-5p,mir-bart5,mir-bart6-5p,and mir-bart17-5p,were significantly up-regulated in both NPC brushing and tissue samples compared with those from healthy/nasopharyngitis controls(P<0.001).EBV DNA was significantly increased in both nasopharyngeal brushing samples(P<0.001)and tissue sam-ples(P<0.001)from NPC patients in comparison with those from healthy ***:Nasopharyngeal brushing can obtain sufficient tumoral materials for the analysis of viral nucleic acid,including EBV-encoded microRNAs and EBV *** the detection of TSG expression,nasopharyngeal brushings was feasible but inferior to tissue *** study confirms nasopharyngeal brushing as an applicable sampling method that can aid in nucleic acid-based NPC research.

关键词： Nasopharyngeal brushing Tissue samples Nasopharyngeal carcinoma Nucleic acid Cancer research

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Down-regulation amyloid β-protein 42 production by interfering with transcript of presenilin 1 gene with siRNA

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Acta Pharmacologica Sinica 2004年第12期25卷 47-52页

作者： Huan-min LUO2, Hui DENG, Fei XIAO, Qin GAO, Wen WENG, pei-fen zhang, Xiao-guang LI Neuropharmacological Research Laboratory, College ofPharmacy, Ji-nan University, Guangzhou 510632, China Neuropharmacological Research Laboratory College of Pharmacy Ji-nan University Guangzhou 510632 Chin

AIM: To investigate the pathogenesis of Aβ42yielding and new drug targets as well as the possibility of RNA interference (RNAi) technique for treatment of Alzheimer disease (AD). METHODS: Human AD presenilin 1 (PS1) cDNA sequence was obtained from NCBI website. The three sites of RNAi action and one missense control site were selected in PS1 cDNA through online design of Ambion company. To confirm specificity of these sites, we conducted a BLAST search of the IMAGE EST library. The corresponding double-stranded DNA was used to construct pSilencer 3.1-H1 plasmid, which could transcribe small interference RNA (siRNA). Then, the pSliencer 3.1-H1 plasmids were transfected into CHO/PS1/APP cells with SuperFect transfection reagent. The cells have been transfected with the mutant PS1 and APP gene of AD. All the CHO/PS1/APP cells with pSliencer 3.1-H1 plasmids were screened out using G418. Transcripts of PS1 gene in CHO/PS1/APP were measured by RT-PCR, the contents of PS1 peptide and Aβ42 production inside CHO/PS1/APP cells were examined through Western blot and the Aβ42 change of secretion by CHO/PS1/APP was determined with ELISA. RESULTS: The site 3 of PS1 mRNA was inhibited by RNAi after 2 d. The effect was more obvious with the time. The peptide corresponding to PS1 gene and Aβ42 production in CHO/PS1/APP cells were both reduced after siRNA interfere for 3 d. Aβ42 secretion by CHO/PS1/APP cells began to reduce on d 3, and reached the most significance on d 5. There was a time-dependent relationship between the transcript of PS1 gene and the production of Aβ42with RNAi action. CONCLUSION: PS1 is essential for γ-secretase activity. Inhibition of the PS1 can decrease the levels of Aβ42. Some sites of PS1 mRNA, for example, the site 3, may serve as a new drug target and RNAi probably can be used for treatment of AD.

关键词： amyloid beta-protein amyloid beta-protein precursor secretase presenilin-1 RNA interference small-interfering RNA Alzheimer disease

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orecast of peak infection and estimate of excess deaths in COVID-19 transmission and prevalence in Taiyuan City,2022 to 2023

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Infectious Disease Modelling 2024年第1期9卷 56-69页

作者： Jia-Lin Wang Xin-Long Xiao fen-fen zhang Xin pei Ming-Tao Li Ju-Ping zhang Juan zhang Gui-Quan Sun Complex Systems Research Center Shanxi UniversityTaiyuan030006China School of Mathematical Sciences Shanxi UniversityTaiyuan030006China School of Mathematics North University of ChinaTaiyuan030051China College of Mathematics Taiyuan University of TechnologyTaiyuan030024China Complex Systems and Data Science Key Laboratory of Ministry of Education Taiyuan030006China

