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Study of ZnO nanoparticle-supported clay minerals for electrochemical sensors,photocatalysis,and antioxidant applications

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chemPhysMater 2024年第1期3卷 83-93页

作者： Mylarappa M n.Raghavendra n.R.Bhumika C.H.chaithra B.n.nagalaxmi K.n.Shravana Kumara Department of chemistry Sri Jagadguru Renukacharya College of ScienceArts&CommerceBengaluru 560009India Department of chemistry East West Institute of TechnologyBengaluru 560091India Department of chemistry Maharani Lakshmi Ammanni College for WomenBengaluru 560012India

In view of the current study’s demonstration of the synthesis of clay-doped ZnO composites,we present a low-cost method for producing clay-metal oxide(clay/ZnO).Utilizing the solution combustion technique,a composite of clay/ZnO was produced utilizing citric acid as both a fuel and a complexing *** hexagonal unit cell structure of the created clay/ZnO may be seen using XRD *** ZnO-infused clay was visible in FE-SEM micrographs as homogenous,sphere-shaped *** possible involvement of clay/ZnO photocatalytic activity in the UV-induced photodegradation of malachite green dye was *** 90%degradation rate shows the composite’s outstanding photocatalytic degradation *** resulting substance was electrochemically analyzed using a constructed electrode in 0.1 M KOH *** increased its sensor capabilities,which.now include chemical and biomolecule sensors,and it excelled in cyclic voltammetry-based redox potential *** efficiently evaluate chemically synthesized nPs for electrochemical,sensing,and photocatalytic applications,this study intends to create a solution combustion procedure for the synthesis of clay/ZnO nanocomposite using urea as fuel.

关键词： Clay Clay/ZnO Photocatalytic Electrochemical sensors

Optimizing laser coupling,matter heating,and particle acceleration from solids using multiplexed ultraintense lasers

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Matter and Radiation at Extremes 2024年第4期9卷 16-28页

作者： Weipeng Yao Motoaki nakatsutsumi Sébastien Buffechoux Patrizio Antici Marco Borghesi Andrea Ciardi Sophia n.ch.n Emmanuel d’Humières Laurent Gremillet Robert Heathcote Vojtech Horny Paul McKenna Mark n.Quinn Lorenzo Romagnani Ryan Royle Gianluca Sarri Yasuhiko Sentoku Hans-Peter Schlenvoigt Toma Toncian Olivier Tresca Laura Vassura Oswald Willi Julien Fuchs LULI-CnRS CEASorbonne UniversitéEcole PolytechniqueInstitut Polytechnique de ParisF-91128 Palaiseau CedexFrance Sorbonne Université Observatoire de ParisUniversité PSLCNRSLERMAF-75005 ParisFrance InRS-EMT 1650 BoulLionel-BouletVarennesQuebec J3X 1S2Canada Center for Plasma Physics School of Mathematics and PhysicsQueen’s University BelfastBelfast BT71NNUnited Kingdom “Horia Hulubei”national Institute for Physics and nuclear Engineering 30 Reactorului StreetRO-077125 Bucharest-MagureleRomania University of Bordeaux Centre Lasers Intenses et ApplicationsCNRSCEAUMR 5107F-33405 TalenceFrance CEA DAMDIFF-91297 ArpajonFrance Université Paris-Saclay CEALMCE91680 Bruyères-le-ChatelFrance Central Laser Facility STFC Rutherford Appleton LaboratoryDidcotUnited Kingdom SUPA Department of PhysicsUniversity of StrathclydeGlasgow G40NGUnited Kingdom Department of Physics University of NevadaRenoNevada 89557USA Institute of Laser Engineering Osaka University2-6 YamadaokaSuitaOsaka 565-0871Japan Institut fur Laser und Plasmaphysik Heinrich Heine Universitat DusseldorfDusseldorfGermany

Realizing the full potential of ultrahigh-intensity lasers for particle and radiation generation will require multi-beam arrangements due to technology ***,we investigate how to optimize their coupling with solid ***,we show that overlapping two intense lasers in a mirror-like configuration onto a solid with a large preplasma can greatly improve the generation of hot electrons at the target front and ion acceleration at the target *** underlying mech.nisms are analyzed through multidimensional particle-in-cell simulations,revealing that the self-induced magnetic fields driven by the two laser beams at the target front are susceptible to reconnection,which is one possible mech.nism to boost electron *** addition,the resistive magnetic field generated during the transport of the hot electrons in the target bulk tends to improve their *** simulations also indicate that such effects can be further enhanced by overlapping more than two laser beams.

