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High‑Entropy Layered Oxide Cathode Enabling High‑Rate for Solid‑State Sodium‑Ion Batteries

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Nano-Micro Letters 2024年第1期16卷 160-171页

作者： Tianxun cai Mingzhi cai Jinxiao Mu Siwei Zhao hui Bi Wei Zhao Wujie Dong Fuqiang Huang State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050People’s Republic of China State Key Laboratory of Rare Earth Materials Chemistry and Applications College of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871People’s Republic of China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049People’s Republic of China Zhongke Institute of Strategic Emerging Materials Yixing 214213JiangsuPeople’s Republic of China

Na-ion O3-type layered oxides are prospective cathodes for Na-ion batteries due to high energy density and ***,such cathodes usually suffer from phase transitions,sluggish kinetics and air instability,making it difficult to achieve high performance solid-state sodium-ion ***,the high-entropy design and Li doping strategy alleviate lattice stress and enhance ionic conductivity,achieving high-rate performance,air stability and electrochemically thermal stability for Na_(0.95)Li_(0.06)Ni_(0.25)Cu_(0.05)Fe_(0.15)Mn_(0.49)O_(2).This cathode delivers a high reversible capacity(141 mAh g^(−1)at 0.2C),excellent rate capability(111 mAh g^(−1)at 8C,85 mAh g^(−1)even at 20C),and long-term stability(over 85%capacity retention after 1000 cycles),which is attributed to a rapid and reversible O3–P3 phase transition in regions of low voltage and suppresses phase ***,the compound remains unchanged over seven days and keeps thermal stability until 279℃.Remarkably,the polymer solid-state sodium battery assembled by this cathode provides a capacity of 92 mAh g^(−1)at 5C and keeps retention of 96%after 400 *** strategy inspires more rational designs and could be applied to a series of O3 cathodes to improve the performance of solid-state Na-ion batteries.

关键词： High-entropy High-rate performance Li-TM interaction Air stability O3 layered oxide cathode

Accurate characterization of bubble mixing uniformity in a circular region using computational geometric theory

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Particuology 2024年第3期86卷 149-159页

作者： hui Sun Jianxin Xu Shibo Wang Guangcheng cai Hua Wang Wuliang Yin State Key Laboratory ofComplex Nonferrous Metal Resources Clean Utilization Kunming University ofScience and TechnologyKunming650093China bFaulty of Metallurgical and Energy Engineering Kunming University ofScience and TechnologyKunming650093China Faculty of Science Kunming University ofScience and TechnologyKunming650500China Department of Elec.and Electronic Engineering.University of Manchester ManchesterM139PL UK

The present study proposes a novel method based on the geometric theory for measuring the distribution of bubble swarms in the circular region of a direct-contact heat *** was determined that the mixing is uniform when the average distance between the bubble swarms in the unit circular region is approximately 0.9054,which is the standard reference *** effect of sample size(i.e.,the number of bubbles)on mixing uniformity was investigated to determine the optimal sample *** was verified that the metric's accuracy and stability were higher with a sample size of ***,it was proposed to increase the sample size by filling irregular bubbles using a segmentation method,which enabled a further accurate assessment of the mixing *** mixing uniformity of bubble swarms in the circular region and its maximum internal connection with the square region was accurately *** was revealed that the relative average error increased by approximately 3.47% due to information *** proposed method was demonstrated to be rotationally *** present study provided novel insights into evaluating mixing uniformity,which would guide enhanced heat transfer and the effective evaluation of the spatiotemporal characteristics of transient mixing in circular regions or the cross-sections of chemical transport pipelines.

关键词： Direct-contact heat exchanger Circular region Bubble swarm Distribution uniformity AD-Circle method

Single depth image 3D face reconstruction via domain adaptive learning

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Frontiers of Computer Science 2024年第1期18卷 259-261页

作者： Xiaoxu cai Jianwen LOU Jiajun BU Junyu DONG Haishuai WANG hui YU College of Computer Science and Technology Zhejiang UniversityHangzhou 310013China School of Creative Technologies University of PortsmouthPortsmouth PO12DJUK College of Computer Science and Technology Ocean University of ChinaQingdao 266100China

1 Introduction In this paper,we propose a novel domain-adaptive reconstruction method that effectively leverages deep learning and synthetic data to achieve robust 3D face reconstruction from a single depth *** method applies two domain-adaptive neural networks for predicting head pose and facial shape,*** networks undergo training with a customized domain adaptation strategy,using a combination of auto-labeled synthetic and unlabeled real data.

