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Spectroscopic investigations on the effect of humic acid on the formation and solubility of secondary solid phases of Ln_2(CO_3)_3

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Journal of Rare Earths 2011年第6期29卷 516-521页

作者： Stella Antoniou Ioannis Pashalidis Andre Gessner michael U Kumke Department of Chemistry University of Cyprus P.O. Box 20537 1678 Nicosia Cyprus Chemistry Department/Physical Chemistry University of Potsdam Karl- Liebknecht-Str. 24-25 14476 Potsdam-Golm Germany

The formation of secondary Ln（III） solid phases （e.g., Nd2（CO3）3 and sm2（CO3）3） was studied as a function of the humic acid concentration in 0.1 mol/L NaClO4 aqueous solution in the neutral pH range （5–6.5）. The solid phases under investigation were prepared by alkaline precipitation under 100% CO2 atmosphere and characterized by attenuated total reflectance Fourier transform infrared spectroscopy （ATR-FTIR）, X-ray diffraction （XRD）, time-resolved laser fluorescence spectroscopy （TRLFS）, diffuse reflectance ultraviolet-visible （DR-UV-Vis）, Raman spectroscopy, and solubility measurements. The spectroscopic data obtained indicated that Nd2（CO3）3 and sm2（CO3）3 were stable and remained the solubility limiting solid phases even in the presence of increased humic acid concentration （0.5 g/L） in solution. Upon base addition in the Ln（III）-HA system, decomplexation of the previously formed Ln（III）-humate complexes and precipitation of two distinct phases occurred, the inorganic （Ln2（CO3）3） and the organic phase （HA）, which was adsorbed on the particle surface of the former. Nevertheless, humic acid affected the particle size of the solid phases. Increasing humic acid concentration resulted in decreasing crystallite size of the Nd2（CO3）3 and increasing crystallite size of the sm2（CO3）3 solid phase, and affected inversely the solubility of the solid phases. However, this impact on the solid phase properties was expected to be of minor relevance regarding the chemical behavior and migration of trivalent lanthanides and actinides in the geosphere.

关键词： lanthanide ions humic acid solid phase solubility Raman TRLFS DR-UV-Vis rare earths

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A Periglacial Palaeoenvionment in the Upper Carboniferous-Lower Permian Tobra Formation of the Salt Range,Pakistan

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Acta Geologica Sinica(English Edition) 2017年第3期91卷 1063-1078页

作者： Irfan U.JAN Shahid IQBAL Sarah J.DA VIES Jan A.ZALASIEWICZ michael H.STEPHENSON michael WAGREICH Muhammad HANEEF Muhammad HANIF Sajjad AHMAD National Centre of Excellence in Geology University of Peshawar Department of Earth Sciences Quaid-i-Azam University Islamabad Department of Geodynamics and Sedimentology University of Vienna Department of Geology University of Leicester British Geological Survey Department of Earth Sciences Comsats Institute of Technology Abbottabad Department of Geology University of Peshawar

The Upper Carboniferous-Lower Permian （Upper Pennsylvanian-Asselian） Tobra Formation is exposed in the Salt and Trans Indus ranges of Pakistan. The formation exhibits an alluvial plain （alluvial fan-piedmont alluvial plain） facies association in the Salt Range and Khisor Range. In addition, a stream flow facies association is restricted to the eastern Salt Range. The alluvial plain facies association is comprised of clast-supported massive conglomerate （Gmc）, diamictite （Dm） facies, and massive sandstone （sm） iithofacies whereas the stream flow-dominated alluvial plain facies association includes fine-grained sandstone and sUtstone （Fss）, fining upwards pebbly sandstone （Sf）, and massive mudstone （Fro） lithofacies. The lack of glacial signatures （particularly glacial grooves and striations） in the deposits in the Tobra Formation, which are, in contrast, present in their time-equivalent and palaeogeographically nearby strata of the Arabian peninsula, e.g. the Al Khlata Formation of Oman and Unayzah B member of the Sandi Arabia, suggests a pro-to periglacial, i.e. glaciofluvial depositional setting for the Tobra Formation. The sedimentology of the Tobra Formation attests that the Salt Range, Pakistan, occupied a palaeogeographic position just beyond the maximum glacial extent during Upper Pennsylvanian-Asselian time.

