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Evidence for particle acceleration approaching PeV energies in the W51 complex

Science Bulletin 2024年第18期69卷 2833-2841页

作者： cao, Zhen Aharonian, F. Axikegu Bai, y.X. Bao, y.W. Bastieri, D. Bi, X.J. Bi, y.J. Bian, W. Bukevich, A.V. cao, Q. cao, W.y. cao, Zhe chang, J. chang, J.F. chen, A.M. chen, E.S. chen, H.X. chen, Liang chen, Lin chen, Long chen, M.J. chen, M.L. chen, Q.H. chen, S. chen, S.H. chen, S.Z. chen, T.L. chen, y. cheng, N. cheng, y.D. cui, M.y. cui, S.W. cui, X.H. cui, y.D. Dai, B.Z. Dai, H.L. Dai, Z.G. Danzengluobu Dong, X.Q. Duan, K.K. Fan, J.H. Fan, y.Z. Fang, J. Fang, J.H. Fang, K. Feng, c.F. Feng, H. Feng, L. Feng, S.H. Feng, X.T. Feng, y. Feng, y.L. Gabici, S. Gao, B. Gao, c.D. Gao, Q. Gao, W. Gao, W.K. Ge, M.M. Geng, L.S. Giacinti, G. Gong, G.H. Gou, Q.B. Gu, M.H. Guo, F.L. Guo, X.L. Guo, y.Q. Guo, y.y. Han, y.A. Hasan, M. He, H.H. He, H.N. He, J.y. He, y. Hor, y.K. Hou, B.W. Hou, c. Hou, X. Hu, H.B. Hu, Q. Hu, S.c. Huang, D.H. Huang, T.Q. Huang, W.J. Huang, X.T. Huang, X.y. Huang, y. Ji, X.L. Jia, H.y. Jia, K. Jiang, K. Jiang, X.W. Jiang, Z.J. Jin, M. Kang, M.M. Karpikov, I. Kuleshov, D. Kurinov, K. Li, B.B. Li, c.M. Li, cheng Li, cong Li, D. Li, F. Li, H.B. Li, H.c. Li, Jian Li, Jie Li, K. Li, S.D. Li, W.L. Li, X.R. Li, Xin Li, y.Z. Li, Zhe Li, Zhuo Liang, E.W. Liang, y.F. Lin, S.J. Liu, B. Liu, c. Liu, D. Liu, D.B. Liu, H. Liu, H.D. Liu, J. Liu, J.L. Liu, M.y. Liu, R.y. Liu, S.M. Liu, W. Liu, y. Liu, y.N. Luo, Q. Luo, y. Lv, H.K. Ma, B.Q. Ma, L.L. Ma, X.H. Mao, J.R. Min, Z. Mitthumsiri, W. Mu, H.J. nan, y.c. Neronov, A. Ou, L.J. Pattarakijwanich, P. Pei, Z.y. Qi, J.c. Qi, M.y. Qiao, B.Q. Qin, J.J. Raza, A. Ruffolo, D. Sáiz, A. Saeed, M. Semikoz, D. Shao, L. Shchegolev, O. Sheng, X.D. Shu, F.W. Song, H.c. Stenkin, yu.V. Stepanov, V. Su, y. Sun, D.X. Sun, Q.N. Sun, X.N. Sun, Z.B. Takata, J. Tam, P.H.T. Key Laboratory of Particle Astrophysics & Experimental Physics Division & computing center Institute of High Energy Physics Chinese Academy of Sciences Beijing 100049 China University of chinese Academy of Sciences Beijing 100049 China TIANFU cosmic Ray Research center Chengdu China Dublin Institute for Advanced Studies 31 Fitzwilliam Place 2 Dublin Ireland Max-Planck-Institut for Nuclear Physics P.O. Box 103980 Heidelberg 69029 Germany School of Physical Science and Technology & School of Information Science and Technology Southwest Jiaotong University Chengdu 610031 China School of Astronomy and Space Science Nanjing University Nanjing 210023 China center for Astrophysics Guangzhou University Guangzhou 510006 China Tsung-Dao Lee Institute & School of Physics and Astronomy Shanghai Jiao Tong University Shanghai 200240 China Institute for Nuclear Research of Russian Academy of Sciences Moscow 117312 Russia Hebei Normal University Shijiazhuang 050024 China University of Science and Technology of china Hefei 230026 China State Key Laboratory of Particle Detection and Electronics China Key Laboratory of Dark Matter and Space Astronomy & Key Laboratory of Radio Astronomy Purple Mountain Observatory Chinese Academy of Sciences Nanjing 210023 China Research center for Astronomical computing Zhejiang Laboratory Hangzhou 311121 China Key Laboratory for Research in Galaxies and cosmology Shanghai Astronomical Observatory Chinese Academy of Sciences Shanghai 200030 China School of Physics and Astronomy Yunnan University Kunming 650091 China Key Laboratory of cosmic Rays (Tibet University) Ministry of Education Lhasa 850000 China National Astronomical Observatories Chinese Academy of Sciences Beijing 100101 China School of Physics and Astronomy (Zhuhai) & School of Physics (Guangzhou) & Sino-French Institute of Nuclear Engineering and Technology (Zhuhai) Sun Yat-sen University Zhuhai 519000 & Guangzhou 510275 Guangdong China Institute of Frontier and

