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Journal of Modern Power Systems and Clean energy 2024年第3期12卷 863-873页

作者： Guanwei Zeng Chengxi liu Minfang Liao Yongjian Luo Xuzhu Dong Hubei engineering and Technology Research Center for AC/DC Intelligent Distribution Network WuhanChina the School of electrical engineering and Automation Wuhan UniversityWuhanChina

We propose an optimal stochastic scheduling strategy for a multi-vector energy complex(MeC),considering a fullblown model of the power-to-biomethane(Pt M)*** conventional optimization that uses a simple efficiency coefficient to coarsely model energy conversion between electricity and biomethane,a detailed Pt M model is introduced to emphasize the reactor kinetics and chemical equilibria of *** model crystallizes the interactions between the Pt M process and MeC flexibility,allowing to adjust the operating condition of the methanation reactor for optimal MeC operation in stochastic *** optimization and flowsheet design of the Pt M process increase the average selectivity of methane(i.e.,ratio between net biomethane production and hydrogen consumption)up to 83.7%in the proposed synthesis *** results can provide information and predictions to operators about the optimal operating conditions of a Pt M unit while improving the MeC flexibility.

关键词： Multi-vector energy complex optimal stochastic scheduling power-to-biomethane unit process synthesis natural gas

Stabilizing zinc anode using zeolite imidazole framework functionalized separator for durable aqueous zinc-ion batteries

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Journal of energy Chemistry 2024年第3期90卷 23-31,I0003页

作者： Weisong Zhang Xinyan Zhu Ling Kang Ziyu Peng Jing Zhu Liang Pan Lei Dai Shude liu Ling Wang Yongguang liu Zhangxing He School of Chemical engineering North China University of Science and TechnologyTangshan 063009HebeiChina Shanghai Key Laboratory of Multidimensional Information Processing East China Normal UniversityShanghai 201620China College of Textiles Donghua UniversityShanghai 201620China

Aqueous zinc-ion batteries(AZIBs) hold great promise as a viable alternative to lithium-ion batteries owing to their high energy density and environmental ***,AZIBs are consistently plagued by the formation of zinc dendrites and concurrent side reactions,which significantly diminish their overall service life,In this study,the glass fiber separator(GF) is modified using zeolite imidazole salt framework-8(ZIF-8),enabling the development of efficient ***-8,which is abundant in nitrogen content,efficiently regulates the desolvation of [Zn(H_(2)O)_(6)]^(2+) to inhibit hydrogen ***,it possesses abundant nanochannels that facilitate the uniform deposition of Zn~(2+) via a localized action,thereby hindering the formation of *** insulating properties of ZIF-8 help prevent Zn^(2+) and water from trapping electron reduction at the layer surface,which reduces corrosion of the zinc ***,ZIF-8-GF achieves the even transport of Zn^(2+) and regulates the homogeneous deposition along the Zn(002) crystal surface,thus significantly enhancing the electrochemical performance of the AZIBs,In particular,the Zn|Zn symmetric cell with the ZIF-8-GF separator delivers a stable cycle life at0.5 mA cm^(-2) of 2300 *** Zn|ZIF-8-GF|MnO_(2) cell exhibits reduced voltage polarization while maintaining a capacity retention rate(93.4%) after 1200 cycles at 1.2 A g^(-1) The unique design of the modified diaphragm provides a new approach to realizing high-performance AZIBs.

关键词： Aqueous zinc-ion batteries Separators modifications ZIF-8 Zn deposition Dendrite-free

1.42-fold enhancement of formate selectivity by linker conversion on the Zn-based metal organic framework catalyst

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Journal of energy Chemistry 2024年第3期90卷 183-190,I0006页

作者： Yayu Guan Yuyu liu Fanghua Ning Jin Yi Jiujun Zhang Institute for Sustainable energy College of SciencesShanghai UniversityShanghai 200444China

electro-reduction of carbon dioxide(eRCO_(2)) is considered an effective method to alleviate the greenhouse effect and produce value-added *** the dominant selectivity of Zn-based catalysts for formate remains a *** this article,the ZnIn-e_(12) catalyst is successfully prepared by solvent assisted ligand exchange(SALe) method to convert organic ligands,achieving a Faradaic efficiency of 72.28% for formate at-1.26 V ***(V_(RHe)),which is 1.42 times higher than the original *** shows that the successful conversion of organic ligands can transform the catalyst from the original large size polyhedron to cross-linked network of particles with a diameter of about 30 *** increased specific surface area can expose more active sites and facilitate the electrocatalytic conversion of CO_(2) to *** work is expected to provide inspiration for the regulation of formate selectivity and catalyst size in Zn-based catalysts.

