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Hydrogen spillover in nonreducible oxides:Mechanism and catalytic utilization

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Nano Research 2022年第12期15卷 10357-10365页

作者： Songhyun Lee Hyungjun Kim Ryong Ryoo Jeong young park minkee Choi Charles D.Davidson School of Chemical Engineering Purdue UniversityWest LafayetteIndiana47907USA Department of Chemical and Biomolecular Engineering Korea Advanced Institute of Science and TechnologyDaejeon34141Republic of Korea Department of Chemistry Korea Advanced Institute of Science and TechnologyDaejeon34141Republic of Korea KENTECH Laboratory for Chemical Environmental and Climate TechnologyKorea Institute of Energy Technology(KENTECH)200 Hyeoksin-roNaju58330Republic of Korea Center for Nanomaterials and Chemical Reactions Institute for Basic Science(IBS)Daejeon34141Republic of Korea

Hydrogen(H)spillover in nonreducible oxides such as zeolites and Al2O3 has been a highly controversial phenomenon in heterogeneous *** industrial catalysts are predominantly prepared using these materials as supports,it is important to understand the mechanism and catalytic functions of H spillover on their *** the past decade,fundamental studies on zeolite-encapsulated metal catalysts have revealed that H spillover and reverse spillover can be utilized in the design of hydrogenation and dehydrogenation catalysts with improved *** experimental and theoretical studies have indicated that H spillover can occur in nonreducible oxides when they possess substantial acid sites that aid the surface migration of active *** the present review,we will discuss the possible mechanisms of H spillover in nonreducible oxides and the unique opportunities of using this phenomenon for the design of advanced hydroprocessing catalysts.

关键词： hydrogen spillover nonreducible oxides zeolites hydroprocessing catalysts

Bile acids and microbes in metabolic disease

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World Journal of Gastroenterology 2022年第48期28卷 6846-6866页

作者： Dhiraj Kumar Sah Archana Arjunan Sun young park young Do Jung Department of Biochemistry Chonnam National UniversityGwangju 501190South Korea Department of Internal Medicine Chonnam National UniversityGwangju 501190South Korea

Bile acids(BAs)serve as physiological detergents that enable the intestinal absorption and transportation of nutrients,lipids and *** are primarily produced by humans to catabolize cholesterol and play crucial roles in gut metabolism,microbiota habitat regulation and cell ***-activated nuclear receptors regulate the enterohepatic circulation of BAs which play a role in energy,lipid,glucose,and drug *** gut microbiota plays an essential role in the biotransformation of BAs and regulates BAs composition and ***,altered gut microbial and BAs activity can affect human metabolism and thus result in the alteration of metabolic pathways and the occurrence of metabolic diseases/syndromes,such as diabetes mellitus,obesity/hypercholesterolemia,and cardiovascular *** and their metabolites are used to treat altered gut microbiota and metabolic *** review explores the increasing body of evidence that links alterations of gut microbial activity and BAs with the pathogenesis of metabolic ***,we summarize existing research on gut microbes and BAs in relation to intracellular pathways pertinent to metabolic ***,we discuss how therapeutic interventions using BAs can facilitate microbiome functioning and ease metabolic diseases.

关键词： Bile acids Metabolic diseases Gut microbe Diabetic mellitus Obesity Hypercholesterolemia

Parallel Iterative FEM Solver with Initial Guess for Frequency Domain Electromagnetic Analysis

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Intelligent Automation & Soft Computing 2023年第5期36卷 1585-1602页

作者： Woochan Lee Woobin park Jaeyoung park young-Joon Kim Moonseong Kim Department of Electrical Engineering Incheon National UniversityIncheon22012Korea Department of Computer Engineering Hongik UniversitySeoul04066Korea Department of Electronic Engineering Gachon UniversitySeongnam13120Korea Department of IT Convergence Software Seoul Theological UniversityBucheon14754Korea

The finite element method is a key player in computational electromag-netics for designing RF(Radio Frequency)components such as *** frequency-domain analysis is fundamental to identify the characteristics of the *** the conventional frequency-domain electromagnetic analysis using FEM(Finite Element Method),the system matrix is complex-numbered as well as indeﬁ*** iterative solvers can be faster than the direct solver when the solver convergence is guaranteed and done in a few ***,such complex-numbered and indeﬁnite systems are hard to exploit the merit of the iterative *** is also hard to beneﬁt from matrix factorization techniques due to varying system matrix parts according to ***,it is hard to adopt conventional iterative solvers even though the system matrix is sparse.A new parallel iterative FEM solver for frequency domain analysis is implemented for inhomogeneous waveguide structures in this *** this implementation,the previous solution of the iterative solver of Matlab(Matrix Laboratory)employ-ing the preconditioner is used for the initial guess for the next step’s solution *** overlapped parallel stage using Matlab’s Parallel Computing Toolbox is also proposed to alleviate the cold starting,which ruins the convergence of early steps in each parallel *** experiments based on waveguide structures have demonstrated the accuracy and efﬁciency of the proposed scheme.

