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Quench-tailored Al-doped V_(2)O_(5) nanomaterials for efficient aqueous zinc-ion batteries

Journal of Energy Chemistry 2022年第7期31卷 52-58,I0003页

作者： Hanmei Jiang Wenbin Gong Yifu Zhang Xin Liu moaz waqar Jingjing Sun Yanyan Liu Xueying Dong Changgong Meng Zhenghui Pan John Wang State Key Laboratory of Fine Chemicals School of Chemical EngineeringDalian University of TechnologyDalian 116024LiaoningChina Department of Materials Science and Engineering National University of SingaporeSingapore 117574Singapore School of Physics and Energy Xuzhou University of TechnologyXuzhou 221018JiangsuChina School of Materials Science and Engineering Tongji UniversityShanghai 201804China

Rechargeable aqueous zinc-ion batteries(ZIBs)are regarded as a promising competition to lithium-ion batteries as energy storage devices,owing to their high safety and low ***,the development of high-performance ZIBs is largely hindered by the shortage of ideal cathode materials with high-rate capability and long-cycle ***,we address this bottleneck issue by the quenching-tailored surface chemistry of V_(2)O_(5) cathode *** rapid quenching from high temperatures,Al ions are doped into V_(2)O_(5) lattice(Al-V_(2)O_(5))and abundant oxygen vacancies are formed on the surface/nearsurface,which facilitate the desired rapid electron *** density functional theory(DFT)simulations elucidate that the doping of Al ions into V_(2)O_(5) remarkably reduces the Zn^(2+)-diffusion barriers and improves the electrical conductivity of V_(2)O_(5).As a proof-of-concept application,the thus-optimized AlV_(2)O_(5) cathode delivers a superior specific capacity of 532 m Ah g^(-1) at 0.1 A g^(-1) and a long-cycling life with76%capacity retention after 5000 cycles,as well as a good rate *** work provides not only a novel strategy for tuning the surface chemistry of V_(2)O_(5) to boost the Zn^(2+)storage but also a general pathway of modifying metal oxides with improved electrochemical performance.

关键词： Quenching-tailored V_(2)O_(5) Aqueous zinc-ion batteries Surface chemistry Long-cycle stability High-rate capability

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Data Information integrated Neural Network (DINN) algorithm for modelling and interpretation performance analysis for energy systems

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Energy and AI 2024年第2期16卷 306-315页

作者： waqar Muhammad Ashraf Vivek Dua The Sargent Centre for Process Systems Engineering Department of Chemical EngineeringUniversity College LondonTorrington PlaceLondon WC1E 7JEUK

Developing a well-predictive machine learning model that also offers improved interpretability is a key challenge to widen the application of artificial intelligence in various application domains. In this work, we present a Data Information integrated Neural Network (DINN) algorithm that incorporates the correlation information present in the dataset for the model development. The predictive performance of DINN is also compared with a standard artificial neural network (ANN) model. The DINN algorithm is applied on two case studies of energy systems namely energy efficiency cooling (ENC) & energy efficiency heating (ENH) of the buildings, and power generation from a 365 MW capacity industrial gas turbine. For ENC, DINN presents lower mean RMSE for testing datasets (RMSE_test = 1.23 %) in comparison with the ANN model (RMSE_test = 1.41 %). Similarly, DINN models have presented better predictive performance to model the output variables of the two case studies. The input perturbation analysis following the Gaussian distribution for noise generation reveals the order of significance of the variables, as made by DINN, can be better explained by the domain knowledge of the power generation operation of the gas turbine. This research work demonstrates the potential advantage to integrate the information present in the data for the well-predictive model development complemented with improved interpretation performance thereby opening avenues for industry-wide inclusion and other potential applications of machine learning.

