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无氢类金刚石薄膜表面H2O和O2分子共同作用的第一性原理计算

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摩擦学学报 2019年第3期39卷 350-356页

作者：王顺花霍磊鞠鹏飞蒲吉斌兰州交通大学机电工程学院甘肃兰州730000 中国科学院宁波材料技术与工程研究所海洋新材料与应用技术重点实验室浙江宁波315201 上海航天设备制造总厂上海200245

无氢类金刚石碳基薄膜(Diamond-like carbon,DLC)在潮湿大气环境中具有较低的摩擦系数,这主要是由于环境中的H2O和O2两种活性分子钝化了无氢DLC薄膜表面的悬键,但迄今两种活性分子对无氢DLC薄膜低摩擦行为的协同影响机制仍不清楚.本文... 详细信息

无氢类金刚石碳基薄膜(Diamond-like carbon,DLC)在潮湿大气环境中具有较低的摩擦系数,这主要是由于环境中的H2O和O2两种活性分子钝化了无氢DLC薄膜表面的悬键,但迄今两种活性分子对无氢DLC薄膜低摩擦行为的协同影响机制仍不清楚.本文中通过第一性原理计算方法研究了H2O和O2分子共存时在金刚石表面的钝化状态,并推测了无氢DLC薄膜实现低摩擦的可能途径.结果表明:H2O和O2两种活性分子在金刚石表面分解形成OH、H及O基团,其中O原子和H原子的相互吸引能够促使其形成OH基团.当H2O分子和O2分子按比例2:1共存时,金刚石表面全部由OH基团钝化,而非2:1比例时,金刚石表面会形成C-OH、C-H和C-O共存的复杂情况.

关键词：第一性原理 DLC 碳悬键钝化

Water molecular activity management towards stable Zn anodes

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Science China Chemistry 2024年

作者： Yun Tan Jun pu Hongpeng Li Dongliang Chao Key Laboratory of Functional Molecular Solids (Ministry of Education) College of Chemistry and Materials Science Anhui Normal University Laboratory of Advanced Materials Fudan University College of Mechanical Engineering Yangzhou University

Zinc-based aqueous batteries(ZABs) have attracted wide interest and become a hot topic in the field of secondary batteries due to their low cost, high safety, and environmental friendliness. However, challenges pertaining to zinc anodes, such as dendrites growth and side reactions, which are associated with the high activity of freedom water molecules in the aqueous electrolyte,significantly hinder the advancement of ZABs. In recent years, strategies aimed at regulating water molecular activity have been demonstrated to address the above issues effectively. Nevertheless, there is a lack of systematic summary regarding the electrolyte engineering and the functional mechanisms for stabilizing zinc anodes from the point of view of water molecular activity management. Hence, this review comprehensively introduces strategies for regulating water activity through the electrolyte engineering to achieve side reaction-suppressed ZABs, including the latest research on aqueous zinc-metal batteries,the origin of critical zinc-related problems, and the development of technological and electrolyte additives. Lastly, various strategies were summarized from different perspectives to improve the performance of zinc metal anodes. This work is expected to present the latest outline and inspire future innovation in electrolyte technologies.

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Aging Behavior of As-Extruded Ti Particles Reinforced VW94 Composites

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Acta Metallurgica Sinica(English Letters) 2024年第3期37卷 401-406页

作者： Dongmei pu Xianhua Chen Jingfeng Wang Jun Tan Jianbo Li Hong Yang Bo Feng Kaihong Zheng Fusheng Pan College of Materials Science and Engineering Chongqing UniversityChongqing 400045China National Engineering Research Center for Magnesium Alloys Chongqing UniversityChongqing 400045China Institute of New Materials Guangdong Academy of SciencesGuangzhou 510650China

The ageing behavior of as-extruded Ti_(P)/VW94 composites was *** peak hardness of the composites increases compared to the matrix alloy and the 5%Ti_(P)/VW94 composite presents the highest peak hardness of 148.7 HV after aging for about 50 ***,the hardness increments first decrease and then slightly increase with increasing Ti particle content due to the introduction of high-density dislocations by Ti particles.

关键词： Magnesium matrix composites Ti particles Ageing behavior Hardness

A Study on Artistic Treatment in Vocal Works

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Journal of Social Science Development Research

Journal of Social Science Development Research 2024年第1期2卷 25-35页

作者： Weiqi pu Geely University of China ChengduChina.

The singing of a vocal work is far more than a simple series of notes,but a delicate artistic process that requires the performer to skillfully use sound,emotion,and *** process is not just about performing music,but also about transmitting emotions,a spiritual dialogue resonating with the *** the wonderful stage of artistic treatment,the performer becomes the second creator of the song,infusing the work with new life through their unique personality and insightful *** the clever concatenation of notes,the performer can unfold the layers of emotion contained within the song,making it richer and deeper.

