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Exploring innovative synthetic solutions for advanced polymer-based electrochromic energy storage devices:Phenoxazine as a promising chromophore

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Journal of Energy Chemistry 2024年第4期91卷 433-452页

作者： Catalin-paul Constantin Mihaela Balan-Porcarasu Gabriela Lisa “Petru Poni”Institute of Macromolecular Chemistry Electroactive Polymers&Plasmochemistry Laboratory41A Grigore Ghica Voda AlleyIasi 700487Romania “Gh.Asachi”Technical University Iasi Faculty of Chemical EngineeringBd.Mangeron 71Iasi 700050Romania

The current investigation offers an innovative synthetic solution regarding electrochromic(EC)and energy storage applications by exploring phenoxazine(POZ)***,three POZ-based polymers(polyimide,polyazomethine,and polyamide)were synthesized to ascertain the superior *** polyamide exhibited remarkable attributes,including high redox stability during 500 repetitive CVs,optical contrast of 61.98%,rapid response times of 1.02 and 1.38 s for coloring and bleaching,EC efficiency of 280 cm^(2)C^(-1).and decays of the optical density and EC efficiency of only 12.18%and 6.23%after 1000 ***,the energy storage performance of polyamide PA was tested,for which the following parameters were obtained:74.7 F g^(-1)(CV,scan rate of 10 mV s^(-1))and 118 F g^(-1)(GCD,charging current of 0.1 A g^(-1)).Then,the polyamide was tested in EES devices,which yielded the following EC parameters:an optical contrast of 62.15%,response times of 9.24 and 5.01 s for coloring and bleaching,EC efficiency of 178 cm^(2)C^(-1),and moderate decays of 20.25%and 23.24%for the optical density and EC efficiency after 500 *** energy storage performance included a capacitance of 106 F g^(-1)(CV,scan rate of 0.1 mV s^(-1))and 9.23 F g^(-1)(GCD,charging current of 0.1 A g^(-1)),capacitance decay of 11.9%after500 cycles,and 1.7 V retention after 2 ***,two EES devices connected in series powered a 3 V LED for almost 30 s.

关键词： Polymers Phenoxazine Electrochromic Energy storage Electrochromi cenergy storage devices

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Geospatial Analysis of Urban Heat Island Effects and Tree Equity

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Open Journal of Forestry 2024年第1期14卷 1-18页

作者： Jillian Gorrell Sharon R. Jean-Philippe paul D. Ries Jennifer K. richards Neelam C. Poudyal Rochelle Butler School of Natural Resources University of Tennessee 203 Third Creek Building Knoxville Tennessee USA

In recent decades, Urban Heat Island Effects have become more pronounced and more widely examined. Despite great technological advances, our current societies still experience great spatial disparity in urban forest access. Urban Heat Island Effects are measurable phenomenon that are being experienced by the world’s most urbanized areas, including increased summer high temperatures and lower evapotranspiration from having impervious surfaces instead of vegetation and trees. Tree canopy cover is our natural mitigation tool that absorbs sunlight for photosynthesis, protects humans from incoming radiation, and releases cooling moisture into the air. Unfortunately, urban areas typically have low levels of vegetation. Vulnerable urban communities are lower-income areas of inner cities with less access to heat protection like air conditioners. This study uses mean evapotranspiration levels to assess the variability of urban heat island effects across the state of Tennessee. Results show that increased developed land surface cover in Tennessee creates measurable changes in atmospheric evapotranspiration. As a result, the mean evapotranspiration levels in areas with less tree vegetation are significantly lower than the surrounding forested areas. Central areas of urban cities in Tennessee had lower mean evapotranspiration recordings than surrounding areas with less development. This work demonstrates the need for increased tree canopy coverage.

关键词： Spatial Analysis Land Cover Urban Heat Island Effect (UHIE) Evapotranspiration Tree Canopy Impervious Surface GIS Prediction Model GIS Machine Learning

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Plant-available water capacity of soils at a regional scale:Analysis of fixed and dynamic field capacities

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Pedosphere 2024年第3期34卷 590-605页

作者： Vinod PHOGAT paul RPETRIE Casandra COLLINS Marcos BONADA South Australian Research and Development Institute GPO Box 397Adelaide SA 5001(Australia) School of Agriculture Food and WineWaite Research InstituteUniversity of AdelaideWaite CampusPMB1Glen Osmond SA 5064(Australia) College of Science and Engineering Flinders UniversityBedford Park SA 5042(Australia) The University of New South Wales Sydney NSW 2052(Australia) ARC Training Centre for Innovative Wine Production University of AdelaidePMB1Glen Osmond SA 5064(Australia)

