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Synergistic effects of constituents in rare earth-based composites:Enhanced structural,electrical and magnetic properties for water splitting applications

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Journal of Rare Earths 2025年第1期43卷 105-114,I0005页

作者： Chitralekha S.Shankar A.p.Singh Functional Materials Research Laboratory Department of PhysicsARSD CollegeUniversity of Delhi1021India Department of physics Multanimal Modi CollegeCh.Charan Singh UniversityMeerutU.PIndia

Rare earth-based Bi_(0.85)La_(0.15)FeO_(3)(BLFO)and NdMnO_(3)(NMO)particles were synthesised using the solidstate route,and their roles affecting structural,electrical,magnetic properties along with hydroelectric application in different concentrations i.e.,(1-x)BLFO:xNMO(where x=0,0.10,0.20,0.30 and 1.0)ceramics composites were investigated.X-ray diffraction analyses confirm the pure-phase formation of BLFO:NMO composites,featuring micrometer-scale crystallite *** transform infrared(FT-IR)spectra of BLFO:NMO composites reveal peak shifts with rising NMO content,indicating composite *** composites exhibit robust Maxwell-Wagner polarization and a pronounced composition-dependent *** addition of NMO to BLFO results in a rise in dielectric permittivity at lower frequencies,confirming relaxor behavior and indicating success in achieving the transition *** spectroscopy facilitates a clearer understanding of how charge carriers contribute to these composites and the impact of grain/grain *** saturation magnetization maximum value(i.e.,0.807 emu/g)was attained in *** coercivity decreases with the addition of NMO in *** results suggest the composite's enhanced suitability for microelectronics and hydropower cells,showing improved hydroelectric cell performance with increased NMO in BLFO,highlighting a notable ion diffusion mechanism.

关键词： Composites X-ray diffraction Relative permittivity Hydroelectric cell Rare earths

Analyses of BioVOCs variation related to vegetation predominance in the Natural park of Ampezzo Dolomites, UNESCO world heritage area of Dolomites

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Journal of Forestry Research 2013年第3期24卷 439-448页

作者： Luca Raveane Francesco Tisato ilena Isak pietro Traldi National Council of Researches ISTM Corso Stati Uniti n°435127 Padova Italy National Council of Researches -ICIS Corso Stati Uniti n°435127 Padova Italy

The determination of emitted Biogenic Volatile Compounds （BioVOCs） profile via Field Air Analysis （FAA） - Solid phase Micro Extraction （75μm Carboxen/pDMS portable field sampler） was performed using GC-MS. The six sampling sites located in the Natural park of Ampezzo Dolomites, part of the UNESCO＇s World Heritage List, are characterized by different predominating vegetation. The ubiquitous compound hexanal was chosen as internal standard, in order to compare the amounts of the different compound in the different sites. The main terpenes identified were α-pinene, 13-pinene, 6-3-carene and d-limonene, while 1,8 cineole was the highest abundant oxygenated terpene. In the site next the＇national road a higher amount of benzene derivatives （ben- zene, toluene, o-xylene, p-xylene and ethylbenzene） were observed. In the site relatively close to the road a marked decrease of benzene deriva- tives was observed. In the sites close to conifers （i.e. Fir, pine and Larch） the terpenic content observed was higher than in the site close to the mixed forest （mainly large-leaf and some conifers）. Some terpenes were observed also in the high-quote meadow site, although of lower abun- dance than in the other sites. The highest abundance of terpenes was ob- served in the pinus cerebra （Swiss pine） site.

关键词： Solid phase microExtraction organic volatile compound Terpene plant emission mass spectrometry gas chromatography.

Investigation of a NO_(x) emission from coal power plants in Texas, United States and its impact on the environment

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China Geology 2025年第1期8卷 107-116页

作者： Mikalai Filonchyk Michael p.peterson Faculty of Geomatics Lanzhou Jiaotong UniversityLanzhou 730070China Gansu provincial Engineering Laboratory for National Geographic State Monitoring Lanzhou 730070China Department of Geography and Geology University of Nebraska OmahaOmaha NE 68182USA

Texas is the largest state by area in the US after Alaska,and one of the top states in the production and consumption of electricity with many coal-fired ***-fired power plants emit greater than 70% of pollutants in the energy *** coal is burned to produce electricity,nitrogen oxides(NO_(x))are released into the air,one of the main pollutants that threaten human health and lead to a large number of premature *** key to effective air quality management is the strict compliance of all plants with emission ***,not all Texas coal plants have the environmental equipment to lower pollutant *** dioxide(NO2)observations from the TROpOspheric Monitoring Instrument(TROpOMI)were used to evaluate the emissions for Texas power *** from both the Emissions and Generation Resource Integrated Database(EGRID)and the Emissions Database for Global Atmospheric Research(EDGAR)were used to examine *** was found that NOx emissions for Texas power plants range from 1.53 kt/year to 10.99 kt/year,with the Martin Lake,Limestone and Fayette power project stations being the top *** parish and Martin Lake stations have the strongest NOx fluxes,with both exhibiting significant seasonal *** of bottom-up inventories for EDGAR and EGRID show a high correlation(r=0.956)and a low root mean square error(0.766).A more reasonable control policy would lead to much reduced NOx emissions.