关键词： laser acceleration particle

Are we ready to use new endoscopic scores for ulcerative colitis?

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World Journal of Gastroenterology 2024年第10期30卷 1466-1469页

作者： Rodrigo Quera Paulina núñez F Universidad de los Andes Inflammatory Bowel Disease ProgramClinica Universidad de los AndesDigestive Disease CenterSantiago 7600976RMChile Digestive Disease Center Inflammatory Bowel Disease ProgramClínica Universidad de los AndesSantiago 7620157Chile Department of Gastroenterology Universidad de Chile-Hospital San Juan de DiosSantiago 770123Chile

For ulcerative colitis(UC),the variability in inflammatory activity along the colon poses a challenge in *** focus on achieving endoscopic healing in UC is evident,where the UC Endoscopic Index of Severity and Mayo Endoscopic Subscore are commonly used for ***,these indices primarily consider the most severely affected *** et al recent study validates the Toronto Inflammatory Bowel Disease Global Endoscopic Reporting(TIGER)score offering a comprehensive assessment of inflammatory activity across diverse segments of the colon and rectum and a reliable index correlating strongly with UC Endoscopic Index of Severity and moderately with Mayo Endoscopic Subscore(MES).Despite recommendation,certain aspects warrant further *** calprotectin,an intermediate target,correlates with TIGER and should be *** TIGER scores defining endoscopic remission and response,evaluating agreement with histological activity,and assessing inter-endoscopist agreement for TIGER require *** the correlation between TIGER and intestinal ultrasound,akin to MES,adds value.

关键词： Ulcerative colitis Sigmoidoscopy Colonoscopy Score index

Empirical model for fusion cross sections of Ca-induced reactions

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ch.nese Physics C 2024年第3期48卷 126-132页

作者： Reddi Rani.L n.Sowmya K.n Sridhar H C.Manjunatha M.M.Armstrong Arasu Department of Physics St.Joseph's College(Autonomous)Affiliated to Bharathidasan UniversityTiruchirappalli620002TNIndia Department of Physics Govt.First.Grade CollegeChikkaballapur-562101KarnatakaIndia Department of Physics Govt.First.Grade CollegeMalur-563160KarnatakaIndia Department of Physics Govt.First.Grade CollegeDevanahalli-562110KarnatakaIndia

A new empirical formula for the astrophysical S-factor has been suggested as a function of the Coulomb interaction parameter,center of mass energy,and barrier *** 22 fusion reactions with ^(40,48)Ca as projectiles were considered for different targets,leading to compound nuclei with atomic and mass numbers varying between 40≤Z≤≤Z≤112 and 88≤A≤27888≤A≤278,*** fusion cross-sections have been estimated using the geometric factor,the Gamow-Sommerfield factor,and the empirical formula for the *** study's findings showed better agreement with those of available experiments when compared to Wong's *** present work leads to a smaller standard deviation value than Wong's formula when used to correlate the experimental data of calcium-induced fusion ***'s formula provides a good approximation of fusion cross-sections when the center of mass energy is below the fusion barrier when compared to above the fusion barrier.

关键词： fusion cross-sections Wong formula Gamow-Sommerfield-factor Geometric-factor S-factor

Alpha7 nicotinic receptors as potential theranostic targets for experimental stroke

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neural Regeneration Research 2024年第5期19卷 939-940页

作者： Maider Garbizu Laura Aguado Abraham Martín Achucarro Basque Center for neuroscience LeioaSpain CIC biomaGUnE Basque Research and Technology AllianceSan SebastianSpain Ikerbasque Basque Foundation for Science BilbaoSpain