Estimation of the plant-available water capacity(PAWC)of soils at a regional scale helps in adopting better land use planning,developing suitable irrigation schedules for crops,and optimizing the use of scarce water *** the current study,72 soil profiles were sampled from the Barossa region of South Australia to estimate pedo-transfer functions deduced from easily estimated soil *** functions were then used to estimate the fixed(10 and 33 kPa)and dynamic pressure head(h_(fc))water contents at field capacity(FC)for minimum drainage flux(0.01 and 0.001 cm d^(-1)),which serves as the upper boundary for plant-available water in *** estimated residual water content was corrected for subsoil constraints,especially the exchangeable sodium percentage(ESP).The results showed that the mean values of h_(fc)in sand-dominated light and medium textured soils(i.e.,sand,loamy sand,sandy loam,and loam)varied in a narrow range(15.8-18.2 kPa),whereas those in the clay-dominated heavy textured soils(i.e.,clay loam)showed a wide range(11.3-49.3 kPa).There were large differences in PAWC for dynamic FC(PAWC_(fc))and fixed FC at 10 kPa(PAWC10),33 kPa(PAWC33),and a mix of 10and 33 kPa(PAWC_(10,33))pressure heads depending on soil ***,the difference between PAWC at 10 kPa and h_(fc)(ΔPAWC_(10))was positive,whereas that between 33 kPa and h_(fc)(ΔPAWC_(33))was negative across all ***,the estimation of PAWC assuming a fixed FC at 10 and 33 kPa pressures(i.e.,PAWC_(10,33))for sandy,clay,and silty soils reduced the difference between fixed and dynamic pressure PAWCs to<10% across the *** estimation of PAWC was improved by incorporating the impact of subsoil constraints,such as high ESP,which was more pronounced for clay and silty *** findings demonstrate the inherent inconsistencies between static pressure and flux-based dynamic FC estimations in *** heterogeneity,intra-texture variability,subsoil constraints,and swell

关键词： crop lower limit drained upper limit pedo-transfer function soil hydraulic parameter soil texture

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Combining neural progenitor cell transplant and rehabilitation for enhanced recovery after cervical spinal cord injury

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Neural Regeneration Research 2024年第7期19卷 1433-1434页

作者： Camila M.Freria paul Lu Department of Neurosciences University of CaliforniaSan DiegoLa JollaCAUSA Veterans Administration San Diego Healthcare System San DiegoCAUSA

Efforts to promote recovery of function after human spinal cord injury(SCI) will likely require interventions to rgeting the corticospinal tract(CST) motor system:the most important pathway for voluntary motor control in *** system has historically been the most refractory to regenerative efforts after *** "nonregeneration" of the CST changed when robust regeneration of the CST into spared tissue was demonstrated by the inactivation of phosphatase and tensin homolog and delivery of inosine.

关键词： cervical progenitor injury

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Governance of decentralized autonomous organizations that produce open source software

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BLOCKCHAIN-RESEARCH AND APPLICATIONS 2024年第1期5卷 10-30页

作者： van Vulpen, paul Siu, Jozef Jansen, Slinger Univ Utrecht Dept Informat & Comp Sci NL-3584 CS Utrecht Netherlands Centric Publ Sect Solut NL-2803 PB Gouda Netherlands

Decentralized autonomous organizations (DAOs) have found use in the governance of open source software (OSS) projects. However, the governance of an OSS producing DAO should match the particularities of OSS production while also overcoming the existing challenges of decentralized governance. The existing decentralized governance frameworks do not include all the governance activities of OSS projects. Therefore, this study presents a governance framework for DAOs that produce OSS. The framework is built upon a total of 34 articles on DAO and OSS governance. The framework was evaluated in three leading DAOs that produce OSS. The evaluation underscores the significance of the framework and proves the potential of the systematic categorization of governance mechanisms. Finally, we list emerging governance practices in various governance domains in this developing field.

