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Transport properties of dilute ammonia-noble gas mixtures from new intermolecular potential energy functions

Chinese Journal of Chemical Engineering 2017年第12期25卷 1727-1734页

作者： Farshid Zargari Delara Mohammad-Aghaie Maryam Lotfi Masoume Ghorbanipour Mohammad Mehdi Alavianmehr omolbanin shahraki Department of Chemistry Shiraz University of Technology Shiraz Iran Medicinal and Natural Products Chemistry Research Center Shiraz University of Medical Sciences Shiraz Iron Department of Physical Chemistry University of Tabriz Tabriz Iran Zahedan University of Medical Sciences Zahedan Iran

Previously we have determined the dilute mixture transport properties of slightly polar fluorocarbons using the inverted intermolecular potential energies(Ind. Eng. Chem. Res. 45(2006) 9211–9223). In the present paper, the corresponding states correlations for reduced viscosity collision integrals were employed to obtain effective unlike interaction potential models for dilute binary mixtures of highly polar molecule ammonia with noble *** inverted potentials were fitted to the Morse–Spline–van der Waals(MSV), model potential. The method of least-squares fitting was then applied to identify best consistence force parameters for each ammonia-noble gas mixture, taking advantage of experimental viscosities, diffusion coefficients and thermal *** proposed potential models were compared with those obtained from other sources, in order to assess the extent of their *** potentials were later employed to calculate transport properties of the studied mixtures. Then, results were compared with those reported in the literature, which led to the acceptable agreement.

关键词： lntermolecular potential energy Transport properties Inversion pmcedure Mixture Ammonia Noble gas

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