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Enhancement of coercivity,permeability,and dielectric properties of Co_(0.2)Zn_(0.3)Ni_(0.5)Eu_(x)Fe_(2-x)O_(4) ferrites for memory and high frequency devices

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Journal of Rare Earths 2024年第6期42卷 1128-1135,I0005页

作者： I.Sardar M.d.Hossain M.S.Sikder M.N.I.Khan M.R.Rahman Physics discipline Khulna UniversityKhulna9208Bangladesh department of Physics Khulna University of Engineering&TechnologyKhulna9203Bangladesh department ofComputer Science and Engineering Northern University of Business&Technology KhulnaKhulna9100Bangladesh Material Science division Atomic Energy CentreDhaka1000Bangladesh

Spinel cubic ferrites have huge applications in me mory and high frequency *** the improvement of these modern devices,the magnetic coercivity,permeability,and dielectric properties of a ferrite are the important *** article focuses on improving the magnetic coercivity,magnetic permeability,and dielectric properties of Co_(0.2)Zn_(0.3)Ni_(0.5)Eu_(x)Fe_(2-x)O_(4) ferrites,where x=0.00,0.06,and *** X-ray diffraction(XRd),Fourier transform infrared spectroscopy(FTIR),field emission scanning electron microscopy(FESEM),energy dispersive X-ray(EdX),vibrating sample magnetometer(VSM),and an impedance analyzer were used to characterize the structural,magnetic,and dielectric properties of the *** XRd patterns indicate the formation of spinel cubic structure of the samples with a secondary peak(EuFeO_(3))for Eu doped *** densities and porosities of the samples follow an inverse trend,where the doped samples’lattice parameters are increased with the increment of rare earth Eu *** FTIR analysis also proves the spinel cubic phase of the *** average grain size of the ferrites is obtained via FESEM images,and it is increased from 121 to 198 *** analysis confirms that doping of the Eu content also changes other hysteresis loop properties of Co_(0.2)Zn_(0.3)Ni_(0.5)Eu_(x)Fe_(2-x)O_(4) ***,the coercivity of the Eu doped samples is greater than that of the mother alloy(x=0.00).The EdX study shows that there is no impurity contamination in the *** permeability and dielectric measurements show an improved quality factor of the Eu-doped samples with low magnetic and dielectric *** dependent resistivity and impedance analysis also show the improved *** the observed properties of the samples,all the investigated ferrites might be strong candidates for potential applications in memory devices,magnetic sensors,and high frequency applications.

关键词： Ferrites Raree arths Coercivity Permeability EdX Resistivity

Highly defective dark TiO_(2) Modified with Pt: Effects of Precursor Nature and Preparation Method on Photocatalytic Properties

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Transactions of Tianjin University 2024年第2期30卷 198-209页

作者： E.d.Fakhrutdinova O.A.Reutova T.A.Bugrova I.Yu.Ovsyuk L.S.Kibis O.A.Stonkus d.B.Vasilchenko O.V.Vodyankina V.A.Svetlychnyi National Research Tomsk State University TomskRussia 634050 Novosibirsk State University NovosibirskRussia 630090 Boreskov Institute of Catalysis NovosibirskRussia 630090 Nikolaev Institute of Inorganic Chemistry NovosibirskRussia 630090

The study focused on the modification with platinum of dark defective titania obtained via pulsed laser ablation. Both the method of Pt introduction and the nature of the Pt precursor were varied. All samples exhibited similar phase compositions, specific surface areas, and Pt contents. High-resolution transmission electron microscopy coupled with pulsed CO adsorption revealed increased dispersity when photoreduction and the hydroxonitrate complex (Me _(4) N) _(2) [Pt _(2) (OH) _(2) (NO _(3) ) _(8) ] were used. The sample featured a high content of single-atom species and subnano-sized Pt clusters. The X-ray photoelectron spectroscopy results showed that the photoreduction method facilitated the appearance of a larger number of Pt ^(2+) states, which appeared owing to the strong metal-support interaction (SMSI) eff ect of the transfer of electron density from the electron-saturated defects on the TiO _(2) surface to Pt ^(4+) . In the hydrogen evolution reaction, samples with a significant fraction of the Pt ^(2+) ionic component, capable of generating short-lived Pt^(0) single-atom sites under irradiation due to the SMSI eff ect, exhibited the highest photocatalytic activity. The 0.5Pt(C)/TiO_(2) -Ph sample exhibited the highest hydrogen yield with a quantum efficiency of 0.53, retaining its activity even after 8 h of operation.