关键词： electrocatalyst Carbon dioxide Formate Linker conversion

Capacitor Voltage Imbalance Mechanism and Balancing Control of MMC When Riding Through PTG Fault

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CSee Journal of Power and energy Systems 2024年第2期10卷 778-785页

作者： Zhen He Maozeng Lu Lijun Hang Pingliang Zeng Yanhua liu Hangzhou Dianzi University Hangzhou 310018China Shandong University of Technology Zibo 255000China State Grid Hangzhou Power Supply Company State GridHangzhou 310000China

Modular multilevel converter (MMC) based fault ride through (FRT) control is a promising solution to deal with the pole-to-ground (PTG) fault in high voltage direct current (HVDC) system. However, when MMC switches to the FRT control, capacitor voltage imbalance between upper and lower arms will occur, resulting in the deterioration of FRT performance. This letter provides a comprehensive analysis for the imbalance issue from the perspective of fundamental frequency circulating current (FFCC). It is found the imbalance during FRT stage will not expand continuously, but converge to a certain value gradually. The specific imbalance degree is closely associated with the amplitude of FFCC. In order to solve the imbalance issue, an open-loop balancing control is proposed. By introducing a fundamental frequency feedforward item to the inherent circulating current control, the proposed method can not only balance the capacitor voltages, but also minimize the amplitude of FFCC, and consequently the power loss of MMC during FRT process can be reduced. Finally, simulation results of PSCAD/ eMTDC verify the validity of theoretical analysis.

关键词： Balancing control capacitor voltage imbalance FFCC FRT control HVDC system PTG fault

Metalenses phase characterization by multidistance phase retrieval

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Light(Science & Applications) 2024年第9期13卷 1898-1907页

作者： Bowen liu Jialuo Cheng Maoxiong Zhao Jin Yao Xiaoyuan liu Shaohu Chen Lei Shi Din Ping Tsai Zihan Geng Mu Ku Chen State Key Laboratory of Surface Physics Key Laboratory of Micro-and Nano-Photonic Structures(Ministry of Education)and Department of PhysicsFudan University200433 ShanghaiChina Department of electrical engineering City University of Hong KongKowloonHong Kong SARChina State Key Laboratory of Terahertz and Millimeter Waves City University of Hong KongKowloonHong Kong SARChina Institute for Nanoelectronic Devices and Quantum Computing Fudan University200438 ShanghaiChina Collaborative Innovation Center of Advanced Microstructures Nanjing University210093 NanjingJiangsuChina Shanghai Research Center for Quantum Sciences 201315 ShanghaiChina Centre for Biosystems Neuroscienceand NanotechnologyCity University of Hong KongKowloonHong Kong SARChina Institute of Data and Information Tsinghua Shenzhen International Graduate SchoolTsinghua University518071 ShenzhenGuangdongChina

Metalens,characterized by their unique functions and distinctive physical properties,have gained significant attention for their potential *** further optimize the performance of metalens,it is necessary to characterize the phase modulation of the *** this study,we present a multi-distance phase retrieval system based on optical field scanning and discuss its convergence and *** findings indicate that the system is capable of retrieving the phase distribution of the metalens as long as the measurement noise is low and the total length of the scanned light field is sufficiently *** system enables the analysis of focal length and aberration by utilizing the computed phase *** extend our investigation to measure the phase distribution of the metalens operating in the near-infrared(NIR)spectrum and identify the impact of defects in the sample on the ***,we conduct a comparative analysis of the phase distribution of the metalens in air and ethanol and observe the variations in the phase modulation of the metalens in different working *** system provides a straightforward method for the phase characterization of metalens,aiding in optimizing the metalens design and functionality.

