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Effect of highland barely germination on thermomechanical, rheological, and micro-structural properties of wheat-oat composite flour dough

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FOOD BIOSCIENCE 2023年第3期53卷 554-563页

作者： AL-Ansi, Waleed Fadhl, Jalal Ahmed Abdullah, Abdulmageed Bagash Al-Adeeb, Abduqader Mahdi, Amer Ali Al-Maqtari, Qais Ali mushtaq, bilal sajid Fan, Mingcong Li, Yan Qian, Haifeng Wang, Li Jiangnan Univ Sch Food Sci & Technol State Key Lab Food Sci & Technol 1800 Lihu Ave Wuxi 214122 Peoples R China Jiangnan Univ Natl Engn Res Ctr Funct Food 1800 Lihu Ave Wuxi 214122 Peoples R China Sanaa Univ Fac Agr Food & Environm Dept Food Sci & Nutr Sanaa Yemen Jiangnan Univ Sch Biotechnol 1800 Lihu Ave Wuxi 214122 Peoples R China Jiangsu Univ Sch Food & Biol Engn Zhenjiang 212013 Peoples R China Sanaa Univ Fac Sci Dept Biol Sanaa Yemen Jiangnan Univ Natl Engn Res Ctr Funct Food Sch Food Sci & Technol State Key Lab Food Sci & Technol 1800 Lihu Ave Wuxi 214122 Peoples R China

This study investigated the effects of highland barley's germination time (24, 48, and 72 h) on the thermomechanical, pasting, fermentation, dynamic rheological, molecular mobility, and protein structural properties of oat-wheat composite flour dough. Germination significantly reduced flour water absorption, freezable water, melting enthalpy, and increased protein weakening compared with native barley (NB) samples. In addition, germination decreased bound and immobilized water and increased the free water compared to the NBcomposite flour dough samples, according to the results of a low-field nuclear magnetic resonance spectrometer (LF-NMR). Germination also increased the protein's extractability and surface hydrophobicity while negatively impacting the starch-protein network;however, it decreased bread-specific volume. Germination for 24 h, on the other hand, had minor effects on dough and bread samples compared to 48 and 72 h. As a result, germination for 24 h under controlled conditions could be used to improve the rheological qualities of highland barley and avoid the adverse rheological effects of the prolonged germination period.

关键词： Germination Mixolab Rheological properties Highland barley Molecular mobility

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Alternative Strategy for Development of Dielectric Calcium Copper Titanate‑Based Electrolytes for Low‑Temperature Solid Oxide Fuel Cells

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Nano-Micro Letters 2025年第1期17卷 310-332页

作者： sajid Rauf Muhammad bilal Hanif Zuhra Tayyab Matej Veis MAKYousaf Shah Naveed mushtaq Dmitry Medvedev Yibin Tian Chen Xia Martin Motola Bin Zhu College of Mechatronics and Control Engineering Shenzhen UniversityShenzhen 518060People’s Republic of China Department of Inorganic Chemistry Faculty of Natural SciencesComenius University BratislavaIlkovicova684215 BratislavaSlovakia Energy Storage Joint Research Center School of Energy and EnvironmentSoutheast UniversityNanjing 210096People’s Republic of China Hydrogen Energy Laboratory Ural Federal University620002 EkaterinburgRussia Laboratory of Electrochemical Devices Based on Solid Oxide Proton Electrolytes Institute of High Temperature Electrochemistry620066 EkaterinburgRussia School of Microelectronics Hubei UniversityWuhan 430062People’s Republic of China

The development of low-temperature solid oxide fuel cells(LT-SOFCs)is of significant importance for realizing the widespread application of *** has stimulated a substantial materials research effort in developing high oxide-ion conductivity in the electrolyte layer of *** this context,for the first time,a dielectric material,CaCu_(3)Ti_(4)O_(12)(CCTO)is designed for LT-SOFCs electrolyte application in this *** individual CCTO and its heterostructure materials with a p-type Ni_(0.8)Co_(0.15)Al_(0.05)LiO_(2−δ)(NCAL)semiconductor are evaluated as alternative electrolytes in LT-SOFC at 450–550℃.The single cell with the individual CCTO electrolyte exhibits a power output of approximately 263 mW cm^(-2) and an open-circuit voltage(OCV)of 0.95 V at 550℃,while the cell with the CCTO–NCAL heterostructure electrolyte capably delivers an improved power output of approximately 605 mW cm^(-2) along with a higher OCV over 1.0 V,which indicates the introduction of high hole-conducting NCAL into the CCTO could enhance the cell performance rather than inducing any potential short-circuiting *** is found that these promising outcomes are due to the interplay of the dielectric material,its structure,and overall properties that led to improve electrochemical mechanism in CCTO–***,density functional theory calculations provide the detailed information about the electronic and structural properties of the CCTO and NCAL and their heterostructure CCTO–*** study thus provides a new approach for developing new advanced electrolytes for LT-SOFCs.

