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MOF glass foam: a blueprint to porous membrane scaling-up

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Science China Chemistry 2024年第3期67卷 746-748页

作者： Yuan peng Weishen Yang State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesBeijing 100049China University of Chinese Academy of Sciences Beijing 100049China

In comparison with conventional energy-intensive separation technologies, such as distillation and crystallization,membrane separation is labelled as an advanced technology with low energy consumption, a small carbon footprint,continuous operation, etc. Metal-organic frameworks(MOFs) are a burgeoning category of crystalline materials consisting of metal ions/clusters coordinated with organic ligands.

关键词： separation porous distillation

Contrasting physical mechanisms of yellowfin tuna fluctuations between the western and eastern Indian Ocean

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Journal of Oceanology and Limnology 2024年第3期42卷 960-971页

作者： peng LIAN Le GAO Key Laboratory of Ocean Observation and Forecasting and Key Laboratory of Ocean Circulation and Waves Institute of OceanologyChinese Academy of SciencesQingdao 266071China University of Chinese Academy of Sciences Beijing 100049China Laboratory for Ocean Dynamics and Climate Laoshan LaboratoryQingdao 266061China

As an economically critical pelagic migratory species,yellowfin tuna(Thunnus albacores,YFT)is very sensible to physical and environmental conditions,such as sea surface temperature(SST),ocean heat content(OHC),and the mixed layer depth(MLD).We investigated the impact of SST,OHC,and MLD on fluctuations of YFT catch in the western/eastern Indian Ocean using the long time series of 63-year environmental and YFT *** found that the impact of SST on YFT was heavily overestimated in the past,and MLD plays a more critical role in the YFT catch *** the MLD deepens(>34.8 m),SST was more influential in predicting the catches of YFT than OHC in the western Indian Ocean,and OHC was more critical to YFT than SST in the eastern Indian ***,when the MLD shallows(<34.8 m),MLD was more vital to predict the catch per unit effort(CPUE)of YFT than SST/OHC in the *** 2000,there was an asynchronous pattern of YFT CPUE induced by higher frequency variations and ocean hiatus of SST/OHC signals in the western and eastern Indian Oceans *** impact of the subsurface hiatus may induce the decrease of YFT in the eastern Indian *** above findings clarified a non-stationary relationship between the environmental factors and catches of YFT and provided new insights into variations in YFT abundance.

关键词： yellowfin tuna Indian Ocean sea surface temperature(SST) ocean heat content(OHC) mixed layer depth(MLD) hiatus

Stabilization and Blow-up in an Infinite Memory Wave Equation with Logarithmic Nonlinearity and Acoustic Boundary Conditions

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Journal of Systems Science & Complexity 2024年第4期37卷 1368-1391页

作者： peng Qingqing ZHANG Zhifei School of Mathematics and Statistics Huazhong University of Science and TechnologyWuhan 430074China Hubei Key Laboratory of Engineering Modeling and Scientific Computing Huazhong University of Science and TechnologyWuhan 430074China

In this paper,the authors consider the stabilization and blow up of the wave equation with infinite memory,logarithmic nonlinearity and acoustic boundary *** authors discuss the existence of global solutions for the initial energy less than the depth of the potential well and investigate the energy decay estimates by introducing a Lyapunov ***,the authors establish the finite time blow up results of solutions and give the blow up time with upper bounded initial energy.

关键词： Acoustic boundary condition finite time blow-up general decay infinite memory logarithmic nonlinearity

Oscillatory solutions in a 3D predation system with time delay and age structure

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International Journal of Biomathematics 2024年第5期17卷 133-175页

作者： peng Yang College of Mathematics and Statistics Northwest Normal University Lanzhou Gansu 730070P.R.China

This paper is concerned with the sustained periodic oscillation phenomenon in a threespecies delayed predation system with Holling type II functional response and age structure in top *** top predator fertility function is regarded as a piecewise continuous smooth function with regard to their maturation period *** complicated dynamic behavior is proved by integrated semigroup theory and Hopf bifurcation theorem for semilinear equations with non-dense *** qualitative analysis and bifurcation study of the system,we yield that this system has a nontrivial periodic solution that bifurcates from the positive equilibrium age distribution when bifurcation parameter T passes through some critical *** simulations are also provided to illustrate theoretically analytical results.

