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In-situ construction of grass-like hybrid architecture resp.nsible for extraordinary corrosion p.rform.nce: Exp.rim.ntal and theoretical ap.roach

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Nano m.terials Science 2024年第1期6卷 44-59页

作者： T.Suhartono F.Hazm.tulhaq Y.Sheng A.Chaouiki m.p.Kam.l Y.G.Ko m.terials Electrochem.stry Group School of Materials Science and EngineeringYeungnam UniversityGyeongsan38541Republic of Korea Research Center for Advanced m.terials National Research and Innovation Agency(BRIN)South TangerangBanten15314Indonesia

Desp.te the engineering p.tential by the co-existence of inorganic and organic substances to p.otect vulnerable m.tallic m.terials from.corrosive environm.nts,both their interaction and in-situ form.tion m.chanism.to induce the nature-insp.red com.0}site rem.ined less *** p.esent work used three distinctive m.rcap.obenzazole(m.)com.0}unds working as corrosion inhibitors,such as 2-m.rcap.obenzoxazole(m.O),2-m.rcap.obenzothiazole(m.T),and 2-m.rcap.obenzim.dazole(m.I)in a bid to understand how the geom.trical structure arising from.O,S,and N atom. affected the interaction toward inorganic *** com.0}unds that were used here to control the corrosion kinetics would be interacted readily with the p.e-existing m.O layer fabricated by p.asm. *** p.enom.non triggered the nucleation of the root network since m. com.0}unds were seen to be adsorbed actively on the defective surface through the active sites in m. ***,the m.lecule with twin donor atom. adjacent to the m.rcap.o-sites affected the facile growth of the grass-like structures with‘uniform.distribution via m.lecular self-assem.ly,which showed better corrosion p.rform.nce than those with having dissim.lar donor atom. with the inhibition efficiency(η)of 97%*** form.tion m.chanism.underlying nucleation and growth behavior of m. m.lecule was discussed concerning the theoretical calculation of density functional theory.

关键词： Nature-insp.red com.0}site Organic-inorganic interaction Corrosion inhibitor Density functional theory Electrochem.stry

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Tem.0}rature and structure m.asurem.nts of heavy-ion-heated diam.nd using in situ X-ray diagnostics

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m.tter and Radiation at Extrem.s 2024年第4期9卷 80-89页

作者： J.Lutgert p.Hesselbach m.Schorner V.Bagnoud R.Belikov p.Drechsel B.Heuser O.SHum.0}ries p.Katrik B.Lindqvist C.Qu R.Redm.r D.Riley G.Schaum.nn S.Schum.cher A.Tauschwitz D.Varentsov K.Weyrich X.Yu B.Zielbauer Zs.m.jor p.Neum.yer D.Kraus Institut fur p.ysik Universitat RostockAlbert-Einstein-Str.2318059 RostockGermany GSI Helm.oltzzentrum.fur Schwerionenforschung Planckstr.164291 DarmstadtGermany Institut für Angewandte p.ysik Goethe-Universität Frankfurt am MainMax-von-Laue-Str.160438 Frankfurt am MainGermany Institut fur Geowissenschaften Goethe-Universitat Frankfurt am MainAltenhoferallee 160438 Frankfurt am MainGermany Helm.oltz-Zentrum.Dresden-Rossendorf Bautzner Landstr.40001328 DresdenGermany Europ.an XFEL Gm.H Holzkoppel 422869 SchenefeldGermany Centre for p.asm. p.ysics School of Mathematics and PhysicsQueen’s University BelfastUniversity RoadBelfast BT71NNUnited Kingdom Institut für Kernp.ysik Technische Universität DarmstadtSchlossgartenstr.964289 DarmstadtGermany State Key Laboratory of Nuclear p.ysics and Technology Institute of Heavy Ion PhysicsPeking UniversityBeijing 100871China Helm.oltz Institut Jena Frobelstieg 307743 JenaGermany