关键词： LT-SOFCs Dielectric CaCu_(3)Ti_(4)O_(12) Semiconductor Ni_(0.8)Co_(0.15)Al_(0.05)LiO_(2−δ) Ionic conductivity Heterostructure electrolyte

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Highly Active Interfacial Sites in SFT-SnO_(2) Heterojunction Electrolyte for Enhanced Fuel Cell Performance via Engineered Energy Bands:Envisioned Theoretically and Experimentally

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Energy & Environmental Materials 2024年第3期7卷 384-397页

作者： sajid Rauf Muhammad bilal Hanif Faiz Wali Zuhra Tayyab Bin Zhu Naveed mushtaq Yatao Yang Kashif Khan Peter D.Lund Martin Motola Wei Xu College of Electronic and Information Engineering and State Key Laboratory of Radio frequency Heterogeneous Integration Shenzhen UniversityShenzhen 518000China Department of Inorganic Chemistry Faculty of Natural SciencesComenius University in BratislavaIlkovicova 684215BratislavaSlovakia College of Physics and Optoelectronic Engineering Shenzhen UniversityShenzhen 518060China School of Energy and Environment Southeast UniversityNo.2 Si Pai LouNanjing 210096China School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731China New Energy Technologies Group Department of Applied PhysicsAalto University School of ScienceP.O.Box 15100Fl-00076AaltoEspoo Finland

Extending the ionic conductivity is the pre-requisite of electrolytes in fuel cell technology for high-electrochemical *** this regard,the introduction of semiconductor-oxide materials and the approach of heterostructure formation by modulating energy bands to enhance ionic conduction acting as an electrolyte in fuel ***(n-type;SnO_(2))plays a key role by introducing into p-type SrFe_(0.2)Ti_(0.8)O_(3-δ)(SFT)semiconductor perovskite materials to construct p-n heterojunction for high ionic ***,two different composites of SFT and SnO_(2)are constructed by gluing p-and n-type SFT-SnO_(2),where the optimal composition of SFT-SnO_(2)(6∶4)heterostructure electrolyte-based fuel cell achieved excellent ionic conductivity 0.24 S cm^(-1)with power-output of 1004 mW cm^(-2)and high OCV 1.12 V at a low operational temperature of 500℃.The high power-output and significant ionic conductivity with durable operation of 54 h are accredited to SFT-SnO_(2)heterojunction formation including interfacial conduction assisted by a built-in electric field in fuel cell ***,the fuel conversion efficiency and considerable Faradaic efficiency reveal the compatibility of SFT-SnO_(2)heterostructure electrolyte and ruled-out short-circuiting ***,the first principle calculation provides sufficient information on structure optimization and energy-band structure modulation of SFT-SnO_(2).This strategy will provide new insight into semiconductor-based fuel cell technology to design novel electrolytes.

关键词： high ionic conductivity interfacial conduction modulated energy band structure p-n heterojunction semiconductors

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Proton transport controlled at surface layer of CeO_(2) by gradient-doping with a built-in-field effect

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Journal of Rare Earths 2023年第12期41卷 2025-2032,I0008页

作者： Yuzheng Lu Naveed mushtaq M.A.K Yousaf Shah sajid Rauf Chen Xia Bin Zhu School of Electronic Engineering Nanjing Xiaozhuang UniversityNanjing21171China School of Physics Electronics and Intelligent ManufacturingHuaihua UniversityHuaihua418008China Jiangsu Provincial Key Laboratory of Solar Energy Science and Technology/Energy Storage Joint Research Center School of Energy and EnvironmentSoutheast UniversityNanjing210096China College of Electronics and Information Engineering Shenzhen UniversityShenzhen58000China Faculty of Physics and Electronic Science Hubei UniversityWuhan430062China

