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Regioselective cation exchange reaction for photoelectrochemical water splitting

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Rare Metals 2024年第7期43卷 3400-3407页

作者： Mo-yan Chen Tai-Song Zhang Zhi yan Jiang-Nan Lv Xiao-Ting Sun Rui-Xia yang mark TSwihart Xiao-Hong Xu yang Liu Research Institute of Materials Science of Shanxi Normal University&Key Laboratory of Magnetic Molecules and Magnetic Information Materials of Ministry of Education Taiyuan 030031China Department of Chemical and Biological Engineering University at Buffalo(SUNY)NY 14260USA Department of Materials Science Fudan UniversityShanghai 200433China

Engineering copper sulfide-based heterostructures via cation exchange(CE)is an appealing approach,as it allows selective combination of distinct compositions and functions of metal *** heterostructures can play a significant role in photoelectrochemical applications,but the effect of the ratio between two or more domains in such heterostructures on the photoresponse has not been well explored.

关键词： exchange sulfide splitting

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Early anticoagulation in patients with stroke and atrial fibrillation is associated with fewer ischaemic lesions at 1 month: the ATTUNE study

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Stroke & Vascular Neurology 2024年第1期9卷 30-37,I0034页

作者： Angelos Sharobeam Longting Lin Christina Lam Carlos Garcia-Esperon Yash Gawarikar Ronak Patel Matthew Lee-Archer Andrew Wong Michael Roizman Amanda Gilligan Andrew Lee Kee Meng Tan Susan Day Christopher Levi Stephen M Davis mark pars.ns.bernard yan Melbourne Brain Centre at Royal Melbourne Hospital ParkvilleVictoriaAustralia University of New South Wales South Western Sydney Clinical School LiverpoolNew South WalesAustralia Department of Neurology John Hunter HospitalNewcastleNew South WalesAustralia Department of Neurology Calvary Public HospitalCanberraAustralian Capital TerritoryAustralia Department of Neurology Northern Hospital EppingEppingVictoriaAustralia Department of Neurology Royal Brisbane and Women's HospitalHerstonQueenslandAustralia The University of Queensland School of Medicine HerstonQueenslandAustralia Neurosciences Clinical Institute Epworth HealthcareRichmondVirginiaAustralia Department of Neurology Austin HealthUniversity of MelbourneHeidelbergVictoriaAustralia Flinders University College of Medicine and Public Health AdelaideSouth AustraliaAustralia Department of Neurology Gold Coast University HospitalSouthportQueenslandAustralia The University of Sydney Northern Clinical School St LeonardsNew South WalesAustralia Department of Neurology and Neurophysiology Liverpool HospitalLiverpoolNew South WalesAustralia

Background The optimal time to commence anticoagulation in patients with atrial fibrillation(AF)after ischaemic stroke or transient ischaemic attack(TIA)is unclear,with guidelines differing in recommendations.A limitation of previous studies is the focus on clinically overt stroke,rather than radiologically obvious diffusion-weighted imaging ischaemic *** aimed to quantify silent ischaemic lesions and haemorrhages on MRI at 1month in patients commenced on early(ns and more haemorrhages in the early anticoagulant group at 1-month *** A prospective multicentre,observational cohort study was performed at 11 Australian stroke *** and MRI data were collected at baseline and follow-up,with blinded imaging assessment performed by two *** of commencement of anticoagulation was at the discretion of the treating stroke *** We recruited 276 patients of whom 208 met the eligibility *** average age was 74.2 years(SD±10.63),and 79(38%)patients were *** National Institute of Health Stroke Scale score was 5(IQR 1–12).Median baseline ischaemic lesion volume was 5mL(IQR 2–17).There were a greater number of new ischaemic lesions on follow-up MRI in patients commenced on anticoagulation≥4days after index event(17%vs 8%,p=0.04),but no difference in haemorrhage rates(22%vs 32%,p=0.10).Baseline ischaemic lesion volume of≤5mL was less likely to have a new haemorrhage at 1month(p=0.02).There was no difference in haemorrhage rates in patients with an initial ischaemic lesion volume of>5mL,regardless of anticoagulation *** Commencing anticoagulationns at 1month in AF *** is no increased rate of haemorrhage with early *** results suggest that early anticoagulation after mild-to-moderate acute ischaemic stroke associated w

关键词： patients lesions ischaemic

High-temperature dielectric polymer composite for high power energy storage applications

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Science China Chemistry 2024年第8期67卷 2425-2426页

作者： Xiangyan Yu Haixue yan School of Engineering and Materials Science Queen Mary University of LondonLondon E14NSUK

Polymer-based dielectric films are the main component of dielectric capacitors due to their high power density, which plays an important role in power electrical systems using renewable energy, such as electric vehicles, solar panel, wind power [1]. However, the energy density of dielectrics is lower than that of other energy storage materials, such as batteries or supercapacitors. High energy density of the dielectric is related to high dielectric permittivity and high dielectric breakdown strength (DBS).