The γ-ray emission from the W51 complex is widely acknowledged to be attributed to the interaction between the cosmic rays (cRs) accelerated by the shock of supernova remnant (SNR) W51c and the dense molecular clouds in the adjacent star-forming region, W51B. However, the maximum acceleration capability of W51c for cRs remains elusive. Based on observations conducted with the Large High Altitude Air Shower Observatory (LHAASO), we report a significant detection of γ rays emanating from the W51 complex, with energies from 2 to 200 TeV. The LHAASO measurements, for the first time, extend the γ-ray emission from the W51 complex beyond 100 TeV and reveal a significant spectrum bending at tens of TeV. By.c.mbining the "π0-decay bump" featured data from Fermi-LAT, the broadband γ-ray spectrum of the W51 region can be well-characterized by a simple pp-collision model. The observed spectral bending feature suggests an exponential cutoff at ∼400 TeV or a power-law break at ∼200 TeV in the cR proton spectrum, most likely providing the first evidence of SNRs serving as cR accelerators approaching the PeV regime. Additionally, two young star clusters within W51B could also be theoretically viable to produce the most energetic γ rays observed by LHAASO. Our findings strongly support the presence of extreme cR accelerators within the W51 complex and provide new insights into the origin of Galactic cRs. © 2024 Science china Press

关键词： cosmic rays

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carbon coated LaFe_(0.92)Pd_(0.08)O_(3) composites for catalytic transfer hydrogenation:Balance in the ability of substrates adsorption and conversion

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nano Research 2024年第5期17卷 3724-3732页

作者： Bowen Wang nan Zhang Ping Xiao Jian Zhang Sónia A.c.carabineiro Junjiang Zhu Hubei Key Laboratory of Biomass Fibers and Eco-dyeing&Finishing College of Chemistry and Chemical EngineeringWuhan Textile UniversityWuhan 430200China college of chemistry and Materials Engineering Wenzhou UniversityWenzhou 325035China LAQV-REQUIMTE Department of ChemistryNOVA School of Science and TechnologyUniversidade NOVA de LisboaLargo da Torre2829-516 CaparicaPortugal