关键词： dark(black)TiO_(2) Pulsed laser ablation Platinum reduction method Precursor type Photocatalysis Hydrogen evolution reaction

Molecular docking Studies on Streptomycin Antileishmanial Activity

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Open Journal of Physical Chemistry 2024年第2期14卷 36-48页

作者： Todd A. Young matthew George Jr. Ayele Gugssa William M. Southerland Yayin Fang Clarence M. Lee department of Biology Howard University Washington DC United States department of Biochemistry and Molecular Biology Howard University Washington DC United States

Resistance to pentavalent antimonial drugs and the lack of vaccines make it urgent to find novel therapeutic options to treat Leishmaniasis, a tropical disease caused by the Leishmania protozoan parasite. The study reported here is to investigate if Streptomycin, an aminoglycoside, and Amphotericin B, the second-line treatment drug, exhibit antileishmanial activity through a similar mechanism. By using MOE (Molecular Operating Environment), we performed molecular docking studies on these drugs binding to a range of targets including ribosome targets in Leishmania and H. sapiens. Our study shows that the two drugs do not bind to the same pockets in Leishmania targets but to the same pockets in the human ribosome, with some differences in interactions. Moreover, our 2d maps indicated that Amphotericin B binds to the A-site in the human cytoplasmic ribosome, whereas streptomycin does not.

关键词： Leishmaniasis Streptomycin Amphotericin B Molecular docking Aminoglycosides Antileishmanial

Experimental measurements of gamma-photon production and estimation of electron/positron production on the PETAL laser facility

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Matter and Radiation at Extremes 2024年第5期9卷 32-47页

作者： F.Brun L.Ribotte G.Boutoux X.davoine P.E.Masson-Laborde Y.Sentoku N.Iwata N.Blanchot d.Batani I.Lantuéjoul L.Lecherbourg B.Rosse C.Rousseaux B.Vauzour d.Raffestin E.d’Humières X.Ribeyre Centre Lasers Intenses et Applications UMR 5107Universitéde Bordeaux-CNRS-CEA33405 TalenceFrance CEA DAMCESTAF-33116 Le BarpFrance CEA DAMDIFF-91297 ArpajonFrance CEA LMCEUniversitéParis-Saclay91680 Bruyères-le-ChâtelFrance Institute of Laser Engineering Osaka University2-6 YamadaokaSuitaOsaka 565-0871Japan

This article reports the first measurements of high-energy photons produced with the high-intensity PETawatt Aquitaine Laser(PETAL)*** experiments were performed during the commissioning of the *** laser had an energy of about 400 J,an intensity of 8×10^(18)W cm^(−2),and a pulse duration of 660 fs(FWHM).It was shot at a 2 mm-thick solid tungsten *** high-energy photons were produced mainly from the bremsstrahlung process for relativistic electrons accelerated inside a plasma generated on the front side of the *** paper reports measurements of electrons,protons and *** electrons up to35 MeV with a few-MeV temperature were recorded by a spectrometer,called SESAME(SpectreÉlectronS Angulaire MoyenneÉnergie).K-and L-shells were clearly detected by a photon spectrometer called SPECTIX(Spectromètre PetalàCristal en TransmIssion pour le rayonnnement X).High-energy photons were diagnosed by CRACC-X(Cassette de RAdiographie Centre Chambre-rayonnement X),a bremsstrahlung *** cannon analysis is strongly dependent on the hypothesis adopted for the spectral *** shapes can exhibit similar reproductions of the experimental *** eliminate dependence on the shape hypothesis and to facilitate analysis of the data,simulations of the interaction were *** model the mechanisms involved,a simulation chain including hydrodynamic,particle-in-cell,and Monte Carlo simulations was *** simulations model the preplasma generated at the front of the target by the PETAL laser prepulse,the acceleration of electrons inside the plasma,the generation of MeV-range photons from these electrons,and the response of the detector impacted by the energetic photon *** this work enabled reproduction of the experimental *** high-energy photons produced have a large emission angle and an exponential distribution *** addition to the analysis of the photon spectra,positron production was also ***,if high

关键词： process positron hypothesis

Community-Level Practice Checklists for Health Protection during Cold Spells in China

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China CdC weekly 2024年第5期6卷 83-87页

作者： Jing Shang Mengzhen Zhao Zhao Liu Xiya Zhang Shiguang Miao Ishaq d.Sulaymon Wenjia Cai Institute of Urban Meteorology CMABeijingChina School of Management and Economics Beijing Institute of TechnologyBeijingChina School of Airport Economics and Management Beijing Institute of Economics and ManagementBeijingChina department of Earth System Science Tsinghua UniversityBeijingChina Sand and dust Storm Warning Regional Center National Center for MeteorologyJeddahSaudi Arabia Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science and TechnologyNanjing CityJiangsu ProvinceChina