关键词： Computational electromagnetics numerical simulation ﬁnite element method parallel processing iterative solvers

Nucleus-Encoded Thylakoid Protein,OsY3IP1,Confers Enhanced Tolerance to Saline and Alkaline Stresses in Rice

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Rice science 2022年第3期29卷 225-236页

作者： Hyeran MOON young-Ah KIM Ryoung SHIN Chang-Jin park Department of Molecular Biology Sejong University Department of Bioresources Engineering Sejong University RIKEN Center for Sustainable Resource Science Plant Engineering Research Institute Sejong University

Abiotic stress confers serious damage to the photosynthetic machinery,often resulting in plant growth *** chloroplast open reading frame 3(Ycf3)-interacting protein 1(Y3IP1)is a nucleus-encoded thylakoid protein and plays an essential role in the assembly of photosystem *** full-length cDNA over-expresser(FOX)gene-hunting system is an approach using systemically generated gain-of-function *** the FOX-rice lines,a line CE175 overexpressing rice Y3IP1gene(Os Y3IP1)displayed less inhibition of root growth under saline(NaCl)*** expression of Os Y3IP1 was up-regulated under saline and alkaline(Na2CO3)stresses in the rice variety *** saline and alkaline treatments,transgenic Kitaake overexpressing OsY3IP1-GFP(OsY3IP1-GFPox/Kit)displayed higher levels of chlorophyll content compared to *** the stress conditions,the maximum quantum yield of photosystem II photochemistry levels was higher in OsY3IP1-GFPox/Kit than in *** increased tolerance conferred by OsY3IP1 overexpression correlated with reduced reactive oxygen species *** data provide new insights into the possible role of OsY3IP1 in the pathway suppressing photooxidative damage under stress *** features can be further exploited to improve saline and alkaline tolerances of rice plants in future.

关键词： alkaline reactive oxygen species rice saline stress tolerance

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Bone Research 2024年第1期12卷 122-136页

作者： Nan-Yu Zou Ran Liu Mei Huang Yu-Rui Jiao Jie Wei Yangzi Jiang Wen-Zhen He min Huang Yi-Li Xu Ling Liu Yu-Chen Sun mi Yang Qi Guo Yan Huang Tian Su Ye Xiao Wei-Shan Wang Chao Zeng Guang-Hua Lei Xiang-Hang Luo Chang-Jun Li Department of Endocrinology Endocrinology Research CenterXiangya Hospital of Central South UniversityChangshaHunan 410008China Department of Orthopaedics Xiangya Hospital of Central South UniversityChangshaHunan 410008China Department of Epidemiology and Health Statistics Xiangya School of Public HealthCentral South UniversityChangshaChina Hunan Key Laboratory of Joint Degeneration and Injury ChangshaHunan 410008China Key Laboratory of Aging-related Bone and Joint Diseases Prevention and Treatment Ministry of EducationXiangya HospitalCentral South UniversityChangshaChina School of Biomedical Sciences Institute for Tissue Engineering and Regenerative MedicineFaculty of MedicineThe Chinese University of Hong KongHong Kong SARChina Department of Orthopaedics The First Affiliated Hospital of Shihezi UniversityShiheziXinjiangChina National Clinical Research Center for Geriatric Disorders Xiangya HospitalCentral South UniversityChangshaHunan 410008China

Skeletal stem/progenitor cell(SSPC)senescence is a major cause of decreased bone regenerative potential with aging,but the causes of SSPC senescence remain *** this study,we revealed that macrophages in calluses secrete prosenescent factors,including grancalcin(GCA),during aging,which triggers SSPC senescence and impairs fracture *** injection of human rGCA in young mice induced SSPC senescence and delayed fracture *** deletion of Gca in monocytes/macrophages was sufficient to rejuvenate fracture repair in aged mice and alleviate SSPC ***,GCA binds to the plexin-B2 receptor and activates Arg2-mediated mitochondrial dysfunction,resulting in cellular *** of Plxnb2 in SSPCs impaired fracture *** of GCA-neutralizing antibody enhanced fracture healing in aged ***,our study revealed that senescent macrophages within calluses secrete GCA to trigger SSPC secondary senescence,and GCA neutralization represents a promising therapy for nonunion or delayed union in elderly individuals.

