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Effect of rare earth on physical properties of Na_(0.5)Bi_(0.5)TiO_(3)system:A density functional theory investigation

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Journal of Rare Earths 2022年第3期40卷 473-481,I0005页

作者： Manal Benyoussef Halima Zaari Jamal Belhadi Youssef el Amraoui Hamid Ez-Zahraouy Abdelilah Lahmar mimoun el marssi Laboratory of Physics of Condensed Matter(LPMC) University of Picardie Jules VerneScientific Pole80039Amiens Cedex 1France Laboratory of Condensed Matter and Indisciplinary Science(LaMCScI) Faculty of ScienceMohammed V UniversityBP 1014RabatMorocco National School of Arts and Crafts Moulay Ismail University50500MeknesMorocco

Na_(0.5)(Bi_(3/4)RE_(1/4))_(0.5)TiO_(3)(RENBT,RE=Nd,Gd,Dy,and Ho)compounds were investigated in the framework of first-principles calculations using the full potential linearized augmented plane wave(FP-LAPW)method based on the spin-polarized density functional theory implemented in the WIEN2k *** charge density distribution and Ti K-edge X-ray absorption spectra reveal that the RENBT compositions with high polarization values are accompanied by a higher TiO_(6)distortion,DyNBT,and NdNBT *** effect of the rare-earth elements on the polarization is confirmed experimentally with the collection of the hysteresis *** investigation of the electronic properties of the compounds highlights the emergence of a magnetization owing to the 4f orbital effect of the rare-earth ***,the investigation of the chemical ordering shows a short-range chemical ordering for the pure composition and an increased A-site disorder for dysprosium doped NBT *** increased disorder may speak for increased relaxor properties in the RE doped compositions.

关键词： Density functional theory Sodium bismuth titanate Rare earths A-site ordering Ferroelectric properties Magnetization

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Novel lead-free BCZT-based ceramic with thermally-stable recovered energy density and increased energy storage efficiency

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Journal of Materiomics 2022年第4期8卷 873-881页

作者： Zouhair Hanani Soukaina Merselmiz M'barek Amjoud Daoud Mezzane Mohammed Lahcini Jaafar Ghanbaja Matjaz Spreitzer Damjan Vengust mimoun el marssi Igor A.Luk'yanchuk Zdravko Kutnjak Brigita Rozic Mohamed Goune IMED-Lab Cadi Ayyad UniversityAvenue Abdelkrim El KhattabiP.B.549Marrakesh40000Morocco ICMCB University of Bordeaux87 Avenue Du Dr Albert SchweitzerPessac33600France Jozef Stefan Institute Jamova Cesta 39Ljubljana1000Slovenia LPMC University of Picardy Jules Verne33 Rue Saint LeuAmiens80039France Mohammed VI Polytechnic University Lot 660-Hay Moulay RachidBen Guerir43150Morocco IJL University of Lorraine54000NancyFrance Department of Building Materials Kyiv National University of Construction and ArchitectureKyiv03680Ukraine

The eco-responsible lead-free piezoelectric ceramics have been intensively searched for more than adecade, however, the final goal to replace toxic ceramics like lead zirconate titanate (PZT) with lead-freecompounds, having comparable or even better performance has not yet been reached. In this road, thelead-free ceramics Ba_(0.85)Ca_(0.15)Zr_(0.1)Ti_(0.9)O_(3) (BCZT), possessing excellent dielectric, ferroelectric, andpiezoelectric properties are regarded as serious candidates for the PZT replacement. Besides, nano-structuring BCZT is of paramount importance to enhance these functionalities even more. Here, BCZTmultipodes are designed by template-growth hydrothermal synthesis using hydrogen zirconate titanatenanowires. We demonstrate that the fabricated BCZT multipodes exhibit high dielectric permittivity of5300 with a temperature stability coefficient of ±5.9% between 20 and 140℃. A significant recoveredenergy density of 315.0 mJ/cm^(3) with high thermal stability and high energy storage efficiency of 87.4%,and enhanced large-signal piezoelectric coefficient d^(*)_(33) (310 pm/V) are found. Compared to the tradi-tional BCZT ceramics reported in the literature, relying on high-temperature processing, our sampleexhibits boosted energy storage parameters at a much lower temperature. These outcomes may offer anew strategy to tailor eco-responsible relaxor ferroelectrics toward superior energy storage performancefor ceramic capacitor applications.

