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Solid-state room-temperature phosphorescence activated by the end-capping strategy of cyano groups

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Aggregate 2024年第4期5卷 367-375页

作者： Jia-Lin Yu Zhaojun Chen Yu-Qi Zhu Yu-Long Jin Xin Wang ming-xue wu Xing-Huo Wang Ying-Wei Yang Institute for Sustainable Energy and Resources College of Chemistry and Chemical EngineeringQingdao UniversityQingdaoP.R.China International Joint Research Laboratory of Nano-Macro Architecture Chemistry College of ChemistryJilin UniversityChangchunP.R.China

Avoiding the tedious process of crystal cultivation and directly obtaining organic crystals with desirable phosphorescent performance is of great signiﬁcance for studying their structure and ***,a set of benzophenone-cored phos-phors with bright green afterglow are obtained on a large scale through in-situ generation via an end-capping strategy to suppress non-radiative triplet excitons and reinforce the intermolecular *** ordered arrangement of phosphors with alkyl-cyano groups as regulators is crucial for the enhancement of room-temperature phosphorescence(RTP)emission,which has been further veriﬁed by the attenuated lifetimes in isolated states through the formation of inclusion complexes upon binding with pillar[5]***,the hierarchical interactions of phos-phors,including hydrogen bonding,π-πstacking interactions,and van der Waals forces,are quantiﬁed by crystal structures and theoretical calculation to deeply inter-pret the origins of RTP *** this study,we provide a potential strategy for the direct acquisition of crystalline organic phosphors and modulation of RTP.

关键词： alkyl-chain length selectivity pillar[n]arenes room-temperature phosphorescence supramolecular interactions

Smart phosphorescence from solid to water through progressive assembly strategy based on dual phosphorescent sources

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Aggregate 2023年第5期4卷 224-234页

作者： Qing-Qing Xia Xing-Huo Wang Jia-Lin Yu Zhong-Yuan Chen Xin-Yue Lou Xiaomin Liu ming-xue wu Ying-Wei Yang College of Chemistry and Chemical Engineering Qingdao UniversityShandongP.R.China International Joint Research Laboratory of Nano-Macro Architecture Chemistry College of ChemistryJilin UniversityChangchunP.R.China

Developing smart room-temperature phosphorescence(RTP)materials with facile and efficient strategies have attracted increasing ***,tunable RTP materials with two phosphorescent sources and stepwise enhanced phosphorescence in water are obtained through an in-situ self-assembly strategy based on the sensitization of phosphors by trimesic acid(TMA)through simple doping and the rigidification of phosphors by hydrogen-bonded organic frameworks(HOFs).As expected,doped TMA+phosphors simultaneously promote the RTP emission of phosphors and maintain TMA ***-situ assembled HOF(MATMA)@phosphors facilitate smart RTP emission in water due to the coexistence of phosphorescent HOF(MA-TMA)host and phosphors ***,such RTP materials with good processability demonstrate the application potential in information security,benefitting from their varied afterglow lifetimes and easy luminous recognition in the *** work will inspire the design of dual phosphorescent source RTP systems and provide new strategies for the development of smart RTP materials in water.

关键词： emissive materials hydrogen-bonded organic frameworks luminescence display room-temperature phosphorescence self-assembly

Observation of acoustic hybrid topological phases induced by the p-d orbital interactions

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Science China(Physics,Mechanics & Astronomy) 2025年第1期Mechanics & Astronomy) .卷 132-139页

作者： Xiao Xiang Feng Gao Yu-Gui Peng Peng wu Zong-Lin Li xue-Feng Zhu School of Physics and Innovation Institute Huazhong University of Science and Technology

In spinless systems,growing attention has recently been attracted to synthetic gauge fields,which redefine the fundamental crystal symmetries by utilizing the projective algebraic ***,synthetic gauge fields have been commonly investigated in single orbital systems,and explorations on hybrid orbitals remain elusive in ***,we report the experimental observation of hybrid topological phases induced by hybrid synthetic gauge flux,which is formed by the interaction between p and d orbitals embedded in acoustic *** breaking the translation symmetries of Lxand/or Ly,we unambiguously demonstrate the first-order M?bius edge states and higher-order corner *** work establishes a platform for seeking exotic topological phases induced by hybrid-orbitals interactions and initializing the framework of hybrid-orbitalsrelated topological *** applications can be anticipated in scenarios such as high-quality sensing and robust wave trapping due to the stepwise energy distribution of the hybrid topological phase.

