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Fe-N_(x) sites coupled with core-shell FeS@C nanoparticles to boost the oxygen catalysis for rechargeable Zn-air batteries

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Journal of energy Chemistry 2024年第3期90卷 565-577,I0013页

作者： Katam Srinivas zhuo Chen Anran Chen Fei Ma Ming-qiang zhu Yuanfu Chen School of Integrated Circuit Science and engineering and State Key Laboratory of Electronic Thin Films and Integrated DevicesUniversity of Electronic Science and Technology of ChinaChengdu 610054SichuanChina College of Mechanical and electronic engineering Northwest A&F UniversityYangling 712100ShaanxiChina School of Materials and energy Yunnan UniversityKunming 650091YunnanChina

The development of efficient single-atom catalysts(SACs) for the oxygen reduction reaction(ORR)remains a formidable challenge,primarily due to the symmetric charge distribution of metal singleatom sites(M-N_(4)).To address such issue,herein,Fe-N_(x) sites coupled synergistic catalysts fabrication strategy is presented to break the uniform electronic distribution,thus enhancing the intrinsic catalytic ***,atomically dispersed Fe-N_(x) sites supported on N/S-doped mesoporous carbon(NSC)coupled with FeS@C core-shell nanoparticles(FAS-NSC@950) is synthesized by a facile hydrothermal reaction and subsequent *** to the presence of an in situ-grown conductive graphitic layer(shell),the FeS nanoparticles(core) effectively adjust the electronic structure of single-atom Fe sites and facilitate the ORR kinetics via short/long-range coupling ***,FAS-NSC@950displays a more positive half-wave potential(e_(1/2)) of 0.871 V with a significantly boosted ORR kinetics(Tafel slope=52.2 mV dec^(-1)),outpacing the commercial Pt/C(e_(1/2)=0.84 V and Tafel slope=54.6 mV dec^(-1)).As a bifunctional electrocatalyst,it displays a smaller bifunctional activity parameter(Δe) of 0.673 V,surpassing the Pt/C-RuO_(2) combination(Δe=0.724 V).Besides,the FAS-NSC@950-based zincair battery(ZAB) displays superior power density,specific capacity,and long-term cycling performance to the Pt/C-Ir/C-based *** work significantly contributes to the field by offering a promising strategy to enhance the catalytic activity of SACs for ORR,with potential implications for energy conversion and storage technologies.

关键词： Fe-N_(x)sites Core-shell FeS@C Synergistic interactions Oxygen reduction reaction Zn-air battery

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Carbon nanotube films with ultrahigh thermal-shock and thermalshock-fatigue resistance characterized by ultra-fast ascending shock testing

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Nano Research 2024年第8期17卷 6777-6784页

作者： Mingquan zhu Shijun Wang Yunxiang Bai Feng Gao Zhenxing zhu Congying Wang Peng Zhang Hao Jin Hui Zhang Luqi Liu Zhiping Xu Xinghong Zhang Fei Wei Zhong Zhang CAS Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China Beijing Key Laboratory of Green Chemical Reaction engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China Department of engineering Mechanics Tsinghua UniversityBeijing 100084China National Key Laboratory of Science and Technology on Advanced Composites in Special environments Center for Composite Materials and StructuresHarbin Institute of TechnologyHarbin 150001China CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Modern MechanicsUniversity of Science and Technology of ChinaHefei 230027China

The exploration of material failure behavior not only involves defining its limits and underlying mechanisms but also entails devising strategies for improvement and protection in extreme ***'ve pioneered an advanced multi-scale,high-speed ascending thermal shock testing platform capable of inducing unprecedented heat shocks at rates surpassing 105℃/*** meticulous examination of the thermal shock responses of carbon nanotube(CNT)films,we've achieved remarkable *** employing an innovative macro-scale synchronous tightening and relaxing approach,we've attained a critical temperature differential in CNT films that exceeds an exceptional 2500℃—surpassing any previously reported metric for highperformance,thermal-shock-resistant ***,these samples have demonstrated exceptional resilience,retaining virtually unchanged strength even after enduring 10,000 thermal shock cycles at temperatures exceeding 1000℃.Furthermore,our research has revealed a novel thermal shock/fatigue failure mechanism that fundamentally diverges from conventional theories centered on thermal stress.

