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Synthesis and Spectroscopic Properties of Ferrocenyl Derivative Containing Donor and Acceptor Groups

International Journal of Organic Chemistry 2017年第3期7卷 284-294页

作者： Makoto Minato Chiharu Sorai Takashi Ito Masashi Kiguchi midori kato Department of Materials Chemistry Faculty of Engineering Yokohama National University Yokohama Japan Advanced Research Laboratory Hitachi Ltd. Hatoyama Japan

Much interest has been devoted to organometallic NLO materials. We have become interested in exploring the utility of ferrocenyl group as the conjugating bridge. Thus, we synthesized 1-{{[1,3-(5-methylbenzo)dithiol]-2-yli- dene}methyl}-1’-[2-(p-nitrophenyl)-(E)-ethenyl]ferrocene (1). This new ferrocenyl compound has a donor and an acceptor group in 1,1’-positions. Investigations of the solvatochromic property of the compound revealed that it has polarized structure in a polar solvent, such as DMF. SHG efficiency of the compound was estimated by an SHEW (second-harmonic generation with the evanescent wave) method.

关键词： Nonlinear Optical Material Ferrocenyl Derivative Solvatochromic Property SHG Efficiency

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Model of the Effects of Improving TB Diagnosis on Infection Dynamics in Differing Demographic and HIV-Prevalence Scenarios

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Journal of Tuberculosis Research 2015年第1期3卷 1-10页

作者： Allison S. Rhines midori kato-Maeda Marcus W. Feldman Department of Biology Stanford University Stanford USA Curry International Tuberculosis Center Division of Pulmonary and Critical Care Medicine University of California San Francisco USA

This paper seeks to examine the sensitivity of tuberculosis transmission (TB) dynamics to the rate at which infectious individuals with active TB begin a TB treatment course, and therefore cease to be infectious to others. We model this by varying both the rate at which individuals are diagnosed and begin treatment, and the demographic conditions in which the epidemic occurs. An agestructured deterministic ordinary differential equation model is used to study the sensitivity of TB transmission dynamics to the implementation of a more effective diagnostic such as Xpert MTB/ RIF in a high HIV prevalence setting. Sensitivity analysis of the effectiveness of the diagnostic (λ) shows the interim disease dynamics in three demographic scenarios defined by differences in HIV prevalence and age structure at a constant transmission rate. In the near future, we expect the diagnostic to have the most effect in areas of high HIV prevalence. In the long term, we expect the diagnostic to have the most significant impact at high transmission rates regardless of HIV prevalence and age structure.

关键词： Tuberculosis Diagnostics Xpert MTB/RIF TB/HIV Co-Infection Demography

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Thrombomodulin in the management of acute cholangitisinduced disseminated intravascular coagulation

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World Journal of Gastroenterology 2015年第2期21卷 533-540页

作者： Keigo Suetani Chiaki Okuse Kazunari Nakahara Yosuke Michikawa Yohei Noguchi midori Suzuki Ryo Morita Nozomi Sato Masaki kato Fumio Itoh Department of Gastroenterology and Hepatology St.Marianna UniversitySchool of MedicineKawasaki 216-8511Japan

AIM: To evaluate the need for thrombomodulin(r TM) therapy for disseminated intravascular coagulation(DIC) in patients with acute cholangitis(AC)-induced DIC. METHODS: Sixty-six patients who were diagnosedwith AC-induced DIC and who were treated at our hospital were enrolled in this study. The diagnoses of AC and DIC were made based on the 2013 Tokyo Guidelines and the DIC diagnostic criteria as defined by the Japanese Association for Acute Medicine, respectively. Thirty consecutive patients who were treated with r TM between April 2010 and September 2013(r TM group) were compared to 36 patients who were treated without r TM(before the introduction of r TM therapy at our hospital) between January 2005 and January 2010(control group). The two groups were compared in terms of patient characteristics at the time of DIC diagnosis(including age, sex, primary disease, severity of cholangitis, DIC score, biliary drainage, and anti-DIC drugs), the DIC resolution rate, DIC score, the systemic inflammatory response syndrome(SIRS) score, hematological values, and outcomes. Using logistic regression analysis based on multivariate analyses, we also examined factors that contributed to persistent DIC. RESULTS: There were no differences between the r TM group and the control group in terms of the patients' backgrounds other than administration. DIC resolution rates on day 9 were higher in the r TM group than in the control group(83.3% vs 52.8%, P < 0.01). The mean DIC scores on day 7 were lower in the r TM group than in the control group(2.1 ± 2.1 vs 3.5 ± 2.3, P = 0.02). The mean SIRS scores on day 3 were significantly lower in the r TM group than in the control group(1.1 ± 1.1 vs 1.8 ± 1.1, P = 0.03). Mortality on day 28 was 13.3% in the r TM group and 27.8% in the control group; these rates were not significantly different(P = 0.26). Multivariate analysis identified only the absence of biliary drainage as significantly associated with persistent DIC(P < 0.01, OR = 12, 95%CI: 2.

关键词： Disseminated intravascular coagulation Acute chola

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Helix Induction to Polysilane Chain Upon Wrapping by Sugar Derivatives and Related Chemistry

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复旦学报（自然科学版） 2007年第5期46卷 618-619页

作者： M.Tanaka T.Sanji Nobu kato Y.Sato Chemical Resources Laboratory Tokyo Institute of Technology 4259-R1-13 NagatsutaMidori-ku Yokohama 226-8503Japan

1 Results Helix induction to polymer chains is an active area of research these days. In most cases,optically-active units are attached to the polymers to induce helical conformation. Scheme 1Since the properties of σ-conjugated polymers like polysilanes are dependent on the conformation of the chain,it is particularly interesting to induce helix to oligo-and polysilanes. We have been working on the helix induction by host-guest complexation with sugar derivatives such as cyclodextrine and *** l...

关键词： polysilane inclusion complex helix supramolecular chemistry

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