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Synergistic integration of self-supported 1T/2H-WS_(2) and nitrogendoped rGO on carbon cloth for pH-universal electrocatalytic hydrogen evolution

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Nano Research 2024年第3期17卷 1267-1280页

作者： Feng ming Yap Jian Yiing Loh Wee-Jun ong School of Energy and Chemical Engineering Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia Center of Excellence for NaNo Energy&Catalysis Technology(CONNECT) Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Gulei Innovation Institute Xiamen UniversityZhangzhou 363200China Shenzhen Research Institute of Xiamen University Shenzhen 518057China

Hydrogen economy based on electrochemical water splitting exemplified one of the most promising means for overcoming the rapid consumption of fossil fuels and the serious deterioration of global *** development of earth-abundant,efficient,and durable electrocatalysts for hydrogen evolution reaction(HER)plays a vital role in the commercialization of water ***,the self-supported electrode with unique nitrogen-doped reduced graphene oxide(N-rGO)nanoflakes and WS_(2) hierarchical nanoflower that were grown directly on carbon cloth(CC)substrate(WS_(2)/N-rGO/CC)was successfully synthesized using a facile dual-step hydrothermal *** as-synthesized 50%1T/2H-WS_(2)/N-rGO/CC(WGC),which possessed high metallic 1T phase of 57%not only efficiently exposed more active sites and accelerated mass/charge diffusion,but also endowed excellent structural lustiness,robust stability,and durability at a high current *** a result,the 50%WGC exhibited lower overpotentials and Tafel slopes of 21.13 mV(29.55 mV∙dec^(-1))and 80.35 mV(137.02 mV∙dec^(-1))as compared to 20%Pt-C/CC,respectively for catalyzing acidic and alkaline hydrogen evolution ***,the as-synthesized 50%WGC also depicted long-term stability for more than 8 h in the high-current-density regions(100 and 220 mA∙cm^(-2)).In brief,this work reveals a self-supported electrode as an extraordinary alternative to Pt-based catalysts for HER in a wide pH range,while paving a facile strategy to develop advanced electrocatalysts with abundant heterointerfaces for practical applications in energy-saving hydrogen production.

关键词： self-supported electrocatalyst carbon-based substrate phase engineering pH-universal water splitting

Guest Editorial:Special issue on advances in representation learning for computer vision

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CAAI Transactions on Intelligence Technology 2024年第1期9卷 1-3页

作者： Andrew Beng Jin Teoh Thian Song ong Kian ming Lim Chin Poo Lee Electrical and Electronic Engineering Department Yonsei UniversitySeoulSouth Korea Faculty of Information Science and Technology Multimedia UniversityMelakaMalaysia

Deep learning has been a catalyst for a transformative revo-lution in machine learning and computer vision in the past *** these research domains,methods grounded in deep learning have exhibited exceptional performance across a spectrum of *** success of deep learning methods can be attributed to their capability to derive potent representations from data,integral for a myriad of downstream *** representations encapsulate the intrinsic structure,fea-tures,or latent variables characterising the underlying statistics of visual *** these achievements,the challenge per-sists in effectively conducting representation learning of visual data with deep models,particularly when confronted with vast and noisy *** special issue is a dedicated platform for researchers worldwide to disseminate their latest,high-quality articles,aiming to enhance readers'comprehension of the principles,limitations,and diverse applications of repre-sentation learning in computer vision.

关键词： spite computer representation

Regulation of aging by NELF-A and RNA polymerase Ⅱ elongation

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Neural Regeneration Research 2024年第7期19卷 1415-1416页

作者： Chin-Tong ong Zhen-Kai Ngian Temasek Life Sciences Laboratory and Department of Biological Sciences National University of SingaporeSingaporeSingapore Department of Genetics Harvard Medical SchoolBostonMAUSA Institute of Molecular and Cell Biology Agency for ScienceTechnology and ResearchSingaporeSingapore

Epigenetic regulation of aging:Aging is defined as the gradual decline of physiological function and cellular integrity,causing o rganismal vulnerability to age-onset diseases and *** in different animal models have l... 详细信息

关键词： aging twelve integrity

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Utility of gastrointestinal ultrasound in functional gastrointestinal disorders:A narrative review

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World Journal of Meta-Analysis 2020年第2期8卷 109-118页

作者： Andrew ming-liang ong Department of Gastroenterology and Hepatology Singapore General HospitalSingapore 169856Singapore Duke-NUS Medical School Singapore 169857Singapore

Gastrointestinal(GI)ultrasound(GIUS)is valuable in the evaluation of GI diseases such as inflammatory bowel disease,but its use in functional GI disorders(FGIDs)is largely unknown although *** order to review the current knowledge on current and potential uses of GIUS in FGIDs,information was obtained via a structured literature search through PubMed,EMBASE and Google Scholar databases with a combination of MESH and keyword search terms:“ultrasound”,“functional GI disorders”,“irritable bowel syndrome”,“functional dyspepsia”,“intestinal ultrasound”,“point of care ultrasonography”,“transabdominal sonography”,“motility”,“faecal loading”,“constipation”.GIUS is currently used for various settings involving upper and lower GI tracts,including excluding organic diseases,evaluating physiology,guiding treatment options and building rapport with *** can be potentially used to correlate mechanisms with symptoms,evaluate mechanisms behind treatment efficacy,and investigate further the origin of symptoms in *** conclusion,GIUS is unique in its real-time,interactive and non-invasive nature,with the ability of evaluating several physiological mechanisms with one test,thus making it attractive in the evaluation and management of ***,there are still limitations and concerns of operator dependence and lack of validation data for widespread implementation of GIUS in FGIDs.