关键词： carbon nanotubes failure behavior thermal shock characterization

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Preface to integrative stratigraphy,biotas,and paleogeographical evolution of the Qinghai-Tibetan Plateau and its surrounding areas

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Science China earth Sciences 2024年第4期67卷 895-898页

作者： Shuzhong SHeN Lin DING Maoyan zhu Xiangdong WANG Tao DeNG State Key Laboratory for Mineral Deposits Research School of Earth Sciences and Engineering and Frontiers Science Center for Critical Earth Material CyclingNanjing UniversityNanjing 210023China State Key Laboratory of Tibetan Plateau earth System Resources and EnvironmentInstitute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China State Key Laboratory of Palaeobiology and Stratigraphy Nanjing Institute of Geology and Palaeontology and Center for Excellence in Life and PalaeoenvironmentChinese Academy of SciencesNanjing 210008China College of earth and Planetary Sciences University of Chinese Academy of SciencesBeijing 100049China Key Laboratory of Vertebrate evolution and Human Origins of Chinese Academy of Sciences Institute of Vertebrate Paleontology and PaleoanthropologyChinese Academy of SciencesBeijing 100044China

The Qinghai-Tibetan Plateau(QTP)is well known as the Roof of the World,the Third Pole and the Asian Water *** spans a vast area from the Pamir Plateau in the west to the Longmenshan-Hengduan Mountains in the east,from the Himalaya Mountains in the south to the Kunlun-Qilian Mountains in the *** stretches approximately 1,200 km from north to south and 2,500 km from east to *** did the QTP start to uplift?This is still controversial between early and late Cenozoic *** some scholars advocated its uplift since the India-Asia continental collision at about 65 million years ago in the Paleogene(e.g.,Ding et al.,2017,2022),and the others suggested its uplift since the Miocene(Zheng and Wu,2018).

关键词： uplift Tibetan north

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explainable-AI-based two-stage solution for WSN object localization using zero-touch mobile transceivers

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Science China(Information Sciences) 2024年第7期67卷 27-45页

作者： Kai FANG Junxin CHeN Han zhu Thippa Reddy GADeKALLU Xiaoping WU Wei WANG School of Mathematics and Computer Science Zhejiang A&F University School of Software Dalian University of Technology Faculty of Applied Sciences Macao Polytechnic University Department of electrical and Computer engineering Lebanese American University School of Information engineering Huzhou University Guangdong-Hong Kong-Macao Joint Laboratory for emotional Intelligence and Pervasive Computing Artificial Intelligence Research Institute Shenzhen MSU-BIT University

Artificial intelligence technology is widely used in the field of wireless sensor networks(WSN).Due to its inexplicability, the interference factors in the process of WSN object localization cannot be effectively eliminated. In this paper, an explainable-AI-based two-stage solution is proposed for WSN object localization. In this solution, mobile transceivers are used to enlarge the positioning range and eliminate the blind area for object localization. The motion parameters of transceivers are considered to be unavailable,and the localization problem is highly nonlinear with respect to the unknown parameters. To address this,an explainable AI model is proposed to solve the localization problem. Since the relationship among the variables is difficult to fully include in the first-stage traditional model, we develop a two-stage explainable AI solution for this localization problem. The two-stage solution is actually a comprehensive consideration of the relationship between variables. The solution can continue to use the constraints unused in the firststage during the second-stage, thereby improving the performance of the solution. Therefore, the two-stage solution has stronger robustness compared to the closed-form solution. experimental results show that the performance of both the two-stage solution and the traditional solution will be affected by numerical changes in unknown parameters. However, the two-stage solution performs better than the traditional solution, especially with a small number of mobile transceivers and sensors or in the presence of high noise. Furthermore,we have also verified the feasibility of the proposed explainable-AI-based two-stage solution.

关键词： explainable AI object localization semidefinite relaxation mobile transceiver two-stage solution closed-form solution

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1D p-type molecular-based coordination polymer semiconductor with ultrahigh mobility

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Science Bulletin 2024年第17期69卷 2705-2711页

作者： Chenhui Yu Xinxu zhu Kefeng Li Guan-e Wang Gang Xu State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China University of Chinese Academy of Sciences Beijing 100049China

One-dimensional(1D)semiconductor nanostructures exhibit exceptional performance in mitigating short-channel effects and ensuring low power ***,the scarcity of high-mobility ptype 1D materials impedes further ***-based materials offer high designability in structure and properties,making them a promising candidate for 1D p-type semiconductor materials.A molecular-based 1D p-type material was developed under the guidance of coordination ***-HT(HT is the abbreviation of p-hydroxy thiophenol)combines the merits of highly orbital overlap between Cu and S,fully covered surface modification with phenol functional groups,and unique cuprophilic(Cu-Cu)*** such,Cu-HT has a remarkable hole mobility of 27.2 cm2V-1s-1,which is one of the highest reported values for 1D molecular-based materials to date and even surpass those of commonly used amorphous silicon as well as the majority of 1D inorganic *** achievement underscores the significant potential of coordination polymers in optimizing carrier transport and represents a major advancement in the synthesis of high-performance,1D p-type semiconductor materials.?2024 Science China *** by elsevier *** Science China *** rights are reserved.

