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The Observed Near-Surface Energy Exchange Processes over Arctic Glacier in Summer

Journal of Meteorological Research 2024年第3期38卷 600-607页

作者： Libo ZHOU Jinhuan ZHU Linlin KONG Peng LI Shupo MA Fei LI Han ZOU meigen zhang Irina REPINA Department of Lower Atmospheric Observation and Research Institute of Atmospheric PhysicsChinese Academy of Sciences State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of Sciences Department of Weather Forecast Aviation Meteorological Centre of Air Traffic Management BureauCivil Aviation Administration of China A.M.Obukhov Institute of Atmospheric Physics Russian Academy of Sciences (RAS)

Under Arctic warming, near-surface energy transfers have significantly changed, but few studies have focused on energy exchange over Arctic glacier due to limitations in available observations. In this study, the atmospheric energy exchange processes over the Arctic glacier surface were analyzed by using observational data obtained in summer 2019 in comparison with those over the Arctic tundra surface. The energy budget over the glacier greatly differed from that over the tundra, characterized by less net shortwave radiation and downward sensible heat flux,due to the high albedo and icy surface. Most of the incoming solar radiation was injected into the glacier in summer,leading to snow ice melting. During the observation period, strong daily variations in near-surface heat transfer occurred over the Arctic glacier, with the maximum downward and upward heat fluxes occurring on 2 and 6 July 2019,respectively. Further analyses suggested that the maximum downward heat flux is mainly caused by the strong local thermal contrast above the glacier surface, while the maximum upward heat transfer cannot be explained by the classical turbulent heat transfer theory, possibly caused by countergradient heat transfer. Our results indicated that the near-surface energy exchange processes over Arctic glacier may be strongly related to local forcings, but a more indepth investigation will be needed in the future when more observational data become available.

关键词： Arctic glacier tundra energy exchange processes

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A progress review of black carbon deposition on Arctic snow and ice and its impact on climate change

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Advances in Polar Science 2024年第2期35卷 178-191页

作者： zhang Zilu ZHOU Libo zhang meigen Department of Lower Atmosphere Observation Research(LAOR) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China College of Earth and Planetary Science University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China

The rapid warming of the Arctic,accompanied by glacier and sea ice melt,has significant consequences for the Earth’s climate,ecosystems,and economy.Black carbon(BC)deposition on snow and ice can trigger a significant reduction in snow albedo and accelerate melting of snow and ice in the Arctic.By reviewing the published literatures over the past decades,this work provides an overview of the progress in both the measurement and modeling of BC deposition and its impact on Arctic climate change.In summary,the maximum value of BC deposition appears in the western Russian Arctic(26 ng·g^(–1)),and the minimum value appears in Greenland(3 ng·g^(–1)).BC records in the Arctic ice core already peaked in 1920s and 1970s,and shows a regional difference between Greenland and Canadian Arctic.The different temporal variations of Arctic BC ice core records in different regions are closely related to the large variability of BC emissions and transportation processes across the Arctic region.Model simulations usually underestimate the concentration of BC in snow and ice by 2–3 times,and cannot accurately reflect the seasonal and regional changes in BC deposition.Wet deposition is the main removal mechanism of BC in the Arctic,and observations show different seasonal variations in BC wet deposition in Ny-Ålesund and Barrow.This discrepancy may result from varying contributions of anthropogenic and biomass burning(BB)emissions,given the strong influence by BC from BB emissions at Barrow.Arctic BC deposition significantly influences regional climate change in the Arctic,increasing fire activities in the Arctic have made BB source of Arctic BC more crucial.On average,BC in Arctic snow and ice causes an increase of+0.17 W·m^(–2)in radiative forcing and 8 Gt·a^(–1)in runoff in Greenland.As stressed in the latest Arctic Monitoring and Assessment Programme report,reliable source information and long-term and high-resolution observations on Arctic BC deposition will be crucial for a more comprehensive understanding and a better mitigation

关键词： Arctic climate black carbon albedo snow deposition

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Modeling study on seasonal variation in aerosol extinction properties over China

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Journal of Environmental Sciences 2014年第1期26卷 97-109页

作者： Yi Gao meigen zhang State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric Physics Chinese Academy of Sciences