Inflammatory reflex and cholinergic anti-inflammatory pathway:Innate immune system triggers a local inflammatory response following an injury or a pathogen ***,this inflammatory response is limited by rapid,localized,and adaptive anti-inflammatory responses which are crucial for maintaining ***,the loss of these responses converts a limited and protective inflammatory response into an excessive and harmful ***-inflammatory responses are integrated into the central nervous system,since the central nervous system accumulates information about harmful events,activates defenses,and builds memory for *** the same time,it has been demonstrated that hypothalamic neuronal signaling can be altered by inflammation in peripheral ***,immune cells release neuropeptides and neurotransmitters such as acetylcholine(Ach),the main neurotransmitter of the parasympathetic autonomic nervous system,evidencing the communication between the immune and nervous systems(Tracey,2002).

关键词： protective invasion Alpha

Developing knn forest data imputation for Catalonia

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Journal of Forestry Research 2024年第4期35卷 142-155页

作者： Timo Pukkala núria Aquilué Ariadna Just Jordi Corbera Antoni Trasobares Forest Science and Technology Centre of Catalonia(CTFC) Crta.de St.Llorençde MorunysKm 225280 SolsonaSpain Cartographic and Geological Institute of Catalonia(ICGC) 08038 BarcelonaSpain

The combined use of LiDAR(Light Detection And Ranging)scanning and field inventories can provide spatially continuous wall-to-wall information on forest *** information can be used in many ways in forest mapping,scenario analyses,and forest manage-ment *** study aimed to find the optimal way to obtain continuous forest data for Catalonia when using knn imputation(knn stands for“k nearest neighbors”).In this method,data are imputed to a certain location from k field-measured sample plots,which are the most similar to the location in terms of LiDAR metrics and topographic *** multidimensional Euclidean distance was used as the similarity *** study tested two different methods to optimize the distance *** first method optimized,in the first step,the set of LiDAR and topographic variables used in the measure,as well as the transformations of these *** weights of the selected variables were optimized in the second *** other method optimized the variable set as well as their transformations and weights in one single *** two-step method that first finds the variables and their transfor-mations and subsequently optimizes their weights resulted in the best imputation *** the study area,the use of three to five nearest neighbors was *** and latitude turned out to be the most important variables when assessing the similarity of two locations of Catalan forests in the context of knn data *** optimal distance measure always included both LiDAR metrics and topographic *** study showed that the optimal similarity measure may be different for different ***,it was suggested that knn data imputation should always be started with the optimization of the measure that is used to select the k nearest neighbors.

关键词： Forest inventory Differential evolution Simulated annealing LiDAR

Simultaneous removal of critical rare earth elements and chalcogen oxyanions by anaerobic granular sludge

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Rare Metals 2024年第9期43卷 4595-4611页

作者： chiara Belloni Mohanakrishnan Logan Stefano Papirio Piet n.L.Lens University of Galway Department of Civil Architectural and Environmental EngineeringUniversity of Naples Federico II

Conventional mining of economically and strategically important critical rare earth elements(REEs)(such as neodymium, lanthanum and dysprosium), and chalcogens(such as selenium and tellurium) are associated with a huge economic and environmental cost. Therefore,the need to recover REEs as well as chalcogens from different waste streams including wastewaters is becoming urgent. Batch assays on synthetic chalcogen/REE-laden wastewater showed that the presence of REEs significantly improved the tellurite removal rate(> 80%) and enhanced selenate removal by 66% ± 10%. Three 3.9 L continuous upflow anaerobic granular sludge bed(UASB) reactors were operated at a hydraulic retention time of 24 h and30 °C. Selenate reduction was achieved with a removal efficiency of ～ 98% with an influent p H of 4.0 for more than 28 days. The effect of REEs on tellurite removal in the UASB bioreactor could not be clearly established since a soluble tellurium removal efficiency of more than 98%was observed already before the addition of REEs at elevated tellurite concentrations. The complete REE removal in both batch assays and UASB reactors at higher pH (7.0 ± 0.5) was attributed to precipitation, whereas chalcogen oxyanions removal was due to microbial reduction. However, at acidic p H, biosorption was responsible for REE's removal, and the Se-enriched sludge exhibited a superior REE's removal efficiency than the non-enriched and Te-enriched sludge.

