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Polarizable Additive with Intermediate Chelation Strength for Stable Aqueous Zinc‑Ion Batteries

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Nano-Micro Letters 2024年第5期16卷 41-55页

作者： Yuting Xia Rongao Tong Jingxi zhang mingjie Xu Gang Shao Hailong Wang Yanhao Dong Chang‑An Wang State Key Lab of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084People’s Republic of China School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001HenanPeople’s Republic of China

Aqueous zinc-ion batteries are promising due to inherent safety,low cost,low toxicity,and high volumetric capacity.However,issues of dendrites and side reactions between zinc metal anode and the electrolyte need to be solved for extended storage and cycle life.Here,we proposed that an electrolyte additive with an intermediate chelation strength of zinc ion—strong enough to exclude water molecules from the zinc metal-electrolyte interface and not too strong to cause a significant energy barrier for zinc ion dissociation—can benefit the electrochemical stability by suppressing hydrogen evolution reaction,overpotential growth,and den-drite formation.Penta-sodium diethylene-triaminepentaacetic acid salt was selected for such a purpose.It has a suitable chelating ability in aqueous solutions to adjust solvation sheath and can be readily polarized under electrical loading conditions to further improve the passivation.Zn||Zn symmetric cells can be stably operated over 3500 h at 1 mA cm^(-2).Zn||NH4V4O10 full cells with the additive show great cycling stability with 84.6%capacity retention after 500 cycles at 1 A g^(-1).Since the additive not only reduces H2 evolution and corrosion but also modifies Zn2+diffusion and deposition,highlyreversible Zn electrodes can be achieved as verified by the experimental results.Our work offers a practical approach to the logical design of reliable electrolytes for high-performance aqueous batteries.

关键词： Aqueous zinc-ion batteries Electrolyte additives DTPA-Na Chelation strength

Post-layout simulation driven analog circuit sizing

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Science China(Information Sciences) 2024年第4期67卷 289-300页

作者： Xiaohan GAO Haoyi zhang Siyuan YE mingjie LIU David Z.PAN Linxiao SHEN Runsheng WANG Yibo LIN Ru HUANG School of Integrated Circuits Peking University School of Computer Science Peking University Department of Electrical and Computer Engineering University of Texas at Austin Institute of Electronic Design Automation Peking University

Post-layout simulation provides accurate guidance for analog circuit design, but post-layout performance is hard to be directly optimized at early design stages. Prior work on analog circuit sizing often utilizes pre-layout simulation results as the optimization objective. In this work, we propose a post-layoutsimulation-driven(post-simulation-driven for short) analog circuit sizing framework that directly optimizes the post-layout simulation performance. The framework integrates automated layout generation into the optimization loop of transistor sizing and leverages a coupled Bayesian optimization algorithm to search for the best post-simulation performance. Experimental results demonstrate that our framework can achieve over 20% better post-layout performance in competitive time than manual design and the method that only considers pre-layout optimization.

关键词： analog EDA transistor sizing Bayesian optimization post-layout simulation

MoS_(2) quantum dots based MoS_(2)/HKUST-1 composites for the highly efficient catalytic oxidation of elementary mercury

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Journal of Environmental Sciences 2022年第6期34卷 163-174页

作者： mingjie zhang Gang Yang Shuai Liu Jiahui Yu Hongzhe Li Liwen zhang Yipei Chen Ruitang Guo Tao Wu College of Environmental and Chemical Engineering Shanghai University of Electric PowerShanghai 200090China New Materials Institute University of Nottingham Ningbo ChinaNingbo 315100China Key Laboratory of Carbonaceous Wastes Processing and Process Intensification of Zhejiang Province University of Nottingham Ningbo ChinaNingbo 315100China Ningbo Institute of Technology Zhejiang UniversityNingbo 315100China

