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A cellulose-based lithium-ion battery separator with regulated ionic transport and high thermal stability for extreme environments

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Nano Research 2025年第1期18卷 315-322页

作者： Kun-Peng Yang Song Xie Zi-meng Han Hao-Cheng Liu Chong-Han Yin Wen-Bin Sun zhang-Chi Ling Huai-Bin Yang De-Han Li Qing-Fang Guan Shu-Hong Yu Department of Chemistry New Cornerstone Science LaboratoryInstitute of Biomimetic Materials&ChemistryAnhui Engineering Laboratory of Biomimetic MaterialsDivision of Nanomaterials&ChemistryHefei National Research Center for Physical Sciences at the MicroscaleUniversity of Science and Technology of ChinaHefei 230026China Institute of Innovative Materials Department of Materials Science and EngineeringDepartment of ChemistrySouthern University of Science and TechnologyShenzhen 518055China

Separators play a critical role in lithium-ion ***,the restrictions of thermal stability and inferior electrical performance in commercial polyolefin separators significantly limit their applications under harsh ***,we report a cellulose-assisted self-assembly strategy to construct a cellulose-based separator massively and *** an ultrahigh ionic conductivity in electrolytes of 3.7 mS·cm^(-1) and the ability to regulate ion transport,the obtained separator is a promising alternative for high-performance lithium-ion *** addition,integrated with high thermal stability,the cellulose-based separator endows batteries with high safety at high temperatures,greatly expanding the application scenarios of energy storage devices in extreme environments.

关键词： lithium-ion batteries bio-inspired materials battery separators cellulose nanofiber ultrahigh ionic conductivity high safety

Metabolic pathway modulation by olanzapine:Multitarget approach for treating violent aggression in patients with schizophrenia

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World Journal of Psychiatry 2025年第1期15卷 37-53页

作者： Yan-Ning Song Shuang Xia Zhi Sun Yong-Chao Chen Lu Jiao Wen-Hua Wan Hong-Wei zhang Xiao Guo Hua Guo Shou-Feng Jia Xiao-Xin Li Shi-Xian Cao Li-Bin Fu meng-meng Liu Tian Zhou Lv-Feng zhang Qing-Quan Jia Department of Pharmacy The Affiliated Encephalopathy Hospital of Zhengzhou University(Zhumadian Second People's Hospital)Zhumadian 463000Henan ProvinceChina Department of Pharmacy The First Affiliated Hospital of Zhengzhou UniversityZhengzhou 450052Henan ProvinceChina Department of Pharmacy Zhumadian First People's HospitalZhumadian 463000Henan ProvinceChina Scientific Education Section The Affiliated Encephalopathy Hospital of Zhengzhou University(Zhumadian Second People's Hospital)Zhumadian 463000Henan ProvinceChina Department of Psychiatry The Affiliated Encephalopathy Hospital of Zhengzhou University(Zhumadian Second People's Hospital)Zhumadian 463000Henan ProvinceChina Clinical Laboratory The Affiliated Encephalopathy Hospital of Zhengzhou University(Zhumadian Second People's Hospital)Zhumadian 463000Henan ProvinceChina Publicity Division The Affiliated Encephalopathy Hospital of Zhengzhou University(Zhumadian Second People's Hospital)Zhumadian 463000Henan ProvinceChina

BACKGROUND The use of network pharmacology and blood metabolomics to study the patho-genesis of violent aggression in patients with schizophrenia and the related drug mechanisms of action provides new directions for reducing the risk of violent aggression and optimizing treatment *** To explore the metabolic regulatory mechanism of olanzapine in treating patients with schizophrenia with a moderate to high risk of violent *** Metabolomic technology was used to screen differentially abundant metabolites in patients with schizophrenia with a moderate to high risk of violent aggression before and after olanzapine treatment,and the related metabolic pathways were *** pharmacology was used to establish protein-protein interaction networks of the core targets of *** Ontology functional analysis and Kyoto Encyclopedia of Genes and Genomes pathway enrichment analysis were subsequently *** Compared with the healthy group,the patients with schizophrenia group presented significant changes in the levels of 24 metabolites related to the disruption of 9 metabolic pathways,among which the key pathways were the alanine,aspartate and glutamate metabolism and arginine biosynthesis *** treatment with olanzapine,the levels of 10 differentially abundant metabolites were significantly reversed in patients with *** effectively regulated six metabolic pathways,among which the key pathways were alanine,aspartate and glutamate metabolism and arginine biosynthesis *** core targets of olanzapine were involved in several key *** The metabolic pathways of alanine,aspartate,and glutamate metabolism and arginine biosynthesis are the key pathways involved in olanzapine treatment for aggressive schizophrenia.