关键词： Pennsylvanian-Asselian Tobra Formation Salt Range Khisor Range glaciofluvial Pakistan

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‘Outbreak Gold Standard’Selection to Provide Optimized Threshold for Infectious Diseases Early-alert Based on China Infectious Disease Automated-alert and Response System

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Journal of Huazhong University of Science and Technology(Medical Sciences) 2017年第6期37卷 833-841页

作者：王瑞平姜永根赵根明郭晓芹 Engelgau michael School of Public Health Fudan UniversityShanghai 200032China Songjiang Center for Disease Control and Prevention Shanghai 201620China Center for Disease Control and Prevention Atlanta 30329-4027USA

The China Infectious Disease Automated-alert and Response System（CIDARS） was successfully implemented and became operational nationwide in 2008. The CIDARS plays an important role in and has been integrated into the routine outbreak monitoring efforts of the Center for Disease Control（CDC） at all levels in China. In the CIDARS, thresholds are determined using the ？Mean＋2SD？ in the early stage which have limitations. This study compared the performance of optimized thresholds defined using the ？Mean ＋2SD？ method to the performance of 5 novel algorithms to select optimal ？Outbreak Gold Standard（OGS）？ and corresponding thresholds for outbreak detection. Data for infectious disease were organized by calendar week and year. The ？Mean＋2 SD？, C1, C2, moving average（MA）, seasonal model（sm）, and cumulative sum（CUSUM） algorithms were applied. Outbreak signals for the predicted value（Px） were calculated using a percentile-based moving window. When the outbreak signals generated by an algorithm were in line with a Px generated outbreak signal for each week, this Px was then defined as the optimized threshold for that algorithm. In this study, six infectious diseases were selected and classified into TYPE A（chickenpox and mumps）, TYPE B（influenza and rubella） and TYPE C [hand foot and mouth disease（HFMD） and scarlet fever]. Optimized thresholds for chickenpox（P_（55））, mumps（P_（50））, influenza（P_（40）, P_（55）, and P_（75））, rubella（P_（45） and P_（75））, HFMD（P_（65） and P_（70））, and scarlet fever（P_（75） and P_（80）） were identified. The C1, C2, CUSUM, sm, and MA algorithms were appropriate for TYPE A. All 6 algorithms were appropriate for TYPE B. C1 and CUSUM algorithms were appropriate for TYPE C. It is critical to incorporate more flexible algorithms as OGS into the CIDRAS and to identify the proper OGS and corresponding recommended optimized threshold by different infectious disease types.

关键词： outbreak gold standard optimized threshold algorithms early-alert signal China Infectious Disease Automated-alert and Response System

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Passive expansion of sub-maximally dilated transjugular intrahepatic portosystemic shunts and assessment of clinical outcomes

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World Journal of Hepatology 2017年第12期9卷 603-612页

作者： michael C Hsu Charles N Weber S William Stavropoulos Timothy W Clark Scott O Trerotola Richard D Shlansky Goldberg michael C Soulen Gregory J Nadolski Department of Radiology Division of Interventional RadiologyMount Sinai Hospital Department of Radiology Division of Interventional RadiologyHospital of the University of Pennsylvania

AIM To assess for passive expansion of sub-maximally dilated transjugular intrahepatic portosystemic shunts(TIPS) and compare outcomes with maximally dilated *** Polytetrafluoroethylene covered TIPS(Viatorr) from July 2002 to December 2013 were retrospectively reviewed at two hospitals in a single institution. Two hundred and thirty patients had TIPS maximally dilated to 10 mm(m TIPS), while 43 patients who were at increased risk for hepatic encephalopathy(HE), based on clinical evaluation or low pre-TIPS portosystemic gradient(PSG), had 10 mm TIPS sub-maximally dilated to 8 mm(sm TIPS). Group characteristics(age, gender, Model for End-Stage Liver Disease score, post-TIPS PSG and clinical outcomes were compared between groups, including clinical success(ascites or varices), primary patency,primary assisted patency, and severe post-TIPS HE. A subset of fourteen patients with sm TIPS underwent follow-up computed tomography imaging after TIPS creation, and were grouped based on time of imaging( 6 mo). Change in diameter and crosssectional area were measured with 3D imaging software to evaluate for passive *** Patient characteristics were similar between the sm TIPS and m TIPS groups, except for pre-TIPS portosystemic gradient, which was lower in the sm TIPS group(19.4 mm Hg ± 6.8 vs 22.4 mm Hg ± 7.1, P = 0.01). Primary patency and primary assisted patency between sm TIPS and m TIPS was not significantly different(P = 0.64 and 0.55, respectively). Four of the 55 patients(7%) with sm TIPS required TIPS reduction for severe refractory HE, while this occurred in 6 of the 218 patients(3%) with m TIPS(P = 0.12). For the 14 patients with follow-up computed tomography(CT) imaging, the median imaging follow-up was 373 d. There was an increase in median TIPS diameter, median percent diameter change, median area, and median percent area change in patients with CT follow-up greater than 6 mo after TIPS placement compared to follow-up within 6 mo(

