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Nanoconfinement-induced water molecules and hydrogen molecules transport behaviors in ball-in-ball structure photocatalysts to improve hydrogen evolution

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Nano Research 2024年第5期17卷 3752-3760页

作者： Ben Chong Baorong Xu He Li Honghui ou Guidong Yang XJTU-Oxford Joint International Research Laboratory of Catalysis School of Chemical Engineering and TechnologyXi’an Jiaotong UniversityXi’an 710049China

The diffusion,adsorption/desorption behaviors of water molecules and hydrogen molecules are of great importance in heterogeneous photocatalytic hydrogen *** the study of structure-property-performance relationships,nanoconfined space provides an ideal platform to promote mass diffusion and transfer due to their extraordinary properties that are different from the bulk ***,we designed and prepared a nanoconfined CdS@SiO_(2)-NH_(2) nanoreactor,whose shell is composed of amino-functionalized silica nanochannels,and encapsulates spherical CdS as a photocatalyst *** and simulated results reveal that the amino-functionalized nanochannels promote water molecules’and hydrogen molecules’directional diffusion and *** molecules are enriched in the nanocavity between the core and the shell,and promote the interfacial photocatalytic *** a result,the maximized water enrichment and minimized hydrogen-occupied active sites enable photocatalyst with optimized mass transfer kinetics and localization electron distribution on the CdS surface,leading to superior hydrogen production performance with activity as high as 37.1 mmol·g^(-1)·h^(-1).

关键词： nanochannels photocatalytic hydrogen evolution mass transfer amino-functionalized CdS

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页岩小层水平井对比及其构造三维可视化表征

西南石油大学学报（自然科学版） 2019年第6期41卷 44-50页

作者：欧成华杨晓梁成钢黄毅朱海燕油气藏地质及开发工程国家重点实验室·西南石油大学四川成都610500 东方地球物理勘探有限责任公司西南物探研究院四川成都610213 中国石油新疆油田分公司准东采油厂新疆阜康831511 中国石油测井有限公司西南分公司重庆渝北400021 油气藏地质及开发工程国家重点实验室·成都理工大学四川成都610059

页岩气建产区是以平台+水平井的井工厂模式运营的,利用水平井开展页岩小层对比及其结构与构造建模,在目前还是一项亟待攻关的技术难题。在解析页岩小层结构特征基础上,建立了页岩小层分层模式和水平井测井多井三维可视化对比方法,依靠井... 详细信息

页岩气建产区是以平台+水平井的井工厂模式运营的,利用水平井开展页岩小层对比及其结构与构造建模,在目前还是一项亟待攻关的技术难题。在解析页岩小层结构特征基础上,建立了页岩小层分层模式和水平井测井多井三维可视化对比方法,依靠井-震结合,实现了页岩小层结构与层面构造的三维建模,形成了井工厂模式下页岩气建产区小层结构与层面构造三维可视化表征新技术。成功完成了四川盆地W页岩气田某典型建产区6个页岩小层分层模式的建立、水平井多井可视化对比,以及页岩小层结构与7个小层层面构造模型的建立。在证实该技术实用性及可靠性的同时,还为研究区后期的精细化生产管理提供了构造模型基础。

关键词：页岩小层井工厂模式水平井小层对比三维可视化表征构造建模

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考虑吸附、变形的煤层气分阶段流动模型

天然气工业 2011年第3期31卷 48-51,110-111页

作者：欧成华梁成钢蒋建立张俊成 "油气藏地质及开发工程"国家重点实验室.西南石油大学中国石油新疆油田公司准东采油厂新疆准东石油技术股份有限公司

煤岩具有微孔—中孔—大孔—裂隙多重孔隙结构,中孔—大孔中的煤层气流动规律是连接微孔解吸和裂隙渗流的桥梁,是揭示煤层气解吸—扩散—渗流分阶段产出机理的关键环节。基于受煤岩变形影响的煤层气分阶段产出特征和规律分析,建立煤层... 详细信息

煤岩具有微孔—中孔—大孔—裂隙多重孔隙结构,中孔—大孔中的煤层气流动规律是连接微孔解吸和裂隙渗流的桥梁,是揭示煤层气解吸—扩散—渗流分阶段产出机理的关键环节。基于受煤岩变形影响的煤层气分阶段产出特征和规律分析,建立煤层气在基质微孔表面解吸、由基质微孔向基质较大孔扩散、在基质较大孔中和裂隙空间中渗流的分阶段流动数学模型,求取裂隙中气—水两相隐式压力显式饱和度有限差分线性方程组,计算出晋试1井煤层气的产出动态,验证了考虑吸附变形的煤层气分阶段流动模型的可靠性,为完善煤层气产出动态分析和预测方法提供了理论依据。

关键词：煤层气流动阶段吸附变形数学模型泌水盆地

Re-examination of statistical relationships between dietary fats and other risk factors,and cardiovascular disease,based on two crucial datasets

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Quantitative Biology 2024年第1期12卷 117-127页

作者： Jiarui ou Le Zhang Xiaoli Ru College of Computer Science Sichuan UniversityChengduChina Department of Gynecology and Obstetrics Beijing Chao-Yang HospitalCapital Medical UniversityBeijingChina