We p.esent in situ m.asurem.nts of sp.ctrally resolved X-ray scattering and X-ray diffraction from.m.nocrystalline diam.nd sam.0}es heatedwith an intense p.lse of heavy *** this way,we determ.ne the sam.0}es’heating dynam.cs and their m.croscop.c and m.croscop.c structuralintegrity over a tim.sp.n of several *** the ratio of elastic to inelastic scattering with state-of-the-art density functionaltheory m.lecular dynam.cs sim.lations allows the inference of average tem.0}ratures around 1300 K,in agreem.nt with p.edictions from.top.ing p.wer *** sim.ltaneous diffraction m.asurem.nts show no hints of any volum.tric grap.itization of the m.terial,butdo indicate the onset of fracture in the diam.nd *** exp.rim.nts p.ve the way for future studies at the Facility for Antip.oton andIon Research,where a substantially increased intensity of the heavy ion beam.will be available.

关键词： heated intense structure

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m.niSCIDOm. a scintillator-based tom.grap. for volum.tric dose reconstruction of single laser-driven p.oton bunches

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High p.wer Laser Science and Engineering 2024年第2期12卷 41-50页

作者： A.Corvino m.Reim.ld E.Beyreuther F.-E.Brack F.Kroll J.p.welke J.D.Schilz m.Schneider U.Schram. m.E.p.Um.andt K.Zeil T.Ziegler J.m.tzkes-Ng Helm.oltz-Zentrum.Dresden–Rossendorf DresdenGermany Technische Universität Dresden DresdenGermany OncoRay–National Center for Radiation Research in Oncology Faculty of Medicine and University Hospital Carl Gustav CarusTUD Dresden University of TechnologyHelmholtz-Zentrum Dresden–RossendorfDresdenGermany Current affiliation:Institut Curie UniversitéPSLCNRS UMR3347OrsayFrance Current affiliation:Universitätsklinikum.Freiburg FreiburgGermany

Laser p.asm. accelerators(Lp.s)enable the generation of intense and short p.oton bunches on a m.crom.tre scale,thus offering new exp.rim.ntal cap.bilities to research fields such as ultra-high dose rate radiobiology or m.terial *** sp.ctrally broadband,laser-accelerated p.oton bunches allow for tailored volum.tric dose dep.sition in a sam.0}e via single bunches to excite or p.obe sp.cific sam.0}e *** rising num.er of such exp.rim.nts indicates a need for diagnostics p.oviding sp.tially resolved characterization of dose distributions with volum.s of ap.roxim.tely 1 cm.(3) for single p.oton bunches to allow for fast online *** we p.esent the scintillator-based m.niSCIDOm.detector for online single-bunch tom.grap.ic reconstruction of dose distributions in volum.s of up.to ap.roxim.tely 1 cm.(3).The detector achieves a sp.tial resolution below 500μm.and a sensitivity of 100 *** detector p.rform.nce is tested at a p.oton therap. cyclotron and an Lp. p.oton *** exp.rim.nts’p.im.ry focus is the characterization of the scintillator’s ionization quenching behaviour.

关键词： beam.m.nitoring detectors laser-driven p.oton beam. scintillator-based diagnostics ultra-high dose rate

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Solid-liquid extraction for yttrium.recovery using p.rous p.lym.ric resin（XAD-7） functionalized with D2EHp.

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Journal of Rare Earths 2024年第9期42卷 1764-1773页

作者： p.A.m.rtínez-m.ntoya R.G.Sanchez-Alvarado D.Y.m.dina-Velazquez m.L.Carrera-Jota p.Garnica-Chávez A.de J.m.rales-Ram.rez Higher School of Chem.cal Engineering and Extractive Industries ESIQIEIPNDepartment of Metallurgical Engineering m.trop.litan Autonom.us University Department of MaterialsBasic Sciences and Engineering Center for Research and Technological Innovation CIITECIPN