关键词： topological insulator synthetic gauge field projective symmetry corner states

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矿区复垦土壤养分变化趋势研究

土壤通报 2003年第1期34卷 58-60页

作者：张乃明武雪萍谷晓滨张学涌云南农业大学资源与环境学院云南昆明650201

系统研究了孝义露天铝矿不同复垦年限的土壤养分变化 ,结果表明 :随着复垦年限的增加 ,复垦土壤有机质、全氮、有效磷均呈逐年增加趋势 ,土壤容重逐年下降 ,土壤全磷、全钾、速效钾、土壤 pH、交换量和Cu、Zn、B、Mn、Fe等微量元素的有... 详细信息

系统研究了孝义露天铝矿不同复垦年限的土壤养分变化 ,结果表明 :随着复垦年限的增加 ,复垦土壤有机质、全氮、有效磷均呈逐年增加趋势 ,土壤容重逐年下降 ,土壤全磷、全钾、速效钾、土壤 pH、交换量和Cu、Zn、B、Mn、Fe等微量元素的有效态含量变化不明显。研究证明通过种植牧草和大量施用有机肥和化肥 ,可加速复垦土壤的熟化、土壤理化性状逐年改善 ,土壤生产力逐年提高。

关键词：矿区复垦土壤养分变化趋势土壤肥力

Dynamic Regulation of Hydrogen Bonding Networks and Solvation Structures for Synergistic Solar‑Thermal Desalination of Seawater and Catalytic Degradation of Organic Pollutants

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Nano-Micro Letters 2025年第2期17卷 548-565页

作者： ming‑Yuan Yu Jing wu Guang Yin Fan‑Zhen Jiao Zhong‑Zhen Yu Jin Qu Beijing Key Laboratory of Advanced Functional Polymer Composites Beijing University of Chemical TechnologyBeijing 100029People’s Republic of China State Key Laboratory of Organic‑Inorganic Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029People’s Republic of China

Although solar steam generation strategy is efficient in desalinating seawater,it is still challenging to achieve continuous solar-thermal desalination of seawater and catalytic degradation of organic ***,dynamic regulations of hydrogen bonding networks and solvation structures are realized by designing an asymmetric bilayer membrane consisting of a bacterial cellulose/carbon nanotube/Co_(2)(OH)_(2)CO_(3)nanorod top layer and a bacterial cellulose/Co_(2)(OH)_(2)CO_(3)nanorod(BCH)bottom ***,the hydrogen bonding networks inside the membrane can be tuned by the rich surface–OH groups of the bacterial cellulose and Co_(2)(OH)_(2)CO_(3)as well as the ions and radicals in situ generated during the catalysis ***,both SO_(4)^(2−)and HSO_(5)−can regulate the solvation structure of Na^(+)and be adsorbed more preferentially on the evaporation surface than Cl^(−),thus hindering the de-solvation of the solvated Na^(+)and subsequent nucleation/growth of ***,the heat generated by the solar-thermal energy conversion can accelerate the reaction kinetics and enhance the catalytic degradation *** work provides a flow-bed water purification system with an asymmetric solar-thermal and catalytic membrane for synergistic solar thermal desalination of seawater/brine and catalytic degradation of organic pollutants.