关键词： Decentralized autonomous organizations Open source software Governance framework Blockchain Decentralized governance Case study research PROJECTS MOTIVATION DESIGN

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Utilization of Pyrrolic Compounds as Indicators of Secondary Migration for Woodford Oils in the Anadarko Basin, Oklahoma, USA

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Journal of Earth Science 2024年第5期35卷 1499-1512页

作者： Mu Liu R.paul Philp Key Laboratory of Cenozoic Geology and Environment Institute of Geology and GeophysicsChinese Academy of Sciences School of Geosciences University of Oklahoma

Migration pathways and distances of the oils in reservoir are thought to affect the distribution of pyrrolic compounds such as carbazole, its alkyl derivatives(alkylated carbazoles) and benzocarbazoles, although other factors, including maturity and depositional environments may also affect the distribution of these organic nitrogen compounds. In this study, 14 oil samples produced from conventional reservoirs in pauls Valley, south Oklahoma were investigated using organic geochemical techniques. The sterane and hopane fingerprints suggest that most of the oils were sourced from the Devonian Woodford shale. Maturity parameters consistently indicate that the maturity level of the studied samples are all of similar maturity(Rc = ～0.7%), suggesting the distribution of the organic nitrogen organic compounds is possibly reflecting variations in relative migration distances. The distribution of alkylcarbazoles revealed a preferential enrichment during migration, with the nitrogen-shielded alkylcarbazole tending to be enriched relative to the nitrogen-semi-shielded alkylcarbozoles particularly in oils produced close to the Arbuckle uplift to the east. Correspondingly, another family of pyrrolic compounds, benzocarbazoles, whose distributions also indicated that the pauls Valley Woodford oils came from deeper part of the Anadarko Basin as the benzo-[a]/([a]+[c])-carbazole ratios decrease eastwards. In more specific migration systems, although the pyrrolic compound indicators are potentially disturbed by the structural complexes, the general migration directions suggest that the studied oils in pauls Valley Hunton uplift were sourced from the deep basin area, and migrate upwards in porous sediments due to the buoyancy. This study investigates the feasibility of using pyrrolic compounds to estimate relative migration distances and will aid in the interpretation of migration history by using the distribution of carbazole, alkylated carbazoles, benzocarbazoles isomers in the An

关键词： carbazole migration oil Oklahoma biomarker organic geochemistry

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The penetration depth of atomic radicals in tubes with catalytic surface properties

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Plasma Science and Technology 2024年第7期26卷 157-164页

作者： Domen paul Miran MOZETIC Rok ZAPLOTNIK Alenka VESEL Gregor PRIMC Denis DONLAGIC Jozef Stefan Institute Jamova Cesta 39Ljubljana 1000Slovenia Jozef Stefan International Postgraduate School Jamova Cesta 39Ljubljana 1000Slovenia Faculty of Electrical Engineering and Computer Science University of MariborKoroska Cesta 46Maribor 2000Slovenia

Catalysis of molecular radicals is often performed in interesting experimental *** possible configuration is tubular *** radicals are introduced into the tubes on one side,and stable molecules are exhausted on the other *** penetration depth of radicals depends on numerous parameters,so it is not always feasible to calculate *** article presents systematic measurements of the penetration depth of oxygen atoms along tubes made from nickel,cobalt,and *** source of O atoms was a surfatron-type microwave *** initial density of O atoms depended on the gas flow and was 0.7×10^(21)m^(-3),2.4×10^(21)m^(-3),and 4.2×10^(21)m^(-3)at the flow rates of 50,300,and 600 sccm,and pressures of 10,35,and 60 Pa,*** gas temperature remained at room temperature throughout the *** dissociation fraction decreased exponentially along the length of the tubes in all *** penetration depths for well-oxidized nickel were 1.2,1.7,and 2.4 cm,*** cobalt,they were slightly lower at 1.0,1.3,and 1.6 cm,respectively,while for copper,they were 1.1,1.3,and 1.7 cm,*** results were explained by gas dynamics and heterogeneous surface *** data are useful in any attempt to estimate the loss of molecular fragments along tubes,which serve as catalysts for the association of various radicals to stable molecules.