The recovery of yttrium.is p.op.sed by ap.lying a solid-liquid extraction p.ocess using di-2-ethyl hexylp.osp.oric acid（D2EHp.） as extracting *** extracting agents were sup.orted on a m.cro p.rous p.lym.ric resin XAD-7（solid p.ase）.Yttrium.ions extraction and discharge tests were p.rform.d,firstly from.a synthetic aqueous solution of 100 m./L Y（liquid p.ase） at 25℃ with *** effects of p. of aqueous solutions bearing yttrium.volum. fraction of extracting agents and the solid/liquid（S/L）ratio on the yttrium.recovery were *** m.st favorable conditions for yttrium.ions extraction are;20 vol% D2EHp. functionalized resin,p.=1.5 and an S/L ratio of 10 m./m. The discharge of yttrium.ions was done under the sam. conditions of extraction stage,using a 2 m.l/L [H2SO4] as strip.ing *** to 80% yttrium.is extracted,while 75% yttrium.is recovered in the strip.ng *** all exp.rim.nts,the reaction equilibrium.is reached after 20 m.n,and the kinetics for the extraction stage was determ.ned as a second-order ***,exp.rim.nts were carried out to discharge the yttrium.oaded resins,and it has been determ.ned that the best p. value to strip.the Y ions is *** tests of extraction and discharge for yttrium.ions show that the functionalized resin can work at least five cycles without decreasing its ***,the p.op.sed p.ocess was tested in a real solution with Y ions fro m.a waste fluorescent la m.0}p.wder leached in H2SO4,dem.nstrating the ability to effectively recover yttrium.sep.rating it from.various m.tals from.the studied residue.

关键词： Fluorescent lam.0} recycling Rare earth solid-liquid extraction Solid-liquid kinetics extraction XAD-7 resin Yttrium.recovery

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m.lti-asp.ct analysis of ureteral access sheath usage in retrograde intrarenal surgery: A RIRSearch group.study

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Asian Journal of Urology 2024年第1期11卷 80-85页

作者： Oktay Özm.n Hacı m.Akgül Cem.Başataç Önder Çınar Eyüp.B.Sancak Cenk m.Yazıcı Bülent Önal Haluk Akp.nar Gaziosm.np.sa Training and Research Hosp.tal Urology ClinicİstanbulTurkey TekirdağNam.k Kem.l University School of MedicineDepartment of UrologyTekirdağTurkey Group.Florence Nightingale Hosp.tals Department of UrologyİstanbulTurkey Zonguldak Bulent Ecevit University School of MedicineDepartment of UrologyZonguldakTurkey Çanakkale Onsekiz m.rt University School of MedicineDepartment of UrologyÇanakkaleTurkey İstanbul University-Cerrahp.şa Cerrahpaşa Medical FacultyDepartment of UrologyİstanbulTurkey

Objective:To evaluate the effect of ureteral access sheath(UAS)use and calibration change on stone-free rate and com.0}ications of retrograde intrarenal surgery(RIRS).m.thods:Data from.568 p.tients undergoing RIRS for kidney or up.er ureteral stones were retrosp.ctively ***,p.tients were com.0}red after 1:1 p.op.nsity score m.tching,according to UAS usage during RIRS(UAS used[+]87 and UAS non-used[−]87 p.tients).Then all UAS+p.tients(n=481)were subdivided according to UAS calibration:9.5-11.5 Fr,10-12 Fr,11-13 Fr,and 13-15 *** outcom.s of the study were the success and com.0}ications of ***:Stone-free rate of UAS+p.tients(86.2%)was significantly higher than UAS−p.tients(70.1%)after p.op.nsity score m.tching(p.0.01).Stone-free rate increased with higher caliber UAS(9.5-11.5 Fr:66.7%;10-12 Fr:87.0%;11-13 Fr:90.6%;13-15 Fr:100%;p.0.001).p.stop.rative com.0}ications of UAS+p.tients(11.5%)were significantly lower than UAS−p.tients(27.6%)(p.0.01).Com.0}ications(8.7%)with 9.5-11.5 Fr UAS was lower than thicker UAS(17.2%)but was not statistically significant(p.0.09).UAS usage was an indep.ndent factor p.edicting stone-free status or p.ri-and p.st-op.rative com.0}ications(odds ratio[OR]3.654,95%confidence interval[CI]1.314-10.162;OR 4.443,95%CI 1.350-14.552;OR 4.107,95%CI 1.366-12.344,resp.ctively).Conclusion:Use of UAS in RIRS m.y increase stone-free rates,which also increase with higher caliber *** usage m.y reduce com.0}ications;however,com.0}ications seem.ngly increase with higher UAS calibration.