关键词： composite dielectric energy

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A robust implicit high-order discontinuous Galerkin method for solving compressible Navier-Stokes equations on arbitrary grids

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Acta Mechanica Sinica 2024年第8期40卷 96-119页

作者： Jia yan Xiaoquan yang Peifen Weng Shanghai Institute of Applied Mathematics and Mechanics Shanghai Key Laboratory of Mechanics in Energy EngineeringSchool of Mechanics and Engineering ScienceShanghai UniversityShanghai200072China College of Energy and Mechanical Engineering Shanghai University of Electric PowerShanghai200090China

The primary impediments impeding the implementation of high-order methods in simulating viscous flow over complex configurations are robustness and *** challenges impose significant constraints on computational efficiency,particularly in the domain of engineering *** address these concerns,this paper proposes a robust implicit high-order discontinuous Galerkin(DG)method for solving compressible Navier-Stokes(ns)equations on arbitrary *** method achieves a favorable equilibrium between computational stability and *** solve the linear system,an exact Jacobian matrix solving strategy is employed for preconditioning and matrix-vector generation in the generalized minimal residual(GMRES)*** approach mitigates numerical errors in Jacobian solution during implicit calculations and facilitates the implementation of an adaptive Courant-Friedrichs-Lewy(CFL)number increasing strategy,with the aim of improving convergence and *** further enhance the applicability of the proposed method for intricate grid distortions,all simulations are performed in the reference *** practice significantly improves the reversibility of the mass matrix in implicit calculations.A comprehensive analysis of various parameters influencing computational stability and efficiency is conducted,including CFL number,Krylov subspace size,and GMRES convergence *** computed results from a series of numerical test cases demonstrate the promising results achieved by combining the DG method,GMRES solver,exact Jacobian matrix,adaptive CFL number,and reference domain calculations in terms of robustness,convergence,and *** analysis results can serve as a reference for implicit computation in high-order calculations.

关键词： Discontinuous Galerkin method Exact Jacobian matrix GMRES solver Adaptive CFL number Reference domain High-order

Voltage rise rate-related generalised probabilistic lifetime model of turn-to-turn insulation in inverter-fed motors

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High Voltage 2024年第1期9卷 46-55页

作者： yan yang Xueyang Bai Yuxing Lei Kai Liu Guangning Wu School of Electrical Engineering Southwest Jiaotong UniversityChengduChina

The lifetime model of turn-to-turn insulation in inverter-fed motors is studied.A lifetime model has been built by considering the effect of inverter-generated high voltage rise rate(dv/dt up to 20 V/ns).This model is followed by the generalised probabilistic model,in which the lifetime is proportional to the nth power of the voltage rise ***,by investigating the effect of voltage rise rate on the partial discharge characteristics,it is found that the effect of voltage rise rate on the charge transport process in a voltage cycle is similar to that of the voltage *** enhanced partial discharge activity and induced charges are responsible for accelerated ageing and thus determine the final lifetime of turn-to-turn *** this case,the generalised probabilistic electric lifetime model is applicable to the voltage rise rate as well as the voltage amplitude.

关键词： lifetime inverter insulation

Inetetamab combined with tegafur as second-line treatment for human epidermal growth factor receptor-2-positive gastric cancer: A case report

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World Journal of Clinical Cases 2024年第4期12卷 820-827页

作者： Jing-Hao Zhou Qi-Jun Yi Ming-yan Li yan Xu Qi Dong Cong-Ying Wang Hai-yan Liu Department of Oncology The Second Affiliated Hospital of Shandong First Medical UniversityTai’an 271000Shandong ProvinceChina

BACKGROUND Human epidermal growth factor receptor-2(HER-2)plays a vital role in tumor cell proliferation and ***,the prognosis of HER2-positive gastric cancer is ***,a novel anti-HER2 targeting drug independently developed in China,exhibits more potent antibody-dependent cell-mediated cytotoxicity than trastuzumab,which is administered as the first-line treatment for HER2-positive gastric cancer in combination with *** this case,the efficacy and safety of inetetamab combined with tegafur was investigated as a second-line treatment for HER2-positive gastric *** SUMMARY A 52-year-old male patient with HER2-positive gastric cancer presented with abdominal distension,poor appetite,and fatigue two years after receiving six cycles of oxaliplatin combined with tegafur as first-line treatment after surgery,followed by tegafur monotherapy for six *** patient was diagnosed with postoperative recurrence of gastric *** received 17 cycles of a combination of inetetamab,an innovative domestically developed anti-HER2 monoclonal antibody,and tegafur chemotherapy as the second-line treatment(inetetamab 200 mg on day 1,every 3 wk combined with tegafur twice daily on days 1–14,every 3 wk).Evaluation of the efficacy of the second-line treatment revealed that the patient achieved a stable condition and progression-free survival of 17 *** tolerated the treatment well without exhibiting any grade 3-4 adverse *** Inetetamab combined with chemotherapy for the treatment of metastatic HER2-positive gastric cancer demonstrates significant survival benefits and acceptable safety.