In this paper,with the method of epidemic dynamics,we assess the spread and prevalence of COVID-19 after the policy adjustment of prevention and control measure in December 2022 in Taiyuan City in China,and estimate the excess population deaths caused by *** on the transmission mechanism of COVID-19 among individuals,a dynamic model with heterogeneous contacts is established to describe the change of control measures and the population's social behavior in Taiyuan *** model is verified and simulated by basing on reported case data from November 8th to December 5th,2022 in Taiyuan city and the statistical data of the questionnaire survey from December 1st to 23rd,2022 in Neijiang *** with reported numbers of permanent residents and deaths from 2017 to 2021 in Taiyuan city,we apply the dynamic model to estimate theoretical population of 2022 under the assumption that there is no effect of *** addition,we carry out sensitivity analysis to determine the propagation character of the Omicron strain and the effect of the control *** a result of the study,it is concluded that after adjusting the epidemic policy on December 6th,2022,three peaks of infection in Taiyuan are estimated to be from December 22nd to 31st,2022,from May 10th to June 1st,2023,and from September 5th to October 13th,2023,and the corresponding daily peaks of new cases can reach 400000,44000 and 22000,*** the end of 2022,excess deaths can range from 887 to 4887,and excess mortality rate can range from 3.06%to 14.82%.The threshold of the infectivity of the COVID-19 variant is estimated 0.0353,that is if the strain infectivity is above it,the epidemic cannot be control with the previous normalization measures.

关键词： Taiyuan city COVID-19 Dynamic model Epidemic scale Epidemic peak Excess death

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High-efficiently doping nitrogen in kapok fiber-derived hard carbon used as anode materials for boosting rate performance of sodium-ion batteries

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Journal of Energy Chemistry 2024年第9期96卷 472-482页

作者： Tianyun zhang Tian zhang Fujuan Wang fen Ran School of Mechanical and Electronical Engineering Lanzhou University of TechnologyLanzhou 730050GansuChina State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals School of Materials Science and EngineeringLanzhou University of TechnologyLanzhou 730500GansuChina

The engineering of plant-based precursor for nitrogen doping has become one of the most promising strategies to enhance rate capability of hard carbon materials for sodium-ion batteries;however,the poor rate performance is mainly caused by lack of pyridine nitrogen,which often tends to escape because of high temperature in preparation process of hard *** this paper,a high-rate kapok fiber-derived hard carbon is fabricated by cross-linking carboxyl group in 2,6-pyridinedicarboxylic acid with the exposed hydroxyl group on alkalized kapok with assistance of zinc ***,a high nitrogen doping content of 4.24%is achieved,most of which are pyridine nitrogen;this is crucial for improving the defect sites and electronic conductivity of hard *** optimized carbon with feature of high nitrogen content,abundant functional groups,degree of disorder,and large layer spacing exhibits high capacity of 401.7 mAh g^(−1)at a current density of 0.05 A g^(−1),and more importantly,good rate performance,for example,even at the current density of 2 A g^(−1),a specific capacity of 159.5 mAh g^(−1)can be *** findings make plant-based hard carbon a promising candidate for commercial application of sodium-ion batteries,achieving high-rate performance with the enhanced pre-cross-linking interaction between plant precursors and dopants to optimize aromatization process by auxiliary pyrolysis.

关键词： Kapok fiber Hard carbon Electrode materials Rate performance Sodium-ion batteries

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Preparation of bifunctional electrocatalyst by recycling heavy metal ions from wastewater using EDTAD-functionalized MOF as highly efficient adsorbent

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Rare Metals 2024年第10期43卷 5105-5116页

作者： Yue Qian pei-Xue Fu Rui-Ze Yin Han-Ni Yang Si-Yang Li Wei-Wei Xiong fen-fen Zheng Jun-Hao zhang Ai-Hua Yuan Huan Pang School of Environmental and Chemical Engineering Jiangsu University of Science and Technology School of Chemistry and Chemical Engineering Yangzhou University

The recovery and subsequent reuse of heavy metal ions from industrial wastewater are crucial for promoting sustainable development,but they also presen significant *** this article,ethylenediaminetetraacetic dianhydride （EDTAD）,which possesses strong metal chelating ability,is covalently attached to MIL-101-NH2（Fe）,resulting in a significant improvement in the removal rate of heavy metal ions in ***,the recovered waste metal ions are transformed into high-performance feni3/NiFe2O4@NC dual-functional oxygen evolution reaction （OER） and oxygen reduction reaction （ORR） ***,feni3/NiFe2O4@NC exhibits outstanding OER performance,with only a264 mV overpotential at 10 mA·*** functiona theory （DFT） calculations reveal that the synergistic effect of the feni3/NiFe2O4@NC heterostructure can enhance conductivity,optimize the free energy of*to OH*during OER reaction,and promote catalytic *** work not only improves the removal rate of heavy metal ions but also obtains high-performance catalysts,while providing a new approach for the treatment and secondary utilization of heavy metal ion wastewater as well as the preparation of low-cost catalysts.

