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CCS Chemistry 2024年第10期6卷 2502-2514页

作者： Kang Huang Hao Wan Zhichao Gong Jianbin Liu Minmin Yan Jun Wu Chunyu Cui Gonglan ye Karsten Reuter Huilong Fei Advanced Catalytic engineering Research Center of the Ministry of education State Key Laboratory for Chemo/Biosensing and ChemometricsCollege of Chemistry and Chemical EngineeringHunan UniversityChangsha 410082 Fritz-Haber-Institut der Max-Planck-Gesellschaft Berlin 14195

The formation of LiOH as the discharge product instead of Li_(2)O_(2)in Li-O_(2)batteries(LOBs)is highly desirable due to the associated drawbacks of Li_(2)O_(2)-based chemistry,which involves the generation of reactive oxygen intermediates responsible for substantial side ***,the current challenge lies in the formation pathway of LiOH,which typically requires the chemical hydrolysis of the hazardous LiO_(2)or Li_(2)O_(2)intermediate,posing risks to the battery ***,we report a direct 4e–electrochemical approach to LiOH enabled by a single atom catalyst(SAC)consisting of CoN_(3)moieties embedded in graphene(CoN_(3)-G),while Li_(2)O_(2)is formed on the metal-free nitrogen-doped graphene(NG).The direct 4e–LiOH pathway significantly reduces the parasitic reactions,resulting in negligible damage to the electrolyte and *** stands in strong contrast to the conventional 2e–Li_(2)O_(2)pathway mediated by NG and the indirect LiOH pathway by MnO_(2).Theoretical calculations further clarify that the presence of CoN_(3)sites enhances the adsorption of oxygen-containing intermediates like*OLiO and*Li_(2)O_(2),promoting the protonation of*Li_(2)O_(2)and the cleavage of the O–O bond to form *** work demonstrates a promising strategy to modulate the reaction pathways in LOBs and broadens the applications of SACs.

关键词： single atom catalyst LiOH Li-O_(2)batteries direct 4-electron oxygen reduction pathway selectivity

On Differential equations of Integrable Billiard Tables

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Acta Mathematica Sinica,english Series 2024年第1期40卷 417-424页

作者： Vladimir DRAGOVIC Andrey e.MIRONOV Department of Mathematical Sciences The University of Texas at DallasRichardson TXUSA Mathematical Institute SANU BelgradeSerbia Novosibirsk State University NovosibirskRussia Sobolev Institute of Mathematics of the Siberian Branch of the Russian Academy of Sciences NovosibirskRussia

We introduce a method to find differential equations for functions which define tables,such that associated billiard systems admit a local first *** illustrate this method in three situations:the case of(locally)integrable wire billiards,for finding surfaces in R^(3)with a first integral of degree one in velocities,and for finding a piece-wise smooth surface in R^(3)homeomorphic to a torus,being a table of a billiard admitting two additional first integrals.

关键词： Polynomial first integrals wire billiards piece-wise smooth surfaces

船舶抵离美国港口出入境申报e-NOA/D7.8版使用详解

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天津航海 2024年第3期 13-15,38页

作者：叶迪中远海运船员管理有限公司天津分公司天津300450

船舶在抵离美国港口时需使用excel workbook e-NOA/D 7.8版进行美国港口抵离港电子申报的相关操作。针对于此,文章进行了详细讲解,并归纳了注意事项,对船舶在美国港口正确地进行抵离港电子申报具有一定的指导意义。

关键词：美国港口出入境电子申报 eNOA/D 操作说明注意事项

Aulacaspis yasumatsui infestations accelerate Cycas leaf litter decomposition and nutrient release

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Pedosphere 2024年第3期34卷 681-684页

作者： Thomas e.MARLeR Bagong Kaalaman Botanikal Institute 15 Rizal StreetBarangay MalabañasAngeles City 2009(Philippines)

Dear editor,Numerous aspects of ecosystem ecology are influenced by insects(Prasad,2022).Herbivory of plant organs by insects may influence the biogeochemistry of forests by changing the speed of litter decomposition(Schowalter,2022).Cycas micronesica *** is the only native gymnosperm in the Mariana *** once-abundant tree experienced no known lethal threats prior to the 2003 invasion of Guam by the scale Aulacaspis yasumatsui Takagi(Marler,2012).This insular case study has been the subject of abundant research(Marler et al.,2021).Changes to leaf litter chemistry improved litter quality following *** infestations(Marler and Dongol,2016),but the prediction of increased decomposition speed has not been confirmed with experimental incubations.

关键词： litter fir release

Octopamine enhances learning

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National Science Review 2024年第6期11卷 82-83页

作者： Yvette e.Fisher Department of Molecular and Cell Biology and Helen Wills Neuroscience Institute University of California

Across the animal kingdom, diverse monoamines actuate and modulate neural circuit function. However, measuring the rapid dynamics of these neuromodulators at cellular resolution has historically presented significant ... 详细信息

关键词： DOPAMINe TYRAMINe FLIeS

Commentary on "Association of daily sitting time and leisure-time physical activity with body fat among ***"

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Journal of Sport and Health Science 2024年第2期13卷 127-129页

作者： Barbara e.Ainsworth School of exercise and Health Shanghai University of SportShanghai 200438China

In their study,association of daily sitting time and leisure-time physical activity (LTPA) with body fat among ***,Liao et al.^(1) analyzed data from the 2011-2018 National Health and examination Survey to examine associations between h/day sitting,meeting (or not meeting) the *** Activity Guidelines of≥150 min/week of moderate-and vigorous-intensity LTPA,and combinations of sitting time and LTPA on totaland trunk percent body fat (BF%).