Ceramic fuel cells hold an important position for the sustainable energy future using renewable energy sources with high *** design and synthesis of active materials,interface engineering and having capability of low operating temperature is considered as an important factor to further increase the power output and stability of ceramic fuel cell devices.A novel methodology has vital importance to develop new functionalities of existing materials by introducing new different *** built-in electric field(BIEF) is one of the most recently used approaches to improve charge transfer and ionic conductivity of solid oxide ***,we demonstrate gradient doping strategy in CeO_(2)-δstructure to produce BIEF effect and to modulate the proton transport effectively at the surface layer rather than bulk *** inclusions of La and Sr metal ions at the surface and Co-metal ions into bulk-layer of CeO_(2)form the gradiently doped *** gradient doping into CeO_(2)highly improves the proton transport properties through the surface layer by modifying the energy ***,unbalanced charge distribution due to gradient doping produces built-in electric-field to provide extra driving force for protons transport through surface *** acquired gradiently doped fluorite structure exhibits remarkable proton conductivity of>0.2 S/cm,as a result ceramic fuel cell shows power output of>1000 mW/cm2while operating at 500℃.This unique work highlights the critical role of gradiently doped electrolyte in electrochemical conversion energy devices and offers new understanding and practices for sustainable energy future.

关键词： La_(0.20)Sr_(0.05)Ce_(0.65)Co_(0.1)0_(2-δ)(LSCC) Gradient doping Fast protonic transport High grain boundary conduction Built-in electric field Rare earths

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Novel LaFe_(2)O_(4)spinel structure with a large oxygen reduction response towards protonic ceramic fuel cell cathode

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Journal of Rare Earths 2023年第3期41卷 413-421,I0004页

作者： Jinping Wang Yuzheng Lu Naveed mushtaq M.A.K Yousaf Shah sajid Rauf Peter D.Lund Muhammad Imran Asghar School of Energy and Power Engineering Nanjing Institute of TechnologyNanjing 211167China School of Electronic Engineering Nanjing Xiao Zhuang UniversityNanjing 211171China Jiangsu Provincial Key Laboratory of Solar Energy Science and Technology/Energy Storage Joint Research Center School of Energy and EnvironmentSoutheast UniversityNanjing 210096China College of Electronics and Information Engineering Shenzhen UniversityShenzhen 518000China New Energy Technologies Group Department of Applied PhysicsAalto University School of ScienceP.O.Box.15100FI00076AaltoEspooFinland Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials Faculty of Physics and Electronic ScienceHubei UniversityWuhan 430062China

Highly active and stable electrocatalysts are mandatory for developing high-performance and longlasting fuel *** current study demonstrates a high oxygen reduction reaction(ORR)electrocatalytic activity of a novel spinel-structured LaFe_(2)O_(4)via a self-doping *** LaFe_(2)O_(4)demonstrates excellent ORR activity in a protonic ceramic fuel cell(PCFC)at temperature range of 350-500℃.The high ORR activity of LaFe_(2)O_(4)is mainly attributed to the facile release of oxide and proton ions,and improved synergistic incorporation abilities associated with interplay of multivalent Fe^(3+)/Fe^(2+)and La^(3+)*** LaFe_(2)O_(4)as cathode over proton conducting BaZr_(0.4)Ce_(0.4)Y_(0.2)O_(3)(BZCY)electrolyte,the fuel cell has delivered a high-power density of 806 mW/cm^(2)operating at 500℃.Different spectroscopic and calculations methods such as UV-visible,Raman,X-ray photoelectron spectroscopy and density functional theory(DFT)calculations were performed to screen the potential application of LaFe_(2)O_(4)as *** study would help in developing functional cobalt-free ORR electrocatalysts for low temperature-PCFCs(LT-PCFCs)and solid oxide fuel cells(SOFCs)applications.

关键词： LaFe_(2)O_(4)cathode Facile Fe^(3+/2+)ions resale Oxygen reductionreaction(ORR) Excellent electrocatalyst Protonic ceramicfuel cell(PCFC) Rare earths

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Current and further trajectories in designing functional materials for solid oxide electrochemical cells:A review of other reviews

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Journal of Energy Chemistry 2024年第7期94卷 302-331页

作者： Stanislav Baratov Elena Filonova Anastasiya Ivanova Muhammad bilal Hanif Muneeb Irshad Muhammad Zubair Khan Martin Motola sajid Rauf Dmitry Medvedev Hydrogen Energy Laboratory Ural Federal University620002 EkaterinburgRussia Institute of Natural Sciences and Mathematics Ural Federal University620002 EkaterinburgRussia Department of Inorganic Chemistry Faculty of Natural SciencesComenius University BratislavaIlkovicova 6Mlynska Dolina84215 BratislavaSlovakia State Key Laboratory for Mechanical Behavior of Materials School of Materials Science and EngineeringXi'an Jiaotong UniversityXi'an 710049ShaanxiChina Department of Physics University of Engineering and TechnologyLahore 54890Pakistan Pak-Austria Fachhochschule:Institute of Applied Sciences and Technology Mang Haripur 22621Khyber PakhtunkhwaPakistan College of Mechatronics and Control Engineering Shenzhen UniversityShenzhen 518000GuangdongChina Laboratory of Electrochemical Devices Based on Solid Oxide Proton Electrolytes Institute of High Temperature Electrochemistry620066 EkaterinburgRussia