关键词： oxygen plasma penetration depth catalysis heterogeneous surface recombination atom loss

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Pressurized environments directly influence friction and wear of dry steel contacts—Investigations in a novel high fluid pressure tribometer

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Friction 2024年第7期12卷 1599-1617页

作者： paul REICHLE Jakob BARZ Georg UMLAUF Günter E.M.TOVAR Institute of Interfacial Process Engineering and Plasma Technology(IGVP) University of StuttgartStuttgart 70569Germany Fraunhofer Institute for Interfacial Engineering and Biotechnology(IGB) Stuttgart 70569Germany

To reduce the usage of classical lubricants in deep drawing,a new tribological system based on volatile lubricants was ***,a volatile medium is injected under high pressure into the interstice between drawing tool and sheet *** on temperature and pressure,the temporary lubricant may exist in its gaseous or liquid *** this study,a novel high fluid pressure tribometer was designed to investigate the friction and wear of dry steel contacts under comparable conditions like in dry deep ***,a new ball-on-disc tribometer was designed and integrated into a high-pressure *** specifically investigate the effects of different environments(technical air,liquid and gaseous carbon dioxide,nitrogen,argon)at atmospheric and high pressure(0.1 MPa,6 MPa)on tribology,the specimens and all components were operating *** the experiments,the friction was measured *** show that the highest friction occurs in air and the lowest in carbon dioxide *** to the experiments,the wear of the specimens was assessed along with changes in surface chemistry related to tribochemical ***,the tribology of the dry sliding contacts is correlated to changes of the surface *** differences as well as similarities regarding the different fluid environments are *** the results show,the differences between the media used are most pronounced at elevated ***,this work gives clear indications on the suitability of volatile lubricants in dry friction or rather gas lubrication,especially for dry deep drawing.

关键词： dry friction and dry wear gas lubrication carbon dioxide tribo-layer dry metal forming

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Quasi-static and dynamic compressive behaviour of additively manufactured Menger fractal cube structures

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Defence Technology（防务技术） 2024年第7期37卷 39-49页

作者： Damith Mohotti Dakshitha Weerasinghe Madhusha Bogahawaththa Hongxu Wang Kasun Wijesooriya paul JHazell School of Engineering and Technology UNSWCanberraACT2600Australia School of Civil Mining and Environmental EngineeringFaculty of Engineering and Information SciencesUniversity of WollongongWollongongNSWAustralia

This paper presents the first-ever investigation of Menger fractal cubes'quasi-static compression and impact *** cubes with different void ratios were 3D printed using polylactic acid(PLA)with dimensions of 40 mm×40 mm×40 *** different orders of Menger cubes with different void ratios were considered,namely M1 with a void ratio of 0.26,M2 with a void ratio of 0.45,and M3with a void ratio of ***-static Compression tests were conducted using a universal testing machine,while the drop hammer was used to observe the behaviour under impact *** fracture mechanism,energy efficiency and force-time histories were *** the structured nature of the void formation and predictability of the failure modes,the Menger geometry showed some promise compared to other alternatives,such as foams and *** the increasing void ratio,the Menger geometries show force-displacement behaviour similar to hyper-elastic materials such as rubber and *** third-order Menger cubes showed the highest energy absorption efficiency compared to the other two geometries in this *** findings of the present work reveal the possibility of using additively manufactured Menger geometries as an energy-efficient system capable of reducing the transmitting force in applications such as crash barriers.

关键词： Additive manufacturing Fractal geometries Menger cube Energy absorption Quasi-static

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New insights into protein–polysaccharide complex coacervation:Dynamics,molecular parameters,and applications

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Aggregate 2024年第1期5卷 148-166页

作者： Jiabao Zheng paul Van der Meeren Weizheng Sun School of Food Science and Engineering South China University of TechnologyGuangzhouChina Department of Green Chemistry and Technology Faculty of Bioscience EngineeringGhent UniversityGhentBelgium Overseas Expertise Introduction Center for Discipline Innovation of Food Nutrition and Human Health(111 Center) GuangzhouChina

For more than a decade,the discovery of liquid–liquid phase separation within living organisms has prompted colloid scientists to understand the connection between coacervate functionality,phase behavior,and dynamics at a multidisciplinary *** the protein–polysaccharide was the first system in which the coacervation phenomenon was discovered and is widely used in food systems,the phase state and relaxation dynamics of protein–polysaccharide complex coacervates(PPCC)have rarely been discussed ***,this review aims to unravel the relationship between PPCC dynamics,thermodynamics,molecular architecture,applications,and phase states in past *** ahead,solving the way molecular architecture spreads to macro-functionality,that is,establishing the relationship between molecular architecture–dynamics–application,will catalyze novel advancements in PPCC research within the field of foods and biomaterials.

关键词： dynamics encapsulation liquid coacervate protein-polysaccharide complex coacervation solid precipitate

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