关键词： Lead-free ceramics Low temperature Piezoelectric Thermal stability Energy storage Nanostructuration

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Enhanced dielectric and electrocaloric properties in lead-free rod-like BCZT ceramics

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Journal of Advanced Ceramics 2020年第2期9卷 210-219页

作者： Zouhair HANANI Soukaina MERSelMIZ Abdelaadim DANINE Nicolas STEIN Daoud MEZZANE M’barek AMJOUD Mohammed LAHCINI Yaovi GAGOU Matjaz SPREITZER Damjan VENGUST Zdravko KUTNJAK mimoun el marssi Igor ALUK'YANCHUK Mohamed GOUNE IMED-Lab Cadi Ayyad UniversityMarrakesh 40000Morocco ICMCB University of 1.BordeauxPessac 33600France IJL University of LorraineNancy 54000France UM6P Ben Guerir 43150Morocco LPMC University of Picardy Jules VerneAmiens 80039France Jozef Stefan Institute Ljubljana 1000Slovenia Physics Faculty Southern Federal UniversityRostov-on-Don 344090Russia

Ba0.85Ca0.15Zr0.10Ti0.90O3(BCZT)lead-free ceramics demonstrated excellent dielectric,ferroelectric,and piezoelectric properties at the morphotropic phase boundary(MPB).So far,to study the effect of morphological changes on dielectric and ferroelectric properties in lead-free BCZT ceramics,researchers have mostly focused on the influence of spherical grain shape *** this study,BCZT ceramics with rod-like grains and aspect ratio of about 10 were synthesized by surfactant-assisted solvothermal route.X-ray diffraction(XRD)and selected area electron diffraction(SAED)performed at room temperature confirm the crystallization of pure perovskite with tetragonal *** electron microscopy(SEM)image showed that BCZT ceramics have kept the 1D rod-like grains with an average aspect ratio of about ***-like BCZT ceramics exhibit enhanced dielectric ferroelectric(εr=11,906,tanδ=0.014,Pr=6.01μC/cm^2,and Ec=2.46 kV/cm),and electrocaloric properties(ΔT=0.492 K andz=0.289(K×mm)/kV at 17 kV/cm)with respect to spherical BCZT ***,rod-like BCZT lead-free ceramics have good potential to be used in solid-state refrigeration technology.

关键词： lead-free Ba0.85Ca0.15Zr0.10Ti0.90O3(BCZT) rod-like Ba0.85Ca0.15Zr0.10Ti0.90O3(BCZT) dielectric ferroelectric electrocaloric effect

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Er3+and Er3+/Yb3+Ions Embedded in Nano-Structure BaTi0.9Sn0.1O3: Structure, Morphology and Dielectric Properties

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World Journal of Nano Science and Engineering 2021年第2期11卷 25-43页

作者： Olfat el Sayed Inas Battisha Abdelilah Lahmar mimoun el marssi Physics Department Faculty of Women for Arts Science and Education Ain Shams University Cairo Egypt Solid State Physics Department Physics Research Division National Research Centre Dokki Giza Egypt Laboratory of Condensed Matter Physics (LPMC) University of Picardie Jules Verne Amiens France

Barium titanate tin oxides BaTi0.9Sn0.1O3 referred to as (BTSO) doped with 0.5Er3+ and co-doped with (0.75 and 1) Yb3+ ions, were prepared using a modified sol-gel method and calcinated at 1050?C in the air for 4 h. The influence of the selected rare earth element on the structure morphology, dielectric properties behavior was investigated. From TEM micrographs, it has appeared that the particles have a spherical shape with a small size in nanoscale. The average particle size is determined both by TEM and XRD diffraction was found to be in agreement and within the range between 45.9 and 57.7 nm. The effects of Lanthanide incorporation on the evolution of these nano-crystalline structures were followed by XRD and (FTIR). The XRD patterns give rise to a single perovskite phase, while the tetragonality was found to decrease gradually with Er3+ and Er3+/Yb3+ ions, respectively. FTIR results showed enhancement of the crystallinity and the absence of carbonates upon increasing Yb3+ ions concentration from 0.75 up to 1 mol%. The dielectric and conductivity properties were found to be enhanced by the nature and the concentration of the lanthanide element (Er3+, Yb3+) in the BTSO host lattice. The Curie temperature (Tc) shifted to a lower value from 117 for BTSO: 0.5Er to 93 for BTSO: 0.5Er/1Yb and the permittivity ε’ increased from 3972 to 6071, so BTSO: 0.5Er/1Yb good crystalline material candidate for capacitors application due to its higher permittivity.