关键词： Explainable AI Model interpretation Scientific machine learning Artificial neural network Loss function

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Experimental Study on Heat Storage Properties Comparison of Paraffin/Metal Foams Phase Change Material Composites

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Journal of Thermal Science 2024年第2期33卷 469-478页

作者： waqar AHMED Abid HUSSAIN Hanzla SHAHID Imran ALI Hafiz Muhammad ALI Department of Mechanical Engineering University of Engineering and TechnologyTaxila47080Pakistan Department of Mechanical Engineering Institute of Space TechnologyIslamabadPakistan Department of Mechanical Mechatronics and Manufacturing EngineeringUniversity of Engineering and Technology LahoreFaisalabad CampusPunjabPakistan Mechanical Engineering Department King Fahd University of Petroleum and MineralsDhahran31261Saudi Arabia Interdisciplinary Research Center for Renewable Energy and Power Systems(IRC-REPS) King Fahd University of Petroleum and MineralsDhahran31261Saudi Arabia

Heat storage properties of phase change materials(PCMs) are essential characteristics that perform a key role in thermal heat energy storage *** thermal properties of PCMs can be improved by developing metal foam/PCM *** addition of metal foam in PCMs has a significant effect on the thermal characteristics of *** this paper,the heat storage properties of two different metal foam/PCM composites were experimentally *** behavior of paraffin in metal foam(copper and iron-nickel)/paraffin composites concerning pure paraffin at a constant heat flux of 1000 W/m^(2) in three directions simultaneously(x,y,and z) was *** was infiltrated into copper and iron-nickel foams to develop composite materials which resulted in enhancing the thermal conductivity of the paraffin.A comparative analysis is made on the heat storage properties of paraffin in copper and iron-nickel foams/paraffin *** temperature distribution during the phase transition process is experimentally *** comparison indicates that temperature uniformity in copper foam/paraffin composite is better than in iron-nickel foam/paraffin composite and pure paraffin at the same heat *** results show that at heat flux of 1000 W/m^(2),the heat storage time for copper foam/paraffin composite is 20.63% of that of iron-nickel foam/paraffin composite.

关键词： heat storage capacity paraffin/metal foam composite temperature uniformity heat storage rate phase transition process

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Sustainable pathways to ammonia:a comprehensive review of green production approaches

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Clean Energy 2024年第2期8卷 60-72页

作者： Hafiz Sharjeel Ahmed Zaid Yahya waqar Ali khan Ali Faraz University of Engineering and Technology(UET) LahorePakistan Chemical Engineering Department NFC Institute of Engineering and Fertilizer ResearchFaislabadPakistan Chemical Engineering Department Punjab UniversityLahorePakistan

Ammonia production is vital in global industries but faces increasing environmental concerns,necessitating a shift towards sustainable *** review comprehensively explores diverse hydrogen production approaches and their potential impact on sustainable ammonia *** primary focus is investigating hydrogen production methods that enhance both efficiency and sustainability in ammonia synthesis,which is crucial for reducing its environmental ***,the review highlights the pivotal role of catalysts in improving Faradaic efficiency in ammonia synthesis,emphasizing their significance in overall process *** study identifies innovative technologies that have the potential to revolutionize ammonia production while aligning with global sustainability *** a thorough examination of hydrogen production methods and catalytic advances,this review provides valuable insight into greener and more efficient ammonia production *** conclusion,it emphasizes the importance of exploring hydrogen production methods and leveraging catalysts to improve ammonia production sustainability and *** addresses a critical research gap and paves the way for an environmentally responsible and globally aligned ammonia production industry.

关键词： ammonia production green alternatives sustainability catalyst

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Flexible pavement longitudinal joint quality evaluation using non-destructive testing

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Journal of Road Engineering 2024年第2期4卷 189-202页

作者： Hamad Bin Muslim Syed waqar Haider Lev Khazanovich Department of Civil and Environmental Engineering Michigan State UniversityEast LansingMI 48824USA Department of Civil and Environmental Engineering University of PittsburghPittsburghPA 15261USA