Communities play a crucial role in protecting the health of vulnerable populations such as the elderly,low-income groups,and high-risk individuals during cold ***,current strategies for responding to cold spells primarily consist of programmatic policies that lack practicality,specificity,and detailed implementation guidelines for community ***,this study aims to identify and analyze the challenges faced by communities in responding to cold spells,review international experiences,and develop a set of practical checklists for community-level health *** checklists will assist community workers and volunteers in effectively preparing for,responding to,and recovering from cold spells.

关键词： preparing income primarily

Photosynthetic response to a winter heatwave in leading and trailing edge populations of the intertidal red alga Corallina offi-cinalis(Rhodophyta)

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Acta Oceanologica Sinica 2024年第7期43卷 70-77页

作者： Regina Kolzenburg Federica Ragazzola Laura Tamburello Katy R.Nicastro Christopher d.McQuaid Gerardo I.Zardi UmeåMarine Sciences Centre UmeåUniversity90571 NorrbynSweden University of Portsmouth Institute of Marine SciencePortsmouth PO49LYUK Stazione Zoologica Anton dohrn Genova Marine CenterGenova 16126Italy Stazione Zoologica Anton dohrn Sicily Marine CenterPalermo 90149Italy department of Zoology and Entomology Rhodes UniversityMakhanda(Grahamstown)6139South Africa Centre of Marine Sciences University of AlgarveFaro 8005-139Portugal Laboratoire d’Océanologie et de Géosciences Universitéde LilleLille 59000France Universitéde Caen Normandie Laboratoire de Biologie des Organismes et des Ecosystèmes AquatiquesCaen 14032France

Marine heatwaves(MHWs)caused by anthropogenic climate change are becoming a key driver of change at the ecosystem *** conditions experienced by marine organisms across their distribution,particularly towards the equator,are likely to approach their physiological limits,resulting in extensive mortality and subsequent changes at the population *** at the margins of their species’distribution are thought to be more sensitive to climate-induced environmental pressures than central populations,but our understanding of variability in fitness-related physiological traits in trailing versus leading-edge populations is *** a laboratory simulation study,we tested whether two leading(Iceland)and two trailing(Spain)peripheral populations of the intertidal macroalga Corallina officinalis display different levels of maximum potential quantum efficiency(Fv/Fm)resilience to current and future winter MHWs *** study revealed that ongoing and future local winter MHWs will not negatively affect leading-edge populations of ***,which exhibited stable photosynthetic efficiency throughout the *** edge populations showed a positive though non-significant trend in photosynthetic efficiency throughout winter MHWs *** and equatorward populations did not produce significantly different results,with winter MHWs having no negative affect on Fv/Fm of either ***,we found no long-term regional or population-level influence of a winter MHWs on this species’photosynthetic ***,we found no statistically significant difference in thermal stress responses between leading and trailing ***,*** showed a trend towards higher stress responses in southern than northern *** responses rest on a variety of local population traits,they are difficult to predict based solely on thermal pressures.

关键词： marginal population coralline algae climate change ecophysiology photophysiology macroalgae Fv/Fm

Advanced strategies for marine antifouling based on nanomaterial-enhanced functional PdMS coatings

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Nano Materials Science 2024年第4期6卷 375-395页

作者： Xiaohui Shi Hao Wei Wenjun Zhou Paul E.d.Soto Rodriguez Cunguo Lin Lei Wang Zhijia Zhang School of Materials Science and Chemical Engineering Harbin Engineering University Qingdao Innovation and development Center of Harbin Engineering University State Key Laboratory for Marin Corrosion and Protection Luoyang Ship Material Research Institute (LSMRI) Instituto de Estudios Avanzados IUdEA Departamento de Física Universidad de La Laguna C/Astrofísico Francisco Sanchez School of Chemistry and Chemical Engineering Harbin Institute of Technology

Marine biofouling seriously affects human marine exploitation and transportation activities, to which marine antifouling(AF) coatings are considered to be the most cost-effective solution. Since the mid-20th century, human beings have dedicated their efforts on developing AF coatings with long cycle and high performance, leading to a large number of non-target organisms? distortion, death and marine environmental pollution. Polydimethylsiloxane(PdMS), is considered as one of the representative environment-friendly AF materials thanks to its non-toxic, hydrophobic, low surface energy and AF properties. However, PdMS AF coatings are prone to mechanical damage, weak adhesion strength to substrate, and poor static AF effect, which seriously restrict their use in the ocean. The rapid development of various nanomaterials provides an opportunity to enhance and improve the mechanical properties and antifouling properties of PdMS coating by embedding *** on our research background and the problems faced in our laboratory, this article presents an overview of the current progress in the fields of PdMS composite coatings enhanced by different nanomaterials, with the discussion focused on the advantages and main bottlenecks currently encountered in this field. Finally, we propose an outlook, hoping to provide fundamental guidance for the development of marine AF field.

