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Nonlinear Rydberg exciton-polaritons in Cu2O microcavities

Light(Science & Applications) 2024年第4期13卷 619-627页

作者： Maxim Makhonin Anthonin Delphan Kok Wee Song Paul Walker Tommi Isoniemi Peter Claronino Konstantinos Orfanakis Sai Kiran Rajendran Hamid Ohadi Julian Heckötter Marc Assmann Manfred Bayer Alexander Tartakovskii maurice skolnick Oleksandr Kyriienko Dmitry Krizhanovskii Department of Physics and Astronomy University of SheffieldSheffield S37RHUK. Department of Physics and Astronomy University of ExeterStocker RoadExeter EX44PYUK. SUPA School of Physics and AstronomyUniversity of St AndrewsSt Andrews KY169SSUK. Fakultät Physik TU DortmundAugust-Schmidt-Straße 444227 DortmundGermany

Rydberg excitons(analogues of Rydberg atoms in condensed matter systems)are highly excited bound electron-hole states with large Bohr *** interaction between them as well as exciton coupling to light may lead to strong optical nonlinearity,with applications in sensing and quantum information ***,we achieve strong effective photon–photon interactions(Kerr-like optical nonlinearity)via the Rydberg blockade phenomenon and the hybridisation of excitons and photons forming polaritons in a Cu2O-filled *** pulsed resonant excitation polariton resonance frequencies are renormalised due to the reduction of the photon-exciton coupling with increasing exciton *** analysis shows that the Rydberg blockade plays a major role in the experimentally observed scaling of the polariton nonlinearity coefficient as∝n4.4±1.8 for principal quantum numbers up to n=*** high principal quantum numbers studied in a polariton system for the first time are essential for realisation of high Rydberg optical nonlinearities,which paves the way towards quantum optical applications and fundamental studies of strongly correlated photonic(polaritonic)states in a solid state system.

关键词： density Rydberg polar

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Observation of Zitterbewegung in photonic microcavities

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Light(Science & Applications) 2023年第6期12卷 1084-1090页

作者： Seth Lovett Paul M.Walker Alexey Osipov Alexey Yulin Pooja Uday Naik Charles E.Whittaker Ivan A.Shelykh maurice S.skolnick Dmitry N.Krizhanovskii Department of Physics and Astronomy University of SheffieldS37RH SheffieldUK Department of Physics and Technology ITMO UniversitySt.Petersburg 197101Russia Science Institute University of IcelandDunhagi 3IS-107 ReykjavikIceland

We present and experimentally study the effects of the photonic spin–orbit coupling on the real space propagation of polariton wavepackets in planar semiconductor microcavities and polaritonic analogues of *** particular,we demonstrate the appearance of an analogue Zitterbewegung effect,a term which translates as‘trembling motion’in English,which was originally proposed for relativistic Dirac electrons and consisted of the oscillations of the centre of mass of a wavepacket in the direction perpendicular to its *** a planar microcavity,we observe regular Zitterbewegung oscillations whose amplitude and period depend on the wavevector of the *** then extend these results to a honeycomb lattice of coupled microcavity *** to the planar cavity,such lattices are inherently more tuneable and versatile,allowing simulation of the Hamiltonians of a wide range of important physical *** observe an oscillation pattern related to the presence of the spin-split Dirac cones in the *** both cases,the experimentally observed oscillations are in good agreement with theoretical modelling and independently measured bandstructure parameters,providing strong evidence for the observation of Zitterbewegung.

关键词： planar versatile analogues

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Spatiotemporal continuum generation in polariton waveguides

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Light(Science & Applications) 2019年第1期8卷 1117-1127页

作者： Paul M.Walker Charles E.Whittaker Dmitry V.Skryabin Emiliano Cancellieri Ben Royall Maksym Sich Ian Farrer David A.Ritchie maurice S.skolnick Dmitry N.Krizhanovskii Department of Physics and Astronomy University of SheffieldSheffield S37RHUK Department of Physics University of BathBath BA27AYUK ITMO University Kronverksky Avenue 49St.Petersburg 197101Russia Department of Physics Lancaster UniversityLancaster LA14YBUK Department of Electronic and Electrical Engineering University of SheffieldSheffield S37HQUK Cavendish Laboratory University of CambridgeCambridge CB30HEUK

We demonstrate the generation of a spatiotemporal optical continuum in a highly nonlinear exciton–polariton waveguide using extremely low excitation powers(2-ps,100-W peak power pulses)and a submillimeter device suitable for integrated optics *** observe contributions from several mechanisms over a range of powers and demonstrate that the strong light–matter coupling significantly modifies the physics involved in all of *** experimental data are well understood in combination with theoretical *** results are applicable to a wide range of systems with linear coupling between nonlinear oscillators and particularly to emerging polariton devices that incorporate materials,such as gallium nitride and transition metal dichalcogenide monolayers that exhibit large light–matter coupling at room *** open the door to low-power experimental studies of spatiotemporal nonlinear optics in submillimeter waveguide devices.

关键词： millimeter waveguide optics

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Nonlinear polaritons in a monolayer semiconductor coupled to optical bound states in the continuum

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Light(Science & Applications) 2020年第1期9卷 1480-1487页

作者： Vasily Kravtsov Ekaterina Khestanova Fedor A.Benimetskiy Tatiana Ivanova Anton K.Samusev Ivan S.Sinev Dmitry Pidgayko Alexey M.Mozharov Ivan S.Mukhin Maksim S.Lozhkin Yuri V.Kapitonov Andrey S.Brichkin Vladimir D.Kulakovskii Ivan A.Shelykh Alexander I.Tartakovskii Paul M.Walker maurice S.skolnick Dmitry N.Krizhanovskii Ivan V.Iorsh ITMO University Saint Petersburg 197101Russia St.Petersburg Academic University Saint Petersburg 194021Russia Saint Petersburg State University ul.Ulyanovskaya 1Saint Petersburg 198504Russia Institute of Solid State Physics RASChernogolovka 142432Russia Science Institute University of IcelandDunhagi 3IS-107ReykjavikIceland Department of Physics and Astronomy University of SheffieldSheffield S37RHUK

Optical bound states in the continuum(BICs)provide a way to engineer very narrow resonances in photonic *** extended interaction time in these systems is particularly promising for the enhancement of nonlinear optical processes and the development of the next generation of active optical ***,the achievable interaction strength is limited by the purely photonic character of optical ***,we mix the optical BIC in a photonic crystal slab with excitons in the atomically thin semiconductor MoSe_(2) to form nonlinear exciton-polaritons with a Rabi splitting of 27 meV,exhibiting large interaction-induced spectral *** asymptotic BIC-like suppression of polariton radiation into the far field toward the BIC wavevector,in combination with effective reduction of the excitonic disorder through motional narrowing,results in small polariton linewidths below 3 *** with a strongly wavevector-dependent Q-factor,this provides for the enhancement and control of polariton–polariton interactions and the resulting nonlinear optical effects,paving the way toward tuneable BIC-based polaritonic devices for sensing,lasing,and nonlinear optics.

关键词： polar nonlinear continuum

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