catalytic transfer hydrogenation(cTH)is a green and efficient pathway for selective hydrogenation of unsaturated aldehydes and ***,managing the abilities of solid catalysts to adsorb substrates and to convert them into desired products is a challenging ***,we report the synthesis of carbon coated LaFe_(0.92)Pd_(0.08)O_(3) composites(LFPO-8@c)for cTH of benzaldehyde(BzH)into benzyl alcohol(BzOH),using isopropanol(IPA)as hydrogen *** coating with carbon improves the ability to adsorb/transfer reactants from solution to active sites,and the doping of Pd2+at Fe3+site strengthens the ability of LaFeO_(3) to convert BzH into BzOH.A balanced point between them(i.e.,abilities to adsorb BzH and to convert BzH into BzOH)is obtained at LFPO-8@c,which exhibits a BzOH formation rate of 3.88 mmol·gcat^(-1)·h^(-1) at 180℃ for 3 h,which is 1.50 and 2.72 times faster than those of LFPO-8 and LaFeO_(3)@c.A reaction mechanism is proposed,in which the acidic sites(e.g.,Fe^(4+),oxygen vacancy)are used for the activation of c=O bond of BzH and O-H bond of IPA,and the basic sites(e.g.,lattice oxygen)for the activation ofα-H(O-H)bond of IPA.

关键词： LaFe_(0.92)Pd_(0.08)O_(3) porous carbon catalytic transfer hydrogenation isopropanol reaction mechanism

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Kinetics and mechanism of propylene hydro-oxidation to acrolein on Au catalysts

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nano Research 2024年第1期17卷 354-363页

作者： Wei Du Zhihua Zhang nan Song Xuezhi Duan Xinggui Zhou State Key Laboratory of chemical Engineering School of Chemical EngineeringEast China University of Science and TechnologyShanghai 200237China

Propylene epoxidation by H_(2)and O_(2)to propylene oxide(PO)over the Au-Ti bifunctional catalysts,as an ideal reaction for PO production,has attracted great *** the mechanism of acrolein formation is of great importance for understanding the mechanism of molecular oxygen activation and the formation of hydroperoxo species on the Au ***,we investigate the reaction mechanism of propylene oxidation to acrolein on the Au/uncalcined TS-1(Au/TS-1-B)catalyst through a combination of multiple characterization,H_(2)/D_(2)exchange,kinetics experiment,and *** Ti sites are found to be non-essential to acrolein ***,the acrolein formation on the Au/TS-1-B catalyst is confirmed to be promoted by H_(2)through hydroperoxo species formation,which includes two main steps:propylene dehydrogenation to*c_(3)H_(5)with the aid of*OOH species,and*c_(3)H_(5)oxidation by*OOH to *** latter step is determined to be the rate-determining step because the corresponding kinetics model gives the best description for experimental *** work not only provides kinetics insights for the propylene hydro-oxidation to acrolein on the Au-Ti bifunctional catalysts,but also facilitates the rational design of Au catalysts with high activity and selectivity in the direct propylene epoxidation with H_(2)and O_(2).

关键词： kinetics mechanism gold acrolein hydro-oxidation

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Photoinduced bismuth vanadate-catalyzed c(sp^(2))-H functionalization

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chinese chemical Letters 2024年第3期35卷 1-2页

作者： Rong-nan yi Wei-Min He Key Laboratory of Food&Environment&Drug Monitoring and Testing of Universities in Hunan Province Hunan Police AcademyChangsha 410138China School of chemistry and chemical Engineering University of South ChinaHengyang 421001China

Visible light-induced organic reactions have gained much attention in recent years due to their mild conditions and high efficiency[1,2].In this context,many efficient photocatalysts including transition metal complex... 详细信息

关键词： bismuth catalyzed gained

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Updated roles of the gut microbiota in exploring shrimp etiology, polymicrobial pathogens, and disease incidence

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Zoological Research 2024年第4期45卷 910-923页

作者： Jin-Bo Xiong Hao-nan Sha Jiong chen State Key Laboratory for Managing Biotic and chemical Threats to the Quality and Safety of Agro-products School of Marine SciencesNingbo UniversityNingboZhejiang 315211China Key Laboratory of Aquacultural Biotechnology Ministry of EducationSchool of Marine SciencesNingbo UniversityNingboZhejiang 315211China Laboratory of Biochemistry and Molecular Biology School of Marine SciencesNingbo UniversityNingboZhejiang 315211China