关键词： Nanomaterials Antifouling PdMS composites Environment-friendly Marine biofouling

Quantitative Mapping of Transient Thermodynamic States in Ultrafast Laser Nanostructuring of Quartz

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Ultrafast Science 2024年第2期4卷 9-18页

作者： H.d.Nguyen A.Tsaturyan S.Sao Joao R.dwivedi A.Melkonyan C.d’Amico E.Kachan J.P.Colombier G.Kermouche R.Stoian Laboratoire Hubert Curien UMR 5516 CNRSUniversite Jean Monnet42000 Saint EtienneFrance Laboratoire George Friedel UMR 5307 CNRSEcole des Mines de Saint Etienne42000 Saint EtienneFrance

Understanding material structural reaction to light is of utmost importance to advance processing resolution in ultrafast laser volume structuring into the *** thermodynamic pathways are required to quench energy transport in the most rapid manner and to confine the process to nanometer lengths,bypassing optical *** material dynamics under confinement,with in situ access to transient local temperature and density parameters,thus becomes key in understanding the *** report in situ reconstruction of thermodynamic states over the entire matter relaxation path in bulkα-quartz irradiated by ultrafast nondiffractive laser beams using time-resolved qualitative and quantitative optical phase *** dynamics indicate rapid spatially confined crystalline-to-amorphous transition to a hot dense fused silica *** exceeds 20%and the matrix temperature rises to more than 2,000 K in the first *** structural state relaxes in hundreds of *** dispersion and time design of the optical beam to picosecond durations increases the spatial confinement and triggers an extreme nanostructuring process based on nanocavitation that occurs within the amorphizing material,where the low-viscosity phase lowers the mechanical requirements for the *** feature scales of less than a tenth of the optical wavelength are obtained in the *** allows for structural and morphological nanoscale material features under 3d confinement that can engineer optical materials.

关键词： Quartz hundreds qualitative

A Room-Temperature Chloride-Conducting Metal-Organic Crystal[Al(dMSO)_(6)]Cl_(3) for Potential Solid-State Chloride-Shuttle Batteries

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Energy & Environmental Materials 2024年第1期7卷 107-113页

作者： Bing Wu Jan Luxa Jiří Šturala Shuangying Wei Lukáš děkanovský Abhilash Karuthedath Parameswaran Min Li Zdenek Sofer department of Inorganic Chemistry University of Chemistry and Technology PragueTechnická 516628Prague Czech Republic

The growing demand for substitutes of lithium chemistries in battery leads to a surge in budding novel anion-based electrochemical energy storage,where the chloride ion batteries(CIBs)take over the *** application of CIBs is limited by the dissolution and side reaction of chloride-based electrode materials in a liquid *** the flipside,its solid-state electrolytes are scarcely reported due to the challenge in realizing fast Cl^(-)*** present study reports[Al(dMSO)_(6)]Cl_(3),a solid-state metal-organic material,allows chloride ion *** strong Al-Cl bonds in AlCl_(3)are broken down after coordinating of Al^(3+)by ligand dMSO,and Cl^(-)in the resulting compound is weakly bound to complexions[Al(dMSO)_(6)]^(3+),which may facilitate Cl^(-)*** partial replacement of Cl^(-)with PF_(6)^(-),the room-temperature ionic conductivity of as-prepared electrolyte is increased by one order of magnitude from 2.172×10^(-5)S cm^(-1)to 2.012×10^(-4)S cm^(-1).When they are assembled with Ag(anode)/Ag-AgCl(cathode)electrode system,reversible electrochemical redox reactions occur on both sides,demonstrating its potential for solid-state chloride ion *** strategy by weakening the bonding interaction using organic ligands between Cl^(-)and central metallic ions may provide new ideas for developing solid chloride-ion conductors.

关键词： [Al(dMSO)_(6)]Cl_(3) chloride-ion batteries ionic conductivity metal-organic solid-state electrolytes