关键词： Bifunctional electrocatalyst Covalently modified MOF Ethylenediaminetetraacetic dianhydride Heavy metals

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Recent Progress in Improving Rate Performance of Cellulose-Derived Carbon Materials for Sodium-Ion Batteries

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Nano-Micro Letters 2024年第8期16卷 102-147页

作者： Fujuan Wang Tianyun zhang Tian zhang Tianqi He fen Ran State Key Laboratory of Advanced Processing and Recycling of Non‑Ferrous Metals Lanzhou University of TechnologyLanzhou 730050People’s Republic of China School of Materials Science and Engineering Lanzhou University of TechnologyLanzhou 730050People’s Republic of China School of Mechanical and Electronical Engineering Lanzhou University of TechnologyLanzhou 730050People’s Republic of China

Cellulose-derived carbon is regarded as one of the most promising candidates for high-performance anode materials in sodium-ion batteries;however,its poor rate performance at higher current density remains a challenge to achieve high power density sodium-ion *** present review comprehensively elucidates the structural characteristics of cellulose-based materials and cellulose-derived carbon materials,explores the limitations in enhancing rate performance arising from ion diffusion and electronic transfer at the level of cellulose-derived carbon materials,and proposes corresponding strategies to improve rate performance targeted at various precursors of cellulose-based *** review also presents an update on recent progress in cellulose-based materials and cellulose-derived carbon materials,with particular focuses on their molecular,crystalline,and aggregation ***,the relationship between storage sodium and rate performance the carbon materials is elucidated through theoretical calculations and characterization ***,future perspectives regarding challenges and opportunities in the research field of cellulose-derived carbon anodes are briefly highlighted.

关键词： Cellulose Hard carbon Anode materials Rate performance Sodium-ion batteries

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A comprehensive research on wear resistance of GH4169 superalloy in longitudinal-torsional ultrasonic vibration side milling with tool wear and surface quality

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Chinese Journal of Aeronautics 2024年第4期37卷 556-573页

作者： Baoqi CHANG Zhaoxi YI fen zhang Lian DUAN Ji-an DUAN School of Mechanical and Electrical Engineering Central South UniversityChangsha 410083China State Key Laboratory of High Performance and Complex Manufacturing Central South UniversityChangsha 410083China School of Physics and Electronics Central South UniversityChangsha 410083China

To improve the service and machining performance of the workpiece, the tool wear mechanisms, surface machining quality, and wear resistance in conventional side milling(CSM)and longitudinal-torsional ultrasonic vibration side milling(LTUVSM) of GH4169 superalloy at different cutting lengths are investigated systematically. Tool wear mechanisms are revealed and the correlation between machined surface quality with tool wear is analyzed correspondingly. Tool wear patterns mainly include adhesive wear, diffusion wear, abrasive wear, and chipping *** surface quality is achieved in LTUVSM due to a maximum reduction of flank wear bandwidth and wear rate by 71.9% and 71.5%, respectively, compared to CSM. The friction coefficient,initial wear stage time, and wear volume of dry sliding wear were measured to evaluate the workpiece wear resistance. The maximum reductions in friction coefficient and wear volume in LTUVSM are 18.2% and 15.8% compared to CSM. The regular ultrasonic vibration textures suppress the friction and the growth of contact nodes in the contact area, decreasing the degree of surface wear, which is demonstrated by a 38.8% increase in initial wear stage time compared to *** conclusion, the workpiece in LTUVSM exhibits higher wear resistance because of the improvement of tool wear and the guarantee of surface quality.

关键词： Dry sliding wear Surface quality Tool wear Ultrasonic vibration Wear resistance

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Evaluation and Projection of Extreme High Temperature Indices in Southwestern China Using NEX-GDDP-CMIP6

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Journal of Meteorological Research 2024年第1期38卷 88-107页

作者： fen zhang Linxiao WEI Yonghua LI Hongyu TANG Tianyu zhang Baogang YANG China Meteorological Administration Key Open Laboratory of Transforming Climate Resource to Economy Chongqing Climate CentreChongqing 401147