关键词： healing union senescence

A novel cytokine consisting of the p40 and EBI3 subunits suppresses experimental autoimmune arthritis via reciprocal regulation of Th17 and Treg cells

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Cellular & Molecular Immunology 2022年第1期19卷 79-91页

作者： Seon-Yeong Lee Su-Jin Moon young-Mee Moon Hyeon-Beom Seo Jun-Geol Ryu A Ram Lee Chae Rim Lee Da-Som Kim Yang-mi Her Jeong Won Choi Seung-Ki Kwok Sung-Hwan park mi-La Cho The Rheumatism Research Center The Catholic University of KoreaSeoulSouth Korea Division of Rheumatology Department of Internal MedicineSeoul St.Mary’s HospitalCollege of MedicineThe Catholic University of KoreaSeoulSouth Korea Department of Biomedicine&Health Sciences College of MedicineThe Catholic University of KoreaSeoulSouth Korea Department of Medical Lifescience College of MedicineThe Catholic University of KoreaSeoulSouth Korea These author contributed equally:Seon-Yeong Lee Su-Jin MoonYoung-Mee Moon

OBJECTIVE:The interleukin(IL)-12 cytokine family is closely related to the development of T helper cells,which are responsible for autoimmune disease enhancement or ***-12 family members are generally heterodimers and share threeα-subunits(p35,p19,and p28)and twoβ-subunits(p40 and EBI3).However,aβ-sheet p40 homodimer has been shown to exist and antagonize IL-12 and IL-23 signaling ***,we assumed the existence of a p40-EBI3 heterodimer in nature and sought to investigate its role in immune ***:The presence of the p40-EBI3 heterodimer was confirmed by ELISA,immunoprecipitation,and western blotting.A p40-EBI3 vector and p40-EBI3-Fc protein were synthesized to confirm the immunological role of this protein in mice with collageninduced arthritis(CIA).The anti-inflammatory effects of p40-EBI3 were analyzed with regard to clinical,histological,and immune cell-regulating features in mice with ***:Clinical arthritis scores and the expression levels of proinflammatory cytokines(e.g.,IL-17,IL-1β,IL-6,and TNF-α)were significantly attenuated in p40-EBI3-overexpressing and p40-EBI3-Fc-treated mice with CIA compared to vehicle-treated mice with *** joint damage and vessel formation-related gene expression were also reduced by p40-EBI3 heterodimer *** vitro,the p40-EBI3-Fc protein significantly suppressed the differentiation of Th17 cells and reciprocally induced CD4+CD25+Foxp3+(regulatory T)cells.p40-EBI3 also inhibited osteoclast formation in a concentrationdependent ***:In this study,p40-EBI3 ameliorated proinflammatory conditions both in vivo and in *** propose that p40-EBI3 is a novel anti-inflammatory cytokine involved in suppressing the immune response through the expansion of Treg cells and suppression of Th17 cells and osteoclastogenesis.

关键词： cytokine p40-EBI3 Rheumatoid arthritis Autoimmune disease regulatory T cell

Incidence and Related Risk Factors of Junctional Ectopic Tachycardia in Infants after Cardiac Surgery for Congenital Heart Disease

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Congenital Heart Disease 2022年第5期17卷 569-578页

作者： Jae Hee Seol Se Yong Jung Jae young Choi Han Ki park young Hwan park Nam Kyun Kim Department of Pediatrics Congenital Heart Disease CenterDivision of Pediatric CardiologySeverance Cardiovascular HospitalYonsei University College of MedicineSeoulKorea Department of Pediatrics Yonsei University Wonju College of MedicineWonjuKorea Department of Thoracic and Cardiovascular Surgery Division of Cardiovascular SurgeryCongenital Heart Disease CenterSeverance Cardiovascular HospitalYonsei University College of MedicineSeoulKorea Department of Pediatrics and Biomedical Engineering School of MedicineEmory UniversityAtlantaUSA

Objective:Junctional ectopic tachycardia is common after cardiac surgery for congenital heart ***,its incidence and related risk factors in infants after cardiac surgery are not well *** objective of this study was to determine the overall incidence and related risk factors for junctional ectopic tachycardia in neonates and ***:We enrolled a total of 271 patients agedmias detected in the perioperative period,and ***:The overall incidence of junctional ectopic tachycardia was 12.9%.The logistic regression analysis revealed that longer cardiopulmonary bypass time,surgery involving atrioventricular node stretching,and the presence of early repolarization on preoperative electrocardiography increased the risk of junctional ectopic *** with junctional ectopic tachycardia had longer intubation time and intensive care unit ***:Junctional ectopic tachycardia is a common arrhythmia after cardiac surgery for congenital heart disease in ***,infants developing junctional ectopic tachycardia after cardiac surgery have specific preoperative electrocardiography *** risk factors for junctional ectopic tachycardia were associated not only with surgical procedural factors but also with preoperative electrocardiographic parameters.