关键词： phase system distribution

enhancement of ionic conductivity and fracture toughness by infiltrating porous Li_(0.33)La_(0.56)TiO_(3) pellets

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Journal of Rare earths 2024年第2期42卷 392-398,I0006页

作者： Xiaojuan Lu Mingyang Duan Jingyu Xiang Yuning Liang Songtao liu Hebei Key Lab of Power Plant Flue Gas Multi-Pollutants Control Department of Environmental Science and EngineeringNorth China Electric Power UniversityBaoding071003China

Although solid-state lithium electrolytes have the potential to reduce the safety issues associated with organic liquid electrolytes,disadvantages such as low total conductivity,large interface impedance,and delamination of the interface due to cyclic stress still need to be *** solid-state lithium-ion conductor Li_(0.33)La_(0.56)TiO_(3)(LLTO) was prepared via a hydrothermal route by using CTAB as templates in this *** LLTO with micro-porous channels was obtained and the total conductivity is comparable to the non-porous *** LLTO pellets are infiltrated with the non-porous LLTO precursor solution,and the total conductivities of the infiltrated porous LLTO are all higher than those without *** infiltration,the porous LLTO calcined at 600℃ achieves the highest total conductivity,7.88×10^(-5) S/*** fracture toughness of the infiltrated LLTO is higher than that of the non-porous *** results demonstrate a new way to prepare solid-state lithium-ion conductors with high ionic conductivity and great tolerance to cyclic stress.

关键词： Perovskite Porous material Infiltration Ionic conductors Fracture toughness Rare earths

Adaptive active inceptor design under shared control architecture for nonlinear pilot-induced oscillations

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Chinese Journal of Aeronautics 2024年第6期37卷 276-292页

作者： Xiaoyu liu Liguo SUN Wenqian TAN Shuting XU Junkai JIAO School of Aeronautic Science and engineering Beihang UniversityBeijing 100191China College of engineering Beijing Forestry UniversityBeijing 100083China

This paper presents a Shared Control Architecture(SCA)between a human pilot and a smart inceptor for nonlinear Pilot Induced Oscillations(PIOs),e.g.,category II or III *** innovation of this paper is that an intelligent shared control architecture is developed based on the intelligent active inceptor technique,i.e.,Smart Adaptive Flight effective Cue(SAFe-Cue).A deep reinforcement learning approach namely Deep Deterministic Policy Gradient(DDPG)method is chosen to design a gain adaptation mechanism for the SAFe-Cue *** doing this,the gains of the SAFe-Cue will be intelligently tuned once nonlinear PIOs triggered;meanwhile,the human pilot will receive a force cue from the SAFe-Cue,and will consequently adapting his/her control *** second innovation of this paper is that the reward function of the DDPG based gain adaptation approach is constructed according to flying *** the premise of considering failure situation,task completion qualities and pilot workload are also taken into ***,the proposed approach is validated using numerical simulation experiments with two types of scenarios:lower actuator rate limits and airframe *** Inceptor Peak Power-Phase(IPPP)metric is adopted to analyze the human-vehicle system simulation *** and analysis show that the DDPG based sharing control approach can well address nonlinear PIO problems consisting of Categories Ⅱ and Ⅲ PIO events.

关键词： Shared control architecture Activeinceptor Deep reinforcement learning Nonlinear pilot-induced oscillations Human-vehicle system

Yolk shell-structured pyrite-type cobalt sulfide grafted by nitrogen-doped carbon-needles with enhanced electrical conductivity for oxygen electrocatalysis

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Chinese Chemical Letters 2024年第7期35卷 212-217页

作者： Jiahao Xie Jin liu Bin liu Xin Meng Zhuang Cai Xiaoqin Xu Cheng Wang Shijie You Jinlong Zou Key Laboratory of Functional Inorganic Material Chemistry Ministry of Education of the People’s Republic of ChinaSchool of Chemistry and Materials ScienceHeilongjiang UniversityHarbin 150080China School of Chemical engineering and Light Industry Guangdong University of TechnologyGuangzhou 510006China State Key Laboratory of Urban Water Resource and environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China

Pyrite-type sulfides(PTS)exhibit promising intrinsic activities for oxygen reduction and evolution reactions(ORR/OeR).However,their poor electrical conductivities may limit the charge transfer rate to inevitably lower ***,yolk-shell structured cobalt-pyrite nanospheres(CoS_(2)YSS)are prepared and modified with amino groups as nucleation sites for coupling highly-conductive needle-like nitrogendoped carbon via a facile solvothermal method(CoS_(2)YSS@NC).The as-marked CoS_(2)YSS@NC-0.5 shows a gap between yolk and shell,and an obvious exterior layer of grafted NC,which can provide an integrated structure,an interior place,and three exposed surfaces on CoS_(2).CoS_(2)YSS@NC-0.5 reveals higher ORR activity(half-wave potential of 0.88 V)and methanol resistance than commercial Pt/*** to in-situ formation of highly-active CoOOH,CoS_(2)YSS@NC-0.5 shows a better overpotential(244 mV at 10 mA/cm^(2))and Tafel slope(135 mV/dec)than ***-air battery with CoS_(2)YSS@NC-0.5 air-cathode exhibits good open circuit potential(1.44 V),specific capacity(772.5 mAh/g)and cycling ***-like NC layer coated on the yolk-shell structure of CoS_(2)effectively lowers the charge transfer resistance to obtain extraordinary ORR/OeR *** indicates that the integration of highly-conductive carbon onto pyritetype sulfides is an effective strategy to acquire durable bifunctional ORR/OeR catalysts.