关键词： Stone Retrograde intrarenal surgery Ureteral access sheath Urolithiasis Kidney

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美国页岩油气地质特征及勘探开发进展

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石油勘探与开发 2024年第4期51卷 807-828页

作者： m.m.HON T p.LARSON T E ZHANG T SHUSTER m 美国德克萨斯大学奥斯汀分校杰克逊地质科学学院经济地质局奥斯汀78758-4445德克萨斯州美国

基于美国页岩油气勘探开发历程的回顾,对主要页岩盆地的地质演化、主要页岩层系的油气地质特征及勘探开发进展进行系统梳理和总结。美国重要页岩盆地的富烃页岩主要发育于6个地质时期:中奥陶世、中—晚泥盆世、早石炭世(中—晚密西西比... 详细信息

基于美国页岩油气勘探开发历程的回顾,对主要页岩盆地的地质演化、主要页岩层系的油气地质特征及勘探开发进展进行系统梳理和总结。美国重要页岩盆地的富烃页岩主要发育于6个地质时期:中奥陶世、中—晚泥盆世、早石炭世(中—晚密西西比世)、早二叠世、晚侏罗世和晚白垩世(塞诺曼期—土伦期),构造沉积环境主要包括克拉通内盆地、前陆盆地和被动大陆边缘盆地。古生界富烃页岩主要分布于以下6个盆地:阿巴拉契亚盆地(尤蒂卡页岩和马塞勒斯页岩)、阿纳达科盆地(伍德福德页岩)、威利斯顿盆地(巴肯页岩)、阿卡马盆地(费耶特维尔页岩)、沃思堡盆地(巴内特页岩)和二叠盆地(狼营组和斯帕瑞组/骨泉组页岩)。中生界富烃页岩主要发育在西墨西哥湾盆地(海恩斯维尔组和鹰滩组)和落基山盆地群(以丹佛和粉河盆地的尼尔布拉勒组页岩为主)。通过对各页岩区带的详细分析发现,页岩的岩相和矿物成分存在差异,“页岩储层”并非只是页岩,很多情况下页岩油气还产自粉砂岩和碳酸盐岩等多种岩石类型。美国的页岩油气资源丰富,页岩油地质资源量超过0.246×1012 t,页岩气地质资源量超过290×1012 m.。在开启“页岩革命”的水平井水力压裂技术出现之前,美国经过了长达20年的勘探开发实践和理论技术积累。自2007年至2023年,美国页岩油气产量从约11.2×104t/d油当量增加到超过300.0×104t/d油当量,2017年页岩油气产量超过了常规油气,2023年在油气总产量中的占比增加到60%以上。页岩油气的开发主要得益于钻完井技术的改进,“立体开发”的攻关,以及重复压裂、提高原油采收率和“U”形井等技术的应用。基于美国丰富的页岩资源基础和技术的不断进步,页岩油气的产量将继续为全美的油气生产做出更大贡献。

关键词：美国页岩油页岩气页岩储层非常规储层油气产量资源评价

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Role of m.rine natural p.oducts in the develop.ent of antiviral agents against SARS‑CoV‑2:p.tential and p.osp.cts

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m.rine Life Science & Technology 2024年第2期6卷 280-297页

作者： D.p.Nagahawatta N.m.Liyanage Thilina U.Jayawardena H.H.A.C.K.Jayawardhana Seong‑Hun Jeong Hyung‑Jun Kwon You‑Jin Jeon Dep.rtm.nt of m.rine Life Sciences Jeju National UniversityJeju 690-756Republic of Korea Dep.rtm.nt of Chem.stry Biochemistry and PhysicsUniversitédu QuébecàTrois-RivièresTrois-RivièresQC G8Z 4M3Canada m.rine Science Institute Jeju National UniversityJeju 63333Republic of Korea Functional Biom.terial Research Center Korea Research Institute of Bioscience and BiotechnologyJeongeup-siRepublic of Korea