Due to the ever-tightening regulation on mercury emission in recent decades,there is an urgent need to develop novel materials for the removal of elemental mercury at coal-fired power plants.In this study,a series of MoS_(2) quantum dots(QDs)-based MoS_(2)/HKUST-1 composite materials were prepared.It is found that MoS_(2)QDs were encapsulated by HKUST-1and enhanced the crystallinity and specific surface area of HKUST-1.The MoS_(2)/HKUST-1 showed excellent performance in catalytic oxidation of Hg~0as compared with pristine HKUST-1.It is found that surface layer of lattice oxygens is active and participates in Hg^(0) oxidation,while the consumption of surface oxygens then leads to the formation of oxygen vacancies on the surface.These vacancies are effective in the adsorption and dissociation of O_(2),which subsequently participates in the oxidation of Hg^(0).Moreover,the study on the influence of commonly seen gas components,such as SO_(2),NO,NH_(3) and H_(2)O,etc.,on Hg^(0) oxidation demonstrated that synergistic effects exist among these gas species.It is found that the presence of NO promotes the oxidation of Hg^(0) using oxygen as the oxidant.

关键词： Core-shell structure HKUST-1 Quantum dots Elemental mercury removal Catalysis

Novel high-voltage cathode for aqueous zinc ion batteries:Porous K_(0.5)VOPO_(4)·1.5H_(2)O with reversible solid-solution intercalation and conversion storage mechanism

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Journal of Energy Chemistry 2024年第6期93卷 71-78,I0003页

作者： Liyu Wang Mingliang Zhao Xiaoyu zhang Menghua Wu Yu Zong Yu Chen Xinliang Huang mingjie Xing Xin Ning Wen Wen Daming Zhu Xiaochuan Ren Industrial Research Institute of Nonwovens&Technical Textiles College of Textiles&ClothingShandong Engineering Research Center for Specialty Nonwoven MaterialsQingdao UniversityQingdao 266071ShandongChina Shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201204China

Cathode materials that possess high output voltage,as well as those that can be mass-produced using facile techniques,are crucial for the advancement of aqueous zinc-ion battery(ZIBs)applications,Herein,we present for the first time a new porous K_(0.5)VOPO_(4)·1.5H_(2)O polyanionic cathode(P-KIVP)with high output voltage(above 1.2 V)that can be manufactured at room temperature using straightforward coprecipitation and etching techniques.The P-KVP cathode experiences anisotropic crystal plane expansion via a sequential solid-solution intercalation and phase co nversion pathway throughout the Zn^(2+)storage process,as confirmed by in-situ synchrotron X-ray diffraction and ex-situ X-ray photoelectron spectroscopy.Similar to other layered vanadium-based polyanionic materials,the P-KVP cathode experiences a progressive decline in voltage during the cycle,which is demonstrated to be caused by the irreversible conversion into amorphous VO_(x).By introducing a new electrolyte containing Zn(OTF)_(2) to a mixed triethyl phosphate and water solution,it is possible to impede this irreversible conversion and obtain a high output voltage and longer cycle life by forming a P-rich cathode electrolyte interface layer.As a proof-of-concept,the flexible fiber-shaped ZIBs based on modified electrolyte woven into a fabric watch band can power an electronic watch,highlighting the application potential of P-KVP cathode.

关键词： Aqueous zinc ion battery Cathode Porous material High voltage platform In-situ synchrotron X-ray diffraction

MOF-derived molybdenum selenide on Ti_(3)C_(2)T_(x) with superior capacitive performance for lithium-ion capacitors

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International Journal of Minerals,Metallurgy and Materials 2022年第5期29卷 1061-1072页

作者： Jianjian Zhong Lu Qin Jianling Li Zhe Yang Kai Yang mingjie zhang State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China State Key Laboratory of Operation and Control of Renewable Energy and Storage Systems China Electric Power Research InstituteBeijing 100192China