Litopenaeus vannamei is the most extensively.c.ltured shrimp species globally,recognized for its scale,production,and economic ***,its aquaculture is plagued by frequent disease outbreaks,resulting in rapid and massive *** research often lags behind the emergence of new diseases,leaving the causal agents of some shrimp diseases unidentified and leading to nomenclature based on symptomatic presentations,especially in cases involving co-and polymicrobial *** data on shrimp disease statuses remain *** this review,we summarize current knowledge on shrimp diseases and their effects on the gut ***,we also propose a workflow integrating primary.c.lonizers,“driver”taxa in gut networks from healthy to diseased states,disease-discriminatory taxa,and virulence genes to identify potential polymicrobial *** examine both abiotic and biotic factors(e.g.,external and internal sources and specific-disease effects)that influence shrimp gut microbiota,with an emphasis on the“holobiome”concept and common features of gut microbiota response to diverse *** excluding the effects of confounding factors,we provide a diagnosis model for quantitatively predicting shrimp disease incidence using disease common-discriminatory taxa,irrespective of the causal *** to the conservation of functional genes used in designing specific primers,we propose a practical strategy applying qPcR-assayed abundances of disease common-discriminatory functional *** review updates the roles of the gut microbiota in exploring shrimp etiology,polymicrobial pathogens,and disease incidence,offering a refined perspective for advancing shrimp aquaculture health management.

关键词： Shrimp disease Gut microbiota Polymicrobial pathogens Diagnosis model Disease common-discriminatory taxa Disease prediction

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Ecological effect of the plantation of Sabina vulgaris in the Mu Us Sandy Land,china

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Journal of Arid Land 2024年第1期16卷 14-28页

作者： nan Weige DONG Zhibao ZHOU Zhengchao LI Qiang cHEN Guoxiang School of Geography and Tourism Shaanxi Normal UniversityXi'an 710062China Shaanxi Key Laboratory of Ecological Restoration in Shaanbei Mining Area Yulin UniversityYulin 719000China college of Prataculture Gansu Agricultural UniversityLanzhou 730070China

Vegetation restoration through artificial plantation is an effective method to combat desertification,especially in arid and semi-arid *** study aimed to explore the ecological effect of the plantation of Sabina vulgaris on soil physical and chemical properties on the southeastern fringe of the Mu Us Sandy Land,*** collected soil samples from five depth layers(0-20,20-40,40-60,60-80,and 80-100 cm)in the *** plantation plots across four plantation ages(4,7,10,and 16 years)in November 2019,and assessed soil physical(soil bulk density,soil porosity,and soil particle size)and chemical(soil organic carbon(SOc),total nitrogen(TN),available nitrogen(AN),available phosphorus(AP),available potassium(AK),cation-exchange capacity.c.c),salinity,p H,and c/N ratio)*** results indicated that the soil predominantly.c.nsisted of sand particles(94.27%-99.67%),with the remainder being silt and *** plantation age increased,silt and very fine sand contents progressively *** 16 years of planting,there was a marked reduction in the mean soil particle *** initial soil fertility was low and declined from 4 to 10 years of planting before witnessing an *** positive correlations were observed for the clay,silt,and very fine sand(mean diameter of 0.000-0.100 mm)with SOc,AK,and p *** contrast,fine sand and medium sand(mean diameter of 0.100-0.500 mm)showed significant negative correlations with these *** findings ascertain that the plantation of *** requires 10 years to effectively act as a windbreak and contribute to sand fixation,and needs 16 years to improve soil physical and chemical ***,these improvements were found to be highly beneficial for vegetation restoration in arid and semi-arid *** research can offer valuable insights for the protection and restoration of the vegetation ecosystem in the sandy lands in china.