Cardiovascular disease(CVD)is the major cause of death in many regions around the world,and several of its risk factors might be linked to *** improve public health and the understanding of this topic,we look at the recent Minnesota Coronary Experiment(MCE)analysis that used t-test and Cox model to evaluate CVD ***,these parametric methods might suffer from three problems:small sample size,right-censored bias,and lack of long-term *** overcome the first of these challenges,we utilize a nonparametric permutation test to examine the relationship between dietary fats and serum total *** address the second problem,we use a resampling-based rank test to examine whether the serum total cholesterol level affects CVD *** the third issue,we use some extra-Framingham Heart Study(FHS)data with an A/B test to look for meta-relationship between diets,risk factors,and CVD *** show that,firstly,the link between low saturated fat diets and reduction in serum total cholesterol is ***,reducing serum total cholesterol does not robustly have an impact on CVD hazards in the diet ***,the A/B test result suggests a more complicated relationship regarding abnormal diastolic blood pressure ranges caused by diets and how these might affect the associative link between the cholesterol level and heart disease *** study not only helps us to deeply analyze the MCE data but also,in combination with the long-term FHS data,reveals possible complex relationships behind diets,risk factors,and heart disease.

关键词： A/B test bioinformatics cardiovascular disease nonparametric statistics

柴达木盆地干柴沟—咸水泉地区中—深层成岩演化及其对储集体性能的影响

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古地理学报 2011年第1期13卷 85-95页

作者：欧成华董兆雄魏学斌西南石油大学油气藏地质及开发工程国家重点实验室四川成都610500 中国石油青海油田分公司勘探开发研究院甘肃敦煌736202

通过剖面观察、岩心描述、分析化验等手段,系统研究了柴达木盆地干柴沟—咸水泉地区中—深层储集体岩石学特征、主要成岩作用类型及特征、储集空间类型及特征、成岩阶段及成岩演化序列,以及成岩作用对储集体性能的影响程度和规律。结果... 详细信息

通过剖面观察、岩心描述、分析化验等手段,系统研究了柴达木盆地干柴沟—咸水泉地区中—深层储集体岩石学特征、主要成岩作用类型及特征、储集空间类型及特征、成岩阶段及成岩演化序列,以及成岩作用对储集体性能的影响程度和规律。结果表明:研究区中—深层储集体主要由成分及结构成熟度均为低—中等的各类砂岩和部分泥灰岩组成;以压实作用、胶结作用、充填作用为主的破坏性成岩作用造成了储集体孔隙空间的大量损失,而以溶蚀作用为主的建设性成岩作用则使部分储集体恢复了储集性能;破坏性成岩作用主要发生在同生成岩、早成岩和中成岩阶段,建设性成岩作用主要发生在褶皱回返引起的表生成岩阶段;受成岩作用影响,主要发育粒间孔、残余粒间孔和溶蚀孔隙,孔隙结构以微细喉型为主,储集层类型以低孔—特低渗储集层为主。

关键词：成岩作用成岩序列储集性能柴达木盆地

Low rank optimization for efficient deep learning:making a balance between compact architecture and fast training

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Journal of Systems Engineering and Electronics 2024年第3期35卷 509-531,F0002页

作者： ou Xinwei CHEN Zhangxin ZHU Ce LIU Yipeng School of Information and Communication Engineering University of Electronic Science and Technology of ChinaChengdu 611731China

Deep neural networks(DNNs)have achieved great success in many data processing ***,high computational complexity and storage cost make deep learning difficult to be used on resource-constrained devices,and it is not environmental-friendly with much power *** this paper,we focus on low-rank optimization for efficient deep learning *** the space domain,DNNs are compressed by low rank approximation of the network parameters,which directly reduces the storage requirement with a smaller number of network *** the time domain,the network parameters can be trained in a few subspaces,which enables efficient training for fast *** model compression in the spatial domain is summarized into three categories as pre-train,pre-set,and compression-aware methods,*** a series of integrable techniques discussed,such as sparse pruning,quantization,and entropy coding,we can ensemble them in an integration framework with lower computational complexity and *** addition to summary of recent technical advances,we have two findings for motivating future *** is that the effective rank,derived from the Shannon entropy of the normalized singular values,outperforms other conventional sparse measures such as the?_1 norm for network *** other is a spatial and temporal balance for tensorized neural *** accelerating the training of tensorized neural networks,it is crucial to leverage redundancy for both model compression and subspace training.