To investigate the seasonal variation of aerosol optical depth （AOD）, extinction coefficient （EXT）, single scattering albedo （SSA） and the decomposed impacts from sulfate （SO42-） and black carbon （BC） over China, numerical experiments are conducted from November 2007 to December 2008 by using WRF-Chem. Comparison of model results with measurements shows that model can reproduce the spatial distribution and seasonal variation of AOD and SSA. Over south China, AOD is largest in spring （0.6-1.2） and lowest in summer （0.2-0.6）. Over north, northeast and east China, AOD is highest in summer while lowest in winter. The high value of EXT under 850 hPa which is the reflection of low visibility ranges from 0.4-0.8 km-1 and the high value area shifts to north during winter, spring and summer, then back to south in autumn. SSA is 0.92-0.94 in winter and 0.94-0.96 for the other three seasons because of highest BC concentration in winter over south China. Over east China, SSA is highest （0.92-0.96） in summer, and 0.88-0.92 during winter, spring and autumn as the concentration of scattering aerosol is highest while BC concentration is lowest in summer over this region. Over north China, SSA is highest （0.9-0.94） in summer and lowest （0.82-0.86） in winter due to the significant variation of aerosol concentration. The SOn2- induced EXT increases about 5%- 55% and the impacts of BC on EXT is much smaller （2%-10%）. The SO42--induced increase in SSA is 0.01-0.08 and the BC-induced SSA decreases 0.02-0.18.

关键词： seasonal variation AOD EXT SSA China WRF-Chem

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Sensitivity analysis of surface ozone to emission controls in Beijing and its neighboring area during the 2008 Olympic Games

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Journal of Environmental Sciences 2012年第1期24卷 50-61页

作者： Yi Gao meigen zhang State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China

The regional air quality modeling system RAMS （Regional Atmospheric Modeling System）-CMAQ （Community Multi-scale Air Quality modeling system） is applied to analyze temporal and spatial variations in surface ozone concentration over Beijing and its surrounding region from July to October 2008.Comparison of simulated and observed meteorological elements and concentration of nitrogen oxides （NOx） and ozone at one urban site and three rural sites during Olympic Games show that model can generally reproduce the main observed feature of wind,temperature and ozone,but NOx concentration is overestimated.Although ozone concentration decreased during Olympics,high ozone episodes occurred on 24 July and 24 August with concentration of 360 and 245 μg/m 3 at Aoyuncun site,respectively.The analysis of sensitive test,with and without emission controls,shows that emission controls could reduce ozone concentration in the afternoon when ozone concentration was highest but increase it at night and in the morning.The evolution of the weather system during the ozone episodes （24 July and 24 August） indicates that hot and dry air and a stable weak pressure field intensified the production of ozone and allowed it to accumulate.Process analysis at the urban site and rural site shows that under favorable weather condition on 24 August,horizontal transport was the main contributor of the rural place and the pollution from the higher layer would be transported to the surface layer.On 24 July,as the wind velocity was smaller,the impact of transport on the rural place was not obvious.

关键词： chemical smoke tropospheric ozone emission control CMAQ process analysis

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The Interannual Variation of Transboundary Contributions from Chinese Emissions of PM_(2.5)to South Korea

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Advances in Atmospheric Sciences 2021年第5期38卷 701-706页

作者： Xiao HAN meigen zhang State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China College of Earth and Planetary Sciences University of Chinese Academy of SciencesBeijing 100049China Center for Excellence in Urban Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China

In recent years,several studies pointed out that anthropogenic emission sources in China which significantly contribute to the PM_(2.5)mass burden was an important cause of particulate pollution in South Korea.However,most studies generally focused upon a single pollution event.It is rare to see comprehensive research that captures those features prone to interannual variations concerning the transboundary pollutant contribution in South Korea using a unified method.In this paper,we establish the emission inventories covering East Asia in 2010,2015,and 2017,and then conduct the source apportionment by applying a coupled regional air quality model called the Integrated Source Apportionment Module(ISAM).Comparison of simulated and observed PM_(2.5)mass concentration at 165 CNEMC(China National Environmental Monitoring Center)sites suggests that the PM_(2.5)concentrations are well represented by the modeling system.The model is used to quantitatively investigate the contribution from emission sources in China to PM_(2.5)concentrations over South Korea and those features found to be prone to interannual variations are then discussed.The results show that the average annual contribution of PM_(2.5)has dropped significantly from 28.0%in 2010 to 15.7%in 2017,which strongly suggests that China has achieved remarkable results in the treatment of atmospheric particulates.