Complex oxides are an important class of materials with enormous potential for electrochemical *** on their composition and structure,such complex oxides can exhibit either a single conductivity(oxygen-ionic or protonic,or n-type,or p-type electronic)or a combination thereof gener-ating distinct dual-conducting or even triple-conducting *** properties enable their use as diverse functional materials for solid oxide fuel cells,solid oxide electrolysis cells,permeable membranes,and gas *** literature review shows that the field of solid oxide materials and related electro-chemical cells has a significant level of research engagement,with over 8,000 publications published since *** manual analysis of such a large volume of material is ***,by examining the review articles,it is possible to identify key patterns,recent achievements,prospects,and remaining *** perform such an analysis,the present article provides,for the first time,a comprehensive summary of previous review publications that have been published since 2020,with a special focus on solid oxide materials and electrochemical ***,this study provides an important reference for researchers specializing in the fields of solid state ionics,high-temperature electrochemistry,and energyconversiontechnologies.

关键词： SOFCs SOECs PCFCS Electrochemistry Energy conversion Hydrogen energy,Carbon neutrality

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Semiconductor Electrochemistry for Clean Energy Conversion and Storage

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Electrochemical Energy Reviews 2021年第4期4卷 757-792页

作者： Bin Zhu Liangdong Fan Naveed mushtaq Rizwan Raza Muhammad sajid Yan Wu Wenfeng Lin Jung‑Sik Kim Peter D.Lund Sining Yun Jiangsu Provincial Key Laboratory of Solar Energy Science and Technology/Energy Storage Joint Research Center School of Energy and EnvironmentSoutheast UniversityNanjing 210096JiangsuChina Shenzhen Key Laboratory of New Lithium‑Ion Batteries and Mesoporous Materials College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhen 518060GuangdongChina Clean Energy Research Lab(CERL) Department of PhysicsCOMSATS University IslamabadLahore CampusLahore 54000Pakistan Engineering Research Center of Nano‑Geo Materials of Ministry of Education Faculty of Materials Science and ChemistryChina University of GeosciencesWuhan 430074HubeiChina Department of Chemical Engineering School of AeronauticalAutomotiveChemical and Materials EngineeringLoughborough UniversityLoughborough LE113TUUK Department of Aeronautical&Automotive Engineering School of AeronauticalAutomotiveChemical and Materials EngineeringLoughborough UniversityLoughborough LE113TUUK Department of Engineering Physics/Advanced Energy Systems School of ScienceAalto University00076 AaltoEspooFinland Functional Materials Laboratory(FML) School of Materials Science and EngineeringXi’an University of Architecture and TechnologyXi’an 710055ShaanxiChina

Semiconductors and the associated methodologies applied to electrochemistry have recently grown as an emerging field in energy materials and *** example,semiconductor membranes and heterostructure fuel cells are new technological trend,which differ from the traditional fuel cell electrochemistry principle employing three basic functional components:anode,electrolyte,and *** electrolyte is key to the device performance by providing an ionic charge flow pathway between the anode and cathode while preventing electron *** contrast,semiconductors and derived heterostructures with electron(hole)conducting materials have demonstrated to be much better ionic conductors than the conventional ionic *** energy band structure and alignment,band bending and built-in electric field are all important elements in this context to realize the necessary fuel cell *** review further extends to semiconductor-based electrochemical energy conversion and storage,describing their fundamentals and working principles,with the intention of advancing the understanding of the roles of semiconductors and energy bands in electrochemical devices for energy conversion and storage,as well as applications to meet emerging demands widely involved in energy applications,such as photocatalysis/water splitting devices,batteries and solar *** review provides new ideas and new solutions to problems beyond the conventional electrochemistry and presents new interdisciplinary approaches to develop clean energy conversion and storage technologies.