关键词： NO_(x)emission Enironmental pollution power plants TROpOMI EDGAR Human health EGRID. Texas

Unlocking hypoglycemia–associated brain microvascular dysfunction:critical insights from proteomic analysis

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Neural Regeneration Research 2025年第6期20卷 1707-1708页

作者： Siva S.V.p.Sakamuri Anil Sakamuri Department of Chemistry Auburn University at MontgomeryMontgomeryALUSA Vascular Biology Center and Department of Medicine Medical College of Georgia at Augusta UniversityAugustaGAUSA

Hypoglycemia-a critical complication linked to worsened brain function in diabetic subjects:Hypoglycemia is characterized by a decline in circulatory glucose levels below sta nda rd physiological *** hypoglycemia,classified as level 1 hypoglycemia,is defined by blood glucose levels below 70 mg/dL and can be effectively addressed through carbohydrate *** hypoglycemia,denoted by blood glucose levels less than 54 mg/dL,poses a life-threatening risk if left *** with type 1 and type 2 diabetes undergoing insulin treatment are particularly susceptible to hypoglycemia due to impaired counterregulatory mechanisms.

关键词： impaired intake critical

Small molecule inhibitor DDQ-treated hippocampal neuronal cells show improved neurite outgrowth and synaptic branching

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Neural Regeneration Research 2025年第9期20卷 2624-2632页

作者： Jangampalli Adi pradeepkiran priyanka Rawat Arubala p.Reddy Erika Orlov pHemachandra Reddy Department of Internal Medicine Texas Tech University Health Sciences CenterLubbockTXUSA Department of Nutritional Sciences College of Human SciencesTexas Tech UniversityLubbockTXUSA Department of pharmacology&Neuroscience Texas Tech University Health Sciences CenterLubbockTXUSA Department of Neurology Texas Tech University Health Sciences CenterLubbockTXUSA Department of Speech Language and Hearing SciencesTexas Tech University Health Sciences CenterLubbockTXUSA Department of public Health Texas Tech University Health Sciences CenterLubbockTXUSA

The process of neurite outgrowth and branching is a crucial aspect of neuronal development and *** and dendrites,sometimes referred to as neurites,are extensions of a neuron's cellular body that are used to start *** we explored the effects of diethyl(3,4-dihydroxyphenethylamino)(quinolin-4-yl)methylphosphonate(DDQ)on neurite developmental features in HT22 neuronal *** this work,we examined the protective effects of DDQ on neuronal processes and synaptic outgrowth in differentiated HT22cells expressing mutant Tau(mTau)*** investigate DDQ chara cteristics,cell viability,biochemical,molecular,western blotting,and immunocytochemistry were *** outgrowth is evaluated through the segmentation and measurement of neural *** neural processes can be seen and measured with a fluorescence microscope by manually tracing and measuring the length of the neurite *** neuronal processes can be observed and quantified with a fluorescent microscope by manually tracing and measuring the length of the neuronal ***-treated mTau-HT22 cells(HT22 cells transfected with cDNA mutant Tau)were seen to display increased levels of synaptophysin,MAp-2,andβ-***,we confirmed and noted reduced levels of both total and p-Tau,as well as elevated levels of microtubule-associated protein 2,β-tubulin,synaptophysin,vesicular acetylcholine transporter,and the mitochondrial biogenesis protein-pe roxisome prolife rator-activated receptor-gamma coactivator-1α.In mTa u-expressed HT22 neurons,we observed DDQ enhanced the neurite characteristics and improved neurite development through increased synaptic *** findings conclude that mTa u-HT22(Alzheimer's disease)cells treated with DDQ have functional neurite developmental chara *** key finding is that,in mTa u-HT22 cells,DDQ preserves neuronal structure and may even enhance nerve development function with mTa u inhibition.

关键词： diethyl(3 4-dihydroxyphenethylamino)(quinolin-4-yl)methylphosphonate(DDQ) hippocampal neuronal cells HT22 neurite outgrowth neuronal development small molecule

Strong resistance to β-cyfluthrin in a strain of the beetle Alphitobius diaperinus: a de novo transcriptome analysis

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INSECT SCIENCE 2025年第1期32卷 209-226页

作者： Gouesbet, Gwenola Renault, David Derocles, Stephane A. p. Colinet, Herve Univ Rennes CNRS UMR 6553 ECOBIO Ecosyst Biodivers Evolut Rennes France Inst Univ France 1 Rue Descartes Paris France