关键词： Periodic oscillations 3D predation system time delay age structure integrated semigroup

Imprints of ultralight axions on the gravitational wave and pulsar timing measurement

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Science China(Physics,Mechanics & Astronomy) 2024年第1期67卷 23-29页

作者： Ning Xie Fa peng Huang MOE Key Laboratory of TianQin Mission TianQin Research Center for Gravitational Physics&School of Physics and AstronomyFrontiers Science Center for TianQinGravitational Wave Research Center of CNSASun Yat-sen University(Zhuhai Campus)Zhuhai 519082China

The axion or axion-like particle motivated from a natural solution of strong CP problem or string theory is a promising dark matter *** study the new observational effects of ultralight axion-like particles by the space-borne gravitational wave detector and the radio *** the neutron star-black hole binary as an example,we demonstrate that the gravitational waveform could be obviously modified by the slow depletion of the axion cloud around the black hole formed through the superradiance *** compare these new effects on the binary with the well-studied effects from dynamical friction with dark matter and dipole radiation in model-independent ***,we discuss the constraints from LIGO/Virgo and study the detectability of the ultralight axion particles at LISA and TianQin.

关键词： gravitational wave axion dark matter

Fabrication of Molecularly Imprinted Electrospun Nanofibers with Mono-amidoxime Functional Ligand for Efficient Decontamination of Toxic Organophosphates

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Chinese Journal of Polymer Science 2024年第4期42卷 446-456页

作者： Lan Wang peng Jiang Ya-Lin Niu Jun-peng Cao Tian-Ying Guo Key Laboratory of Functional Polymer Materials Ministry of EducationInstitute of Polymer ChemistryCollege of Chemistry and Frontier Science Center for the Creation of New Organic SubstancesNankai UniversityTianjin300071China

There is an urgent imperative to discover practical and efficacious artificial catalysts for the expeditious decontamination of toxic organophosphates. Herein, we propose a novel molecularly imprinted approach utilizing electrospun fiber scaffolds. Specifically, an amidoxime-based functional polymer (PMAOX) has been synthesized, which contains amidoxime groups that can act as nucleophiles and ligands for the formation of catalytic active sites. This polymer was blended with polyacrylonitrile (PAN), a well-processable material, to prepare a nanofiber mat using electrospinning techniques. Then, the amidoxime side groups on fiber surface were further cross-linked after the molecular coordination of templates to complete the molecularly imprinting process. This approach can not only enhance the content of functional molecularly imprinted polymers without affecting structural stability, but also combines surface MI technology to fully expose and leverage the advantages of active sites. The as prepared molecularly imprinted electrospun nanofibers MIF-Zn-PMAOX/PAN-6/4 catalyzes the degradation of paraoxon with a half-life of 32 min, and MIF-Ag-PMAOX/PAN catalyzes the degradation of parathion with a half-life of 18 min. The maximum catalytic rate evidence rate enhancements nearly 3700-fold of the self-hydrolysis. Thus, the mono-amidoxime based molecularly imprinted fibers demonstrate the versatility and superiority as self-detoxifying for organophosphates.

关键词： Organophosphateshydrolysis Electrospinning Molecular imprinting

3D Foam-Based MXene Architectures:Structural and Electrolytic Engineering for Advanced Potassium-Ion Storage

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Energy & Environmental Materials 2024年第4期7卷 64-73页

作者： peng Zhang Yanmeng peng Qizhen Zhu Razium Ali Soomro Ning Sun Bin Xu State Key Laboratory of Organic-Inorganic Composites Beijing Key Laboratory of Electrochemical Process and Technology for Materials Beijing University of Chemical Technology Beijing Advanced Innovation Centre for Soft Matter Science and Engineering Beijing University of Chemical Technology

MXenes are emerging rapidly as promising electrode materials for energy storage due to their high electronic conductivity and rich surface chemistry,but their potassium storage performance is unsatisfactory because of... 详细信息