关键词： Schizophrenia Violent aggression Olanzapine Metabolomics Network pharmacology

Establishment of a pig model with enteric and portal venous drainage of pancreatoduodenal transplantation

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World Journal of Gastroenterology 2005年第35期11卷 5475-5479页

作者： Zhao-da zhang Fang-Hai Han Ling-Xiang meng Third GeneralDepartment West China Hospital of Sichuan University Chengdu610041 Sichuan Province China

AIM： To establish the pig model of pancreatoduodena transplantation with enteric drainage （ED） and porta venous drainage （PVD）. METHODS： Forty-six hybrid Landrace pigs were divided into two groups （donors and recipients） randomly, and pancreatoduodenal allotransplantation was performed. Donors were perfused via abdominal aorta without clamping the portal venous outflow with UW solution at 80-100 cm H2O after heparinization. Whole pancreatoduodenal grafts were harvested with segments of abdominal aorta and portal vein, and shaped under 4℃ UW solution. Then, end-to-end anastomosis was performed with the donor iliac artery bifurcation Y graft to the recipient superior mesenteric artery and celiac artery. Furthermore, type I diabetes model was made by removal of the recipient pancreas. The venous anastomosis was reconstructed between the donor portal vein and the recipient superior mesentery vein. Meanwhile, end-toside anastomosis was performed with the donor common iliac artery bifurcation Y graft to the recipient abdominal aorta, and side-to-side intestinal anastomosis was performed between the donor duodenum and the recipient jejunum. External jugular vein was intubated for transfusion. Levels of plasma glucose, insulin and glucagon were measured during the operation and on the 1^st 3^rd 5^th and 7^th d after operation. RESULTS： Pancreatoduodenal allotransplantation was performed on 23 pigs of which 1 died of complication of anesthesia. The success rate of operation was 95.6%. Complications of operation occurred in two cases in which one was phlebothrombosis with an incidence of 4.6%, and the other was duodenojejunal anastomotic leak with an incidence of 4.6%. The level of plasma glucose decreased within 30 min, after removal of pancreas and recovered on the 2^nd after operation. The level of plasmainsulin and glucagon increased within 30 min after removal of pancreas and recovered on the 2^nd d after operation. Rejection occurred on the 1^st and reached the worst le

关键词： Pancreatoduodenal transplantation Entericdrainage Portal venous drainage

Sulfolane‑Based Flame‑Retardant Electrolyte for High‑Voltage Sodium‑Ion Batteries

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Nano-Micro Letters 2025年第2期17卷 498-516页

作者： Xuanlong He Jie Peng Qingyun Lin meng Li Weibin Chen Pei Liu Tao Huang Zhencheng Huang Yuying Liu Jiaojiao Deng Shenghua Ye Xuming Yang Xiangzhong Ren Xiaoping Ouyang Jianhong Liu Biwei Xiao Jiangtao Hu Qianling zhang Graphene Composite Research Center College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhen 518060People’s Republic of China Center of Electron Microscopy State Key Laboratory of Silicon and Advanced Semiconductor MaterialsSchool of Materials Science and EngineeringZhejiang UniversityHangzhou 310027People’s Republic of China GRINM(Guangdong)Research Institute for Advanced Materials and Technology FoshanGuangdong 528051People’s Republic of China College of Energy Engineering Zhejiang UniversityHangzhouZhejiang 310027People’s Republic of China School of Materials Science and Engineering Xiangtan UniversityXiangtan 411105People’s Republic of China Shenzhen Eigen-Equation Graphene Technology Co.Ltd Shenzhen 518000People’s Republic of China