关键词： U.S. adult among

exploration of chromene-based BioAIegens

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National Science Review 2024年第3期11卷 47-48页

作者： Fritz e.Kühn Department of Chemistry&Catalysis Research Center School of Natural Sciences Technical University of Munich

Photoemission efficiency is usually higher in solution than in solid *** compounds however, display a reverse behavior. Such a behavior is called aggregation-induced emission(AIe).

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Performance analysis of deep borehole heat exchangers for decarbonization of heating systems

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Deep Underground Science and engineering 2024年第3期3卷 349-357页

作者： Andreas e.D.Lund Department of electrical engineering and Automation Aalto UniversityEspooFinland

Meeting the climate change mitigation targets will require a substantial shift from fossil to clean fuels in the heating *** pumps with deep borehole exchangers are a promising solution to reduce *** the thermal behavior of deep borehole exchangers(DBHes)ranging from 1 to 2 km was analyzed for various heat flow profiles.A strong correlation between thermal energy extraction and power output from DBHes was found,also influenced by the heating profile *** operating time over the year typically resulted in higher energy production,while shorter one yielded higher average thermal power output,highlighting the importance of the choice of heating strategy and system design for optimal performance of *** breaks in operation for regenerating the borehole,for example,with waste heat,proved to be favorable for the performance yielding an overall heat output close to the same as with continuous extraction of *** results demonstrate the usefulness of deep boreholes for dense urban areas with less available *** the heat production from a single DBHe in Finnish conditions ranges from half up to even a few GWh a year,the technology is best suitable for larger heat loads.

关键词： clean energy deep borehole exchangers energy transition geothermal heat ground-coupled heat pump

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Mechanically strong porous bioceramic tubes facilitate large segmental bone defect repair by providing long-term structurally stability and promoting osteogenesis

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engineered Regeneration 2024年第1期5卷 1-10页

作者： Lijun Xie Jiahao Zhang Hangxiang Sun Zehao Chen Wangsiyuan Teng Xupeng Chai Cong Wang Xianyan Yang Yifan Li Sanzhong Xu Zhongru Gou Zhaoming ye Department of Orthopedic Surgery the Second Affiliated HospitalZhejiang University School of MedicineHangzhou 310000PR China Orthopedics Research Institute of Zhejiang University Hangzhou 310000PR China Key Laboratory of Motor System Disease Research and Precision Therapy of Zhejiang Province Hangzhou 310000PR China Bio-nanomaterials and Regenerative Medicine Research Division Zhejiang-California International Nanosystem InstituteZhejiang UniversityHangzhou 310058PR China Department of Orthopedics the First Affiliated HospitalZhejiang University School of MedicineHangzhou 310003PR China

Mechanically strong magnesium-doped Ca-silicate bioceramic scaffolds have many advantages in repairing large segmental bone *** we combine β-TCP with 6 mol%magnesium-doped calcium silicate(Mg6)at three different ratios(TCP,TCP+15%Mg6,TCP+85%Mg6)to find an appropriate ratio which can exert considerable influence on bone *** this study,the bioceramic scaffolds were assessed for mechanical strength,bioactive ion release,biocompatibility,and osteogenic capacity through in vitro ***,the potential for promoting bone regeneration was investigated through in vivo implantation of porous tube-like *** results showed that the compressive strength increased with the augmentation of Mg6 *** the compressive strength of the TCP+85%Mg6 group reached 38.1±3.8 MPa,three times that of the other two ***,extensive in vivo investigations revealed that the TCP+85%Mg6 bioceramic scaffolds were particularly beneficial for the osteogenic capacity of critical-sized femoral defects(20 mm in length).Altogether,magnesium doping in bioceramic implants is a promising strategy to provide stronger mechanical support and enhance osteogenesis to accelerate the repair of large defects.

关键词： Bioceramic tubes Mg-doped calcium silicate Porous structural stability Large segmental bone defects Digital light processing

Climate refugia along Lake Superior’s shores:disjunct arctic-alpine plants rely on cool shoreline temperatures but are restricted to highly exposed habitat under climate warming

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Journal of Plant ecology 2024年第4期17卷 23-41页

作者： Ashley Hillman Scott e.Nielsen Department of Renewable Resources University of AlbertaEdmontonAB T6G 2R3Canada

Climate refugia can serve as a remnant habitat or stepping stones for species dispersal under climate *** largest freshwater lake by surface area,Lake Superior,USA and Canada,serves as a model system for understanding cooling-mediated local refugia,as its cool water temperatures and wave action have maintained shoreline habitats suitable for southern disjunct populations of arctic-alpine plants since ***,we seek to explain spatial patterns and environmental drivers of arctic-alpine plant refugia along Lake Superior’s shores,and assess future risk to refugia under moderate(+3.5℃)and warmest(+5.7℃)climate warming ***,we examined how the interactive effects of summer surface water temperatures and wind affected onshore temperatures,resulting in areas of cooler ***,we developed an ecological niche model for the presence of disjunct arctic-alpine refugia(pooling 1253 occurrences from 58 species)along the lake’s ***,we fit species distribution models for 20 of the most common arctic-alpine disjunct species and predicted presence to identify refugia ***,we used the two climate warming scenarios to predict changes in the presence of refugia and disjunct *** type,elevation above water,inland distance,July land surface temperature from MODIS/Terra satellite and near-shore depth of water were the best predictors of disjunct ***,we predicted 2236 km of the shoreline(51%)as disjunct refugia habitat for at least one species under current conditions,but this was reduced to 20% and 7% with moderate(894 km)and warmest(313 km)climate change projections.

关键词： climate refugia disjunct populations lake effect Lake Superior species distribution models