关键词： Molecular-basedmaterials Hole mobility Coordinationpolymer Field-effecttransistors

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A novel optical emission spectroscopy method for diagnostics of contribution of different ionization mechanisms and flux of ions in different valences in discharge channel of a Hall thruster

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Chinese Journal of Aeronautics 2024年第4期37卷 294-307页

作者： Yanfei WANG Ximing zhu Renqiu ZOU Shilin YAN Junwei JIA Zhongxi NING Daren YU School of energy Science and engineering Harbin Institute of TechnologyHarbin 150001China Key Laboratory of Aerospace Plasma Propulsion Ministry of Industry and Information TechnologyHarbin 150001China Beijing Orient Institute of Measurement and Test Beijing 100094China Beijing Aerospace Long March Aircraft Research Institute Beijing 100076China

The mass application of Hall thrusters poses the need for a diagnostic method of ionization mechanism in the discharge channel to boost the iteration and optimization of thruster *** work presents an Optical emission Spectroscopy (OeS) method for diagnostics of the contribution of different ionization mechanisms and the flux of ions in different valences in the discharge channel of a Hall *** emission spectra in the discharge channel are analyzed by jointly utilizing a collisional-radiative model,an ionization-excitation model,and a flux-conservation *** is found that the intensities of some spectral lines can be converted into the reaction rates of collision processes,e.g.,electron-induced excitation and ionization *** latter can further be used to determine the evolutions of particle fluxes by utilizing the conservation law of *** novel method is demonstrated on a kilo-watt Hall *** evolutions of several parameters are determined using this method along the discharge channel,including the ionization rates of different mechanisms,particle fluxes,particle densities,and particle *** novel method can be further developed by being jointly utilized with spectral imaging and tomography techniques,enabling diagnostics of multi-dimensional distributions of the above-mentioned parameters in the discharge channel and near-field plume.

关键词： Hall thruster Optical emission spectroscopy Ionization mechanism Particle flux Divalent ion

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Toughening ultrastrong low-density steel by textured δ-ferrite lamellas

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Defence Technology（防务技术） 2024年第2期32卷 405-411页

作者： Bin Hu Guosen zhu Guohui Shen Zheng Wang Qinghua Wen Xiao Shen Haiwen Luo School of Metallurgical and ecological engineering University of Science and Technology BeijingXue Yuan Rd.30Beijing 100083China Shougang Research Institute of Technology Yangzhuang Street 69Beijing 100043China Steel Institute RWTH Aachen UniversityIntzestraße 152072AachenGermany

By both the Charpy V-notched impact and the projectile tests, we here investigated the dynamic fracture behavior of a recently developed ultrastrong lightweight steel comprising a hierarchical martensitic matrix, dispersed ultra-fine-retained austenite grains and oriented δ-ferrite lamellas, the latter being due to high Al and Si contents employed for low-density design. This steel shows a superior combination of specific ultimate tensile strength and impact toughness to other ultrastrong steels and has successfully arrested a real steel-cored bullet shot. These are attributed to the densely textured δ-ferrite lamellas that can deflect the propagating cracks until they are trapped and enclosed besides austenite-to-martensite transformation crack closure, leading to more energy consumed before failure. These results suggest a new pathway for toughening ultrastrong lightweight steels.

关键词： Ultrastrong and light steel d-Ferrite lamellas Crack propagation Toughness

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elemental Compositions of Clinopyroxenes from Southern Okinawa Trough Basalt:Implications for Magmatism and Structural environment in an Initial Back-Arc Basin

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Journal of Ocean University of China 2024年第3期23卷 643-653页

作者： GUO Kun ZHAI Shikui FAN Di ZHANG Xia ZHANG Yu zhu Zhimin Laoshan Laboratory Qingdao 266237China Key Laboratory of Submarine Geosciences and Prospecting Techniques Ministry of EducationCollege of Marine GeosciencesOcean University of ChinaQingdao 266100China Key Laboratory of Submarine Geosciences&Second Institute of Oceanography Ministry of Natural ResourcesHangzhou 310012China