关键词： Solar steam generation Seawater desalination Catalytic degradation Bacterial cellulose Cobalt hydroxycarbonate nanorods

Resting-state brain network remodeling after different nerve reconstruction surgeries:a functional magnetic resonance imaging study in brachial plexus injury rats

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Neural Regeneration Research 2025年第5期20卷 1495-1504页

作者： Yunting Xiang Xiangxin Xing Xuyun Hua Yuwen Zhang Xin xue Jiajia wu Mouxiong Zheng He Wang Jianguang Xu School of Rehabilitation Science Shanghai University of Traditional Chinese MedicineShanghaiChina Engineering Research Center of Traditional Chinese Medicine Intelligent Rehabilitation Ministry of EducationShanghaiChina Department of Rehabilitation Medicine Yueyang Hospital of Integrated Traditional Chinese and Western MedicineShanghai University of Traditional Chinese MedicineShanghaiChina Department of Traumatology and Orthopedics Yueyang Hospital of Integrated Traditional Chinese and Western MedicineShanghai University of Traditional Chinese MedicineShanghaiChina Institute of Science and Technology for Brain-Inspired Intelligence Fudan UniversityShanghaiChina Key Laboratory of Computational Neuroscience and Brain-Inspired Intelligence(Fudan University) Ministry of EducationShanghaiChina Human Phenome Institute Fudan UniversityShanghaiChina

Distinct brain remodeling has been found after different nerve reconstruction strategies,including motor representation of the affected ***,differences among reconstruction strategies at the brain network level have not been *** study aimed to explore intranetwork changes related to altered peripheral neural pathways after different nerve reconstruction surgeries,including nerve repair,endto-end nerve transfer,and end-to-side nerve ***–Dawley rats underwent complete left brachial plexus transection and were divided into four equal groups of eight:no nerve repair,grafted nerve repair,phrenic nerve end-to-end transfer,and end-to-side transfer with a graft sutured to the anterior upper ***-state brain functional magnetic resonance imaging was obtained 7 months after *** independent component analysis algorithm was utilized to identify group-level network components of interest and extract resting-state functional connectivity values of each voxel within the *** in intra-network resting-state functional connectivity were compared among the *** muscle reinnervation was assessed by behavioral observation(elbow flexion)and *** results showed that alterations in the sensorimotor and interoception networks were mostly related to changes in the peripheral neural *** repair was related to enhanced connectivity within the sensorimotor network,while end-to-side nerve transfer might be more beneficial for restoring control over the affected limb by the original motor *** thalamic-cortical pathway was enhanced within the interoception network after nerve repair and end-to-end nerve *** areas related to cognition and emotion were enhanced after end-to-side nerve *** study revealed important brain networks related to different nerve *** networks may be potential targets for enhancing motor recovery.

关键词： brain functional networks end-to-end nerve transfer end-to-side nerve transfer independent component analysis nerve repair peripheral plexus injury resting-state functional connectivity

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熔化极气体保护焊引弧时间预测模型

上海交通大学学报 2009年第5期43卷 697-699,703页

作者：华学明吴毅雄张勇付延安上海交通大学焊接工程研究所上海200240 上海交通大学上海市激光制造与材料改性重点实验室上海200240

通过分析熔化极气体保护焊(GMAW)引弧过程中焊丝与工件接触处的加热过程,建立了GMAW接触引弧时间预测计算模型,并实验验证了该计算模型的准确性和可靠性.结果表明:引弧时间不仅与焊丝的热性能和电性能有关,而且与焊丝直径、引弧电流和... 详细信息

通过分析熔化极气体保护焊(GMAW)引弧过程中焊丝与工件接触处的加热过程,建立了GMAW接触引弧时间预测计算模型,并实验验证了该计算模型的准确性和可靠性.结果表明:引弧时间不仅与焊丝的热性能和电性能有关,而且与焊丝直径、引弧电流和接触电压有关;基于预测模型计算的引弧时间与实验所得引弧时间基本一致,该计算模型具有一定的准确性和可靠性,为进一步认识GMAW引弧机制以及对焊接电源引弧阶段的合理设计提供指导.