关键词： Semiconductor electrochemistry Fuel cells Lithium-ion batteries Solar cells Built-in electric field Energy system integration

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A Review of Image Steganography Based on Multiple Hashing Algorithm

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Computers, Materials & Continua 2024年第8期80卷 2463-2494页

作者： Abdullah Alenizi Mohammad sajid Mohammadi Ahmad A.Al-Hajji Arshiya sajid Ansari Department of Information Technology College of Computer and Information SciencesMajmaah UniversityAl-Majmaah11952Saudi Arabia Department of Computer Science College of Engineering and Information TechnologyOnaizah CollegesQassim56312Saudi Arabia

Steganography is a technique for hiding secret messages while sending and receiving communications through a cover *** ancient times to the present,the security of secret or vital information has always been a significant *** development of secure communication methods that keep recipient-only data transmissions secret has always been an area of ***,several approaches,including steganography,have been developed by researchers over time to enable safe data *** this review,we have discussed image steganography based on Discrete Cosine Transform(DCT)algorithm,*** have also discussed image steganography based on multiple hashing algorithms like the Rivest–Shamir–Adleman(RSA)method,the Blowfish technique,and the hash-least significant bit(LSB)*** this review,a novel method of hiding information in images has been developed with minimal variance in image bits,making our method secure and effective.A cryptography mechanism was also used in this *** encoding the data and embedding it into a carry image,this review verifies that it has been ***,embedded text in photos conveys crucial signals about the *** review employs hash table encryption on the message before hiding it within the picture to provide a more secure method of data *** the message is ever intercepted by a third party,there are several ways to stop this operation.A second level of security process implementation involves encrypting and decrypting steganography images using different hashing algorithms.

关键词： Image steganography multiple hashing algorithms Hash-LSB approach RSA algorithm discrete cosine transform(DCT)algorithm blowfish algorithm

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One-dimensional quantum walks with a position-dependent coin

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Communications in Theoretical Physics 2020年第6期72卷 18-28页

作者： Rashid Ahmad Uzma Sajjad Muhammad sajid Department of Physics Kohat University of Science and TechnologyKohat 26000Khyber-PakhtunkhwaPakistan

We investigate the evolution of a discrete-time one-dimensional quantum walk driven by a position-dependent *** rotation angle,which depends upon the position of a quantum particle,parameterizes the coin *** different values of the rotation angle,we observe that such a coin leads to a variety of probability distributions,***,periodic,classicallike,semi-classical-like,and ***,we study the Shannon entropy associated with position and the coin space of a quantum particle,and compare them with the case of the position-independent *** results show that the entropy is smaller for most values of the rotation angle as compared to the case of the position-independent *** also study the effect of entanglement on the behavior of probability distribution and Shannon entropy by considering a quantum walk with two identical position-dependent entangled *** observe that in general,a wave function becomes more localized as compared to the case of the positionindependent coin and hence the corresponding Shannon entropy is *** results show that a position-dependent coin can be used as a controlling tool of quantum walks.

关键词： quantum walk position-dependent coin Shannon entropy

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Size-controlled synthesis of Fe3O4 and Fe3O4@SiO2 nanoparticles and their superparamagnetic properties tailoring

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Progress in Natural Science:Materials International 2023年第1期33卷 116-119页

作者： Muhammad sajid Sidra Shuja Hongpan Rong Jiatao Zhang Beijing Key Laboratory of Construction-Tailorable Advanced Functional Materials and Green Applications School of Materials Science & Engineering Beijing Institute of Technology Beijing Key Laboratory of Construction-Tailorable Advanced Functional Materials and Green Applications Key Laboratory of Medical Molecule Science and Pharmaceutics Engineering School of Chemistry and Chemical Engineering Institute of Engineering Medicine Beijing Institute of Technology

Superparamagnetic properties and fine-tuning of colloidal Fe3O4nanoparticles are important for their widespread biomedical applications. Herein, colloidal Fe3O4nanoparticles(NPs) of different sizes(8–20 nm) were prepared,and their hydrophilization with SiO2shell coating to be Fe3O4@SiO2core-shell had been realized *** size of Fe3O4NPs was controlled by different heating rates. Transmission electron microscope(TEM), powder X-ray diffractometry(XRD), and vibrating sample magnetometer(VSM) were performed to examine the morphology, crystallinity, and magnetic properties of the prepared Fe3O4and Fe3O4@SiO2core-shell NPs,respectively. In addition, high resolution transmission electron microscope(HRTEM) results suggested that Fe3O4NPs had well crystallization. Enabled by such, their superparamagnetic properties can be fine-tuned accordingly and cater to their potential applications.

关键词： Fe3O4 nanoparticles Fe3O4@SiO2 hydrophilization Superparamagnetic Core-shell Aqueous inverse microemulsion

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