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Light-induced halide segregation in perovskites with wrinkled morphology

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Journal of Energy Chemistry 2022年第8期31卷 83-88,I0003页

作者： Eduardo G.Machado Paulo E.Marchezi Eralci M.Therézio JoséCarlos Germino Rodrigo Szostak Caique Sde Brito Yara G.Gobato Ernesto C.Pereira michael f.toney Raphael Nagao Ana flávia Nogueira Institute of Chemistry University of CampinasCampinas 13083-970 SPBrazil Center for Innovation on New Energies University of CampinasCampinas 13083-970SPBrazil Institute of Physics Federal University of Mato GrossoCuiaba 78060-900MTBrazil Department of Physics Federal University of Sao CarlosSao Carlos 13565-905SPBrazil Department of Physics and i3N–Institute for Nanostructures Nanomodulation and NanofabricationUniversity of AveiroAveiro 3810-193Portugal Department of Chemistry Federal University of Sao CarlosSao Carlos 13565-905SPBrazil Renewable and Sustainable Energy Institute(RASEI) University of Colorado BoulderBoulder CO 80309ColoradoUnited States of America

In this work, it is proposed that, upon light incidence, a halide segregation event takes place, where iodine anions move towards the hills of a wrinkled mixed-halide perovskite.

关键词： halide perovskite iodine

Like a G6-nal:transcriptional control of G-protein coupled receptors during oligodendroglial development

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Neural Regeneration Research 2025年第7期20卷 2001-2002页

作者： Tim Aberle michael Wegner Institut für Biochemie Friedrich-Alexander-Universität Erlangen-NürnbergErlangenGermany

Multilayered control of myelination:Quick,saltatory conduction of action potentials along nerve fibers requires the electrical insulation of axons by myelinating *** the central nervous system,this role is taken up by *** are marked by the expression of the lineage determinants Sox10 and Olig2 and arise from oligodendrocyte precursor cells(OPCs)during embryonal *** the majority of OPCs differentiate into mature oligodendrocytes when nearby axonal segments require myelination,a small subpopulation of OPCs persist as a progenitor ***,the timing of myelination and maintenance of the OPC pool both need to be precisely *** transcription factors either positively or negatively affect oligodendrocyte differentiation and maintenance of the OPC pool as components of a complex gene regulatory network(reviewed in Sock and Wegner,2021).Network activity is additionally influenced by extracellular signaling molecules that bind to receptors on the oligodendroglial cell surface and activate intracellular signaling *** the receptors are linked to the network is poorly understood so far,but pivotal to understanding the overall regulation of central nervous system(CNS)myelination in response to environmental *** insights were recently gained for Gpr37(Schmidt et al.,2024),a G-protein coupled receptor(GPCR)with known relevance in differentiating oligodendrocytes(Yang et al,2016).

关键词： gained insulation conduction

Low bend loss,high index,composite morphology ultra-fast laser written waveguides for photonic integrated circuits

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Light(Advanced Manufacturing) 2024年第1期5卷 50-59页

作者： Andrew Ross-Adams toney Teddy fernandez michael Withford Simon Gross MQ Photonics School of Mathematics and Physical SciencesMacquarie University2109Australia School of Engineering Macquarie University2109Australia

We demonstrate a novel,composite laser written 3D waveguide,fabricated in boro-aluminosilicate glass,with a refractive index contrast of 1.12×10^(−2).The waveguide is fabricated using a multi-pass approach which leverages the respective refractive index modification mechanisms of both the thermal and athermal inscription *** present the study and optimisation of inscription parameters for maximising positive refractive index change and ultimately demonstrate a dramatic advancement on the state of the art of bend losses in laser-written *** 1.0 dB cm−1 bend loss cut-off radius is reduced from 10 mm to 4 mm,at a propagation wavelength of 1550 nm.