Longitudinal joint construction quality is critical to the life of flexible *** deteriorated longitudinal joints has become a challenge for many highway *** the joint's quality through better compaction during construction can help achieve flexible pavements with longer service lives and less *** quality control(QC)and quality assurance(QA)plans provide limited ***,the risk of missing areas with poor joint compaction is significant.A density profiling system(DPS)is a non-destructive alternative to conventional destructive evaluation *** can provide quick and continuous real-time coverage of the compaction during construction in *** paper presents several case studies comparing various types of longitudinal joints and demonstrating the use of DPS to evaluate the joint's compaction *** paper shows that dielectric measurements can provide valuable insight into the ability of various construction techniques to achieve adequate levels of compaction at the longitudinal *** paper proposes a dielectric-based longitudinal joint quality index(LJQI)to evaluate the relative compaction of the joint during *** also shows that adopting DPS for assessing the compaction of longitudinal joints can minimize the risk of agencies accepting poorly constructed joints,identify locations of poor quality during construction,and achieve better-performing flexible pavements.

关键词： Sustainable pavements Dielectric/density profiling system Quality assurance Non-destructive testing Asphalt longitudinal joint

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Comparative analysis of jet and underlying event properties across various models as a function of charged particle multiplicity at 7 TeV

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Chinese Physics C 2024年第9期48卷 118-125页

作者： Maryam waqar Haifa I.Alrebdi Muhammad Waqas K.S.Al-mugren Muhammad Ajaz Department of Physics Abdul Wali Khan University MardanMardan 23200Pakistan Department of Physics College of SciencePrincess Nourah bint Abdulrahman UniversityP.O.Box 84428Riyadh 11671Saudi Arabia School of Nuclear Science and Technology University of Chinese Academy of SciencesBeijing 100049China

In this study,a comprehensive analysis of jets and underlying events as a function of charged particle multiplicity in proton-proton(pp)collisions at a center-of-mass energy of √s=7 TeV is *** Monte Carlo(MC)event generators,including Pythia8.308,EPOS 1.99,EPOSLHC,EPOS4_(Hydro),and EPOS4_(noHydro),are employed to predict particle *** predictions from these models are compared with experimental data from the CMS *** charged particles are categorized into those associated with underlying events and those linked to jets,and the analysis is restricted to charged particles with|η|0.25 GeV/*** comparing the MC predictions with CMS data,we find that EPOS4_(Hydro),EPOSLHC,and Pythia8 consistently reproduce the experimental results for all charged particles,underlying events,intrajets,and leading charged *** charged jet rates with p_T^(***)>5 GeV/c,EPOS4_(Hydro)and Pythia8 perform exceptionally *** the case of charged jet rates with p_T^(***)→30 GeV/c,EPOSLHC reproduces satisfactorily good results,whereas EPOS4 Hydro exhibits good agreement with the data at higher charged particle multiplicities compared to the other *** can be attributed to the conversion of energy into flow when"Hydro=on"leading to an increase in *** EPOSLHC model describes the data better owing to the new collective flow effects,correlated flow treatment,and parameterization compared to EPOS ***,the examination of the jet p_T spectrum and normalized charged p_T density reveals that EPOS4_(Hydro),EPOS4_(noHydro),and EPOSLHC exhibit good agreement with the experimental results,whereas Pythia8 and EPOS 1.99 do not perform as well owing to the lack of correlated flow treatment.

关键词： Monte Carlo models underlying event jets charged particle multiplicity

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Condition indices for rigid pavements: A comparative analysis of state DOTs using Michigan PMS data

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Journal of Road Engineering 2024年第3期4卷 348-360页

作者： Rahul Raj Singh Mumtahin Hasnat Muhammed Emin Kutay Syed waqar Haider James Bryce Bora Cetin Department of Civil and Environmental Engineering Michigan State UniversityEast LansingMI 48824USA Wadsworth Department of Civil and Environmental Engineering West Virginia UniversityMorgantownWV 26506USA

