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Wastewater degradation by iron/copper nanoparticles and the microorganism growth rate

Journal of Environmental Sciences 2018年第12期30卷 19-31页

作者： Tareq W.M.Amen osama eljamal Ahmed M.E.Khalil Nobuhiro Matsunaga Earth System Science and Technology Interdisciplinary Graduate School of Engineering Sciences Kyushu University Department of Chemical Engineering Faculty of Engineering Cairo University

Nowadays, trends in wastewater treatment by zero-valent iron（ZVI） were turned to use bimetallic NZVI particles by planting another metal onto the ZVI surface to increase its reactivity. Nano size zero-valent iron/copper（NZVI/Cu0） bimetallic particles were synthesized in order to examine its toxicity effects on the wastewater microbial life, kinetics of phosphorus, ammonia stripping and the reduction of chemical oxygen demand（COD）.Various concentrations of NZVI/Cu0 and operation conditions both aerobic and anaerobic were investigated and compared with pure NZVI experiment. The results showed that addition10 mg/L of NZVI/Cu0 significantly increased the numbers of bacteria colonies under anaerobic condition, conversely it inhibited bacteria activity with the presence of oxygen. Furthermore,the impact of nanoparticles on ammonia stripping and phosphorus removal was also linked to the emitted iron ions electrons. It was found that dosing high concentration of bimetallic NZVI/Cu0 has a negative effect on ammonia stripping regardless of the aeration condition. In comparison to control, dosing only 10 mg/L NZVI/Cu0, the phosphorus removal increased sharply both under aerobic and anaerobic conditions, these outcomes were obtained as a result of complete dissolution of bimetallic nanoparticles which formed copper-iron oxides components that are attributed to increasing the phosphorus adsorption rate.

关键词： Iron bimetallic Wastewater biodegradation Bacterial life Contaminants removal

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Removal of Phosphorus from Water Using Marble Dust as Sorbent Material

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Journal of Environmental Protection 2012年第8期3卷 709-714页

作者： osama eljamal Junya Okawauchi Kazuaki Hiramatsu Laboratory of Water Environment Engineering Kyushu University 6-10-1 Hakozaki Higashi-ku Fukuoka 812-8581 Japan

The removal of phosphorus from water using marble dust as sorbent material was studied by conducting batch tests, kinetic sorption model and isotherm model. The kinetic sorption model based on a pseudo equation was applied to predict the rate constant of sorption. Thorough investigations to understand the mechanism of phosphorus sorption onto the marble dust using kinetic sorption models, pseudo first order and pseudo second order kinetic sorption models showed that the kinetic sorption is consistent with the second order model, from which it can be inferred that the mechanism of sorption is chemisorption. The Langmuir and Freundlich isotherm models were applied to describe the equilibrium isotherms. The results of isotherm models showed that the Langmuir isotherm agrees very well with the experimental data compare with Freundlich isotherm. Batch tests and kinetic sorption models results showed that using the marble dust as sorbent material could be remove more than 94.3% of phosphorus from water.

关键词： Removal of Phosphorus Marble Dust Kinetic Model Pseudo Equation Isotherm Model

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Sorption Kinetic of Arsenate as Water Contaminant on Zero Valent Iron

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Journal of Water Resource and Protection 2013年第6期5卷 563-567页

作者： osama eljamal Keiko Sasaki Tsuyoshi Hirajima Department of Earth Resources Engineering Kyushu University Fukuoka Japan

This study investigates the sorption of arsenate from water using zero-valent iron ZVI as sorbent. Batch experiments were carried out to study the sorption kinetics of arsenate under different concentrations of arsenate varies from 0.5 to 200 mg/l. A kinetic model was considered to describe the arsenates sorption on ZVI material. The kinetics of the arsenate sorption processes were described by the Langmuir kinetic model. The sorption capacity increases with high initial concentration which obtained the maximum sorption 2.1 mg/g at 200 mg/l of arsenate initial concentration. The results show that the rapid initial sorption rates of arsenate were occurred at the beginning of experiments running time, followed by a slower removal that gradually approaches an equilibrium condition. The data from laboratory batch experiments were used to verify the simulation results of the kinetic model resulting in good agreement between measured and modeled results. The results indicate that ZVI could be employed as sorbent materials to enhance the sorption processes and increase the removal rate of arsenate from water.

关键词： Arsenic Sorption Langmuir Kinetic Model Zero-Valent Iron Removal of Arsenate Iron(III)

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