关键词： networks image learning

Theoretical understanding of correlation between magnetic phase transition and the superconducting dome in high-Tc cuprates

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Science China(Physics,Mechanics & Astronomy) 2024年第2期67卷 167-173页

作者： Chen Zhang cai-Xin Zhang Su-Huai Wei Haiqing Lin hui-Xiong Deng State Key Laboratory of Superlattices and Microstructures Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Beijing Computational Science Research Center Beijing 100193China

Many issues concerning the origin of high-temperature superconductivity(HTS)are still under *** example,how the magnetic order varies with doping and its relationship with the superconducting temperature(Tc);and why Tcalways peaks near the quantum critical *** this paper,taking hole-doped La_(2)CuO_(4)as a classical example,we employ the first-principles band structure and total energy calculations with Monte Carlo simulations to explore how the symmetry-breaking magnetic ground state evolves with hole doping and the origin of a dome-shaped superconductivity region in the phase *** demonstrate that the local antiferromagnetic order and doping play key roles in determining the electron-phonon coupling,thus ***,the La_(2)CuO_(4)possesses a checkerboard local antiferromagnetic ground *** the hole doping increases,Tcincreases with the enhanced electron-phonon coupling *** as the doping increases further,the strength of the antiferromagnetic interaction weakens and spin fluctuation *** the critical doping level,a magnetic phase transition occurs that reduces the local antiferromagnetism-assisted electron-phonon coupling,thus diminishing the *** superconductivity disappears in the heavily overdoped region when the ferromagnetic order *** observations could account for why cuprates have a dome-shaped superconductivity region in the phase *** study,thus,contributes to a fundamental understanding of the correlation between doping,local magnetic order,and superconductivity of HTS.

关键词： high-temperature superconductivity antiferromagnetic order electron-phonon coupling doping effect cuprates

Study on cumulative effects of biological craniocerebral trauma under repeated blast

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Theoretical & Applied Mechanics Letters 2024年第3期14卷 174-183页

作者： Xingyuan Huang Bingchen Xia Lijun Chang Zhikang Liao hui Zhao Zhihua cai Hunan Provincial Key Laboratory of Health Maintenance for Mechanical Equipment Hunan University of Science and TechnologyXiangtan 411201China School of Mechanical and Electrical Engineering Foshan UniversityFoshan 528231China Institute for Traffic Medicine PLA Army Characteristic Medical CenterChongqing 400042China

Repeated blast impacts on personnel in explosive environments can exacerbate craniocerebral *** existing studies focus on the injury effects of a single blast,lacking in-depth analysis on the injury effects and cumulative effects of repeated ***,rats were used as the experimental samples to suffer from explosion blasts with different peak air overpressures(167 kPa~482 kPa)and varying number of repeated *** cumulative effect of craniocerebral trauma was most pronounced for moderate repeated blast,showing approximately 95%increase of trauma severity with penta blast,and an approximately 85%increase of trauma severity with penta minor *** cumulative effect of craniocerebral trauma from severe,repeated blast has a smaller rate of change compared to the other two *** severity of trauma from penta blast increased by approximately 69%compared to a single *** physiological,pathological and biochemical analysis show that the degree of neurological trauma caused by repeated blasts is higher than that of single blasts,and the pathological trauma to brain tissue is more extensive and *** trauma degree remains unchanged after double blast,increases by one grade after triple or quadruple blast,and increases by two grades after penta blast.

关键词： Repeated blast Craniocerebral trauma Trauma severity grade Cumulative effects

Numerical and experimental research on axial injection end-burning hybrid rocket motors with polyethylene fuel

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Chinese Journal of Aeronautics 2024年第8期37卷 91-105页

作者： Xiangyu MENG hui TIAN Lingfei HE Jingfei GAO Xiaoting NIU Guobiao cai School of Astronautics Beihang UniversityBeijing 100191China Key Laboratory of Spacecraft Design Optimization&Dynamic Simulation Technologies Ministry of EducationBeijing 100816China