关键词： CMAQ PM_(2.5) transboundary contribution air quality

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Simulation of atmospheric aerosols in East Asia using modeling system RAMS-CMAQ:Model evaluation

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China Particuology 2007年第5期5卷 321-327页

作者： meigen zhang Zhiwei Han Lingyun Zhu State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of Sciences Beijing 100029 China Key Laboratory of Regional Climate Environment Research for Temperate East Asia Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China Graduate School of the Chinese Academy of Sciences Beijing 100049 China Shanxi Province Meteorological Institute Taiyuan 030002 China

The modeling system RAMS-CMAQ is applied in this paper to East Asia to simulate the temporo-spatial concentration distributions of atmospheric aerosols. For evaluating its performances, modeled concentrations of aerosols such as sulfate, nitrate, ammonium, black carbon and organic carbon were compared with observations obtained in East Asia on board of two aircrafts in the springtime of 2001. The comparison showed generally good agreement, and, in particular, that the modeling system captured most of the important observed features, including vertical gradients of the aerosols of the Asian outflow over the western Pacific. The evaluation results provide us with much confidence for further use of the modeling system to investigate the transport and transformation processes of atmospheric aerosols over East Asia and to assess their impacts on the Earth＇s radiation budget.

关键词： East Asia CMAQ TRACE-P ACE-Asia

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Modeling nitrate aerosol distributions and its direct radiative forcing in East Asia with RAMS-CMAQ

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Particuology 2013年第3期11卷 256-263页

作者： Xiao Han meigen zhang Baorong Zhou State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of Sciences Xinghua Meteorological Bureau

The geographical and seasonal characteristics in nitrate aerosol and its direct radiative forcing over East Asia are analyzed by using the air quality modeling system RAMS-CMAQ coupled with an aerosol optical properties/radiative transfer module. For evaluating the model performance, nitrate ion concentration in precipitation, and mixing ratios of PMl0, and some gas precursors of aerosol during the whole year of 2007 are compared against surface observations at 17 stations located in Japan, Korea, and China, and the satellite retrieved NO2 columns, The comparison shows that the simulated values are generally in good agreement with the observed ones. Simulated monthly averaged values are mostly within a factor of 2 of the measurements at the observation stations. The distribution patterns of NO2 from simulation and satellite measurement are also similar with each other. Analysis of the distribution features of monthly and yearly averaged mass concentration and direct radiative forcing （DRF） of nitrate indicates that the nitrate aerosol could reach about 25-30% of the total aerosol mass concentration and DRF in Sichuan Basin, Southeast China, and East China where the high mass burden of all major aerosols concentrated. The highest mass concentration and strongest DRF of nitrate could exceed 40 μg/m^3 and -5 Wire2, respectively. It also indicates that other aerosol species, such as carbonaceous and mineral particles, could obviously influence the nitrate DRF for they are often internally mixed with each other.

关键词： Nitrate aerosolDirect radiative forcing CMAQEAN ET AOD

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Impacts of the meteorological condition versus emissions reduction on the PM_(2.5) concentration over Beijing-Tianjin-Hebei during the COVID-19 lockdown

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Atmospheric and Oceanic Science Letters 2021年第4期14卷 38-44页

作者： Yanqing zhang Zhaokun Ma Yi Gao meigen zhang State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijingChina College of Earth and Planetary Sciences University of Chinese Academy of SciencesBeijingChina Shandong Academy for Environmental Planning JinanChina

本研究从气象条件和减排两方面探讨了COVID-19封锁期间严重雾霾发生的原因[研究目的],并定量的分析了气象条件和减排对PM_(2.5)浓度的相对影响[创新点].使用WRF-Chem在2019年2月3日–16日和2020年2月3日–16日进行了三个数值模拟试验,... 详细信息

本研究从气象条件和减排两方面探讨了COVID-19封锁期间严重雾霾发生的原因[研究目的],并定量的分析了气象条件和减排对PM_(2.5)浓度的相对影响[创新点].使用WRF-Chem在2019年2月3日–16日和2020年2月3日–16日进行了三个数值模拟试验,分别为2019年气象场与MEIC-2019(2019年中国多分辨率月度排放清单),2020年气象场与MEIC-2019,2020年气象场与MEIC-2020[研究方法].结果表明COVID-19封锁期间严重雾霾的原因是不利气象条件增加的PM_(2.5)浓度大于减排减少的PM_(2.5)浓度[重要结论].