Two-dimensional Ti_(3)C_(2)T_(x) exhibits outstanding rate property and cycle performance in lithium-ion capacitors(LICs)due to its unique layered structure,excellent electronic conductivity,and high specific surface area.However,like graphene,Ti_(3)C_(2)T_(x) restacks during electrochemical cycling due to hydrogen bonding or van der Waals forces,leading to a decrease in the specific surface area and an increase in the diffusion distance of electrolyte ions between the interlayer of the material.Here,a transition metal selenide MoSe_(2) with a special three-stacked atomic layered structure,derived from metal-organic framework(MOF),is introduced into the Ti_(3)C_(2)T_(x) structure through a solvo-thermal method.The synergic effects of rapid Li+diffusion and pillaring effect from the MoSe_(2) and excellent conductivity from the Ti_(3)C_(2)T_(x) sheets endow the material with excellent electrochemical reaction kinetics and capacity.The composite Ti_(3)C_(2)T_(x)@MoSe_(2) material exhibits a high capacity over 300 mAh·g^(-1) at 150 mA·g^(-1) and excellent rate property with a specific capacity of 150 mAh·g^(-1) at 1500 mA·g^(-1).Addition-ally,the material shows a superior capacitive contribution of 86.0%at 2.0 mV·s^(-1) due to the fast electrochemical reactions.A Ti_(3)C_(2)T_(x)@MoSe_(2)//AC LIC device is also fabricated and exhibits stable cycle performance.

关键词： two-dimensional titanium carbide molybdenum selenide solvothermal method electrochemical kinetics

Landscape of human organoids:Ideal model in clinics and research

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The Innovation 2024年第3期5卷 146-164页

作者： Xinxin Han Chunhui Cai Wei Deng Yanghua Shi Lanyang Li Chen Wang Jian zhang mingjie Rong Jiping Liu Bangjiang Fang Hua He Xiling Liu Chuxia Deng Xiao He Xin Cao Organ Regeneration X Lab Lisheng East China Institute of BiotechnologyPeking UniversityJiangsu 226200China Shanghai Lisheng Biotech Shanghai 200092China LongHua Hospital Shanghai University of Traditional Chinese Medicine725 Wanping South RoadXuhui DistrictShanghai 200032China Department of Oncology Shanghai Ninth People’s HospitalShanghai Jiao Tong University School of MedicineShanghai 200125China Department of Neurosurgery Third Affiliated HospitalNaval Medical UniversityShanghai 200438China Shanghai Key Laboratory of Forensic Medicine Shanghai Forensic Service PlatformAcademy of Forensic ScienceMinistry of JusticeShanghai 200063China Cancer Center Faculty of Health SciencesUniversity of MacaoTaipaMacao SARChina Ministry of Education Frontiers Science Center for Precision Oncology University of MacaoTaipaMacao SAR 999078China CAS Key Lab for Biomedical Effects of Nanomaterials and Nanosafety Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China Zhongshan Hospital Institute of Clinical Science Fudan University Shanghai Medical CollegeShanghai 200032China

In the last decade,organoid research has entered a golden era,signifying a pivotal shift in the biomedical landscape.The year 2023 marked a milestone with the publication of thousands of papers in this arena,reflecting exponential growth.However,amid this burgeoning expansion,a comprehensive and accurate overview of the field has been conspicuously absent.Our review is intended to bridge this gap,providing a panoramic view of the rapidly evolving organoid landscape.We meticulously analyze the organoid field from eight distinctive vantage points,harnessing our rich experience in academic research,industrial application,and clinical practice.We present a deep exploration of the advances in organoid technology,underpinned by our long-standing involvement in this arena.Our narrative traverses the historical genesis of organoids and their transformative impact across various biomedical sectors,including oncology,toxicology,and drug development.We delve into the synergy between organoids and avant-garde technologies such as synthetic biology and single-cell omics and discuss their pivotal role in tailoring personalized medicine,enhancing high-throughput drug screening,and constructing physiologically pertinent disease models.Our comprehensive analysis and reflective discourse provide a deep dive into the existing landscape and emerging trends in organoid technology.We spotlight technological innovations,methodological evolution,and the broadening spectrum of applications,emphasizing the revolutionary influence of organoids in personalized medicine,oncology,drug discovery,and other fields.Looking ahead,we cautiously anticipate future developments in the field of organoid research,especially its potential implications for personalized patient care,new avenues of drug discovery,and clinical research.We trust that our comprehensive review will be an asset for researchers,clinicians,and patients with keen interest in personalized medical strategies.We offer a broad view of the present and prospective capabilities of organoi

关键词： landscape intended advances

On the effects of urban-like intersections on ventilation and pollutant dispersion

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Building Simulation 2022年第3期15卷 419-433页

