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Science China Chemistry 2025年第1期 192-200页

作者： Dongying Wang Shulan pu Yongmin Chen Ke Lei Yujie Duan Linjiao Mao Xuhui Zeng Xi Luo Yuntao Zhang Yuqin Dong Jin Zhong Zhang Yan Sun School of Mechanical Engineering Chengdu University Department of Chemistry and Biochemistry University of California

Potassium ions （K+） doped graphitic carbon nitride （g-C3N4） was prepared by a thermal etching method using potassium hydroxide （KOH） as an ion *** transform infrared spectroscopy （FTIR） and X-ray photoelectron spectroscopy （XPS）results showed that the generation of the cyano group was detected while introducing K+.Under simulated sunlight irradiation,the sample with a K+doping amount of 10%showed the highest hydrogen peroxide （H2O2） generation rate of2,140.2μmol *** apparent quantum yield （AQY） at 400 nm and the solar-to-chemical conversion （SCC） are 4.35%and1.23%,respectively.K+acted as a bridge between g-C3N4layers,which enhanced charge transfer ***,the cyano group enhanced the adsorption capacity of protons （H+） and promoted the yield of *** catalyst exhibited excellent photocatalytic stability based on four-cycle *** addition,a mechanism study showed that superoxide radicals （·O2-）were the most important active species in the reaction *** production of H2O2was achieved through consecutive single-electron *** study deepens the understanding of the oxygen reduction reaction process and opens up a new venue for improving H2O2generation.

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Maintaining moderate levels of hypochlorous acid promotes neural stem cell proliferation and differentiation in the recovery phase of stroke

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Neural Regeneration Research 2025年第3期20卷 845-857页

作者： Lin-Yan Huang Yi-De Zhang Jie Chen Hai-Di Fan Wan Wang Bin Wang Ju-Yun Ma Peng-Peng Li Hai-Wei pu Xin-Yian Guo Jian-Gang Shen Su-Hua Qi School of Medical Technology Xuzhou Key Laboratory of Laboratory DiagnosticsXuzhou Medical UniversityXuzhouJiangsu ProvinceChina School of Pharmacy Xuzhou Medical UniversityXuzhouJiangsu ProvinceChina Department of Laboratory Medicine Branch Hospital of Huai’an First People’s HospitalHuai’anJiangsu ProvinceChina Department of Laboratory Medicine the Affiliated Hospital of Xuzhou Medical UniversityXuzhouJiangsu ProvinceChina School of Chinese Medicine The University of Hong KongHong Kong Special Administrative RegionChina

It has been shown clinically that continuous removal of ischemia/reperfusion-induced reactive oxygen species is not conducive to the recovery of late ***,previous studies have shown that excessive increases in hypochlorous acid after stroke can cause severe damage to brain *** previous studies have found that a small amount of hypochlorous acid still exists in the later stage of stroke,but its specific role and mechanism are currently *** simulate stroke in vivo,a middle cerebral artery occlusion rat model was established,with an oxygen-glucose deprivation/reoxygenation model established in vitro to mimic *** found that in the early stage(within 24 hours)of ischemic stroke,neutrophils produced a large amount of hypochlorous acid,while in the recovery phase(10 days after stroke),microglia were activated and produced a small amount of hypochlorous ***,in acute stroke in rats,hypochlorous acid production was prevented using a hypochlorous acid scavenger,taurine,or myeloperoxidase inhibitor,4-aminobenzoic acid *** results showed that high levels of hypochlorous acid(200μM)induced neuronal apoptosis after oxygen/glucose deprivation/***,in the recovery phase of the middle cerebral artery occlusion model,a moderate level of hypochlorous acid promoted the proliferation and differentiation of neural stem cells into neurons and *** suggests that hypochlorous acid plays different roles at different phases of cerebral ischemia/reperfusion *** levels of hypochlorous acid(5 and 100μM)promoted nuclear translocation ofβ-*** transfection of single-site mutation plasmids,we found that hypochlorous acid induced chlorination of theβ-catenin tyrosine 30 residue,which promoted nuclear ***,our study indicates that maintaining low levels of hypochlorous acid plays a key role in the recovery of neurological function.

