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Large-area flexible nanostripe electrodes featuring plasmon hybridization engineering

Nano Research 2021年第3期14卷 858-867页

作者： Carlo Mennucci Debasree Chowdhury Giacomo Manzato matteo barelli Roberto Chittofrati Christian Martella Francesco Buatier de Mongeot Dipartimento di Fisica Universitàdegli Studi di Genovavia Dodecaneso 33I-16146GenovaItaly

Multifunctional flexible Au electrodes based on one-dimensional(1D)arrays of plasmonic gratings are nanofabricated over large areas with an engineered variant of laser interference lithography optimized for low-cost transparent *** nanostripe(NS)arrays achieve sheet resistance in the order of 20 Ohm/square on large areas(∼cm^(2))and are characterized by a strong and dichroic plasmonic response which can be easily tuned across the visible(VIS)to near-infrared(NIR)spectral range by tailoring their cross-sectional *** vertically a second nanostripe,separated by a nanometer scale dielectric gap,we form near-field coupled Au/SiO_(2)/Au dimers which feature hybridization of their localized plasmon resonances,strong local field-enhancements and a redshift of the resonance towards the NIR *** possibility to combine excellent transport properties and optical transparency on the same plasmonic metasurface template is appealing in applications where low-energy photon management is mandatory like e.g.,in plasmon enhanced spectroscopies or in photon harvesting for ultrathin photovoltaic *** remarkable lateral order of the plasmonic NS gratings provides an additional degree of freedom for tailoring the optical response of the multifunctional electrodes via the excitation of surface lattice resonances,a Fano-like coupling between the broad localised plasmonic resonances and the collective sharp Rayleigh modes.

关键词： nanofabrication nanostripes transparent electrodes plasmonic dimers interference lithography surface lattice resonances

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Plasmon hybridization engineering in self-organized anisotropic metasurfaces

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Nano Research 2018年第7期11卷 3943-3956页

作者： Maria C. Giordano Stefano Longhi matteo barelli Andrea Mazzanti Francesco Buatier de Mongeot Giuseppe Della Valle Dipartimento di Fisica Universita di Genova Via Dodecaneso 33 Genova I-16146 Italy Dipartimento di Fisica and IFN-CNR Politecnico di Milano Piazza L. da Vinci 32 Milano 1-20133 Italy

The engineering of self-organized plasmonic metasurfaces is demonstrated using a maskless technique with defocused ion-beam sputtering and kinetically controlled deposition. The proposed reliable, cost-effective, and controllable approach enables large-area （order of square centimeter） sub-wavelength periodic patterning with close-packed gold nanostrips. A multi-level variant of the method leads to high-resolution manufacturing of vertically stacked nanostrip dimer arrays, without resorting to lithographic approaches. The design of these self-organized metasurfaces is optimized by employing plasmon hybridization methods. In particular, preliminary results on the so-called gap-plasmon configuration of the nanostrip dimers, implementing magnetic dipole resonance in the near-infrared range, are reported. This resonance offers a superior sensitivity and field enhancement, compared with the more conventional electric dipole resonance. The translational invariance of the nanostrip configuration leads to a high filling factor of the hot spots. These advanced features make the large-area metasurface based on gap-plasmon nanostrip dimers very attractive for surface-enhanced linear and nonlinear spectroscopy （e.g., surface-enhanced Raman scattering） and plasmon-enhanced photon harvesting in solar and photovoltaic cells.

关键词： metasurfaces self-organization gold nanostructures plasmon hybridization gap plasmon resonances

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