关键词：熔化极气体保护焊引弧时间预测模型

Enhancement of motor functional recovery in thoracic spinal cord injury: voluntary wheel running versus forced treadmill exercise

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Neural Regeneration Research 2025年第3期20卷 836-844页

作者： Do-Hun Lee Dan Cao Younghye Moon Chen Chen Nai-Kui Liu Xiao-ming Xu Wei wu Spinal Cord and Brain Injury Research Group Stark Neurosciences Research InstituteIndiana University School of MedicineIndianapolisINUSA Department of Neurological Surgery Indiana University School of MedicineIndianapolisINUSA Department of Neuroscience Baylor College of MedicineHoustonTXUSA

Spinal cord injury necessitates effective rehabilitation strategies, with exercise therapies showing promise in promoting recovery. This study investigated the impact of rehabilitation exercise on functional recovery and morphological changes following thoracic contusive spinal cord injury. After a 7-day recovery period after spinal cord injury, mice were assigned to either a trained group(10 weeks of voluntary running wheel or forced treadmill exercise) or an untrained group. Bi-weekly assessments revealed that the exercise-trained group, particularly the voluntary wheel exercise subgroup, displayed significantly improved locomotor recovery, more plasticity of dopaminergic and serotonin modulation compared with the untrained group. Additionally, exercise interventions led to gait pattern restoration and enhanced transcranial magnetic motor-evoked potentials. Despite consistent injury areas across groups, exercise training promoted terminal innervation of descending axons. In summary, voluntary wheel exercise shows promise for enhancing outcomes after thoracic contusive spinal cord injury, emphasizing the role of exercise modality in promoting recovery and morphological changes in spinal cord injuries. Our findings will influence future strategies for rehabilitation exercises, restoring functional movement after spinal cord injury.

关键词： behavioral assessment motor function neural plasticity running wheel exercise spinal cord injury treadmill exercise voluntary exercise

Regulation and function of endoplasmic reticulum autophagy in neurodegenerative diseases

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Neural Regeneration Research 2025年第1期20卷 6-20页

作者： Xiu-Yun Zhao De-En Xu ming-Lei wu Ji-Chuan Liu Zi-Ling Shi Quan-Hong Ma Department of Neurology and Clinical Research Center of Neurological Disease the Second Affiliated Hospital of Soochow UniversitySuzhouJiangsu ProvinceChina Institute of Neuroscience&Jiangsu Key Laboratory of Translational Research and Therapy for Neuro-Psycho-Diseases Soochow UniversitySuzhouJiangsu ProvinceChina Department of Neurology Jiangnan University Medical CenterWuxiJiangsu ProvinceChina

The endoplasmic reticulum,a key cellular organelle,regulates a wide variety of cellular *** reticulum autophagy,one of the quality control systems of the endoplasmic reticulum,plays a pivotal role in maintaining endoplasmic reticulum homeostasis by controlling endoplasmic reticulum turnover,remodeling,and *** this review,we briefly describe the endoplasmic reticulum quality control system,and subsequently focus on the role of endoplasmic reticulum autophagy,emphasizing the spatial and temporal mechanisms underlying the regulation of endoplasmic reticulum autophagy according to cellular *** also summarize the evidence relating to how defective or abnormal endoplasmic reticulum autophagy contributes to the pathogenesis of neurodegenerative *** summary,this review highlights the mechanisms associated with the regulation of endoplasmic reticulum autophagy and how they influence the pathophysiology of degenerative nerve *** review would help researchers to understand the roles and regulatory mechanisms of endoplasmic reticulum-phagy in neurodegenerative disorders.

关键词： autophagy endoplasmic reticulum endoplasmic reticulum autophagy endoplasmic reticulum quality control system endoplasmic reticulum receptors endoplasmic reticulum-associated degradation neurodegeneration neurodegenerative disease selective autophagy unfolded protein response