关键词： cell differentiation cerebral ischemia/reperfusion injury chlorination hypochlorous acid microglia neural stem cell neurogenesis nuclear translocation stroke β-catenin

Progress of crystalline carbon nitride in synthesis,atomic structure characterization and photocatalysis

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Nano Research 2025年第1期18卷 455-476页

作者： Yueyang Tan Zhongyan Zhang Yayun pu Zongzhao Sun Limin Huang School of Materials Science and Engineering Harbin Institute of TechnologyHarbin 150001China Department of Chemistry Southern University of Science and TechnologyShenzhen 518055China School of Traffic and Environment Shenzhen Institute of Information TechnologyShenzhen 518172China College of Chemistry and Chemical Engineering Linyi UniversityLinyi 276000China School of Optoelectronic Engineering Chongqing University of Posts and TelecommunicationsChongqing 400065China

Crystalline carbon nitride(CCN)has emerged as a highly promising semiconductor photocatalyst with unique properties,such as enhanced charge migration rate,reduced carrier recombination probability,narrow band gap and improved light-harvesting efficiency,which are suitable for a wide range of applications in solar-to-chemical conversion,energy storage,therapeutic and environmental pollution *** the past few years,there has been an increasing number of reviews on CCN ***,most of these reviews mainly focus on synthesis methods,modification and applications,with less emphasis on the relationship between structures and properties,as well as on indepth exploration of the crystalline *** electronic instability of CCN presents challenges for conventional characterization techniques to directly and thoroughly investigate the relationship between its intrinsic atom structure and photocatalytic *** mini-review not only highlights the progress in CCN-based photocatalysts,with a focus on molten-salt synthesis(including solid-salt-induced crystallization),but also emphasizes the atomic structure characterization by specifically introducing the differential phase contrast(DPC)scanning transmission electron microscopy(STEM)technique,which is essential for enhancing our understanding of the crystal structure and photocatalytic mechanisms of ***,the review outlines the photocatalytic performance and puts forward potential challenges on CCN *** review will provide a clearer understanding of the relationship in developing precise customization strategies for CCN materials and ultimately explain the regularity and specificity of the enhanced performance in targeted photocatalytic systems.

关键词： crystalline carbon nitride synthesis characterization photocatalysis

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运动干预与细胞焦亡在骨关节炎中的作用

中国组织工程研究 2025年第8期29卷 1667-1675页

作者：王秋月靳攀蒲锐长江大学教育与体育学院湖北省荆州市434023 长江大学医学部湖北省荆州市434023 长江大学运动人体科学实验室湖北省荆州市434023

背景:细胞焦亡参与软骨细胞外基质降解、滑膜炎症以及疼痛,在骨关节炎防治中发挥重要作用。此外,运动可通过抑制细胞焦亡调控骨关节炎的发生,已成为防治骨关节炎的研究热点。目的:总结细胞焦亡在骨关节炎中的调控作用,以及运动介导细胞... 详细信息