Pavement infrastructure is vital in providing services and links between various sectors of society. Therefore, thepreservation and maintenance of these roads are critical to attaining a pavement network in good conditionthroughout its service life. Various performance indicators like the international roughness index (IRI), pavementcondition index (PCI), and present serviceability rating (PSR) have been used by the state department of transportation (DOT) and highway agencies for evaluating pavement surface conditions and planning future maintenance strategies. Limited data availability, multiple distresses depending on region, lack of correlation of thesecondition indices to maintenance strategies, and data collection limitations pose a challenge for applying theseindices to local conditions. This paper compares condition indices of different states for rigid pavements. Further,using a specific condition index for local conditions is also highlighted. For this purpose, five states and theircorresponding condition indices were evaluated and compared to the Michigan DOT distress index (DI). Thesestates include Virginia, Minnesota, North Dakota, Louisiana, and Oregon. The corresponding distresses of eachcondition index were converted to make them compatible with the MDOT DI. This study used the MDOT'spavement management system (PMS) database to evaluate each condition index for 433 rigid pavement *** distress index was plotted against MDOT DI and compared using a paired t-test. Results show that thecondition indices of Virginia and Minnesota are comparable to DI in terms of the Spearman correlation value. Thet-test results show that except for Virgina, condition indices from other states statistically differ from ***, one can't use those directly for local conditions in Michigan. This paper presents the evaluation anddata requirements for each condition index and its impact on selecting a maintenance treatment.

关键词： Rigid pavement Pavement management Condition index Distress index

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Soil erosion susceptibility mapping of Hangu Region,Kohat Plateau of Pakistan using GIS and RS-based models

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Journal of Mountain Science 2024年第8期21卷 2547-2561页

作者： Fakhrul ISLAM Liaqat Ali WASEEM Tehmina BIBI waqar AHMAD Muhammad SADIQ Matee ULLAH Walid SOUFAN Aqil TARIQ Department of Geology Khushal Khan Khattak UniversityKarak 27200Pakistan Department of Geography Government College University FaisalabadPunjab 38000Pakistan Institute of Geology The University of Azad Jammu&KashmirMuzaffarabad 13100Pakistan Department of Earth Sciences Changan UniversityXi’an 710003China NCEG University of PeshawarPeshawar 25120Pakistan Faculty of Earth Sciences Geography and AstronomyUniversity of ViennaVienna 1090Austria Plant Production Department College of Food and Agriculture SciencesKing Saud UniversityRiyadh 11451Saudi Arabia Department of Wildlife Fisheries and AquacultureCollege of Forest ResourcesMississippi State UniversityMS 39762USA

Soil erosion is a crucial geo-environmental hazard worldwide that affects water quality and agriculture,decreases reservoir storage capacity due to sedimentation,and increases the danger of flooding and ***,this study uses geospatial modeling to produce soil erosion susceptibility maps(SESM)for the Hangu region,Khyber Pakhtunkhwa(KPK),*** Hangu region,located in the Kohat Plateau of KPK,Pakistan,is particularly susceptible to soil erosion due to its unique geomorphological and climatic ***,the Hangu region is characterized by a combination of steep slopes,variable rainfall patterns,diverse land use,and distinct soil types,all of which contribute to the complexity and severity of soil erosion *** factors necessitate a detailed and region-specific study to develop effective soil conservation *** this research,we detected and mapped 1013 soil erosion points and prepared 12 predisposing factors(elevation,aspect,slope,Normalized Differentiate Vegetation Index(NDVI),drainage network,curvature,Land Use Land Cover(LULC),rainfall,lithology,contour,soil texture,and road network)of soil erosion using GIS ***,GIS-based statistical models like the weight of evidence(WOE)and frequency ratio(FR)were applied to produce the SESM for the study *** SESM was reclassified into four classes,i.e.,low,medium,high,and very high *** results of WOE for SESM show that 16.39%,33.02%,29.27%,and 21.30%of areas are covered by low,medium,high,and very high zones,*** contrast,the FR results revealed that 16.50%,24.33%,35.55%,and 23.59%of the areas are occupied by low,medium,high,and very high ***,the reliability of applied models was evaluated using the Area Under Curve(AUC)*** validation results utilizing the area under curve showed that the success rate curve(SRC)and predicted rate curve(PRC)for WOE are 82%and 86%,respectively,while SRC and PRC for FR are 85%and 96%,res

关键词： Soil erosion Geospatial technology Statistical models Hangu Pakistan

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Electronic and thermoelectric properties of YbMg_(2)X_(2)(X=P,As,Sb,Bi)zintl compounds by first-principles method