关键词： Ultrasound Functional gastrointestinal disorders Irritable bowel syndrome Functional dyspepsia Constipation

Enhancing MXene-based supercapacitors:Role of synthesis and 3D architectures

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Journal of Energy Chemistry 2024年第4期91卷 1-26页

作者： Wen Siong Poh Wen Jie Yiang Wee-Jun ong Pau Loke Show Chuan Yi Foo School of Energy and Chemical Engineering Xiamen University MalaysiaSelangor Darul EhsanMalaysia&College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005FujianChina Kelip-kelip!Center of Excellence for Light Enabling Technologies Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia Center of Excellence for NaNo Energy&Catalysis Technology(CONNECT) Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia Department of Chemical Engineering Khalifa UniversityShakhbout Bin Sultan St-Zone 1Abu DhabiUnited Arab Emirates Zhejiang Provincial Key Laboratory for Subtropical Water Environment and Marine Biological Resources Protection Wenzhou UniversityWenzhou 325035ZhejiangChina Department of Chemical and Environmental Engineering Faculty of Science and EngineeringUniversity of Nottingham MalaysiaJalan Broga43500 SemenyihSelangor Darul EhsanMalaysia Department of Sustainable Engineering Saveetha School of EngineeringSIMATSChennai 602105India

MXene has been the limelight for studies on electrode active materials,aiming at developing supercapacitors with boosted energy density to meet the emerging influx of wearable and portable electronic *** its various desirable properties including intrinsic flexibility,high specific surface area,excellent metallic conductivity and unique abundance of surface functionalities,its full potential for electrochemical performance is hindered by the notorious restacking phenomenon of MXene *** to its two-dimensional(2D)nature and surface functional groups,inevitable Van der Waals interactions drive the agglomeration of nanosheets,ultimately reducing the exposure of electrochemically active sites to the electrolyte,as well as severely lengthening electrolyte ion transport *** a result,energy and power density deteriorate,limiting the application versatility of MXene-based *** 3D architectures using 2D nanosheets presents as a straightforward yet ingenious approach to mitigate the fatal flaws of ***,the sheer number of distinct methodologies reported,thus far,calls for a systematic review that unravels the rationale behind such 3D MXene structural ***,this review aims to serve this purpose while also scrutinizing the structure–property relationship to correlate such structural modifications to their ensuing electrochemical performance ***,the physicochemical properties of MXene play fundamental roles in determining the effective charge storage capabilities of 3D MXene-based *** largely depends on different MXene synthesis techniques and synthesis condition variations,hence,elucidated in this review as ***,the challenges and perspectives for achieving viable commercialization of MXene-based supercapacitor electrodes are highlighted.

关键词： MXene 3D architectures Synthesis design Supercapacitor Energy storage

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Apolipoprotein E elicits targetdirected miRNA degradation to maintain neuronal integrity

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Neural Regeneration Research 2025年第9期20卷 2577-2578页

作者： Jiazi Tan Chin-Tong ong Temasek Life Sciences Laboratory National University of SingaporeSingapore Department of Biological Sciences National University of SingaporeSingapore

Apolipoprotein E has diverse functions in neurons:Apolipoprotein E(ApoE)is a glycoprotein that primarily regulates lipid metabolism and transport in the central nervous *** are three predominant human ApoE protein isoforms with cysteine and arginine substitutions at amino acid positions 112 and 158 that impact their lipidation and related functions(Flowers and Rebeck,2020).ApoE2 is characterized by Cys112 and Cys158,ApoE3 by Cys112 and Arg158,whereas ApoE4 contains Arg112 and Arg158.

关键词： metabolism glycoprotein maintain

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释放多孔纳米结构的活力:可持续电催化水分解

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Chinese Journal of Catalysis 2024年第3期58卷 37-85页

作者：罗健颖傅捷叶丰铭梁汉锋王伟俊厦门大学马来西亚分校能源与化工学院马来西亚雪兰莪州厦门大学马来西亚分校纳米能源与催化技术卓越中心(CONNECT)马来西亚雪兰莪州厦门大学化学与化工学院固体表面物理化学国家重点实验室福建厦门361005 厦门大学古雷创新学院福建漳州363200 厦门大学深圳研究院广东深圳518057

电化学整体水分解(OWS)作为一种很有应用前景的能源转换技术,可用于生产清洁的可再生氢燃料,引起了人们的广泛关注.然而,水分解反应的半反应,即析氧反应(OER),因动力学缓慢、水分解热力学势垒高和能量消耗大等问题制约了OWS的广泛应用.... 详细信息