关键词： Sabina vulgaris plantation age soil physical and chemical properties soil particle size soil fertility vegetation restoration Mu Us Sandy Land

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Porous S-doped carbon nitride foam with accelerated charge dynamics for sy.c.ronous photocatalytic hydrogen production and highly selective oxidation of amines

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nano Research 2024年第8期17卷 6860-6869页

作者： yu He Aiping Wu nan Wang ying Xie chungui Tian Honggang Fu Key Laboratory of Functional Inorganic Material chemistry(Ministry of Education of the People’s Republic of china) Heilongjiang UniversityHarbin 150080China

Photocatalytic hydrogen evolution coupled with organic oxidation holds great promise for converting solar energy into high-valueadded chemicals,but it is hampered by sluggish charge dynamics and limited redox ***,a porous S-doped carbon nitride(S-c_(3)N_(4−y))foam assembled from ultrathin nanosheets with rich nitrogen vacancies was synthesized using a molecular selfassembly *** S dopants and N vacancies synergistically adjusted the band structure,facilitating light absorption and enhancing the oxidation ***,the ultrathin nanosheets and porous structure provided more exposed active sites and facilitated mass and charge ***,S-c_(3)N_(4−y) foam exhibited enhanced photocatalytic activities for sy.c.ronous hydrogen evolution(4960μmol/(h·g))and benzylamine oxidation to N-benzylidenebenzylamine(4885μmol/(h·g))with high selectivity of>99%,which were approximately 17.6 and 72.9 times higher than those of bulk cN,*** photocatalytic coupling pairing reaction promotes the water splitting by.c.nsuming H2O2,thereby improving the hydrogen evolution efficiency and achieving the production of high value-added *** study provides an effective route for regulating the morphology and band structure of carbon nitride for synthesizing highly valuable chemicals.

关键词： photocatalysis S-doped carbon nitride band structure regulation hydrogen evolution coupled with benzylamine oxidation reaction mechanism

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Using Natural Radionuclides to Trace Sources of Suspended Particles in the Lower Reaches of the yellow River

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Journal of Ocean University of china 2024年第1期23卷 99-108页

作者： ZHANG Han BURNETT cWilliam ZHANG Xiaojie ZHAO Shibin yANG Disong nan Haiming yU Zhigang XU Bochao Frontiers Science center for Deep Ocean Multispheres and Earth System and Key Laboratory of Marine Chemistry Theory and TechnologyMinistry of EducationOcean University of ChinaQingdao 266100China Laboratory for Marine Ecology and Environmental Science Qingdao National Laboratory for Marine Science and TechnologyQingdao 266071China college of chemistry and chemical Engineering Ocean University of ChinaQingdao 266100China Department of Earth Ocean and Atmospheric ScienceFlorida State UniversityTallahasseeFL 32306USA North china Sea Environmental Monitoring center State Oceanic AdministrationKey Laboratory of Ecological Prewarning and Protection of Bohai SeaMNRQingdao 266033China Shandong Provincial Key Laboratory of Marine Ecological Environment and Disaster Prevention and Mitigation Qingdao 266033China

Natural radionuclides are powerful tools for understanding the sources and fate of suspended particulate matter(SPM).Particulate matter with different particle sizes behaves differently with respect to adsorption and *** analyzed the activi-ties and distribution characteristics of multiple natural radionuclides(238U,226Ra,40K,228Ra,7Be and 210Pbex)on size-fractionated SPM at the Lijin Hydrographic Station(Huanghe or yellow River)every month over a one-year *** showed that medium silt(16–32µm)was the main *** expected,the activity of each radionuclide decreased with an increase of particle *** examined the sources of SPM with different particle sizes using activity ratios of 226Ra/238U,228Ra/226Ra,40K/238U and 7Be/210Pbex,and concluded that SPM with different particle sizes originated from different *** results indicate that fine SPM(y from the erosion of soil along the lower reaches of the yellow River,while coarse SPM(>32µm)was mainly derived from resuspension of riverbed *** high runoff periods,the concentration of SPM increased significantly,and the pro-portion of fine particles originating upstream *** occurring radioactive isotopes,especially on size-fractionated par-ticles,are therefore seen as useful tracers to understand the sources and behaviors of riverine particles transported from land to sea.