关键词： Adsorption Bioreduction Rare earth elements Selenium Tellurium

Comparison of Perovskite Systems Based on AFeO_(3)(A=Ce,La,Y)in CO_(2) Hydrogenation to CO

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Transactions of Tianjin University 2024年第4期30卷 337-358页

作者： Anna n.Matveyeva Shamil O.Omarov Laboratory of Materials and Processes for Hydrogen Energy Ioff e Institute194021 St.PetersburgRussia

CO_(2) is the most cost-eff ective and abundant carbon resource,while the reverse water-gas reaction(rWGS)is one of the most eff ective methods of CO_(2) *** work presents a comparative study of rWGS activity for perovskite systems based on AFeO_(3)(where A=Ce,La,Y).These systems were synthesized by solution combustion synthesis(SCS)with diff erent ratios of fuel(glycine)and oxidizer(φ),diff erent amounts of nH 4 nO_(3),and the addition of alumina or silica as *** techniques,including X-ray diff raction analysis,thermogravimetric analysis,Fourier transform infrared spectroscopy(FTIR),scanning electron microscopy,energy-dispersive X-ray spectroscopy,n 2-physisorption,H_(2) temper-ature-programmed reduction,temperature-programmed desorption of H_(2) and CO_(2),Raman spectroscopy,and in situ FTIR,were used to relate the physicochemical properties with the catalytic performance of the obtained *** specifi c perovskite-containing system(either bulk or supported)has its own optimalφand nH_(4) nO_(3) amount to achieve the highest yield and dispersion of the perovskite *** all synthesized systems,bulk SCS-derived La-Fe-O systems showed the highest resistance to reducing environments and the easiest hydrogen desorption,outperforming La-Fe-O produced by solgel combustion(SGC).CO_(2) conversion into CO at 600°C for bulk ferrite systems,depending on the A-cation type and preparation method,follows the order La(SGC)nces in properties between La-Fe-O obtained by the SCS and SGC methods can be attributed to diff erent ratios of oxygen and lanthanum vacancy contributions,hydroxyl coverage,morphology,and free iron oxide *** situ FTIR data revealed that CO_(2) hydrogenation occurs through formates generated under reaction conditions on the bulk system based on La-Fe-O,obtained by the SCS method.γ-Al_(2)O_(3) improves the dispersion of CeFeO_(3) and LaFeO_(3) phases,the specifi c surface area,and the quant

关键词： Perovskites LaFeO_(3) CeFeO_(3) YFeO_(3) Solution combustion synthesis CO_(2) hydrogenation Reverse water–gas reaction(rWGS)

Formation of diffuse and spark discharges between two needle electrodes with the scattering of particles

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Plasma Science and Technology 2024年第9期26卷 32-39页

作者： Victor F TARASEnKO Dmitry V BELOPLOTOV Alexei n PAnch.nKO Dmitry A SOROKIn Institute of High Current Electronics Siberian BranchRussian Academy of SciencesTomsk 634055Russia national Research Tomsk State University Tomsk 634050Russia

The development of a nanosecond discharge in a pin-to-pin gap filled with air at atmospheric pressure has been studied with high temporal and spatial resolutions from a breakdown start to the spark *** and negative nanosecond voltage pulses with an amplitude of tens of kilovolts were ***-resolved images of the discharge development were taken with a fourch.nnel Intensified charge Coupled Device(ICCD)*** minimum delay between the camera ch.nnels could be as short as≈0.1 *** made it possible to study the gap breakdown process with subnanosecond *** was observed that a wide-diameter streamer develops from the high-voltage pointed *** ionization processes near the grounded pin electrode started when the streamer crossed half of the *** bridging the gap by the streamer,a diffuse discharge was *** development of spark leaders from bright spots on the surface of the pointed electrodes was observed at the next *** was found that the rate of development of the spark leader is an order of magnitude lower than that of the wide-diameter *** thin luminous tracks were observed against the background of a discharge plasma *** has been established that the tracks are adjacent to brightly glowing spots on the electrodes and are associated with the flight of small particles.

关键词： needle electrodes short voltage pulses atmospheric air streamer breakdown diffuse and spark discharges scattering metal particles