电化学整体水分解(OWS)作为一种很有应用前景的能源转换技术,可用于生产清洁的可再生氢燃料,引起了人们的广泛关注.然而,水分解反应的半反应,即析氧反应(OER),因动力学缓慢、水分解热力学势垒高和能量消耗大等问题制约了OWS的广泛应用.研究发现,采用地球储量丰富的元素设计的多孔材料可以显著提高活性位点数量及其可及性,增大比表面积,优化反应物的吸附/脱附,改善传质,进而表现出较好的电催化活性.因此,系统梳理总结多孔纳米材料在电催化分解水领域的研究进展具有重要的意义.本文综述了近年来用于析氢反应,OER和OWS的多孔电催化剂的研究进展.聚焦于合成策略的最新进展,并结合多孔结构在电催化剂中的独特作用进行了讨论.概述了各种新兴的多孔电催化剂改性策略,包括结构工程、相工程、缺陷工程和应变工程;重点介绍了合成方法、多孔材料性能提升、机理理解、集成实验、水分解的理论研究和先进的改性策略,并提出了合成工艺.特别总结了结构-活性关系的研究成果,为设计和改性具有独特性能的多孔材料提供参考.最后,本文强调了当前多孔电催化剂所面临的科学挑战和未来发展方向,旨在为推动多孔电催化剂在电化学水分解领域的应用和发展提供借鉴.

关键词：多孔材料电催化析氢反应析氧反应水分解

Treatment options for rumination syndrome: A systematic review

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World Journal of Meta-Analysis 2019年第6期7卷 297-308页

作者： Andrew ming-liang ong Shu-Wen Tay Yu-Tien Wang Department of Gastroenterology and Hepatology Singapore General HospitalSingapore 169856Singapore Duke-NUS Graduate Medical School Singapore 169856Singapore

BACKGROUND Rumination syndrome (RS) is characterized by recurrent effortless postprandial regurgitation of recently ingested food from the stomach to the oral cavity and has been associated with quality of life impairment and malnutrition. There is a general lack of consensus on the most appropriate treatment options for RS. AIM To summarize the literature on treatment options for RS. METHODS We conducted a systematic review according to PRISMA guidelines. We searched Medline (1946 to February 2019), EMBASE (1947 to February 2019), PsycINFO (1806 to February 2019) and Cochrane central register of controlled trials for articles discussing treatment options for adult patients (> 18 years) with RS. All relevant articles were accessed in full text. We extracted data on study designs, patient profiles, duration of symptoms, follow up periods, date, diagnostic criteria, interventions and outcomes. Risk of bias assessment was carried out independently by 3 reviewers via Cochrane Risk of Bias tool and Newcastle Ottawa Scale for randomized controlled trials and Cohort studies respectively. RESULTS Twelve articles were identified. A total of 254 patients were included in the analysis, with a mean age of 36.1 (range 18-89). 185 patients (72.8%) were females. 5 studies looked into behavioral therapies, primarily diaphragmatic breathing (DB) 2 studies looked at baclofen, 1 fundoplication and 1 supportive lifestyle changes. 3 studies looked at a combination of therapies involving pharmacological, behavioral and psychotherapies. CONCLUSION Although evidence for treatment options is still limited, the strongest evidence point towards the use of DB and Baclofen, and both should be considered depending on their availabilities.

关键词： Rumination Rumination syndrome Diaphragmatic breathing Treatment Systematic review

计及故障持续时间的电力系统暂态稳定分布式控制

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控制理论与应用 2024年第5期41卷 905-913页

作者：陈世明余翔张微刘江钱成龙华东交通大学电气与自动化工程学院江西南昌330013

针对电力系统故障持续时间会影响暂态稳定控制的问题,本文提出了一种使系统在固定时间内恢复暂态稳定运行的策略.该策略通过电力系统通信拓扑建模方法为每个发电机建立“邻居发电机”,利用发电机本地信息和其邻居发电机的信息设计分布... 详细信息

针对电力系统故障持续时间会影响暂态稳定控制的问题,本文提出了一种使系统在固定时间内恢复暂态稳定运行的策略.该策略通过电力系统通信拓扑建模方法为每个发电机建立“邻居发电机”,利用发电机本地信息和其邻居发电机的信息设计分布式控制器,通过控制储能装置作用于受扰动后的系统,使其在固定时间内恢复稳定运行.其次,此控制策略还解决了一些实际挑战,如控制器的输入延时、外部的干扰、储能装置的容量限制等.通过构建李雅普诺夫函数并利用图论知识对该策略展开了稳定性分析,推导出了稳定系统的时间界限.最后,将控制器投入新英格兰39节点测试系统中,并与其它控制器进行比较,仿真结果验证了在低容量储能装置限制下和抗干扰性上控制器性能的优势.

关键词：故障持续时间暂态稳定控制固定时间电力系统通信拓扑建模分布式控制器储能装置

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