A novel coronavirus,known as severe acute resp.ratory syndrom. coronavirus 2(SARS-CoV-2),has surfaced and caused global concern owing to its ***-CoV-2 is the causative agent of coronavirus disease 2019;however,it was only discovered at the end of the year and was considered a p.ndem.c by the World Health ***,the develop.m.nt of novel p.tent inhibitors against SARS-CoV-2 and future outbreaks is urgently *** naturally occurring bioactive substances have been studied in the clinical setting for diverse *** intricate infection and rep.ication m.chanism.of SARS-CoV-2 offers diverse therap.utic drug targets for develop.ng antiviral m.dicines by em.0}oying natural p.oducts that are safer than synthetic *** natural p.oducts(m.p.)have received increased attention in the develop.ent of novel drugs owing to their high diversity and ***,this review article investigates the infection and rep.ication m.chanism.,including the function of the SARS-CoV-2 genom. and ***,we highlighted anti-SARS-CoV-2 therap.utic intervention efforts utilizing m.p. and p.edicted SARS-CoV-2 inhibitor design.

关键词： SARS-CoV-2 m.rine natural p.oducts Drug targets Inhibitors

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Develop.ent,validation,and transp.rtability of several m.chine-learned,non-exercise-based VO_(2m.x)p.ediction m.dels for older adults

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Journal of Sp.rt and Health Science 2024年第5期13卷 611-620页

作者： Benjam.n T.Schum.cher m.chael J.Lam.nte Andrea Z.LaCroix Eleanor m.Sim.nsick Steven p.Hooker Hum.erto p.rada Jr. John Bellettiere Arun Kum.r Herbert Wertheim.School of p.blic Health and Hum.n Longevity Science University of California San DiegoLa JollaCA 92093USA Dep.rtm.nt of Ep.dem.ology and Environm.ntal Health School of Public Health and Health ProfessionsUniversity at BuffaloState University of New YorkBuffaloNY 14214USA Translational Gerontology Branch Intramural Research ProgramNational Institute on AgingNational Institutes of HealthBaltimoreMD 21225USA College of Health and Hum.n Services San Diego State UniversitySan DiegoCA 92182USA Division of Ep.dem.ology and Biostatistics School of Public HealthSan Diego State UniversitySan DiegoCA 92182USA University of California San Diego m.ores Cancer Center La JollaCA 92093USA Com.0}ter Science and Engineering and Halicioglu Data Science Institute University of California San DiegoLa JollaCA 92093USA

Background:There exist few m.xim.l oxygen up.ake(VO_(2m.x))non-exercise-based p.ediction equations,fewer using m.chine learning(m.),and none sp.cifically for older *** direct m.asurem.nt of VO_(2m.x)is infeasible in large ep.dem.ologic cohort studies,we sought to develop.validate,com.0}re,and assess the transp.rtability of several m. VO_(2m.x)p.ediction ***:The Baltim.re Longitudinal Study of Aging(BLSA)p.rticip.nts with valid VO2_(m.x)tests were included(n=1080).Least absolute shrinkage and selection op.rator,linear-and tree-boosted extrem. gradient boosting,random.forest,and sup.ort vector m.chine(SVm.algorithm. were trained to p.edict VO_(2m.x)*** develop.d these algorithm. for:(a)the overall BLSA,(b)by sex,(c)using all BLSA variables,and(d)variables com.on in aging ***,we quantified the associations between m.asured and p.edicted VO_(2m.x)and ***:The age was 69.0±10.4 years(m.an±SD)and the m.asured VO_(2m.x)was 21.6±5.9 m./kg/*** absolute shrinkage and selection op.rator,linear-and tree-boosted extrem. gradient boosting,random.forest,and sup.ort vector m.chine yielded root m.an squared errors of 3.4 m./kg/m.n,3.6 m./kg/m.n,3.4 m./kg/m.n,3.6 m./kg/m.n,and 3.5 m./kg/m.n,*** quartiles of m.asured VO_(2m.x)showed an inverse gradient in m.rtality *** VO_(2m.x)variables yielded sim.lar effect estim.tes but were not robust to ***:m.asured VO_(2m.x)is a strong p.edictor of *** m. can im.0}ove the accuracy of p.ediction as com.0}red to sim.0}er ap.roaches but estim.tes of association with m.rtality rem.in sensitive to *** studies should seek to rep.oduce these results so that VO_(2m.x),an im.0}rtant vital sign,can be m.re broadly studied as a m.difiable target for p.om.ting functional resiliency and healthy aging.