关键词： Ultrafast laser inscription Thermal inscription Cumulative heating Athermal inscription Multi-scan Multi-pass Half-scan Bend loss High index contrast Photonic integrated circuit

A re-evaluation of the average chain length of lacustrine sedimentary n-alkanes as a paleoproxy on the Qinghai-Tibet Plateau

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frontiers of Earth Science 2023年第4期17卷 905-919页

作者： Mingda WANG Qin LI Jaime toney David HENDERSON Juzhi HOU School of Geography Liaoning Normal UniversityDalian 116029China Alpine Paleoecology and Human Adaptation(ALPHA)Group State Key Laboratory of Tibetan Plateau Earth SystemResources and EnvironmentInstitute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China School of Geographical and Earth Sciences University of GlasgowGlasgow G128QQScotlandUK CAS Center for Excellence in Tibetan Plateau Earth Sciences Beijing 100101China

Long-chain n-alkanes are one of the most common organic compounds in terrestrial plants and they are well-preserved in various geological archives.n-alkanes are relatively resistant to degradation and thus they can provide high-fidelity records of past vegetation and climate ***,previous studies have shown that the interpretation of n-alkane proxies,such as the average chain length(ACL),is often ambiguous since this proxy depends on more than one *** vegetation and climate could exert controls on the n-alkane ACL,and hence its interpretation requires careful consideration,especially in regions like the Qinghai-Tibet Plateau(QTP)where topography,biome type and moisture source are highly *** further evaluate the influences of vegetation and climate on the ACL in high-elevation lakes,we examined the n-alkane distributions of the surface sediments of 55 lakes across the *** results show that the ACL across a climatic gradient is significantly affected by precipitation,rather than by *** positive correlation between ACL and precipitation may be because of the effect of microbial degradation during ***,we suggest that more caution is needed in the interpretation of ACL data in different regions.

关键词： ACL average chain length n-alkanes leaf wax lake sediments Qinghai-Tibet Plateau

Building geospatial infrastructure

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Geo-Spatial Information Science 2020年第1期23卷 1-9页

作者： Jack Dangermond michael f.Goodchild Esri RedlandsCAUSA Department of Geography University of CaliforniaSanta BarbaraCAUSA

Many visions for geospatial technology have been advanced over the past half *** researchers saw the handling of geospatial data as the major problem to be *** vision of geographic information systems arose as an early international *** visions included spatial data infrastructure,Digital Earth,and a nervous system for the *** accelerating advances in information technology,a new vision is needed that reflects today’s focus on open and multimodal access,sharing,engagement,the Web,Big Data,artificial intelligence,and data *** elaborate on the concept of geospatial infrastructure,and argue that it is essential if geospatial technology is to contribute to the solution of problems facing humanity.

关键词： Spatial data handling National Spatial Data Infrastructure Digital Earth Big Data citizen engagement

Linking water and nutrients through the vadose zone: a fungal interface between the soil and plant systems

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Journal of Arid Land 2011年第3期3卷 155-163页

作者： michael f ALLEN Center for Conservation Biology University of California

Plant water availability, use, and management have largely focused on physical processes of infiltration and the role of roots in uptake and transpiration. However, roots and mycorrhizal fungi redistribute water in complex patterns. Here I describe some of our observations and experiments showing that mycorrhizal fungi play key roles in moving water for both transpiration and to facilitate nutrient acquisition under dry conditions. Mycorrhizal fungal hyphae grow from both surface and deep roots even into bedrock to help extract water under dry conditions. In both deep and surface roots, mycorrhizal fungi acquire water from pores too small for roots and root hairs to access, and at distances from roots and root hairs. Mycorrhizal fungi are also able to utilize hydraulic-lifted water from plants to obtain nutrients in extremely dry surface soils. The importance of these root symbionts in water and nutrient dynamics, and as integrators of surface and deeper water dynamics need further investigation.