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Journal of Rare Earths 2024年第1期42卷 147-154,I0006页

作者： Sajid Khan Dil Faraz Khan R.Neffati Tariq Usman Muhammad waqar Ahsraf Shamim Khan Saeed Ullah Jan G.Murtaza Department of Physics University of Science&Technology BannuBannu28100Pakistan Department of Physics Faculty of ScienceKing Khalid UniversityP.O.Box 9004AbhaSaudi Arabia Laboratoire de Physique de La Matiere Condensee Departement de PhysiqueFaculte des Sciences de TunisUniversite Tunis El ManarCampus Universitaire1060TunisTunisia Department of Physics Shaoxing UniversityShaoxing312000China Department of Mathematics&Natural Sciences Prince Mohammad Bin Fahd UniversityAlkhobar31952Saudi Arabia Materials Modeling Lab Department of PhysicsIslamia College Peshawar25120KhyberPakhtunkhwaPakistan

In this work the structural,electronic and thermoelectric properties of YbMg_(2)X_(2)(X=P,As,Sb,Bi)zintl compounds were investigated comprehensively using first principles *** electronic properties were studied using PBE GGA,TB-mBJ and hybrid(YS-PBE0)*** the structural parameters of optimized structures are in harmonious agreement to the available *** band structure study illustrates that the titled materials manifest metallic and semi metallic nature using PBE and TB-mBJ potentials while they show wide band gap semiconducting behavior by following hybrid(YS-PBE0)*** density of states(TDOS)and partial density of states(PDOS)were also calculated to glimpse the contribution of orbitals of atoms in the formation of *** properties were studied by using BoltzTraP2 code employed to *** get enormous values of Seebeck coefficient(S),power factor(PF)and thermoelectric figure of merit(ZT)for all the samples YbMg_(2)X_(2)(X=P,As,Sb,Bi),Moreover,the overwhelming transport properties for the titled compounds indicate the optimum level of carriers’concentration which pinpoints these materials to be better thermoelectrics in the 1-2-2 zintl family.

关键词： Zintl compounds Hybrid functional Band structure Thermoelectrics Rare earths

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刈割对豆科和非豆科植物叶片内稳性及叶片土壤化学计量特征的影响

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草地学报 2024年第5期32卷 1513-1521页

作者：杜艺宋佼阳张玉林柴旭田张志浩 ISLAM waqar 曾凡江中国科学院新疆生态与地理研究所新疆荒漠植物根系生态与植被修复重点实验室新疆乌鲁木齐830011 中国科学院新疆生态与地理研究所荒漠与绿洲生态国家重点实验室干旱区生态安全与可持续发展重点实验室新疆乌鲁木齐830011 新疆策勒荒漠草地生态系统国家野外科学观测研究站新疆策勒848300 中国科学院大学北京100049 新疆大学生态与环境学院新疆乌鲁木齐830046

为了明确豆科和非豆科植物在生长发育过程中养分利用策略的差异。本试验以典型豆科植物苜蓿(Medicago sativa)和非豆科植物菊苣(Cichorium intybus)为研究对象。分别于2021年7月14日(播种后第60 d)、2021年8月3日(播种后第80 d)和2021年... 详细信息

为了明确豆科和非豆科植物在生长发育过程中养分利用策略的差异。本试验以典型豆科植物苜蓿(Medicago sativa)和非豆科植物菊苣(Cichorium intybus)为研究对象。分别于2021年7月14日(播种后第60 d)、2021年8月3日(播种后第80 d)和2021年8月24日(播种后第100 d)采集地上部分和土壤样品,计算生态化学计量内稳性。结果表明:2种植物叶片氮钾比在播种后第80 d刈割显著高于播种后第100 d刈割,而叶片磷钾比表现相反趋势(PH K>H P,表明植物对氮元素的调控能力更强。这项研究发现叶片化学计量特征存在物种间差异,这种差异是物种对环境长期适应的结果,与自身遗传特征有关,具有相对稳定性,并非全部受制于土壤养分的影响。

关键词：生态化学计量植物养分内稳性指数土壤特性

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