关键词： Variceal hemorrhage Portal hypertension Transjugular intrahepatic portosystemic shunts Ascites Sub-maximal dilation Underdilated Passive expansion Hepatic encephalopathy

A Cytogenetic Analysis of Enteromius parablabes (Daget, 1957) from Aho Stream, Ile-Ife, Nigeria

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Open Journal of Genetics 2022年第3期12卷 25-32页

作者： michael Olaoluwa Popoola Oluwatomisin Awe Idowu Isaac Adeniran Department of Zoology Obafemi Awolowo University Ile-Ife Nigeria

In this study, Enteromius parablabes [1] was analyzed with the aim of providing baseline information regarding the diploid chromosome number and karyotype differences of both sexes. The diploid chromosome number (2n) was 50 for both sexes, and this corresponds to the diploid chromosome number reported for most small African Barbus species. The fundamental number (NFa) of the male and female was 81 and 98 respectively. The first pair of metaphase chromosomes which has been suggested to be a marker for the small African Barbus group was conspicuously larger in the female karyotype. The karyotype of the female consisted more of metacentric (39m + 7sm + 2st + 2t) which is common in the group while the karyotype of the male which consisted more of telocentric chromosomes (10m + 21st + 19T) is scarce. The chromosomal number obtained for E. parablabes demonstrates its diploid status in the context of the ploidy lines characteristic of the African Barbus assemblage.

关键词： Karyotype Barbus Taxonomy Africa Chromosome

Neural EGF-like protein 1(NELL-1):Signaling crosstalk in mesenchymal stem cells and applications in regenerative medicine

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Genes & Diseases 2017年第3期4卷 127-137页

作者： Mikhail Pakvasa Alex Alverdy Sami Mostafa Eric Wang Lucy Fu Alexander Li Leonardo Oliveira Aravind Athiviraham michael J.Lee Jennifer Moriatis Wolf Tong-Chuan He Guillermo A.Ameer Russell R.Reid The University of Chicago Pritzker School of MedicineChicagoIL 60637USA Laboratory of Craniofacial Biology and Development Section of Plastic and Reconstructive SurgeryDepartment of SurgeryThe University of Chicago Medical CenterChicagoIL 60637USA Rosalind Franklin University Chicago Medical SchoolNorth ChicagoIL 60064USA Molecular Oncology Laboratory Department of Orthopaedic Surgery and Rehabilitation MedicineThe University of Chicago Medical CenterChicagoIL 60637USA Department of Biomedical Engineering Northwestern UniversityEvanstonIL 60208USA Center for Advanced Regenerative Engineering Northwestern UniversityEvanstonIL 60208USA Department of Surgery Feinberg School of MedicineNorthwestern UniversityChicagoIL 60611USA

Bone tissue regeneration holds the potential to solve both osteoporosis and large skeletal defects,two problems associated with significant *** differentiation of mesenchymal stem cells into the osteogenic lineage requires a specific microenvironment and certain osteogenic growth *** EGF Like-Like molecule 1(NELL-1)is a secreted glycoprotein that has proven,both in vitro and in vivo,to be a potent osteo-inductive ***,it has been shown to repress adipogenic differentiation and ***-1 can work synergistically with other osteogenic factors such as Bone Morphogenic Protein(BMP)2 and9,and has shown promise for use in tissue engineering and as a systemically administered drug for the treatment of *** we provide a comprehensive up-to-date review on the molecular signaling cascade of NELL-1 in mesenchymal stem cells and potential applications in bone regenerative engineering.

关键词： Bone tissue engineering Mesenchymal stem cells NELL-1 NEL-like protein 1 Osteogenic differentiation

Genotype-Specific Microsatellite (SSR) Markers for the Sugarcane Germplasm from the Karst Region of Guizhou, China

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American Journal of Plant Sciences 2016年第15期7卷 2209-2220页

作者： Yuhua Fu Yongbao Pan Chaoyun Lei michael P. Grisham Chenglong Yang Qiuyi Meng Guizhou Institute of Subtropical Crops Guizhou Academy of Agricultural Sciences Xingyi Guizhou China Sugarcane Research Unit Southeast Area USDA-ARS Houma LA USA

Genetic variability among sugarcane genotypes from the Karst region of China was evaluated using genotype-specific microsatellite (SSR) markers. Eighteen sugarcane genotypes including 13 active cultivars and five elite QT-series clones bred locally were screened for genetic variability with 21 SSR primer pairs. All the primer pairs were highly polymorphic and amplified a total of 167 alleles with an average of eight alleles per primer pair. The average polymorphism information content (PIC) value was 0.86 with a range of 0.68 and 0.92. A UPGMA dendrogram categorized the 18 sugarcane genotypes into three major groups containing three, ten and five genotypes, respectively. No geographical affinity was observed among genotypes within the same group. Eight SSR primer pairs produced cultivar-specific alleles, of which five alleles were unique to the QT-series clones, namely, smC334BS-165 and smC851MS-145 in QT 08-558, mSSCIR43-229 in QT 4, sm597CS-182 in QT 08-536 and smC7CUQ-168 in QT 06-212. The clone-specific SSR alleles will be useful in identifying elite QT-series clones for use in the sugarcane crossing programs in China.