Sodium-ion batteries hold great promise as next-generation energy storage ***,the high instability of the electrode/electrolyte interphase during cycling has seriously hindered the development of *** particular,an unstable cathode–electrolyte interphase(CEI)leads to successive electrolyte side reactions,transition metal leaching and rapid capacity decay,which tends to be exacerbated under high-voltage ***,constructing dense and stable CEIs are crucial for high-performance *** work reports localized high-concentration electrolyte by incorporating a highly oxidation-resistant sulfolane solvent with non-solvent diluent 1H,1H,5H-octafluoropentyl-1,1,2,2-tetrafluoroethyl ether,which exhibited excellent oxidative stability and was able to form thin,dense and homogeneous *** excellent CEI enabled the O3-type layered oxide cathode NaNi_(1/3)Mn_(1/3)Fe_(1/3)O_(2)(NaNMF)to achieve stable cycling,with a capacity retention of 79.48%after 300 cycles at 1 C and 81.15%after 400 cycles at 2 C with a high charging voltage of 4.2 *** addition,its nonflammable nature enhances the safety of *** work provides a viable pathway for the application of sulfolane-based electrolytes on SIBs and the design of next-generation high-voltage electrolytes.

关键词： Sodium-ion batteries Sulfolane-based electrolyte High voltage Layered oxide cathode Flame retardant

Multivariable Dynamic Modeling for Molten Iron Quality Using Incremental Random Vector Functional-link Networks

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Journal of Iron and Steel Research International 2016年第11期23卷 1151-1159页

作者： Li zhang Ping ZHOU He-da SONG meng YUAN Tian-you CHAI State Key Laboratory of Synthetical Automation for Process Industries Northeastern University Department of Mechanical Engineering University of Melbourne

Molten iron temperature as well as Si, P, and S contents is the most essential molten iron quality （MIQ） indices in the blast furnace （BF） ironmaking, which requires strict monitoring during the whole ironmaking production. However, these MIQ parameters are difficult to be directly measured online, and large-time delay exists in off-line analysis through laboratory sampling. Focusing on the practical challenge, a data-driven modeling method was presented for the prediction of MIQ using the improved muhivariable incremental random vector functional-link net- works （M-I-RVFLNs）. Compared with the conventional random vector functional-link networks （RVFLNs） and the online sequential RVFLNs, the M-I-RVFLNs have solved the problem of deciding the optimal number of hidden nodes and overcome the overfitting problems. Moreover, the proposed M I RVFLNs model has exhibited the potential for multivariable prediction of the MIQ and improved the terminal condition for the multiple-input multiple-out- put （MIMO） dynamic system, which is suitable for the BF ironmaking process in practice. Ultimately, industrial experiments and contrastive researches have been conducted on the BF No. 2 in Liuzhou Iron and Steel Group Co. Ltd. of China using the proposed method, and the results demonstrate that the established model produces better estima ting accuracy than other MIQ modeling methods.

关键词： molten iron quality multivariable incremental random vector functional-link network blast furnace iron-making data-driven modeling principal component analysis

Optimization Study on the Blade Profiles of A Horizontal Axis Tidal Turbine Based on BEM-CFD Model

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China Ocean Engineering 2019年第4期33卷 436-445页

作者： zhang da-hai DING Lan HUANG Bin CHEN Xue-meng LIU Jin-tao Ocean College Zhejiang University Zhoushan 316021 China Beijing Institute of Control Engineering Beijing 100190 China

In order to increase the performance of horizontal tidal turbines, a multi-objective optimization model was proposed in this study. Firstly, the prediction model for horizontal tidal turbines was built, which coupled the blade element momentum (BEM) theory and the CFD calculation. Secondly, a multi-objective optimization method coupled the response surface method (RSM) with the multi-objective genetic algorithm NSGA-II was applied to obtain the optimal blade profiles. The pitch angle and the chord length distribution were chosen as the design variables, while the mean power coefficient and the variance of power coefficient were chosen as the objective functions. With the mean power coefficient improved by 4.1% and the variance of power coefficient decreased by 46.7%, results showed that both objective functions could be improved.