关键词： 3D foam-like scaffold electrolyte chemistry electrostatic neutralization MXene potassium-ion batteries

Divergent contributions of spring and autumn photosynthetic phenology to seasonal carbon uptake of subtropical vegetation in China

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Journal of Geographical Sciences 2024年第7期34卷 1280-1296页

作者： peng Ying LI peng ZHOU Xiaolu LUO Yunpeng ZHANG Cicheng WANG Longjun LI Tong peng Changhui School of Geographic Sciences Hunan Normal UniversityChangsha410081China Department for Biogeochemical Integration Max-Planck-Institute for BiogeochemistryJena07745Germany Department of Biology Sciences Institute of Environment SciencesUniversity of Quebec at MontrealC.P.8888Succ.Centre-VilleMontrealH3C 3P8Canada

Phenological changes play a central role in regulating seasonal variation in the ecological processes,exerting significant impacts on hydrologic and nutrient cycles,and ultimately influencing ecosystem functioning such as carbon ***,the potential impact mechanisms of phenological events on seasonal carbon dynamics in subtropical regions are *** knowledge gaps hinder from accurately linking photosynthetic phenology and carbon sequestration *** chlorophyll fluorescence remote sensing and productivity data from 2000 to 2019,we found that an advancement in spring phenology increased spring gross(GPP)and net primary productivity(NPP)in subtropical vegetation of China by 2.1 gC m^(-2)yr^(-1)and 1.4 gC m^(-2)yr^(-1),respectively.A delay in autumn phenology increased the autumnal GPP and NPP by 0.4 gC m^(-2)yr^(-1)and 0.2 gC m^(-2)yr^(-1),***,the contribution of the spring phenology to spring carbon uptake increased significantly during the study period,while this positive contribution showed a nonsignificant trend in *** comparison,the later autumn phenology could significantly contribute to the increase in autumnal carbon uptake;however,this contributing effect was *** analysis indicated that these phenomena have been caused by the increased leaf area and enhanced photosynthesis due to earlier spring and later autumn phenology,*** results demonstrate the diverse impacts of vegetation phenology on the seasonal carbon sequestration ability and it is imperative to consider such asymmetric effects when modeling ecosystem processes parameterized under future climate change.

关键词： subtropics vegetation phenology remote sensing carbon cycle climate change

Edge and lithium concentration effects on intercalation kinetics for graphite anodes

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Journal of Energy Chemistry 2024年第3期90卷 337-347,I0009页

作者： Keming Zhu Denis Kramer Chao peng School of Mechanical and Precision Instrument Engineering Xi'an University of TechnologyXi'an 710048ShanxiChina Faculty of Mechanical Engineering Helmut-Schmidt UniversityHamburg 22043Germany School of Engineering University of SouthamptonSouthampton SO171BJUK Multiscale Crystal Materials Research Center Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055GuangdongChina

Graphite interfaces are an important part of the anode in lithium-ion batteries(LIBs),significantly influencing Li intercalation *** anodes adopt different stacking sequences depending on the concentration of the intercalated Li *** this work,we performed first-principles calculations to comprehensively address the energetics and dynamics of Li intercalation and Li vacancy diffusion near the no n-basal edges of graphite,namely the armchair and zigzag-edges,at high Li *** find that surface effects persist in stage-Ⅱ that bind Li strongly at the edge ***,the pronounced effect previously identified at the zigzag edge of pristine graphite is reduced in LiC_(12),penetrating only to the subsurface site,and eventually disappearing in LiC_(6).Consequently,the distinctive surface state at the zigzag edge significantly impacts and restrains the charging rate at the initial lithiation of graphite anodes,whilst diminishes with an increasing degree of *** diffusion time for Li hopping to the bulk site from either the zigzag edge or the armchair edge in LiC_(6) was observed during high state of charge due to charge *** controlling Li occupation and diffusion kinetics at this stage is also crucial for enhancing the charge rate.

关键词： Graphite anode Edge Interface Lithium-ion batteries Density functional theory