关键词： Junctional ectopic tachycardia congenital heart disease early re-polarization

Case mistaken for leukemia after mRNA COVID-19 vaccine administration:A case report

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World Journal of Clinical Cases 2022年第33期10卷 12268-12277页

作者： Seul Bi Lee Chi young park Sang-Gon park Hee Jeong Lee Department of Internal Medicine Hemato-oncologyChosun University HospitalGwangju 501-717South Korea

BACKGROUND Following the global outbreak of coronavirus disease 2019(COVID-19),unlike other vaccines,COVID-19 vaccines were developed and commercialized in a relatively short period of *** large-scale administration of this vaccine in a short time-period led to various unexpected side effects,including severe cytopenia and thrombosis with thrombocytopenia *** many reports on adverse reactions,vaccination was necessary to prevent the spread of COVID-19;thus,it is essential to understand and discuss various cases of adverse reactions after *** SUMMARY A 77-year-old woman was administered the second dose of Pfizer mRNA COVID-19 *** vaccination she experienced fever,myalgia,and *** were subsequently administered for several days,but there was no improvement in the *** patient showed severe thrombocytopenia and *** and abdominopelvic computed tomography showed no infection related findings,but splenomegaly and cirrhotic liver features were observed.A large number of immature cells were observed in the peripheral blood smear;thus,bone marrow examination was performed for acute ***,there were no *** patient recovered after administration of hepatotoxins and transfusion treatment for cytopenia and was diagnosed with an adverse reaction to COVID-19 *** Adverse reactions of vaccination could be mistaken for hematologic malignancies including *** report a patient with leukocytosis following COVID-19 vaccination.

关键词： COVID-19 Vaccine mRNA Leukocytosis Adverse reaction Case report

Intrinsic electrochemical activity of Ni in Ni_(3)Sn_(4) anode accommodating high capacity and mechanical stability for fast-charging lithium-ion batteries

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Journal of Energy Chemistry 2022年第8期31卷 470-477,I0013页

作者： Janghyuk Moon Trung Dinh Hoang Seong Soo park Seowan park Dong young Rhee Junwon Lee Sang A Han min-Sik park Jung Ho Kim School of Energy Systems Engineering Chung-Ang UniversityHeukseok-RoDongjak-guSeoul 06974Republic of Korea Department of Advanced Materials Engineering for Information and Electronics Integrated Education Institute for Frontier Science&Technology(BK21 Four)Kyung Hee University1732 Deogyeong-daeroGiheung-guYongin 17104Republic of Korea Institute for Superconducting&Electronic Materials(ISEM) Australian Institute of Innovative Materials(AIIM)University of WollongongInnovation CampusSquires WayNorth WollongongNSW 2500Australia

Fast interfacial kinetics derived from bicontinuous three-dimensional(3D)architecture is a strategic feature for achieving fast-charging lithium-ion batteries(LIBs).One of the main reasons is its large active surface and short diffusion ***,understanding of unusual electrochemical properties still remain great challenge due to its *** this study,we proposed a nickel–tin compound(Ni_(3)Sn_(4))supported by 3D Nickel scaffolds as main frame because the Ni_(3)Sn_(4) clearly offers a higher reversible capacity and stable cycling performance than bare tin(Sn).In order to verify the role of Ni,atomic-scale simulation based on density functional theory systematically addressed to the reaction mechanism and structural evolution of Ni_(3)Sn_(4) during the lithiation *** findings are that Ni enables Ni_(3)Sn_(4) to possess higher mechanical stability in terms of reactive flow stress,subsequently lead to improve Li storage *** study elucidates an understanding of the lithiation mechanism of Ni_(3)Sn_(4) and provides a new perspective for the design of high-capacity and high-power 3D anodes for fast-charging LIBs.

关键词： Lithium-ion batteries Ni_(3)Sn_(4) High-capacity anode 3D-structured electrode Inverse opal structure Density functional theory