This study investigates the end-burning hybrid rocket motors with polyethylene fuel by the numerical simulation and *** on computational fluid dynamics,a numerical model is *** model is validated by two firing tests in this hybrid rocket motor,which uses oxygen and polyethylene as *** results show that the numerical and experimental data are in good agreement,and the error of the chamber pressure is less than 2.63%.Based on the simulation mode,the blowoff limit of the end-burning hybrid rocket motors is *** the nozzle throat diameter and the inner diameter of grain are large,it is more difficult for the hybrid rocket motor to achieve end-burning mode,i.e.,the flame spreading is prevented in the narrow *** main reason is that when the nozzle throat and the grain port are large,chamber pressure and oxidizer flow velocity are ***,the friction velocity considering the pressure and flow velocity is *** critical friction velocity is about 4.054–4.890 m/s in the hybrid rocket *** the friction velocity exceeds the critical friction velocity,the combustion mode in hybrid rocket motors changes from the flame spreading mode to the end-burning ***,the regression rate formula is obtained by fitting,which shows that the regression rate has a good correlation with combustion chamber *** critical friction velocity and regression rate formula can provide an important reference for end-burning hybrid rocket motors.

关键词： Hybrid rocket motor End burning Blowoff limit Flame propagation Regression rate

Combining systemic inflammatory response index and albumin fibrinogen ratio to predict early serious complications and prognosis after resectable gastric cancer

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World Journal of Gastrointestinal Oncology 2024年第3期16卷 732-749页

作者： Jing-Yao Ren Da Wang Li-hui Zhu Shuo Liu Miao Yu hui cai School of Clinical Medicine Ningxia Medical UniversityYinchuan 750000Ningxia Hui Autonomous RegionChina General Surgery Clinical Medical Center Gansu Provincial HospitalLanzhou 730000Gansu ProvinceChina Key Laboratory of Molecular Diagnostics and Precision Medicine for Surgical Oncology in Gansu Province Gansu Provincial HospitalLanzhou 730000Gansu ProvinceChina NHC Key Laboratory of Diagnosis and Therapy of Gastrointestinal Tumor Gansu Provincial HospitalLanzhou 730000Gansu ProvinceChina Medical College of Jiangsu University Jiangsu UniversityZhenjiang 212013Jiangsu ProvinceChina The First Clinical Medical School Lanzhou UniversityLanzhou 730000Gansu ProvinceChina

BACKGROUND Gastric cancer has a high incidence and fatality rate,and surgery is the preferred course of ***,patient survival rates are still low,and the incidence of major postoperative complications cannot be *** systemic inflammatory response,nutritional level,and coagulation status are key factors affecting the postoperative recovery and prognosis of gastric cancer *** systemic inflammatory response index(SIRI)and the albumin fibrinogen ratio(AFR)are two valuable comprehensive indicators of the severity and prognosis of systemic inflammation in various medical *** To assess the clinical importance and prognostic significance of the SIRI scores and the AFR on early postoperative outcomes in patients undergoing radical gastric cancer *** We conducted a retrospective analysis of the clinicopathological characteristics and relevant laboratory indices of 568 gastric cancer patients from January 2018 to December *** calculated and compared two indicators of inflammation and then examined the diagnostic ability of combined SIRI and AFR values for serious early postoperative *** scored the patients and categorized them into three groups based on their SIRI and AFR *** analysis was used to compare the three groups of patients the prognostic value of various preoperative SIRI-AFR scores for 5-year overall survival(OS)and disease-free survival(DFS).RESULTS SIRI-AFR scores were an independent risk factor for prognosis[OS:P=0.004;hazards ratio(HR)=3.134;DFS:P<0.001;HR=3.543]and had the highest diagnostic power(area under the curve:0.779;95%confidence interval:0.737-0.820)for early serious complications in patients with gastric *** tumor-node-metastasis stage(P=0.001),perioperative transfusion(P=0.044),positive carcinoembryonic antigen(P=0.014)findings,and major postoperative complications(P=0.011)were factors associated with *** Preoperative SIRI and AFR values were s

关键词： Inflammation Albumin fibrinogen ratio Gastric cancer Complications Prognosis

Potential risks of organic contaminated soil after persulfate remediation:Harmful gaseous sulfur release

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Journal of Environmental Sciences 2024年第1期135卷 1-9页