The major and trace elemental compositions of clinopyroxene from basalt were used to characterize the nature of the primitive magma and structural environment beneath the southern Okinawa Trough(SOT),which is an initial back-arc basin at a continental *** clinopyroxenes in the basalt were augite with variable Mg^(#)contents(73.37-78.22).The regular variations in major oxide contents(i.e.,CaO,FeO,TiO_(2),and Cr)with decreasing Mg#implied that the clinopyroxenes evolved from being enriched in Mg,Ca,and Cr to being enriched in Fe and *** clinopyroxenes had relatively low rare earth element concentrations(7.51×10^(-6) to 12.68×10^(-6))and negative eu anomalies(δeu=0.67-0.95).The Kd_(cpx) values of clinopyroxenes(0.2-0.26),which were used to examine whether the clinopyroxene was equilibrated with its host basalt,demonstrate that these clinopyroxene phenocrysts were not captured crystals but were instead produced by crystallization differentiation of the *** calculated clinopyroxene crystallization temperatures showed a narrow range of 990-1061℃,and their crystallization pressures ranged from 2.0 to 3.2 *** geochemistry features of these clinopyroxenes indicated that the parent magma belonged to the subalkaline tholeiitic magma series and suggested that the magma experienced crystallization differentiation of olivine,plagioclase,and clinopyroxene,where the crystallization of plagioclase occurred earlier than that of *** with geophysical data,this research on primitive magma and its crystallization differentiation from clinopyroxene indicates that the SOT is in the stage of‘seafloor spreading’and that basaltic rocks produced from tholeiitic magma represent the generation of oceanic crust.

关键词： trace elements clinopyroxenes southern Okinawa Trough seafloor spreading back-arc basin

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Strip flatness prediction of cold rolling based on ensemble methods

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Journal of Iron and Steel Research International 2024年第1期31卷 237-251页

作者： Wu-quan Yang Zhi-ting Zhao Liang-yu zhu Xun-yang Gao Li Wang School of Mechanical and Power engineering Shenyang University of Chemical TechnologyShenyang110142LiaoningChina

Aiming at the problem of insufficient prediction accuracy of strip flatness at the outlet of cold tandem rolling,the prediction performance of strip flatness based on different ensemble methods was studied and a high-precision prediction ensemble model of strip flatness at the outlet was ***,based on linear regression(LR),K nearest neighbors(KNN),support vector regression,regression trees(RT),and backpropagation neural network(BPN),bagging,boosting,and stacking ensemble methods were used for ensemble ***,three existing ensemble models,i.e.,random forest,extreme random tree(eT)and extreme gradient boosting,were used to conduct experiments and compare the *** research shows that bagging,boosting,and stacking three ensemble methods have the most significant improvement in the prediction accuracy of the regression trees model,which is increased by 5.28%,6.51%,and 5.32%,*** the same time,the stacking ensemble method improves both the simple model and the complex model,and the improvement effect on the simple base model is the greatest,which is 4.69%higher than that of the base model *** all of the ensemble models,the stacking ensemble model of level-1(eT,AdaBoost-RT,LR,BPN)paired with level-2(LR)was discovered to be the best model(eALB-LR)and can be further studied for industrial applications.

关键词： Tandem cold rolling Flatness prediction Machine learning ensemble method

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Tipping Point Detection Using Reservoir Computing

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Research 2024年第1期2023卷 779-790页

作者： Xin Li Qunxi zhu Chengli Zhao Xuzhe Qian Xue Zhang Xiaojun Duan Wei Lin College of Science National University of Defense TechnologyChangshaHunan 410073China Research Institute of Intelligent Complex Systems and MOe Frontiers Center for Brain Science Fudan UniversityShanghai 200433China Shanghai Artificial Intelligence Laboratory Shanghai 200232China School of Mathematical Sciences SCMSSCAMand CCSBFudan UniversityShanghai 200433China

Detection in high fidelity of tipping points,the emergence of which is often induced by invisible changes in internal structures or/and external interferences,is paramountly beneficial to understanding and predicting complex dynamical systems(CDSs).Detection approaches,which have been fruitfully developed from several perspectives(e.g.,statistics,dynamics,and machine learning),have their own advantages but still encounter difficulties in the face of high-dimensional,fluctuating ***,using the reservoir computing(RC),a recently notable,resource-conserving machine learning method for reconstructing and predicting CDSs,we articulate a model-free framework to accomplish the detection only using the time series observationally recorded from the underlying unknown CDSs.

关键词： computing record ping

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