关键词： Inetetamab Gastric cancer Human epidermal growth factor receptor-2 protein Tegafur Case report

Sn-fused perylene diimides: Synthesis, mechanism, and properties

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Chinese Chemical Letters 2024年第10期35卷 270-274页

作者： Wenzhong Zhang Zirui yan Lingcheng Chen Yi Xiao State Key Laboratory of Fine Chemicals Dalian University of Technology

The first example of metal Sn-fused perylene diimides(PDI) derivative(Sn-PDI) was designed, synthesized, and investigated. To obtain this type compound, a simple one-pot synthesis, named stannylative cycloaddition reaction, has been successfully developed via a palladium-based catalyst system. The novel mechanism exhibits that the reaction experiences oxidative addition, Pd-cyclization, stannylation, Pd-Sn-cyclization, and reductive elimination processes successively. This stannylative cycloaddition does realize unique σ-π hyperconjugation effect and therefore significantly influencing on the photophysical, electrochemical and excited state properties. Compared with those of PDI, both of the absorption and fluorescence spectra of Sn-PDI display large red-shifts over 20 nm. The electron energy levels of Sn-PDI have changed with an uncommon regulation. And Sn-PDI gives a considerably raised highest occupied molecular orbital(HOMO) level of-6.00 eV More importantly, the singlet excitons of Sn-PDI could efficiently intersystem cross(ISC) into triplet state with a long lifetime of 17.8 μs, which is far longer than that(4.4 ns) of PDI.

关键词： Functional dyes Hyperconjugation Organometallic heterocyclics Perylene diimides Triplet state

Characteristics and genetic mechanism of the Mesoproterozoic rift system,Ordos Basin,China

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Energy Geoscience 2024年第1期5卷 141-152页

作者： Meng Li Xiangbin yan Wei Zhang Yuanling Guo Chaoying Liu Lingling Fan Shuang yang Petroleum Exploration and Production Research Institute SINOPECBeijing100083China Exploration and Development Research Institute SINOPEC North China CompanyZhengzhouHenan450006China

The Mesoproterozoic rifts are developed in the Ordos Basin located in the western margin of the North China *** on the latest 3D seismic data and previous research results,this study intends to discuss the zonal differential deformation characteristics and genetic mechanism of the Mesoproterozoic rifts in the Ordos ***-trending rifts are developed in the Mesoproterozoic in the south-central Ordos Basin,the main part of which are located near the western margin of the North China ***-trending rifts are developed in the north of the basin,while NW-NNW rifts in the Mesoproterozoic in Hangjinqi *** genetic mechanism of the Mesoproterozoic rifts is related to regional extensional stress field,plate boundary conditions and internal preexisting *** main extensional stress direction strikes NWW-SSE(120°)in the western margin of the North China Plate,based on the forward rift trend of the northern *** Hangjinqi area,the reactivation of the existing NWtrending Wulansu fault and NW-NW-trending Daolao fault,results in dextral shear stress *** boundary between the western margin of the North China Plate and its adjacent plates forms a nearly ns-trending preexisting basement tectonic belt,which intersects with the NWW-SSE(120°)extensional stress at an acute angle of 60°.Therefore,the western margin of the North China Plate is formed by oblique normal faults under oblique *** to the long time span of Columbia Supercontinent breakup(1.8e1.6 Ga),the oblique rift in the south-central Ordos Basin is formed under the continuous oblique extension at the western margin of the North China Plate.

关键词： Columbia Supercontinent Ordos Basin Rift system Mesoproterozoic Genetic mechanism

Investigating the neutron star physics through observations of several young pulsars in the dipole-field re-emergence scenario

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Science China(Physics,Mechanics & Astronomy) 2024年

作者： Yu-Long yan Quan Cheng Xiao-Ping Zheng Institute of Astrophysics Central China Normal University Department of Astronomy Huazhong University of Science and Technology

The observed timing data, magnetic tilt angle χ, and age of young pulsars could be used to probe some important issues about neutron star（ns） physics, e.g., the ns internal magnetic field configuration, and the number of precession cycles ξ. Both quantities are critical in studying the continuous gravitational wave emission from pulsars, and the latter generally characterizes the mutual interactions between superfluid neutrons and other particles in the ns interior. The timing behavior of pulsars can be influenced by the dipole field evolution, which instead of decaying, may increase with time. An increase in the dipole field may result from the re-emergence of the initial dipole field Bd,ithat was buried into the ns interior shortly after the birth of the *** this work, the field re-emergence scenario ξ and the internal field configuration of several young pulsars, as well as their Bd,iare investigated by assuming typical accreted masses △M. Moreover, since the Crab pulsar has an exactly known age and its tilt angle change rate can be inferred from observations, we can set stringent constraints on its ξ, Bd,i, and △M. Although for other young pulsars without exactly known ages and tilt angle change rates, these quantities cannot be accurately determined, we find that their ξ are generally within ～10～4-10～6, and some of them probably have magnetar-strength Bd,i. Our work could be important for investigating the transient emissions associated with nss, the origin of strong magnetic fields of nss, pulsar population,continuous gravitational wave emission from pulsars, and accretion under extreme conditions in principle.

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