背景:细胞焦亡参与软骨细胞外基质降解、滑膜炎症以及疼痛,在骨关节炎防治中发挥重要作用。此外,运动可通过抑制细胞焦亡调控骨关节炎的发生,已成为防治骨关节炎的研究热点。目的:总结细胞焦亡在骨关节炎中的调控作用,以及运动介导细胞焦亡在改善骨关节炎中的机制。方法:以“pyroptosis,osteoarthritis,chondrocyte pyroptosis,synovial cell pyroptosis,exercise”和“细胞焦亡,骨关节炎,软骨细胞焦亡,滑膜细胞焦亡,运动”为关键词,检索pubMed与中国知网数据库1992-2024年间发表的相关文献,根据纳入及排除标准选择71篇文献进行综述。结果与结论:①骨关节炎是以软骨细胞外基质降解、滑膜炎症和软骨下骨重塑等为特点的慢性退行性关节疾病,易引起骨的器质性病变、疼痛并引发功能障碍。②细胞焦亡作为一种特殊的程序性死亡机制,其特征为细胞裂解死亡释放炎症因子引发强烈的炎症反应,与骨关节炎的发生发展关系密切。细胞焦亡可导致大量炎症因子释放,进而激活核因子κB转录,增加焦亡蛋白的产生,进而加剧骨关节炎的发生发展,因此细胞焦亡可作为骨关节炎防治的新方向。③运动可通过下调焦亡蛋白信号通路和抑制相关炎症因子表达等途径抑制软骨细胞和滑膜细胞的焦亡,从而在骨关节炎防治中发挥重要作用。有氧和无氧运动可通过抑制细胞焦亡的发生延缓骨关节炎的病理进程,中等强度的有氧运动通过抑制细胞焦亡信号通路改善骨关节炎的效果较好,无氧运动可通过提高肌肉质量进而对骨关节炎产生有益效应。

关键词：细胞焦亡骨关节炎运动运动调控信号通路综述

PREDICTION OF MAXIMUM SCOUR DEPTH AROUND LARGE DIAMETER CYLINDER UNDER THE EFFECTS OF BOTH WAVE AND CURRENT

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Journal of Hydrodynamics 2005年第1期17卷 74-79页

作者： LILin-pu CUILi SchoolofCivilandHydraulicEngineering~DalianUniversityofTechnology Dalian116024china

Physical model tests were counducted to predict local scour and maximum scour depth around the large diameter cylinders located in the (sand) seabed under the action of both wave and current . According to the result of tests, an analysis was made on all the factors influencing the scour. The results shows that for the seabed with relative fine grains in shallow water (0.07

关键词： offshore engineering the effects of both wave and current large diameter cylinder local scour

A Large Dynamic Range Floating Memristor Emulator With Equal Port Current Restriction

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IEEE/CAA Journal of Automatica Sinica 2020年第1期7卷 237-243页

作者： Yifei pu Bo Yu Computer Science Sichuan UniversityChengdu 610065China College of Physics and Engineering Chengdu Normal UniversityChengdu 611130China

In this paper, a large dynamic range floating memristor emulator(LDRFME) with equal port current restriction is proposed to be achieved by a large dynamic range floating voltage-controlled linear resistor(VCLR). Since real memristors have not been largely commercialized until now, the application of a LDRFME to memristive systems is reasonable. Motivated by this need, this paper proposes an achievement of a LDRFME based on a feasible transistor model. A first circuit extends the voltage range of the triode region of an ordinary junction field effect transistor(JFET). The idea is to use this JFET transistor as a tunable linear resistor. A second memristive non-linear circuit is used to drive the resistance of the first JFET transistor. Then those two circuits are connected together and, under certain conditions, the obtained "resistor" presents a hysteretic behavior,which is considered as a memristive effect. The electrical characteristics of a LDRFME are validated by software simulation and real measurement, respectively.

关键词： Floating voltage-controlled linear resistor fracmemristance fracmemristor two-port ordinary memristor three-port mirror memristor

Material and device design for organic solar cells: towards efficiency and stability

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Science China Chemistry 2023年第12期66卷 3484-3494页

作者： Mingrui pu Feng He Shenzhen Grubbs Institute and Department of Chemistry Southern University of Science and TechnologyShenzhen 518055China Guangdong Provincial Key Laboratory of Catalysis Southern University of Science and TechnologyShenzhen 518055China