作者： Xin Guo Riccardo Buccolieri Zhi Gao mingjie zhang Tong Lyu Liyan Rui Jialei Shen School of Architecture and Urban Planning Nanjing University22 Hankou RoadNanjing 210093Jiangsu ProvinceChina Dipartimento di Scienze e Tecnologie Biologiche ed Ambientali Laboratory of MicrometeorologyUniversity of SalentoS.P.6 Lecce-Monteroni73100LecceItaly Department of Green Building and Low-Carbon Development Shanghai Research Institute of Building Sciences568 Shenfu RoadShanghai201108China Department of Mechanical and Aerospace Engineering Syracuse UniversitySyracuseNY13210USA

Focusing on the effect of street morphology on the ventilation efficiency,this paper presents 3D computational fluid dynamics(CFD)simulations of airflow and pollutant dispersion within urban-like three-way intersections,four-way intersections and roundabouts.The steady-state Reynolds-averaged Navier-Stokes(RANS)k-εturbulence model is adopted and eight directions of the approaching wind are considered.The ventilation efficiency is evaluated using the ventilation indices purging flow rate(PFR)and the net escape velocity(NEV).Results show the sensitivity of the ventilation efficiency to the type of intersection,to the wind direction and to the number of branches.Specifically,the ventilation efficiency of the investigated three-way intersections is found to be better than that of the other intersections,especially when the angle between the streets is large,while that of roundabouts is also considerable,even with a similar average wind velocity,among the cases evaluated in this paper.Further,the influence of the wind direction for the three-way and four-way intersections is greater than that on roundabouts.Studies on the ventilation efficiency at urban intersections are not common in the literature and this work may help urban planners to better design such hub nodes of urban traffic,where traffic-related pollutants are not easily dispersed,thus avoiding harm to the health of pedestrians and surrounding residents.

关键词： urban-like intersections ventilation efficiency CFD simulations traffic-related pollutants

An Affective EEG Analysis Method Without Feature Engineering

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Journal of Electronic Research and Application 2024年第1期8卷 36-45页

作者： Jian zhang Chunying Fang Yanghao Wu mingjie Chang Heilongjiang University of Science and Technology Harbin 150022Heilongjiang ProvinceChina

Emotional electroencephalography(EEG)signals are a primary means of recording emotional brain activity.Currently,the most effective methods for analyzing emotional EEG signals involve feature engineering and neural networks.However,neural networks possess a strong ability for automatic feature extraction.Is it possible to discard feature engineering and directly employ neural networks for end-to-end recognition?Based on the characteristics of EEG signals,this paper proposes an end-to-end feature extraction and classification method for a dynamic self-attention network(DySAT).The study reveals significant differences in brain activity patterns associated with different emotions across various experimenters and time periods.The results of this experiment can provide insights into the reasons behind these differences.

关键词： Dynamic graph classification Self-attention mechanism Dynamic self-attention network SEED dataset

The efficiency and toxicity of dodecafluoro-2-methylpentan-3-one in suppressing lithium-ion battery fire

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Journal of Energy Chemistry 2022年第2期31卷 532-540页

作者： Yujun Liu Kai Yang mingjie zhang Shi Li Fei Gao Qiangling Duan Jinhua Sun Qingsong Wang State Key Laboratory of Fire Science University of Science and Technology of ChinaHefei 230026AnhuiChina State Key Laboratory of Operation and Control of Renewable Energy&Storage Systems China Electric Power Research InstituteBeijing 100192China

Currently,the effective and clean suppression of lithium-ion battery(LIB)fires remains a challenge.The present work investigates the use of various inhibitor doses(Xin)of dodecafluoro-2-methylpentan-3-one(C_(6) F_(12)O)in 300 Ah LIBs,and systematically examines the thermal and toxic hazards of the extinguished batteries via real scale combustion and gas analysis.The inhibitor is shown to be completely effective.The inhibition mechanism involves a combination of chemical inhibition and physical cooling.While the chemical inhibition effect tends to saturate with increasing Xin,the physical cooling remains effective at higher inhibitor doses.However,extinguishing the battery fire with a high Xin of C_(6)F_(12)O is found to incur serious toxicity problems.These results are expected to provide a guideline for the design of inhibitor doses for the suppression of LIB fires.

关键词： Lithium ion battery safety Thermal runaway Fire suppression C_(6)F_(12)O