关键词： Vocal music works Artistic treatment Singing skill

High power tunable Raman fiber laser at 1.2μm waveband

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Frontiers of Optoelectronics 2024年第1期17卷 1-8页

作者： Yang Zhang Jiangming Xu Junrui Liang Jun Ye Sicheng Li Xiaoya Ma Zhiyong Pan Jinyong Leng pu Zhou College of Advanced Interdisciplinary Studies National University of Defense TechnologyChangsha 410073China Nanhu Laser Laboratory National University of Defense TechnologyChangsha 410073China Hunan Provincial Key Laboratory of High Energy Laser Technology National University of Defense TechnologyChangsha 410073China

Development of a high power fiber laser at special waveband,which is difficult to achieve by conventional rare-earth-doped fibers,is a significant *** of the most common methods for achieving lasing at special wavelength is Raman ***-doped fiber(PDF),due to the phosphorus-related large frequency shift Raman peak at 40 THz,is a great choice for large frequency shift Raman ***,by adopting 150 m large mode area triple-clad PDF as Raman gain medium,and a novel wavelength-selective feedback mechanism to suppress the silica-related Raman emission,we build a high power cladding-pumped Raman fiber laser at 1.2μm waveband.A Raman signal with power up to 735.8 W at 1252.7 nm is *** the best of our knowledge,this is the highest output power ever reported for fiber lasers at 1.2μm ***,by tuning the wavelength of the pump source,a tunable Raman output of more than 450 W over a wavelength range of 1240.6–1252.7 nm is *** work proves PDF’s advantage in high power large frequency shift Raman conversion with a cladding pump scheme,thus providing a good solution for a high power laser source at special waveband.

关键词： Phosphosilicate fiber Raman fiber laser 1.2μm waveband Wavelength tunable

Betaine addition to the diet alleviates intestinal injury in growing rabbits during the summer heat through the AAT/mTOR pathway

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Journal of Animal Science and Biotechnology 2024年第4期15卷 1623-1637页

作者： Zimei Li Junning pu Xiang Chen Yanbin Chen Xiaoyan Peng Jingyi Cai Gang Jia Hua Zhao Gang Tian Animal Nutrition Institute Sichuan Agricultural UniversityChengduSichuan 611130China

Background The aim of this experiment was to investigate the effect of different levels of betaine(Bet)inclusion in the diet on the intestinal health of growing rabbits under summer heat.A total of 100 weaned Qixing meat rabbits aged 35 d with body weight of 748.61±38.59 g were randomly divided into 5 treatment groups:control group(basal diet)and Bet groups(basal diet+0.75,1.0,1.5 or 2.0 g/kg Bet).The average daily temperature in the rabbitry during the experiment was 30.48°C and the relative humidity was 69.44%.Results Dietary addition of Bet had no significant effect on growth performance and health status of growing rabbits(P>0.05),but it increased ileal secretory immunoglobulin A content compared to the control under summer heat(P<0.05).Addition of 0.75 g/kg Bet up-regulated jejunal IL-4,down-regulated ileal TNF-αexpression(P<0.05).The addition of 1.0 g/kg Bet increased the villi height(VH)in the jejunum(P<0.05).Serum glucose levels were reduced,and the expression of SLC6A20 was up-regulated in jejunum and ileum of rabbits fed with 1.5 g/kg Bet(P<0.05).When added at 2.0 g/kg,Bet reduced serum HSP70 content,increased jejunal VH,and up-regulated duodenal SLC7A6,SLC38A2,mTOR and 4EBP-2 expression(P<0.05).Correlation analysis revealed that intestinal mTOR expression was significantly and positively correlated with SLC7A6,SLC38A2,SLC36A1 and IL-4 expression(P<0.05).Conclusions Dietary addition of Bet can up-regulate the expression of anti-inflammatory factors through the AAT/mTOR pathway,improve the intestinal immune function,alleviate intestinal damage in growing rabbits caused by summer heat,and improve intestinal health.

关键词： AAT/mTOR Betaine Growing rabbits Intestinal injury Summer heat

The generation and use of animal models of osteosarcoma in cancer research

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Genes & Diseases 2024年第2期11卷 664-674页

作者： Feifei pu Haoyu Guo Deyao Shi Fengxia Chen Yizhong Peng Xin Huang Jianxiang Liu Zhicai Zhang Zengwu Shao Department of Orthopedics Wuhan Hospital of Traditional Chinese and Western Medicine (Wuhan No.1 Hospital)Tongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei 430022China Department of Orthopedics Union HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei 430022China Department of Radiation and Medical Oncology Zhongnan HospitalWuhan UniversityWuhanHubei 430071China Hubei Cancer Clinical Study Center Zhongnan HospitalWuhan UniversityWuhanHubei 430071China

Osteosarcoma is the most common malignant bone tumor affecting children and ***,the most common treatment is surgery combined with neoadjuvant *** the survival rate of patients with osteosarcoma has improved in recent years,it remains poor when the tumor(s)progress and distant metastases ***,better animal models that more accurately replicate the natural progression of the disease are needed to develop improved prognostic and diagnostic markers,as well as targeted therapies for both primary and metastatic *** present review described animal models currently being used in research investigating osteosarcoma,and their characteristics,advantages,and *** models may help elucidate the pathogenic mechanism(s)of osteosarcoma and provide evidence to support and develop clinical treatment strategies.