Organic solar cells(OSCs) have garnered significant attention as a novel photovoltaic technology and have been extensively investigated. In recent years, OSCs have made rapid strides in power conversion efficiency(PCE), demonstrating their significant potential in practical applications. In addition to high PCE, the practical application of OSCs demands a prolonged operating lifespan. The rational design of materials and devices to achieve efficient and stable OSCs is pivotal. This feature article presents a thorough analysis of our group's studies on enhancing efficiency and stability through material and device design. We introduce a range of exceptional chlorine-mediated organic photovoltaic materials and systematically summarize chlorine atom(Cl) induced effects on energy levels, molecular stacking, active layer film morphology and photovoltaic performance. Furthermore, the use of single-crystal diffraction technology allows for a comprehensive understanding of intermolecular packing and interaction at the molecular level. A series of highly efficient non-fullerene acceptors(NFAs) with threedimensional(3D) network packing structures are developed and discussed. Subsequently, based on efficient 3D network brominated NFAs, the studies on polymer and oligomer acceptor materials are carried out and achieve efficient and stable *** addition to materials design, the development of the “quasiplanar heterojunction”(Q-PHJ) based OSC device also plays an important role in achieving superior efficiency and stability. These design experiences of materials and devices hope to provide valuable guidance for the development of efficient and stable OSCs.

关键词： chlorine-mediated photovoltaic materials single-crystal 3D network efficiency stability

Categorical resolutions of a class of derived categories

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Science China Mathematics 2018年第2期61卷 391-402页

作者： pu Zhang School of Mathematical Sciences Shanghai Jiao Tong University

We clarify the relation between the subcategory D_(hf)~b(A) of homological finite objects in D^b(A)and the subcategory K^b(P) of perfect complexes in D^b(A), by giving two classes of abelian categories A with enough projective objects such that D_(hf)~b(A) = K^b(P), and finding an example such that D_(hf)~b(A)≠K^b(P). We realize the bounded derived category D^b(A) as a Verdier quotient of the relative derived category D_C^b(A), where C is an arbitrary resolving contravariantly finite subcategory of A. Using this relative derived categories, we get categorical resolutions of a class of bounded derived categories of module categories of infinite global *** prove that if an Artin algebra A of infinite global dimension has a module T with *** <∞ such that ~⊥T is finite, then D^b(modA) admits a categorical resolution; and that for a CM(Cohen-Macaulay)-finite Gorenstein algebra, such a categorical resolution is weakly crepant.

关键词： homologically finite object perfect complex smooth triangulated category (weakly crepant)categorical resolution (relative) derived category CM-finite Gorenstein algebra

Weighted Estimates for Multilinear Commutators of Marcinkiewicz Integral

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Acta Mathematica Sinica,English Series 2008年第8期24卷 1387-1400页

作者： pu ZHANG Department of Mathematics Mudanjiang Teachers College Mudanjiang 157012 P. R. China

Let μ be the n-dimensional Marcinkiewicz integral and μb the multilinear commutator of μ. In this paper, the following weighted inequalities are proved for ω ∈ A∞ and 0 〈 p 〈 ∞,｜｜μ（f）｜｜LP（ω）≤C｜Mf｜LP（ω） and ｜｜μb（f）｜｜LP（ω）≤C｜｜ML（log L）^1/r f｜｜LP（ω）.The weighted weak L（log L）^1/r -type estimate is also established when p=1 and ω∈A1.

关键词： Marcinkiewicz integral multilinear commutator sharp function Ap weights

Multiple Weighted Estimates for Commutators of Multilinear Maximal Function

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Acta Mathematica Sinica,English Series 2015年第6期31卷 973-994页

作者： pu ZHANG Department of Mathematics Mudanjiang Normal University

Let M be the multilinear maximal function and = （b1, . . . , bm） be a collection of locally integrable functions. Denote by M and [,M] the maximal commutator and the commutator of M with , respectively. In this paper, the multiple weighted strong and weak type estimates for operators M and [,M] are studied. Some characterizations of the class of functions bj are given, for which these operators satisfy some strong or weak type estimates.

关键词： Multilinear maximal function multiple weights commutator BMO