作者： Yuyang Long Zixiao Wu Xiaodong Ding Jiansong Chen Dongsheng Shen Jiali Shentu cai hui Zhejiang Provincial Key Laboratory of Solid Waste Treatment and Recycling Zhejiang Engineering Research Center of Non-ferrous Metal Waste RecyclingInstrumental Analysis CenterSchool of Environmental Science and EngineeringZhejiang Gongshang UniversityHangzhou 310012China Shangyu Yingtai Fine Chemical Co. Ltd.Shaoxing 312000China Hangzhou Ecological Environment Monitoring Center Hangzhou 310007China

Persulfate is considered a convenient and efficient remediation agent for organic contaminated ***,the potential risk of sulfur into the soil remediation by persulfate remains *** this study,glass bottles with different persulfate dosages and groundwater tables were set up to simulate persulfate remediation of organic pollutants(aniline).The results found sulfate to be the main end-product(83.0%–99.5%)of persulfate remediation after10 ***,H_(2)S accounted for 93.4%–99.4%of sulfur reduction end-products,suggesting that H_(2)S was the final fate of sulfur.H_(2)S was released rapidly after one to three days at a maximum concentration of 33.0 ppm,which is sufficient to make a person *** to the fitted curve results,H_(2)S concentration decreased to a safe concentration(0.15 ppm)after 20–85 ***,the maximum concentration of methanethiol reached 0.6 *** results indicated that secondary pollution from persulfate remediation could release harmful gases over a long ***,persulfate should be used more carefully as a remediation agent for soil contamination.

关键词： Gaseous sulfur release H_2S Long period potential risk Organic contaminated soil remediation Persulfate

TSPO deficiency exacerbates acute lung injury via NLRP3 inflammasome-mediated pyroptosis

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Chinese Medical Journal 2024年第13期137卷 1592-1602页

作者： Jingyi Han Xue Zhang Menghua cai Feng Tian Yi Xu hui Chen Wei He Jianmin Zhang hui Tian Department of Thoracic Surgery Qilu Hospital of Shandong UniversityJinanShandong 250012China CAMS Key Laboratory of T Cell and Immunotherapy Department of ImmunologyInstitute of Basic Medical SciencesChinese Academy of Medical Sciences and School of Basic MedicinePeking Union Medical CollegeState Key Laboratory of Medical Molecular BiologyBeijing 100005China Changzhou Xitaihu Institute for Frontier Technology of Cell Therapy ChangzhouJiangsu 213000China Haihe Laboratory of Cell Ecosystem Chinese Academy of Medical Sciences&Peking Union Medical CollegeTianjin 300020China

Background:Acute respiratory distress syndrome(ARDS)is a common cause of respiratory failure in many critically ill *** inflammasome activation plays an important role in the induction of acute lung injury(ALI)and ARDS,the regulatory mechanism of this process is still *** cells are stimulated by inflammation,the integrity and physiological function of mitochondria play a crucial part in ***,the underlying mechanisms and function of mitochondrial proteins in the process of pyroptosis are largely not yet ***,we identified the 18-kDa translocator protein(TSPO),a mitochondrial outer membrane protein,as an important mediator regulating nucleotide-binding domain,leucine-rich repeat,and pyrin domain-containing protein 3(NLRP3)inflammasome activation in macrophages during ***:TSPO gene knockout(KO)and lipopolysaccharide(LPS)-induced ALI/ARDS mouse models were employed to investigate the biological role of TSPO in the pathogenesis of *** macrophages were used to further characterize the effect of TSPO on the NLRP3 inflammasome *** of NLRP3 inflammasome was preformed through LPS+adenosine triphosphate(ATP)co-stimulation,followed by detection of mitochondrial membrane potential,reactive oxygen species(ROS)production,and cell death to evaluate the potential biological function of *** between two groups were performed with a two-sided unpaired ***:TSPO-KO mice exhibited more severe pulmonary inflammation in response to LPS-induced *** deficiency resulted in enhanced activation of the NLRP3 inflammasome pathway,promoting more proinflammatory cytokine production of macrophages in LPS-injured lung tissue,including interleukin(IL)-1β,IL-18,and macrophage inflammatory protein(MIP)-*** in TSPO-KO macrophages tended to depolarize in response to cellular *** increased production of mitochondrial damage-associated molecular pattern led to enhanced mitochondrial membr

关键词： Acute respiratory distress syndrome Acute lung injury 18-kDa translocator protein Macrophage NLRP3 inflammasome Inflammation