关键词： tidal turbine BEM-CFD multi-objective optimization power coefficient

The rhythmic expression of genes controlling flowering time in southern and northern populations of invasive Ambrosia artemisiifolia

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Journal of Plant Ecology 2015年第2期8卷 207-212页

作者： Xiao-meng Li da-Yong zhang Wan-Jin Liao State Key Laboratory of Earth Surface Processes and Resource Ecology and MOE Key Laboratory for Biodiversity Science and Ecological Engineering College of Life SciencesBeijing Normal University19 Xinjiekouwai StreetHaidianBeijing 100875China

Aims Flowering time has been suggested to be an important adaptive trait during the dispersal of invasive species,and identifying the molecu-lar mechanisms underlying flowering time may provide insight into the local adaptation during the process of ***,we con-ducted a preliminary exploration on the genetic basis of the differ-entiation of flowering time in Ambrosia *** using relative real-time fluorescent quantitative polymerase chain reaction,we investigated the expression levels of eight flowering-related genes,including AP1,FT,SOC1,CRY2,FKF1,GI,CO2 and SPY,in leaves and flowers at different time points in individuals from northern beijing and southern Wuhan populations that exhibit significant differences in flowering times to identify any rhythmic changes in gene expression and their association with differential flowering *** Findings The differentiation of flowering time in the *** popula-tions was closely associated with five genes involved in flowering *** floral pathway integrators FT and SOC1 and floral meristem identity gene AP1 exhibited increased expression during *** photoreceptor CRY2 in the light-dependent path-way and the SPY gene in the gibberellin pathway displayed specific expression patterns over *** earlier-flowering beijing plants,CRY2 expression was lower and SPY expression was higher than in Wuhan *** expression patterns of these five genes sug-gest a molecular basis for the differentiation of flowering time in ***.

关键词： Ambrosia artemisiifolia flowering time adaptation flowering pathway gene expression

Balanced solubility product and enthalpies of formation of Nb compounds in 0.09 % oriented silicon steel

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Rare Metals 2013年第3期32卷 318-322页

作者： Hui Li Yun-Li Feng dan zhang meng Song da-Qiang Cang School of Metallurgical and Ecological Engineering University of Science and Technology Beijing School of Metallurgy and Energy Hebei United University

Balance solubility products and enthalpy of for- mation for NbC0.75, NbC0.85, NbC0.88, NbC and NbN in oriented silicon steels were calculated and compared quali- tatively. Meanwhile, the mixing enthalpies of these five Nb compounds were calculated based on Miedema Model. The results show that the solubility products of Nb compounds in ferrite and austenite meet the following relationship, NbC0.75 〉 NbC0.85 〉 NbC0.88 〉 NbC 〉 NbN and NbN has the minimum enthalpy of formation. It indicates that NbN easily precipitate out, but it is more difficult for NbC0.75.

关键词： Oriented silicon steel Nb compounds Solubility formula Enthalpy of formation

A practical synthesis of (-)fosfomycin from its enantiomer

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Chinese Chemical Letters 2008年第11期19卷 1297-1300页

作者： meng zhang Zheng Yu Ji Jun Li da Li Yin Beijing Collab Pharma Co. Ltd. Beijing 102600 China Institute of Materia Medica Peking Union Medical College Beijing 100050 China

（＋）-cis-（1S, 2R）-Epoxypropylphosphonic acid, the enantiomer of fosfomycin, which is the industrial side-product in the preparation of the antibiotic fosfomycin, was converted into （-）fosfomycin by a seven-step procedure. The esterification of the dihydroxyphosphonic intermediate was the key step. The title compound was obtained in good yield and its optical purity was up to the medicine quality standard of Chinese Pharmacopoeia.

关键词： Fosfomycin Enantiomer Phosphonate