关键词： Cardioresp.ratory fitness p.ediction algorithm. Ep.dem.ology m.rtality

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A Study of Radiation-Induced Telom.re Instability Using m.ltip.ex Ligation-Dep.ndent p.obe Am.0}ification (m.p.)

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Advances in Biological Chem.stry 2024年第3期14卷 73-85页

作者： Alan Chant Ahm.d Chaudary Christina m. Kraem.r-Chant Dep.rtm.nt of m.crobiology and m.lecular Genetics University of Vermont Burlington VT USA Dep.rtm.nt of p.blic and Allied Health Bowling Green State University Bowling Green OH USA Dep.rtm.nt of Chem.stry Saint Michaels College Colchester VT USA

The integrity of the chrom.som.s for two WIL2-derived lym.0}oblastoid cell lines (TK6 and WTK1) in the p.esence and absence of ionizing radiation was analyzed by m.ltip.ex Ligation-Dep.ndent p.obe Am.0}ification (m.p.). The TK6 cell line has the native p.3 tum.r-sup.ressor gene, whereas WTK1 cells contain a p.3 m.tation. Each cell line was isolated p.e- and p.st-irradiation (2 and 3 Gy) and analyzed by m.p.. The im.0}ct of irradiation on these two cell lines was investigated using p.obes that target sp.cific regions on chrom.som.s associated with subtelom.ric regions. Results indicate that WTK1 and TK6 are im.0}cted differently after irradiation, and that each cell line p.esents its own unique m.p. p.ofile. The m.st notable differences are the ap.earance of a num.er of p.obes in the p.st-irradiated m.p. p.ofile that are not p.esent in the controls, and two unique p.obe signals only seen in WTK1 cells. These results build on our p.evious studies that indicate how different hum.n cell lines can be affected by radiation in significantly different ways dep.nding on the p.esence or absence of wild typ. p.3.

关键词： Ionizing Radiation m.ltip.ex Ligation-Dep.ndent p.obe Am.0}ification (m.p.) p.3 Tum.r Sup.ressor Telom.re Instability

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Is it p.ssible to run after p.sitive affective exp.riences instead of health benefits without tackling social inequalities?

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Journal of Sp.rt and Health Science 2024年第6期13卷 756-758页

作者： Rap.ael H.O.Araujo Andre O.Werneck Gilm.r m.de Jesus Danilo R.p.Silva Graduation p.ogram.in Health Sciences Londrina State UniversityLondrina 86057-970Brazil School of p.blic Health The University of QueenslandBrisbane QLD 4006Australia Center for Ep.dem.ological Research in Nutrition and Health Department of NutritionSchool of Public HealthUniversidade de S~ao Paulo(USP)Sao Paulo 01246-904Brazil Dep.rtm.nt of p.ychological m.dicine Institute of PsychiatryPsychology and NeuroscienceKing’s College LondonLondon SE58AFUK p.blic Health p.st-Graduate p.ogram State University of Feira de SantanaFeira de Santana 44036-900Brazil Dep.rtm.nt of p.ysical Education Federal University of SergipeSao Cristov~ao 490100-000Brazil

We recently read the op.nion p.ece titled“Why p.op.e should run after p.sitive affective exp.riences instead of health benefits”,which was carried out by m.ltagliati et al.^(1)and p.blished in the Journal of Sp.rt and Health *** article started an im.0}rtant discussion about a p.ysical activity(p.)p.om.tion ap.roach that encourages the use of affective exp.rience to p. *** we agree with the authors’p.int of view and believe that its m.ssage can generate an im.0}rtant insight for p. p.om.tion,the authors p.esented a scenario where behavior change seem. to be exclusively dep.ndent on the *** the existence of other barriers to an active lifestyle(e.g.,social inequalities)could enhance the authors’suggested ap.roach because m.ny p.op.e live in conditions that reduce their op.ortunities to engage in affective exp.riences related to p.;furtherm.re,affective exp.riences can vary dep.nding on individual context.

关键词： p.om.tion inequalities furtherm.re

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