Based on the recently released NASA Earth Exchange Global Daily Downscaled Projections(NEX-GDDP)Coupled Model Intercomparison Project Phase 6(CMIP6) dataset and the gridded observational daily dataset CN05.1, this study evaluates the performance of 26 CMIP6 models in simulating extreme high temperature(EHT) indices in southwestern China and estimates future changes in the EHT indices under the Shared Socioeconomic Pathways(SSPs) SSP1-2.6, SSP2-4.5, and SSP5-8.5 using 11 optimal CMIP6 models. Five EHT indices are employed:annual maximum value of daily maximum temperature(TXX), high temperature days(T35), warm days(TX90P),heat wave frequency(HWF), and heat wave days(HWD). The main results are as follows.(1) NEX-GDDP-CMIP6 is highly capable of simulating the spatial patterns of TXX and T35 in southwestern China but it presents a weaker ability to simulate the spatial patterns of TX90P, HWF, and HWD.(2) The simulated time series of T35, TX90P, HWF,and HWD in southwestern China exhibit consistent upward trends with the observations. The linear trends of increase in TX90P and HWD are much greater than those of increase in TXX, T35, and HWF.(3) The estimated increases in TXX and T35 in southwestern China are significantly greater in Chongqing and the adjacent areas of Sichuan than in the other regions. Spatial distributions of the increases in TX90P, HWF, and HWD generally show higher values in the west and lower values in the east.(4) In the three different scenarios, the projected future TXX,T35, TX90P, and HWD in southwestern China all display a continuous increase with time and radiative forcing levels, whereas HWF initially increases but then decreases under the SSP5-8.5 scenario. By the end of the 21st century, under the SSP5-8.5 scenario, TXX and T35 are projected to increase by 6.0℃ and 45.0 days, respectively. The duration of individual heat waves is also expected to increase.

关键词： NEX-GDDP-CMIP6 extreme high temperature(EHT) southwestern China evaluation projection

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Double contrast-enhanced ultrasonography improves diagnostic accuracy of T staging compared with multi-detector computed tomography in gastric cancer patients

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World Journal of Gastroenterology 2024年第23期30卷 3005-3015页

作者： Yan-fen Xu Hui-Yun Ma Gui-Ling Huang Yu-Ting zhang Xue-Yan Wang Ming-Jie Wei Xiao-Qing pei Department of Ultrasound State Key Laboratory of Oncology in South ChinaGuangdong Key Laboratory of Nasopharyngeal Carcinoma Diagnosis and TherapyGuangdong Provincial Clinical Research Center for CancerSun Yat-sen University Cancer CenterGuangzhou 510060Guangdong ProvinceChina Department of Radiology State Key Laboratory of Oncology in South ChinaGuangdong Key Laboratory of Nasopharyngeal Carcinoma Diagnosis and TherapyGuangdong Provincial Clinical Research Center for CancerSun Yat-sen University Cancer CenterGuangzhou 510060Guangdong ProvinceChina Department of Medical Ultrasound State Key Laboratory of Oncology in South ChinaGuangdong Key Laboratory of Nasopharyngeal Carcinoma Diagnosis and TherapyGuangdong Provincial Clinical Research Center for CancerSun Yat-sen University Cancer CenterGuangzhou 510060Guangdong ProvinceChina

BACKGROUND Gastric cancer(GC)is the most common malignant tumor and ranks third for cancer-related deaths among the *** disease poses a serious public health problem in China,ranking fifth for incidence and third for *** of the invasive depth of the tumor is vital to treatment *** To evaluate the diagnostic performance of double contrast-enhanced ultrasonography(DCEUS)for preoperative T staging in patients with GC by comparing with multi-detector computed tomography(MDCT).METHODS This single prospective study enrolled patients with GC confirmed by preoperative gastroscopy from July 2021 to March *** underwent DCEUS,including ultrasonography(US)and intravenous contrast-enhanced ultrasonography(CEUS),and MDCT examinations for the assessment of preoperative T *** of GC were identified on DCEUS and criteria developed to evaluate T staging according to the 8th edition of AJCC cancer staging *** diagnostic performance of DCEUS was evaluated by comparing it with that of MDCT and surgical-pathological findings were considered as the gold *** A total of 229 patients with GC(80 T1,33 T2,59 T3 and 57 T4)were *** accuracies were 86.9%for DCEUS and 61.1%for MDCT(P<0.001).DCEUS was superior to MDCT for T1(92.5%vs 70.0%,P<0.001),T2(72.7%vs 51.5%,P=0.041),T3(86.4%vs 45.8%,P<0.001)and T4(87.7%vs 70.2%,P=0.022)staging of *** DCEUS improved the diagnostic accuracy of preoperative T staging in patients with GC compared with MDCT,and constitutes a promising imaging modality for preoperative evaluation of GC to aid individualized treatment decision-making.

关键词： Double contrast-enhanced ultrasonography Multi-detector computed tomography Gastric cancer T staging

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