关键词： Animal model Cancer Osteosarcoma Pathogenic mechanism Translational research

Re-usable Cd_(0.9)Zn_(0.1)S-ZnO@C/PVDF piezo-photocatalytic film with exceptional hydrogen evolution capability triggered by the synergetic advantages of piezoelectricity and S-Scheme heterojunction

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Journal of Energy Chemistry 2024年第9期96卷 164-176页

作者： Ping Su Dong Zhang Minghui Zhu Tengteng Liang Nan Yang Huaihao Zhao Dafeng Zhang Junchang Liu Peiqing Cai Xipeng pu School of Materials Sciencend Engineering Shandong Provincial Key Laboratory of Chemical Energy Storagend Novel Cell TechnologyLiaocheng UniversityLiaocheng 252000ShandongChina School of Physics Sciencend Information Technology Shandong Key Laboratory of Optical Communication Sciencend TechnologyLiaocheng UniversityLiaocheng 252000ShandongChina College of Opticalnd Electronic Technology China Jiliang UniversityHangzhou 310018ZhejiangChina

Piezoelectric materials have advantages of fine-tuning photocatalytic performance through harvesting mechanical energy and open a new avenue in facilitating green catalytic ***,polyvinylidene fluoride(PVDF),a flexible piezoelectric material,was introduced to synthesize a novel Cd_(0.9)Zn_(0.1)S-ZnO@C/PVDF(CZS-ZO@C/PVDF)piezo-photocatalytic film by spin coating and immersion phase conversion *** from the piezoelectricity of PVDF and the internal electric field(IEF)of CZS-ZO@C Step-scheme(S-Scheme)heterojunction,CZS-ZO@C/PVDF was able to induce a hydrogen generation rate of 34.9 mmol g^(−1)h^(−1)activated by ultrasound and visible light(U-L),which is∼17.5 times of Cd_(0.9)Zn_(0.1)S/PVDF(CZS/PVDF)and∼7.4 times of the photocatalysis rate activated by visible light only(L).Piezoelectric measurements and COMSOL simulation illustrated the excellent piezoelectricity of CZS-ZO@C/PVDF film,which exhibits a piezoelectric coefficient(d33)of 9.9 pm V−1 and a piezoelectric potential of 874 mV(under 0.5 MPa).The reaction mechanism for the exceptional piezo-photocatalytic performance was finally disclosed through density functional theory(DFT)calculation and electrochemical *** study enriches the application scope of piezoelectric materials in sustainable energy catalysis and provides a new direction to develop efficient piezoelectric photocatalysts.

关键词： Piezo-photocatalysis Heterojunction Cd_(0.9)Zn_(0.1)S Zno@c PVDF

Modulation of phase boundary and domain structures to engineer strain properties in BNT-based ferroelectrics

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Journal of Advanced Ceramics 2024年第7期13卷 967-975页

作者： Yule Yang Zhiyong Liu Pengrong Ren Yuqing Mao Haijun Sun Bingliang Liang pu Mao Kun Guo Bing Xie Longlong Shu School of Materials Science and Engineering Nanchang Hangkong UniversityNanchang 330063China School of Materials Science and Engineering Xi'an University of TechnologyXi’an 710048China School of Aircraft Engineering Nanchang Hangkong UniversityNanchang 330063China School of Physics and Materials Science Nanchang UniversityNanchang 330031China

Bismuth sodium titanate(BNT)ceramics exhibit outstanding strain responses but are unfavorable for application in high-sensitivity displacement actuators due to the large negative strain resulting from irreversible changes in their phase transition and domain ***,(1−x)Bi_(0.50)Na_(0.41)K_(0.09)TiO_(3)-xNaNbO_(3)(BNKT−xNN)solid solutions were prepared to improve the strain properties through the strategy of modulating the phase boundary and domain *** introduction of sodium niobate could effectively regulate the relative content of the tetragonal(P4bm)and rhombohedral(R3c)phases in the phase boundary *** ferroelectric-to-relaxor phase transition(TF−R)was reduced,and the ergodic relaxor(ER)state was nurtured at room *** zero-negative strain properties of S=0.41%and d33*=742 pm/V were achieved from the reversible transition between the ER and ferroelectric states under an applied electric field(x=0.04).Additionally,understanding the domain states via piezoelectric force microscopy(PFM)and firstorder reversal curve(FORC)revealed that the superior strain responses originated from the reversible inter-transformation of substable macrodomains and polar nanoregions(PNRs)in the phase *** study provides new insight into the interplay between the evolution of phase boundaries and domain structures and the strain properties of BNT-based ceramics.

关键词： bismuth sodium titanate(BNT) domain structure phase boundary strain response relaxor state