关键词： PM_(2.5) WRF-Chem 气象条件减排

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Accounting for CO2 Variability over East Asia with a Regional Joint Inversion System and Its Preliminary Evaluation

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Journal of Meteorological Research 2017年第5期31卷 834-851页

作者： xingxia kou xiangjun tian meigen zhang zhen peng xiaoling zhang institute of urban meteorology china meteorological administrationBeijing 100089 state key laboratory of atmospheric boundary layer physics and atmospheric chemistry institute of atmospheric physicschinese academy of sciencesBeijing 100029 international center for climate and environment sciences institute of atmospheric physicschinese academy of sciencesNanjing 210093 school of atmospheric sciences nanjing university school of atmospheric sciences chengdu university of information technologyChengdu 610225

A regional surface carbon dioxide （C02） flux inversion system, the Tan-Tracker-Region, was developed by incor- porating an assimilation scheme into the Community Multiscale Air Quality （CMAQ） regional chemical transport model to resolve fine-scale CO2 variability over East Asia. The proper orthogonal decomposition-based ensemble four-dimensional variational data assimilation approach （POD-4DVar） is the core algorithm for the joint assimilation framework, and simultaneous assimilations of CO2 concentrations and surface CO2 fluxes are applied to help reduce the uncertainty in initial CO2 concentrations. A persistence dynamical model was developed to describe the evolu- tion of the surface CO2 fluxes and help avoid the ＂signal-to-noise＂ problem; thus, CO2 fluxes could be estimated as a whole at the model grid scale, with better use of observation information. The performance of the regional inversion system was evaluated through a group of single-observation-based observing system simulation experiments （OSSEs）. The results of the experiments suggest that a reliable performance of Tan-Tracker-Region is dependent on certain assimilation parameter choices, for example, an optimized window length of approximately 3 h, an ensemble size of approximately 100, and a covariance localization radius of approximately 320 km. This is probably due to the strong diurnal variation and spatial heterogeneity in the fine-scale CMAQ simulation, which could affect the perform- ance of the regional inversion system. In addition, because all observations can be artificially obtained in OSSEs, the performance of Tan-Tracker-Region was further evaluated through different densities of the artificial observation net- work in different CO2 flux situations. The results indicate that more observation sites would be useful to systematic- ally improve the estimation of CO2 concentration and flux in large areas over the model domain. The work presented here forms a foundation for future research in which a thorough estimation of CO2 flux variabili

关键词： surface CO2 flux inversion proper orthogonal decomposition （PDO） four-dimensional variational dataassimilation （4DVar） joint assimilation regional transport model

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NUMERICAL SIMULATION WITH A COMPREHENSIVE CHEMICAL TRANSPORT MODEL OF NITRATE,SULFATE,AND AMMONIUM AEROSOL DISTRIBUTIONS OVER EAST ASIA

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China Particuology 2005年第5期3卷 255-259页

作者： meigen zhang State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 P.R.China

The transport and chemical production processes of nitrate, sulfate, and ammonium aerosols over East Asia were investigated by use of the Models-3 Community Multi-scale Air Quality （CMAQ） modeling system coupled with the Regional Atmospheric Modeling System （RAMS）. For the evaluation of the model＇s ability in depicting their 3-dimensional concentration distributions and temporal variations, modeled concentrations of nitrate, sulfate, and ammonium aerosols are compared with the observations obtained at a ground station in Japan in March 2001 and onboard of an aircraft DC-8 on 18 and 21 March 2001 during the Transport and Chemical Evolution over the Pacific （TRACE-P） field campaign. Comparison shows that simulated values of nitrate, sulfate, and ammonium aerosols are generally in good agreement with their observed data, and the model captures most important observed features, and reproduces temporal and spatial variations of nitrate, sulfate, and ammonium aerosol concentrations reasonably well, e.g., the timing and locations of the concentration spikes of nitrate, sulfate, and ammonium aerosols are well reproduced, but large discrepancies between observed and simulated values are also clearly seen at some points and some times due to the coarse grid resolution and uncertainties of the emissions used in this study. This comparison results indicate that CMAQ is able to simulate the distributions of nitrate, sulfate, and ammonium aerosols and their related species in the troposphere over East Asia reasonably well.

关键词： long-range transport regional pollution Community Multi-scale Air Quality （CMAQ） East Asia

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