关键词： Sol-Gel Nano-Structure BaTiSnO3-Doped “Er3+ Ion” or “Er3+/Yb3+ Ion” Dielectric Properties

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Attenuation of coda waves in the SW of High-Atlas area, Morocco

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Geodesy and Geodynamics 2019年第4期10卷 297-306页

作者： Roumaissae Azguet Ghizlane Bouskri Youssef Timoulali mimoun Harnafi Younes el.Fellah Scientific Institute Mohamed V University in RabatMorocco Faculty of Science Mohammed V University in RabatMorocco Rural Engineering Department Institut agronomique et veterinaire hassan IIRabatMorocco

We investigate attenuation scattering and loss properties in Souss basin(SW of High-Atlas) as a transition zone between the High and Anti Atlas ranges. This district consists in a thinned crustal patch with shallow seismicity and loose sedimentary trenches that perform an important contribution to augment seismic attenuation. So far, no coda waves approach in our knowledge have been used to draw satisfying outputs about the attenuation properties in the region. Therefore, this update suggests to correlate the lateral changes of seismic attenuation to different characteristics and asperities i.e. seismic activity,crustal age and thickness, heat flow, and ground deformation rate. To do so, we analysed coda waves derived from waveform data of more than 23 local earthquakes from seven broadband seismometers recorded during 2010 e2012 period. As a starter, we utilized the backscattering model which defines theseismic attenuation as inversely proportional to quality factor by the equation A ?1=. QQcestimates c were deducted at various central frequency bands 1.5, 3.0, 6.0, 9.0, 12.0 and 18.0 Hz according to different lapses times. The estimated average frequency dependence quality factor gives relation Qc? 120 f1;01,while the average Qcvalues vary from 149 at 1.5 Hz to 1895 at 18 Hz central frequencies. We observed an intimate dependence between quality factor and frequency ranges, which reflects the complexity of geological/geophysical pattern in the Souss basin and the presence of a variety of heterogeneities within the underlying crust.

关键词： Attenuation Coda waves Quality factor Frequency Souss basin Morocco

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Spatial variation of coda wave attenuation using aftershocks of the Al Hoceima earthquake of 24 February, 2004, Morocco

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Natural Science 2013年第8期5卷 72-77页

作者： Abderrahim Boulanouar Lahcen el Moudnib mimoun Harnafi Taj-Eddine Cherkaoui Abdelaali Rahmouni Mohamed Boukalouch Jamal Sebbani Earth Science Department Scientific Institute Mohammed V University-Agdal Rabat Morocco Physics Department Faculty of Science Mohammed V University-Agdal Rabat Morocco Physics Department Faculty of Science Mohammed V University-Agdal Rabat Morocco Earth Science Department Scientific Institute Mohammed V University-Agdal Rabat Morocco

On 24th February 2004 a significant earthquake (Md = 6.4) occurred in the north of Moroccocausing great damage in the vicinity of Al Hoceima region. This area is characterized by a complex faulting system as a result of compressional tectonic forces. Three short period seismic stations are set in this area of interest and recordings from these stations were used in this study. In order to complete our knowledge of attenuation, 60 local earthquakes are recorded a few days after the great earthquake with magnitude Ml 2.6 - 5.0 to estimate seismic attenuation. For this purpose, we applied the single backscattering model of Aki & Chouet 1975 inthe frequency range for 1 to 8 Hz. The study of coda waves was limited to a relatively short lapse time (20 Seconds) in order to sample the earth’s crust only. The values of Qc estimated for all the three stations show a strong frequency dependent relationship of the form Qc = Q0fn, where Q0 is Qc at 1 Hz , and n represents the degree of frequency dependence, and reflects the level of crustal heterogeneities to varying degrees. The average frequency dependent attenuation relationship has been obtained which indicates that the attenuation is high in this region. Finally to conclude our work, the values of Q0 suggest that Al Hoceima area is highly heterogeneous and the n parameter indicates a meaning frequency dependence of Qc.

关键词： Attenuation Coda Waves Single Backscattering Model Al Hoceima Morocco Seismic Earthquake

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