关键词： mycorrhiza vadose zone hydraulic redistribution drought

A potpourri of pancreatic issues

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World Journal of Gastroenterology 2007年第47期13卷 6327-6332页

作者： Iman Zandieh michael f Byrne Division of Gastroenterology Department of MedicineUniversity of British ColumbiaVancouverBritish ColumbiaCanada

Autoimmune pancreatitis has emerged over the last 40 years from a proposed concept to a well established and recognized entity. As an efficient mimicker of pancreatic carcinoma, its early and appropriate recognition are crucial. With mounting understanding of its pathogenesis and natural history, significant advances have been made in the diagnosis of autoimmune pancreatitis. The characteristic laboratory features and imaging seen in autoimmune pancreatitis are reviewed along with some of the proposed diagnostic criteria and treatment algorithms.

关键词： Autoimmune pancreatitis Chronic pancreatitis Idiopathic pancreatitis Sclerosing pancreatitis

Influence of lanthanum level and interactions with nitrogen source on early development of Juglans nigra

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Journal of Rare Earths 2009年第2期27卷 270-279页

作者： Nicodemus michael A Salifu K francis Jacobs Douglass f Department of forestty and Natural Resources Hardwood Tree Improvement and Regeneration Center Purdue University West Lafayette IN 47907 USA

Rare earth elements have been used for 30 years in Chinese agriculture to improve growth and yield. Numerous scientific studies have shown improvements in physiology, mineral nutrition, and growth, though deleterious effects may also occur. Very few studies have been performed on woody species. We exponentially fertilized one-year old black walnut （Juglans nigra L.） seedlings with 0, 0.1, 1, 10, or 100 mg lanthanum （La） and 800 mg nitrogen （N） as NaNO3, （NH4）2SO4, NH4NO3, or no N. One month following final fertilization, growth, mineral nutrition, photosynthesis, chlorophyll, and nitrate reductase activity were assessed. Plants fertilized with the highest level of La had reduced fine root growth, concentrations of magnesium, calcium, nickel, and phosphorus, photosynthesis levels, and chlorophyll a content. foliar La concentration showed an interaction effect, with three to four times greater concentration in plants fed at 100 mg La to those given 10 mg La for （NH4）2SO4 and NHaNO3 treatments. The results suggested no beneficial effects of La addition at levels used in this study and interactions between N source and La levels did not have an important impact on the growth, mineral nutrition, or physiology of black walnut seedlings.

关键词： lanthanum nitrate reductase chlorophyll photosynthesis Jugians nigra rare earths

电化学去合金化Pt(Pd)-Cu对氧的电催化还原活性的研究

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电化学 2012年第2期18卷 146-150页

作者：杨瑞枝 Peter Strasser michael toney 苏州大学能源学院江苏苏州215006 斯坦福大学材料和能源科学研究所美国斯坦福94025 斯坦福美国国家同步辐射光源中心美国斯坦福94025 柏林科技大学化学化工学院德国柏林10623

应用电化学去合金法制备了表面覆盖有Pt(Pd)原子层的Pt(Pd)-Cu合金催化剂.研究该催化剂在0.1mol.L-1HClO4酸性溶液中对氧气电化学还原的催化活性,并采用同步辐射反常X-射线衍射法(Anomalous X-ray Diffraction,AXRD)和表面X-射线散射法(... 详细信息

应用电化学去合金法制备了表面覆盖有Pt(Pd)原子层的Pt(Pd)-Cu合金催化剂.研究该催化剂在0.1mol.L-1HClO4酸性溶液中对氧气电化学还原的催化活性,并采用同步辐射反常X-射线衍射法(Anomalous X-ray Diffraction,AXRD)和表面X-射线散射法(Surface X-ray Scattering,SXS)从原子尺度研究了去合金化后催化剂的结构.分析对比纳米颗粒、薄膜和单晶3种不同形式的去合金化Pt-Cu的结构和催化活性以及Pt-Cu和Pd-Cu两种不同合金薄膜的结构和催化活性.结果表明,表面应力是影响催化剂催化活性的关键因素,而应力大小则与去合金化后所形成的表面Pt(Pd)层的厚度相关,材料尺寸和组成元素等都影响表面Pt(Pd)层的厚度.提出可利用调控材料表面的应力来设计高催化活性的催化剂.

关键词：氧电化学还原电化学去合金 Pt(Pd)-Cu合金电催化剂