The lesser mealworm, Alphitobius diaperinus, is an invasive tenebrionid beetle and a vector of pathogens. Due to the emergence of insecticide resistance and consequent outbreaks that generate significant phytosanitary and energy costs for poultry farmers, it has become a major insect pest worldwide. To better understand the molecular mechanisms behind this resistance, we studied a strain of A. diaperinus from a poultry house in Brittany that was found to be highly resistant to the beta-cyfluthrin. The strain survived beta-cyfluthrin exposures corresponding to more than 100 times the recommended dose. We used a comparative de novo RNA-Seq approach to explore genes expression in resistant versus sensitive strains. Our de novo transcriptomic analyses showed that responses to beta-cyfluthrin likely involved a whole set of resistance mechanisms. Genes related to detoxification, metabolic resistance, cuticular hydrocarbon biosynthesis and proteolysis were found to be constitutively overexpressed in the resistant compared to the sensitive strain. Follow-up enzymatic assays confirmed that the resistant strain exhibited high basal activities for detoxification enzymes such as cytochrome p450 monooxygenase and glutathione-S-transferase. The in-depth analysis of differentially expressed genes suggests the involvement of complex regulation of signaling pathways. Detailed knowledge of these resistance mechanisms is essential for the establishment of effective pest control.

关键词： Alphitobius diaperinus de novo transcriptome insecticide resistance p450 xenobiotic metabolism

Application of feedforward and recurrent neural networks for model-based control systems

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CONTROL THEORY AND TECHNOLOGY 2025年第1期23卷 91-104页

作者： Krok, Marek Hunek, Wojciech p. Mielczarek, Szymon Buchwald, Filip Kolender, Adam Opole Univ Technol Dept Control Sci & Engn Opole Poland

In this paper, a new study concerning the usage of artificial neural networks in the control application is given. It is shown, that the data gathered during proper operation of a given control plant can be used in the learning process to fully embrace the control pattern. Interestingly, the instances driven by neural networks have the ability to outperform the original analytically driven scenarios. Three different control schemes, namely perfect, linear-quadratic, and generalized predictive controllers were used in the theoretical study. In addition, the nonlinear recurrent neural network-based generalized predictive controller with the radial basis function-originated predictor was obtained to exemplify the main results of the paper regarding the real-world application.

关键词： predictive control Linear-quadratic control Inverse problems Feedforward network Recurrent neural network Optimization

Adding new dimension to non-directed C（sp3）–H functionalizations

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Science China Chemistry 2025年

作者： Konstantin p.Bryliakov Laboratory of Selective Oxidation Catalysis N.D.Zelinsky Institute of Organic Chemistry RAS

Aliphatic C–H groups are among the most abundant yet least reactive functional groups in organic molecules. Nature has evolved metalloenzymes such as those of the cytochrome p450 superfamily that efficiently activate individual tertiary（3） and secondary （2） C（sp3）–H bonds in complex molecules with the highest level of regio-and stereoselectivity [1], thus encouraging studies aimed at engineering artificial metalloenzymes for synthetic applications [2].

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Microstructure and mechanical properties of welds of AZ31B magnesium alloy produced by different gas tungsten arc welding variants

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Defence Technology(防务技术) 2025年第2期44卷 98-110页

作者： S.Srinivasan R.Ravi Bharath A.Atrens p.Bala Srinivasan School of Mechanical Engineering SASTRA Deemed to be UniversityThanjavur 613401India Welding Research Institute Bharat Heavy Electricals LimitedTiruchirappalli 620014India School of Mechanical and Mining Engineering Centre for Advanced Materials Processing and Manufacturing(AMPAM)University of QueenslandSt LuciaQLD 4072Australia High Energy Batteries(India)Limited MathurTiruchirappalli 622515India

This work aimed to(i)understand conventional and pulse gas tungsten arc welding(GTAW)of AZ31B,and(ii)explore high frequency welding(100 Hz-1500 Hz).GTA welding with alternating current(AC)and direct current electrode positive(DCEp)polarities yielded crack-free partial penetration welds for6 mm thick AZ31B alloy *** under direct current electrode negative(DCEN)polarity with identical parameters as that for AC and DCEp resulted in full penetration welds that had ***-free full-penetration welds could be accomplished with pulse GTA welding using DCEN polarity at a pulse frequency of 1 Hz with a pulse duration ratio of 1:*** resultant DCEN p 1:1 weld metal had a microstructure finer than the conventional DCEN *** produced with pulse duration ratios of 1:2and 1:4 lacked penetration but had a much finer microstructures because of the lower heat *** arc constriction by the high frequency pulsing in the Activ Arc■-High frequency(AA-HF)mode welding was responsible for deeper *** produced under DCEN pulsing and AA-HF conditions had hardness higher than conventional DCEN,DCEp and AC GTA welds,attributed to the finer ***-HF GTA welding produced defect free deeper penetration welds with good microstructural features/mechanical properties and also gave an advantage of 50%enhanced productivity when welded at1500 Hz.

关键词： AZ31B alloy pulse GTAW High frequency Microstructure Mechanical properties productivity