关键词： the yellow River suspended particulate matter size-fractions radionuclides sediment sources water elutriator

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Simulating gamma-ray production from cosmic rays interacting with the solar atmosphere in the presence of coronal magnetic fields

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chinese Physics c 2024年第4期48卷 159-173页

作者：李哲吳震宇陈松战南云程何会海 Institute of High Energy Physics Chinese Academy of ScienceBeijing 100049China Department of Physics The Chinese University of Hong KongShatinNew TerritoriesHong KongChina School of Physical Sciences University of Chinese Academy of ScienceBeijing 100049China

cosmic rays can interact with the solar atmosphere and produce a slew of secondary messengers,making the Sun a bright gamma-ray source in the *** observations with Fermi-LAT have shown that these interactions must be strongly affected by solar magnetic fields in order to produce a wide range of observational features,such as a high flux and hard ***,the detailed mechanisms behind these features are still a *** this study,we tackle this problem by performing particle-interaction simulations in the solar atmosphere in the presence of coronal magnetic fields using the potential field source surface(PFSS)*** find that low-energy(~GeV)gamma-ray production is significantly enhanced by the coronal magnetic fields,but the enhancement decreases rapidly with *** enhancement directly.c.rrelates with the production of gamma rays with large deviation angles relative to the input cosmic-ray *** conclude that coronal magnetic fields are essential for correctly modeling solar disk gamma rays below 10 GeV,but above that,the effect of coronal magnetic fields *** magnetic field structures are needed to explain the high-energy disk emission.

关键词： solar gamma-ray corona magnetic field Geant4 simulation hadronic interaction

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A Scalable Pillar Layered Metal-Organic Framework for Natural Gas Purification

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chemical Research in chinese Universities 2024年第4期40卷 675-681页

作者： LU nan LAN Lan GAO Qiang LI Na BU Xian-He School of Materials Science and Engineering Nankai UniversityTianjin300350P.R.China State Key Laboratory of Elemento-Organic chemistry College of ChemistryNankai UniversityTianjin300071P.R.China School of Environmental and chemical Engineering Jiangsu University of Science and TechnologyZhenjiang212003P.R.China

One-step harvest of high-purity methane(cH_(4))from ternary propane/ethane/methane(c_(3)H_(8)/c_(2)H_(6)/cH_(4))mixtures remains a desirable yet challenging goal for natural gas ***,adsorbents either suffer from high capacity and selectivity,or are caught in a dilemma of scalable ***,we demonstrate a scalable pillar layered metal-organic framework Ni-MOF for highly efficient one-step cH_(4)***-MOF exhibits high c_(2)H_(6)and c_(3)H_(8)uptakes of 83.3 and 86.1 cm^(3)/g at 298 K and 100 kPa and remarkable c_(2)H_(6)/cH_(4)(50/50,volume ratio,21.5)and c_(3)H_(8)/cH_(4)(50/50,volume ratio,212.0)***,high c_(2)H_(6)(42.2 cm^(3)/g at 10 kPa)and c_(3)H_(8)(64.7 cm^(3)/g at 5 kPa)capacities in the low-pressure region at 298 K were realized on Ni-MOF,suggesting the strong affinities of Ni-MOF towards c_(2)H_(6)and c_(3)H_(8).Furthermore,the dynamic breakthrough experiments revealed that purifying cH_(4)from natural gas in one-step can be achieved in Ni-MOF with high-purity(>99.8%)and productivity(346.0 cm^(3)/g).Most significantly,the production of Ni-MOF can be scalably synthesized at room temperature,rendering it promising potential for industrial *** combined advantages of exceptional separation performance,scalability,and cycle stability of Ni-MOF pave the way for one-step cH_(4)purification from natural gas.

关键词： Metal-organic framework Adsorption and separation Natural gas purification Scale-up synthesis

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