关键词： model compression subspace training effective rank low rank tensor optimization efficient deep learning

Ultrathin two-dimensional medium-entropy oxide as a highly efficient and stable electrocatalyst for oxygen evolution reaction

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Nano Research 2024年第4期17卷 2555-2562页

作者： Guangyuan Yan Tianlu Wang Biwei Zhao Wenjing Gao Tong Wu Liming ou School of Mechanical Electronic and Control EngineeringBeijing Jiaotong UniversityBeijing 100044China

Medium-entropy oxides(MEOs)with broad compositional tunability and entropy-driven structural stability,are receiving booming attention as a promising candidate for oxygen evolution reaction(OER)***,ultrathin two-dimensional(2D)nanostructure offers extremely large specific surface area and is therefore considered to be an ideal catalyst ***,it remains a grant challenge to synthesize ultrathin 2D MEOs due to distinct nucleation and growth kinetics of constituent multimetallic elements in 2D anisotropic *** this work,an ultrathin 2D MEO(MnFeCoNi)O was successfully synthesized by a facile and low-temperature ionic layer epitaxy *** from multi-metal synergistic effects within ultrathin 2D nanostructure,this 2D MEO(MnFeCoNi)O revealed excellent OER electrocatalytic performance with a quite low overpotential of 117 mV at 10 mA·cm^(-2) and an impressive stability for 120 h continuous operation with only 6.9%***,the extremely high mass activity(5584.3 A·g^(-1))was three orders of magnitude higher than benchmark RuO_(2)(3.4 A·g^(-1))at the same overpotential of 117 *** work opens up a new avenue for developing highly efficient and stable electrocatalysts by creating 2D nanostructured MEOs.

关键词： medium-entropy oxide two-dimensional nanomaterials ionic layer epitaxy oxygen evolution reaction electrocatalysis

Alleviating the anisotropic microstructural change and boosting the lithium ions diffusion by grain orientation regulation for Ni-rich cathode materials

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Journal of Energy Chemistry 2024年第1期88卷 213-222,I0005页

作者： Xinyou He Shilin Su Bao Zhang Zhiming Xiao Zibo Zhang Xing ou Engineering Research Center of the Ministry of Education for Advanced Battery Materials School of Metallurgy and EnvironmentCentral South UniversityChangsha 410083HunanChina Zhejiang Power New Energy Co.Ltd Zhuji 311899ZhejiangChina

Generally,layered Ni-rich cathode materials exhibit the morphology of polycrystalline secondary sphere composed of numerous primary *** the arrangement of primary particles plays a very important role in the properties of Ni-rich *** disordered particle arrangement is harmful to the cyclic performance and structural stability,yet the fundamental understanding of disordered structure on the structural degradation behavior is ***,we have designed three kinds of LiNi_(0.83)Co_(0.06)Mn_(0.11)O_(2) cathode materials with different primary particle orientations by regulating the precursor coprecipitation *** finite element simulation and in-situ characterization,the Li^(+)transport and structure evolution behaviors of different materials are ***,the smooth Li^(+)diffusion minimizes the reaction heterogeneity,homogenizes the phase transition within grains,and mitigates the anisotropic microstructural change,thereby modulating the crack evolution ***,the optimized structure evolution ensures radial tight junctions of the primary particles,enabling enhanced Li^(+)diffusion during dynamic ***-loop bidirectional enhancement mechanism becomes critical for grain orientation regulation to stabilize the cyclic *** precursor engineering with particle orientation regulation provides the useful guidance for the structural design and feature enhancement of Ni-rich layered cathodes.

关键词： Ni-rich cathode Grain orientation regulation Anisotropic microstructural change Precursor engineering Li~+-ions diffusion

A Video Captioning Method by Semantic Topic-Guided Generation

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Computers, Materials & Continua 2024年第1期78卷 1071-1093页

作者： ou Ye Xinli Wei Zhenhua Yu Yan Fu Ying Yang College of Computer Science and Technology Xi’an University of Science and TechnologyXi’an710054China

In the video captioning methods based on an encoder-decoder,limited visual features are extracted by an encoder,and a natural sentence of the video content is generated using a ***,this kind ofmethod is dependent on a single video input source and few visual labels,and there is a problem with semantic alignment between video contents and generated natural sentences,which are not suitable for accurately comprehending and describing the video *** address this issue,this paper proposes a video captioning method by semantic topic-guided ***,a 3D convolutional neural network is utilized to extract the spatiotemporal features of videos during the ***,the semantic topics of video data are extracted using the visual labels retrieved from similar video *** the decoding,a decoder is constructed by combining a novel Enhance-TopK sampling algorithm with a Generative Pre-trained Transformer-2 deep neural network,which decreases the influence of“deviation”in the semantic mapping process between videos and texts by jointly decoding a baseline and semantic topics of video *** this process,the designed Enhance-TopK sampling algorithm can alleviate a long-tail problem by dynamically adjusting the probability distribution of the predicted ***,the experiments are conducted on two publicly used Microsoft Research Video Description andMicrosoft Research-Video to Text *** experimental results demonstrate that the proposed method outperforms several state-of-art ***,the performance indicators Bilingual Evaluation Understudy,Metric for Evaluation of Translation with Explicit Ordering,Recall Oriented Understudy for Gisting Evaluation-longest common subsequence,and Consensus-based Image Description Evaluation of the proposed method are improved by 1.2%,0.1%,0.3%,and 2.4% on the Microsoft Research Video Description dataset,and 0.1%,1.0%,0.1%,and 2.8% on the Microsoft Research-Video to Text dataset

关键词： Video captioning encoder-decoder semantic topic jointly decoding Enhance-TopK sampling