关键词： Cobalt sulfides Cycle stability electrical conductivity Pyrite Yolk-shell structure

Configuration and Kinematics of a 3-DOF Generalized Spherical Parallel Mechanism for Ankle Rehabilitation

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Chinese Journal of Mechanical engineering 2024年第1期37卷 176-188页

作者： Jianjun Zhang Shuai Yang Chenglei liu Xiaohui Wang Shijie Guo School of Mechanical engineering Hebei University of TechnologyTianjin 300401China Key Laboratory of Robot Perception and Human-Machine Fusion Tianjin 300401China

The kinematic equivalent model of an existing ankle-rehabilitation robot is inconsistent with the anatomical structure of the human ankle,which influences the rehabilitation ***,this study equates the human ankle to the UR model and proposes a novel three degrees of freedom(3-DOF)generalized spherical parallel mechanism for ankle *** parallel mechanism has two spherical centers corresponding to the rotation centers of tibiotalar and subtalar *** screw theory,the mobility of the parallel mechanism,which meets the requirements of the human ankle,is *** inverse kinematics are presented,and singularities are identified based on the Jacobian *** workspaces of the parallel mechanism are obtained through the search method and compared with the motion range of the human ankle,which shows that the parallel mechanism can meet the motion demand of ankle ***,based on the motion-force transmissibility,the performance atlases are plotted in the parameter optimal design space,and the optimum parameter is obtained according to the demands of practical *** results show that the parallel mechanism can meet the motion requirements of ankle rehabilitation and has excellent kinematic performance in its rehabilitation range,which provides a theoretical basis for the prototype design and experimental verification.

关键词： Ankle rehabilitation Parallel mechanism Kinematic analysis Parameter optimization

Cu,N codoped carbon nanosheets encapsulating ultrasmall Cu nanoparticles for enhancing selective 1,2-propanediol oxidation

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Journal of energy Chemistry 2024年第4期91卷 27-35页

作者： Yonghai Feng Min Yu Minjia Meng Lei liu Dewei Rao Institute for Advanced Materials School of Materials Science and EngineeringJiangsu UniversityZhenjiang 212013JiangsuChina School of Chemistry and Chemical engineering Jiangsu UniversityZhenjiang 212013JiangsuChina

In the selective oxidation of biomass-based 1,2-propanediol(PDO)with oxygen as the terminal oxidant,it is challenging to improve the lactic acid(LA)selectivity for nonnoble metal nanoparticles(NPs)due to their limited oxygen reduction rate and easy C-C *** the high economic feasibility of nonnoble metals,i.e.,Cu,in this work,copper and nitrogen codoped porous carbon nanosheets encapsulating ultrafine Cu nanoparticles(Cu@Cu-N-C)were developed to realize highly selective of PDO oxidation to *** carbon-encapsulated ultrasmall Cu^(0)NPs in Cu@Cu-N-C have high PDO dehydrogenation activity while N-coordinated Cu(Cu-N)sites are responsible for the high oxygen reduction ***,the performance of catalytic PDO conversion to LA is optimized by a proposed pathway of PDO→hydroxylacetone→lactaldehyde→***,the enhanced LA selectivity is 88.5%,and the PDO conversion is up to 75.1%in an O_(2)-pressurized reaction system(1.0 MPa O_(2)),superior to other Cu-based catalysts,while in a milder nonpressurized system(O_(2)flow rate of 100 mL min-1),a remarkable LA selectivity(94.2%)is obtained with 39.8%PDO conversion,2.2 times higher than that of supported Au nanoparticles(1%Au/C).Moreover,carbon encapsulation offers Cu@Cu-N-C with strong leaching resistance for better recycling.

关键词： Selective oxidation Copper and nitrogen doped carbon 1,2-Propanediol Ultrasmall Cu nanoparticles Lactic acid