关键词： Sugarcane Clone-Specific SSR Markers Genetic Diversity Karst Region

Rural congestive heart failure mortality among US elderly, 1999-2013: Identifying counties with promising outcomes and opportunities for implementation research

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Family Medicine and Community Health 2015年第2期3卷 27-38页

作者： Maria C.Mejia de Grubb Robert S.Levine Barbara Kilbourne Baqar A.Husaini Tyler Skelton Lisa Gittner michael A.Langston George E.Rust Department of Family and Community Medicine Baylor College of MedicineHoustonTXUSA Department of Sociology Tennessee State UniversityNashvilleTennesseeUSA Center for PreventionResearch Tennessee State University College of AgricultureNashvilleTennesseeUSA Department of Political Science Texas Tech UniversityLubbockTXUSA Department of Electrical Engineering and Computer Science University of TennesseeKnoxvilleTennesseeUSA Department of Family Medicine National Center for Primary CareMorehouse School of MedicineAtlantaGeorgiaUSA

Objective:Describe modern trends in congestive heart failure(CHF)among elderly(>65 years of age)in the United States,to identify potentially successful rural *** CHF mortality using multiple-(MCOD)versus underlying-(UCOD)cause of death ***:*** for Disease Control and Prevention mortality files(WONDER internet site).Results:Using MCOD data,overall mortality rates/100,000 population(and 95%confidence intervals)for CHF among persons>65 years of age(1999-2013)were 482.0(481.2-482.8)for large central and large fringe metropolitan(LCLF)counties,549.6(548.6-550.7)in small and medium metropolitan(sm)counties,and 652.6(650.9-654.0)in micropolitan and non-core,non-metropolitan(MNCNM)*** positive deviance NCNM counties(collectively including 198,581 residents>65 years of age)had an overall CHF rate of 300.9(275.0-326.9)in *** was significantly lower than the LCLF rate for 2013(482.0[481.2-482.8]),and rep-resented a reduction of 47%since *** CHF occurrence as estimated with MCOD was 3.4-fold higher than that obtained with ***:These data illustrate underestimation of CHF by UCOD data and the importance of correct death *** CHF mortality rates are higher than urban rates,but some positive deviance counties demonstrate that this is not *** research is needed to understand the relative contribution of research innovation,medical care,and public health to rural-urban disparities and the relative success of positive deviance counties.

关键词： Congestive heart failure elderly mortality rural

QUASI STEADY-STATE HURRICANES REVISITED

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Tropical Cyclone Research and Review 2019年第1期8卷 1-17页

作者： JOHN PERSING michael T.MONTGOMERY ROGER K.smITH JAMES C.MCWILLIAMS Department of Meteorology Naval Postgraduate School Meteorological Institute Ludwig-Maximilians University of Munich Department of Atmospheric and Oceanic Sciences University of California at Los Angeles

We revisit the theoretical possibility of long-term, sustained tropical cyclone solutions using a state-of-the-art numerical model that incorporates the most recent observational guidance for subgrid scale parameters and airsea exchange coefficients of heat and momentum. Emphasis is placed on the realism of such solutions and the sources of cyclonic relative angular momentum(RAM) that are necessary to replenish that lost by friction at the surface. For simplicity, we confine our attention to strictly axisymmetric numerical *** are able to replicate Hakim's long-term simulation of a quasi-steady state cyclone in a 1500 km radial domain. The structure of the wind field is found to be somewhat realistic compared to observations, but sustained by unrealistic processes. Artificial sources of cyclonic RAM are quantified and the lateral damping of the anticyclonic wind near the outer boundary is found to make the largest contribution to the source of cyclonic RAM. When the domain size is extended to 9,000 km radius and lateral damping is removed altogether, a quasi-steady vortex emerges, but the structure of this vortex has many unrealistic features. In this solution, the remaining upper-level Rayleigh damping contributes a major portion of the needed source of cyclonic RAM. In a simulation in which the upper-level damping is removed also, the solution is found to be neither quasi-steady nor *** findings call into question the realism of long-term, sustained tropical cyclone simulations, which require a sufficiently large source of cyclonic RAM to facilitate the existence of a quasi-steady state.

关键词： tropical cyclones steady-state angular momentum